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1.
悬浮颗粒物和沉积物是湖泊有机污染物的主要承载物质,其稳定同位素研究对有效识别有机质污染导致的湖泊富营养化具有重要意义.本研究选取乌梁素海为研究区,于2019年4月（融冰期）、7月（夏灌期）和10月（秋灌期）对湖区及入湖渠道的表层沉积物和悬浮颗粒物中有机碳的δ13C、C/N比及总有机碳（TOC、POC）和总氮（TON、PON）含量进行测定分析,联合采用δ13C、C/N及同位素多元混合模型研究湖泊有机碳来源及其贡献率.结果表明,乌梁素海悬浮颗粒物有机碳δ13CPOC的变化范围为-23.29‰~-29.75‰,呈现10月>4月>7月、入湖渠道>湖区的趋势,悬浮颗粒物POC/PON比变化范围为4.10~21.35,呈现出4月<7月<10月的时间变化,悬浮颗粒有机质主要来源于浮游植物（51.59%）、入湖渠道泥沙（34.60%）和大型水生植物（13.76%）.沉积物有机碳δ13CTOC变化范围为-27.58‰~-22.68‰,呈现4月<10月<7月的变化,沉积物TOC/TON比变化范围为3.06~23.77,时空变化明显,沉积物有机质则主要源于入湖渠道挟带的泥沙,贡献达72.79%以上,而浮游植物与大型水生植物的贡献率相差较小,分别为11.85%和15.36%.本研究可以初步判定受入湖渠道影响的富营养化湖泊中悬浮颗粒物和沉积物有机碳来源,为改善湖泊有机污染和研究有机碳来源提供更多理解. 相似文献
2.
Cascadia边缘与天然气水合物共生沉积物中有机质碳、氮同位素组成及意义 总被引：1，自引：1，他引：1
Hydrate Ridge南高点ODP204航次5个站位54个沉积物样品中有机碳C, N同位素组成及C/N比值表明沉积物中的有机质主要来自海洋. 对1245B孔的系统分析表明天然气水合物的发育改变了沉积物中有机碳和氮同位素的成岩演化轨迹, 水合物发育处δ15N值和C/N比值同时变低, 且δ13C值相对较重; 在水合物稳定带内δ15N值的亏损将近2‰. 水合物发育处沉积物中氮含量的增加和δ15N值的亏损, 推断可能与天然气水合物发育处沉积物中细菌(包括古细菌)的固氮作用有关. 沉积物中有机质中碳、氮同位素的分布与沉积环境的变化同步响应, 同时亦反映流体活动的变化. 相似文献
3.
δ13C和δ15N指示不同生态类型湖泊无机氮及有机质来源 总被引：2，自引：0，他引：2
为了探讨不同生态类型湖泊(天然湖泊、城市湖泊)中无机氮和有机质来源,分别采集湖泊中水体、表层沉积物、水生植物、底栖动物进行碳、氮同位素特征分析.结果表明:蚌湖水体δ15N-NH4均值为-1.8‰±1.0‰,δ15N-NO3-均值为-0.5‰±1.7‰,说明蚌湖水体氮表现为雨水和农业肥料氮污染;象湖δ15 N-NH4+均值为6.8‰±8.6‰,其中养殖废水和管道排污口δ15N-NH4+值分别为13.5‰和25.4‰,表现出污水氮同位素特征,象湖δ15 N-NO3-均值为-2.9‰±4.2‰,是氨的硝化作用引起的氮同位素分馏所致.蚌湖表层沉积物、水生植物δ15N差别不大,分别为6.6‰±0.3‰、7.1‰±0.7‰,水生植物δ13C均值为-27.5‰±0.3‰,比沉积物δ13C偏负3‰.有机C/N为9.4±0.5,比沉积物C/N明显偏高6,反映水生植物是蚌湖有机质的主要来源.象湖表层沉积物δ15N、δ13C及有机C/N分布范围大,δ15N在3.6‰～8.3‰之间,均值为5.9‰±1.6‰,δ13C在-27.1‰～-24.7‰之间,均值为-26.0‰±1.0‰,有机C/N在2.6 ～10.8之间,均值为6.2±2.7,表明城市湖泊沉积有机质来源复杂.2个湖泊蚌类δ15N组成与各自湖泊表层沉积物δ15N组成相对应. 相似文献
4.
鄱阳湖候鸟栖息地湖泊悬浮有机质的碳氮分布及来源分析——以大湖池和沙湖为例 总被引：1，自引：0，他引：1
以江西鄱阳湖国家级自然保护区的2个湖泊——大湖池和沙湖为研究对象，分析不同季节和水位悬浮有机质的碳氮稳定同位素（δ13C和δ15N）及碳氮比值（C/N）的变化特征，甄别悬浮有机质的来源.结果表明：在不同水位条件下，悬浮有机质的δ13C和δ15N均存在差异显著性.沙湖5月水位上涨时，悬浮有机质δ13C最正，均值为-26.4‰±0.9‰，10月退水后，δ13C最负，均值为-31.2‰±1.1‰.悬浮有机质δ15N值在5月和8月较低（范围为3.5‰~5.5‰），10月也相对较低，均值为6.1‰±0.6‰，而12月相对较高（7.3‰~10.8‰）.悬浮有机质C/N值在10月最低，均值为6.5±0.6，小于7，与其他各月的C/N有显著差异，而其他各月C/N在7.8~8.7之间，不存在显著差异.大湖池悬浮有机质δ13C、δ15N各月的变化趋势与沙湖类似，并且两个湖泊在相同月份的δ13C、δ15N或C/N均不存在显著差异，但大湖池的δ13C和δ15N比沙湖的δ13C和δ15N均值略偏正0.1‰~0.5‰，C/N比沙湖的C/N略偏低0~0.4.有机δ13C、δ15N结合C/N示踪表明，大湖池和沙湖的悬浮有机质在5月水位上涨和8月丰水期主要来源于河流运输的土壤有机质，表层沉积物对5月悬浮有机质也有一定贡献（16%），水生浮叶植物对8月悬浮有机质有一定贡献（25%）；10月秋季退水后悬浮有机质主要来源于藻类（77%），表层沉积物有一定贡献（23%）；12、3和4月冬、春季枯水期悬浮有机质主要来源于表层沉积物，候鸟粪便对12月悬浮有机质有较大贡献（40%），湿地植物碎屑对3和4月有较大贡献（47%和51%）. 相似文献
5.
基于多指标分析的博斯腾湖表层沉积物有机碳来源 总被引：3，自引：0，他引：3
通过有机碳稳定同位素(δ13Corg)、有机碳、氮含量及其比值(C∶N)的测定,结合已有的正构烷烃空间分布特征数据,对新疆博斯腾湖表层沉积物的有机碳来源进行综合研究.结果表明:博斯腾湖表层沉积物δ13Corg值在-26.7‰~-24.1‰之间波动,变幅较小;C∶N的波动范围为4.8~8.5,平均值约为7.4;正构烷烃的碳数分布范围为n C13~n C35,所有采样点样品的主峰碳以n C17和n C23为主.参考博斯腾湖文献调查资料,基于δ13Corg值、C∶N及正构烷烃等指标的空间分布状况,发现博斯腾湖表层沉积物中的有机碳主要来自湖泊内部浮游生物的残体;而不同湖区沉积物有机碳的内、外源贡献比例不同,其中陆源碎屑、挺水植物、沉水植物的贡献空间差异较大.博斯腾湖有机碳来源的空间差异主要表现在湖泊东部近岸水域表层沉积物有机碳主要为外源贡献,中心湖泊东部和西部浅水区表层沉积物有机碳由外源和内源共同贡献,而其余大部分水域表层沉积物有机碳则主要为内源贡献. 相似文献
6.
碳氮稳定同位素示踪鄱阳湖流域蚌湖丰水期的氮污染 总被引：2，自引：1，他引：1
鄱阳湖边缘深水区是鄱阳湖水位上涨时扩散而成的低洼湖区,通过对其一典型边缘湖泊——蚌湖丰水期的氮浓度和同位素特征值的检测,分析这类洪泛湖泊在水位最高时期水体颗粒有机质及无机氮的氮同位素变化特征,并识别氮污染来源及转化途径.结果表明:6月悬浮颗粒有机质碳氮同位素值(δ~(13)C:-26.7‰~-23.7‰,δ~(15)N:2.6‰~6.2‰)介于土壤有机质(δ~(13)C:-25.21‰±0.52‰,δ~(15)N:3.79‰±0.37‰)和水生植物的碳氮同位素值(δ~(13)C:-28.8‰~-24.9‰,δ~(15)N:5.3‰~8.2‰)之间.7月相比于6月,降低的δ~(13)C(-27.6‰~-23.2‰)和升高的δ~(15)N(4.3‰~7.7‰)表明暴雨冲刷带来更多的周边陆地碎屑输入.无机氮在6月以铵态氮(NH_4~+-N)为主要形态,7月以硝态氮(NO_3~--N)为主要形态.6月δ~(15)NH_4~+较负的特征值(-18.6‰±5.2‰)表明铵态氮主要来源于雨水,硝态氮(δ~(15)NO_3~-:1.4‰±3.0‰)主要来源于农业化肥和雨水.7月相比于6月,铵态氮和硝态氮的浓度和同位素值都大幅升高(分别升高了0.3和2倍,6‰和3‰),是暴雨冲刷陆地使农业化肥、城镇生活废水和畜禽养殖废水输入的结果.水生植物的δ~(15)N在7月(8.8‰±1.1‰)相比于6月(6.6‰±1.1‰)也升高了较多,是由于水生植物吸收了更高δ~(15)N废水无机氮的结果.通过颗粒有机质和无机氮的δ~(15)N分析可知,湖区水体氮的矿化作用和硝化作用较强,藻类对湖泊的内源氮贡献较弱,沿河湖的畜禽养殖在暴雨时对水域污染的威胁较大.本研究提供了洪泛湖泊氮污染治理的科学依据. 相似文献
7.
通过对鱼苗时期鄱阳湖网箱养殖区沉积物、饵料及鱼粪等样品总有机碳(TOC)含量、总氮(TN)含量、碳氮比(C/N)、δ^13 C及δ^15 N的测定,分析探讨了鄱阳湖网箱养殖区沉积物有机质来源,量化了网箱养殖废物对养殖区沉积物有机质的贡献.结果表明,网箱养殖区沉积物的δ^13 C和δ^15 N值分别为-27.67‰~-25.65‰和5.19‰~7.27‰,饵料的δ^13 C和δ^15 N值分别为-24.73‰和10.28‰,鱼粪的δ^13 C和δ^15 N值分别为-26.30‰和15.54‰.网箱养殖区沉积物有机质来源主要有残饵、浮游生物及其他来源,其贡献率分别为48.3%±11.4%、25.6%±11.3%及26.0%±5.8%,而鱼粪的贡献几乎可以忽略不计.在水动力平流引起的扩散及沉积物的再悬浮的影响下,网箱养殖源有机质的扩散距离达1500 m.在鱼苗时期,鱼类网箱养殖的残饵是鄱阳湖网箱养殖区沉积物有机质的主要来源. 相似文献
8.
太湖梅梁湾富营养化过程的同位素地球化学证据 总被引：4，自引：0，他引：4
以浅水湖泊太湖为研究对象,通过湖泊水体、水生生物同位素以及相应湖泊水体营养指标的比较分析,并根据梅梁湾钻孔沉积物TN,TP,TOC,C/N,δ15N,δ13C等多项指标记录,恢复了湖泊富营养化过程.研究结果表明,不同湖区植物碳、氮同位素值和水体NH4+的δ15N值变化反映了植物组成和营养水平的差异.梅梁湾水体NH4+的δ15N和水环境参数不同月份的变化反映了外部营养载荷的输入对湖泊环境有明显的影响.1950～1990年湖泊沉积物有机质碳、氮同位素同步变化的趋势说明湖泊初级生产力的增长和湖泊逐渐富营养化的过程,而1990年之后二者之间反相关关系的出现表明在富营养条件下,大量浮游植物生长对富15N的无机氮的吸收及表层沉积物有机质分解和反硝化作用,代表湖泊富营养化加剧.以同位素示踪,并结合元素地球化学指标变化,将太湖梅梁湾富营养化过程分为三阶段,以20世纪50年代和20世纪90年代为营养状态的转换时段,揭示了人类活动不断加强的影响,与近50年来的湖泊环境监测结果一致. 相似文献
9.
湖泊沉积物氮同位素(δ15N)在古环境、古气候变化方面有着指示气候干湿变化的重要作用,但目前学界对于δ15N记录作为气候代用指标所指示的气候干湿变化特征仍缺乏深入探索。本文以贵州省梵净山九龙池湖泊沉积物为研究对象,分析并探讨δ15N所记录的梵净山地区气候干湿变化过程与特征,并结合总有机碳(TOC)、总氮(TN)和碳氮比值(C/N)数据进行对比研究,结果表明:(1)由于九龙池湖泊沉积物有机质受流域输入影响,气候湿润时,陆生植物增多,土壤湿度增大,外源输入对湖泊沉积物有机质影响增大,沉积物δ15N值偏负;气候干旱时,陆生植物减少,土壤湿度降低,外源输入对湖泊沉积物有机质影响减小,沉积物δ15N值偏正;(2)九龙池湖泊沉积物δ15N记录很好地揭示了梵净山地区全新世的气候干湿变化过程,即早期(11.5—9.2 ka B.P.)亚洲夏季风增强,气候从干旱期向湿润期转变,中期(9.2—3.0 ka B.P.)亚洲夏季风强盛,气候整体处于湿润期,晚期(3.0—2.2 k... 相似文献
10.
通过对内蒙古高原呼伦湖沉积物样品总有机碳含量(TOC)及其稳定同位素(δ13Corg)、总氮含量(TN)和TOC/TN(C/N)值的测定,结合沉积岩芯AMS14C年代标尺,分析了中全新世以来呼伦湖沉积物有机碳埋藏速率随时间变化的趋势及有机质的来源,并探讨了影响呼伦湖有机碳埋藏的主要因素.结果表明,中全新世以来呼伦湖有机碳埋藏速率平均值约为2.06 g/(m~2·a),碳储量约为35.25 Tg C,且总体上呈现增加趋势.呼伦湖沉积物中有机质主要来源于外源输入,但近1000 a以来内源输入逐渐增加并占据优势.呼伦湖有机碳埋藏速率与温度和降水均呈负相关,表明在长时间尺度上,升温及降水量的增加可能对呼伦湖的碳埋藏起到一定的抑制作用. 相似文献
11.
Seasonal and annual trends of changes in rainfall, rainy days, heaviest rain and relative humidity have been studied over the last century for nine different river basins in northwest and central India. The majority of river basins have shown increasing trends both in annual rainfall and relative humidity. The magnitude of increased rainfall for considered river basins varied from 2–19% of mean per 100 years. The maximum increase in rainfall is observed in the Indus (lower) followed by the Tapi river basin. Seasonal analysis shows maximum increase in rainfall in the post‐monsoon season followed by the pre‐monsoon season. There were least variations in the monsoon rainfall during the last century and winter rainfall has shown a decreasing trend. Most of the river basins have experienced decreasing trends in annual rainy days with a maximum decrease in the Mahanadi basin. The heaviest rain of the year has increased from 9–27 mm per 100 years over different river basins with a maximum of 27 mm for the Brahamani and Subaranrekha river basins. A combination of increase in heaviest rainfall and reduction in the number of rainy days suggest the possibility of increasing severity of floods. Such information is useful in the planning, development and management of water resources in the study area. Further, the majority of river basins have also experienced an increasing trend in relative humidity both on seasonal and annual scales. An increase in annual mean relative humidity for six river basins has been found in the range of 1–18% of mean per 100 years, while a decrease for three river basins from ? 1 to ? 13% of mean per 100 years was observed, providing a net increase in the study area by 2·4% of mean per 100 years. It is understood that an increase in areal extent of vegetation cover as well as rainfall over the last century has increased the moisture in the atmosphere through enhanced evapotranspiration, which in turn has increased the relative humidity. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
12.
Although changes in rainfall characteristics have been noted across the world, few studies have reported those in mountainous areas. This study was undertaken to clarify spatial and temporal variations in rainfall characteristics such as annual rainfall amount (Pr), mean daily rainfall intensity (η), and ratio of rain days (λ) in mountainous and lowland areas in Taiwan. To this aim, we examined spatial and year‐to‐year variations and marginal long‐term trends in Pr, η, and λ, based on rainfall data from 120 stations during the period 1978–2008. The period mean rainfall () at the lowland stations had strong relationships with the period mean daily rainfall intensity () and the period mean ratio of rain days () during those 31 years. Meanwhile, was only strongly related to at mountainous stations, indicating that influences on spatial variations in were different between lowland and mountainous stations. Year‐to‐year variations in Pr at each station were primarily determined from the variation in η at most stations for both lowland and mountainous stations. Long‐term trend analysis showed that Pr and η increased significantly at 10% and 31% of the total 120 stations, respectively, and λ decreased significantly at 6% of the total. The increases in Pr were mostly accompanied by increases in η. Although stations with significant η increases were slightly biased toward the western lowland area, increases or decreases in Pr and λ were not common. These results contribute to understanding the impacts of possible climate changes on terrestrial hydrological cycles. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
13.
Phosphorus dynamics in water and sediments in urbanized and non-urbanized rivers in Southern Brazil 总被引：1，自引：0，他引：1
Pagliosa PR Fonseca A Bosquilha GE Braga ES Barbosa FA 《Marine pollution bulletin》2005,50(9):965-974
Phosphorus flux models show that the removal tends to be a common feature in polluted estuarine systems whereas the release of P to the adjacent coastal area occurs in pristine environments. This study analyzes the distribution of P in water and sediments along six rivers in the south coast of Brazil. Three rivers located inside protected areas were considered non-polluted and used as a control of urbanization. The other three, situated within urbanized areas, were considered as having highly elevated concentrations of P. Results showed a different behavior of P in water and sediments located in urbanized and non-urbanized areas. The concentrations of dissolved organic (P-org) and inorganic (P-inorg) phosphorus in water, and the total phosphorus (P-tot) and polyphosphate (P-poly) in sediments where higher in the urbanized rivers compared to the non-urbanized ones. Both P of punctual origin and of diffuse origin contributed to the maintenance of elevated concentrations and disturbed the natural fluxes along the polluted rivers. The minimum and maximum concentrations in urbanized areas varied from 0.39 to 12.45 (microM) for P-org and 0.00 to 5.92 (microM) for P-inorg in water, and in sediments from 89.90 to 808.16 (microM g(-1)) for P-tot and 0.00 to 76.51 (microM g(-1)) for P-poly. In non-urbanized areas concentrations in water varied from 0.22 to 1.20 (microM) for P-inorg and 4.43 to 5.56 (microM) for P-org, and in sediments from 45.91 to 652.26 (microM g(-1)) for P-tot and 0.00 to 8.61 (microM g(-1)) for P-poly. Using a hierarchical sampling design and a simple model of variation of P (K(d) model) it was possible to demonstrate that urbanized and non-urbanized estuaries may act as sinks or sources of P. The variation of P analysis in different points along each of the six rivers showed that release and removal areas may occur within a same river independently of its urbanization. 相似文献
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Jurassic and Lower Cretaceous radiolarian zonation in Japan and in the western Pacific 总被引：7，自引：0，他引：7
Abstract A radiolarian zonal scheme for the entire Jurassic and Lower Cretaceous using biostratigraphic data from both Japanese Island sections and the western Pacific seafloor is documented. The zonation is applicable to low and middle paleolatitude portions of the Paleo-Pacific ocean. Radiolarian bio-events such as the evolutionary first appearance biohorizon, first occurrence biohorizon, and last occurrence biohorizon were used to define zones. The 11 zones proposed are, in ascending order, Parahsuum simplum, Trillus elkhornensis, Laxtorum(?) jurassicum, Tricolocapsa plicarum, Tricolocapsa conexa, Stylocapsa(?) spiralis, Hsuum maxwelli, Pseudodictyomitra primitiva, Pseudodictyomitra carpatica, Cecrops sep-temporatus, and Acanthocircus carinatus zones. Preliminary age assignments for these zones are presented. 相似文献
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This Special Issue of Earth Surface Processes and Landforms develops from the ‘Geomorphology: a 2020 Vision’ Annual Conference of the British Society for Geomorphology, organised at the University of Birmingham, UK, in July 2007. Entitled ‘New Developments in Process Understanding and Modelling in Geomorphology’, the Issue comprises a vibrant selection of 10 ‘process’ papers from leading researchers in geomorphological processes who presented at Birmingham. It aims to provide a readily accessible source of new and emerging ideas in understanding different landform processes across a range of space and time scales, based on innovations in geomorphological modelling and monitoring. The last few years have seen significant and exciting changes in geomorphology, especially in conceptual developments, numerical simulations, monitoring methodologies, data‐acquisition strategies and dating techniques. The resultant empirical datasets, theory development and modelling results have generated substantial advances in the understanding of geomorphological processes, form‐process feedbacks, scale impacts, long‐term landform evolution, the effects of climate and environmental change, and human impacts and management strategies. The Special Issue attempts to address the following key challenges: (a) to build on our Conference theme ‘Geomorphology: a 2020 Vision’, by identifying fundamental areas where doors need to be opened, for example in theory development, conceptual understanding, model evaluation, integration of the chemistry, physics, biology and mathematics of geomorphological processes, experimental validation, data needs and monitoring requirements; (b) to look forward to the next decade and beyond, and critically examine some of the approaches we will need for the questions ahead; and (c) to stimulate new research in the geomorphological sciences by highlighting both research gaps and promising developments, including emerging process modelling approaches, monitoring technologies and robust datasets. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
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本文对中国石油、天然气资源作了重点的介绍.强调了这些资源对我国国民经济和国防建设的重要性.目前,我国油气资源短缺的现象日益严重.作者指明了在前第三纪海相残留盆地中勘探这些资源,会带来光明的前景. 相似文献
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