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1.
Changes in bed topography that build and maintain channel morphology are driven by the displacements of individual particles, either though their entrainment or deposition. However, the linkages between these topographic changes and individual grain displacements have not been comprehensively addressed, as many historical tracer studies have not included coincident topographic data. In this study, we compare the movements of bedload tracers to the differences in repeat topographic surveys across four gravel-bed river reaches. To do this, we apply a 1-D Bayesian survival process model to the starting and ending locations of tracers. This model estimates downstream trapping probabilities, which represent the likelihood that a given segment of channel will “trap” an entrained particle. We then adapt this model to estimate downstream trapping probabilities using digital elevation models of difference and compare the results. The estimates from the tracer and topographic trapping models showed general alignment, meaning that tracers were preferentially trapped in segments that experienced deposition along the channel. Thus, tracers in this study were able to identify downstream differences in bedload transport. The comparison also highlighted that tracer-estimated trapping probabilities were larger than topographically estimated ones. This supports previous observations that sediment travel distances estimated using tracers are shorter than those estimated using morphological methods. We find that the differences between these two estimates vary systematically across study environments. These variations are attributable to either study design (i.e., tracers being larger than the median size of the sediment that deforms the bed) or differences in compensating scour and fill. We explore potential causes for differences in compensating scour and fill, including hydrograph shape, sediment delivery regime, channel deformation style, and channel width, highlighting that morphodynamics needs to be considered in designing bedload tracer studies.  相似文献   

2.
This paper reports results from bedload transport investigations with active (radio) and passive (iron, magnetic) tracers in the Lainbach, a step-pool mountain river, in Bavaria, Southern Germany. The spatial distributions of the iron tracers after flood events can be best described by exponential or Gamma distributions. There is some indication of a tendency of size-selective transport of the iron tracers, but there is also a considerable amount of scatter in the correlations between weight (size) and travel length owing to the masking influence of other variables, such as the shape of the particles and different positions in the river bed. The experiments with artificial magnetic tracers showed that elongated pebbles (rods) had the longest mean transport distance, platy ones (discs) remained relatively close to the starting points. The particles from the pool showed the greatest transport lengths and a 100 per cent chance of being eroded. The Pebble Transmitter System (PETSY) consists of transmitters implanted into individual pebbles, a computerized receiver, a stationary antenna system with an antenna switchboard, and a data logging system. The particles do not move continuously but in a series of transport steps and non-movement intervals. A single value for a given size-class is not adequate to describe the critical conditions of entrainment under natural circumstances. A probability approach is much more suitable. The critical unit discharges (total discharge divided by active channel width) along the measuring reach are dependent on river bed morphology. In the steps bedload needs higher unit discharges to be entrained. Once entrained, the transport of bedload is stochastic in nature and the single particle transport is controlled by the step lengths and the duration of rest periods. The distributions of both parameters can be approximated by exponential functions. Applying the stochastic concept proposed by Einstein the mean values of the random variables [step length] and [duration of rest period] measured with the PETSY technique were used for the simulation of spatial distributions of bedload particles from point sources. More field and laboratory data are needed to include varying flow and roughness conditions with tracers representing different particle characteristics.  相似文献   

3.
In gravel‐bed rivers with well‐de?ned pool–bar morphology, the path length of transported bed particles must be, at least during ‘channel‐forming’ ?ows, equal to the length scale of the morphology. This is the basis for some methods for estimating bed material transport rates. However, previous data, especially from ?eld tests, are often strongly positively skewed with mean much shorter than the pool–bar spacing. One possible explanation is that positively skewed distributions occur only in channels lacking distinct pool–bar topography or only at lower discharges in pool–bar channels. A series of ?ume experiments using ?uorescent tracers was used to measure path length distributions in low‐sinuosity meandering channels to assess the relation with channel morphology and ?ow conditions. At channel‐forming ?ows, 55 to 75 per cent of the tracer grains were deposited on the ?rst point bar downstream of the point of tracer input, with 15 per cent passing beyond the ?rst bar. Path length distributions are symmetrical with mean equal to the pool–bar spacing and can be described with a Cauchy distribution. In some cases there was a secondary mode close to the point of tracer introduction; this bimodal distribution ?ts a combined gamma–Cauchy distribution. Only when discharge was reduced below the channel‐forming ?ow were frequency distributions unimodal and positively skewed with no relation to the pool–bar spacing. Thus, path length distributions become more symmetrical, and mean path length increases to coincide with pool–bar spacing, as ?ow approaches channel‐forming conditions. This is a substantial modi?cation of existing models of particle transfer in gravel‐bed rivers. Copyright © 2003 John Wiley & Sons, Ltd.  相似文献   

4.
This paper reports a radiofrequency identification (RFID) tracing experiment implemented in a high‐sediment‐load mountain stream typical of alpine gravel‐bed torrents. The study site is the Bouinenc Torrent, a tributary to the Bléone River in southeast France that drains a 38·9‐km² degraded catchment. In spring 2008, we deployed 451 tracers with b‐axis ranging from 23 to 520 mm. Tracers were seeded along eight cross‐sections located in the upstream part of the lowest 2·3 km of the stream. Three tracer inventories were implemented in July 2008, 2009 and 2010. Recovery rates calculated for mobile tracers declined from 78% in 2008 to 45% in 2009 and 25% in 2010. Observations of tracer displacement revealed very high sediment dispersion, with frontrunners having travelled more than 2 km only three months after their deployment. The declining recovery rate over time was interpreted as resulting from rapid dispersion rather than deep burial. We evaluated that 64% of the tracers deployed in the active channel were exported from the 2·3‐km study reach three years after the onset of the tracing experiment. Travel distances were characterized by right‐skewed and heavy‐tailed distributions, correctly fitted by a power‐law function. This supports the idea that in gravel‐bed rivers with abundant sediment supply relative to transport capacity, bedload transport can be viewed as a superdiffusive sediment dispersion process. It is also shown that tracers initially deployed in the low‐flow channel were characterized by a 15‐ to 30‐fold increase of mobility compared to tracers deployed in gravel bars. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

5.
Unsteady bedload transport was measured in two c. 5 m wide anabranches of a gravel‐bed braided stream draining the Haut Glacier d'Arolla, Switzerland, during the 1998 and 1999 melt seasons. Bedload was directly sampled using 152 mm square Helley–Smith type samplers deployed from a portable measuring bridge, and independent transport rate estimates for the coarser size fractions were obtained from the dispersion of magnetically tagged tracer pebbles. Bedload transport time series show pulsing behaviour under both marginal (1998) and partial (1999) transport regimes. There are generally weak correlations between transport rates and shear stresses determined from velocity data recorded at the measuring bridge. Characteristic parameters of the bedload grain‐size distributions (D50, D84) are weakly correlated with transport rates. Analysis of full bedload grain‐size distributions reveals greater structure, with a tendency for transport to become less size selective at higher transport rates. The bedload time series show autoregressive behaviour but are dif?cult to distinguish by this method. State–space plots, and associated measures of time‐series separation, reveal the structure of the time series more clearly. The measured pulses have distinctly different time‐series characteristics from those modelled using a one‐dimensional sediment routing model in which bed shear stress and grain size are varied randomly. These results suggest a mechanism of pulse generation based on irregular low‐amplitude bedforms, that may be generated in‐channel or may represent the advection of material supplied by bank erosion events. Copyright © 2003 John Wiley & Sons, Ltd.  相似文献   

6.
Sodium bromide and Rhodamine WT were used as conservative tracers to examine the hydrologic characteristics of seven tundra streams in Arctic Alaska, during the summers of 1994–1996. Continuous tracer additions were conducted in seven rivers ranging from 1st to 5th order with samples collected from instream, hyporheic, and parafluvial locations. Tracer data was used as input for a computer model to estimate hydrologic characteristics of each study reach. While solute concentrations during the tracer additions indicated that steady-state or “plateau” conditions had been reached, interstitial samples indicated that there were additional hyporheic and parafluvial zones that had not been fully labeled at the time of apparent steady state in the stream channel (plateau). Exchange between channel and hyporheic water was a function of location within a pool–riffle sequence, with rapid downwelling at the head of riffles and delayed upwelling in riffle tails. The extent of exchange between channel and hyporheic water was positively correlated with apparent streambed hydraulic conductivity. Tracer additions indicated interstitial velocities ranging from 0.030 to 0.075 cm s−1 and hydraulic conductivities from 2.4 to 12.2 cm s−1. Hyporheic and in-channel samples were collected for N, P, DO, and CO2 analyses in conjunction with conservative tracer additions in four of the stream reaches for which the interstitial velocities were also determined. Transformation rates based on these data indicated that there was rapid nitrification of mineralized organic N and production of ammonium, phosphate, and carbon dioxide in the interstitial zones of all four reaches. Dissolved oxygen did not appear to be limiting in the reaches studied. The hyporheic zone of all four reaches was a source of nitrate, carbon dioxide, and ammonium to the channel water based on the average concentration of upwelling waters. Increased contact time with hyporheic and parafluvial zones was related to decreased temperature and increased conductivity. Net nitrogen flux from the hyporheic zone was equivalent to 14–162% of benthic N uptake requirements for the Kuparuk River. These observations are important because we expected that the presence of continuous permafrost in this Arctic environment would limit the importance of hyporheic processes, either physically (i.e., through the presence of a restricting thaw bulb in the permafrost) or biogeochemically (i.e., through low temperatures). Instead, we found that biogeochemical processes in the hyporheic zone of these Arctic streams are at least as important as it is in similar temperate stream ecosystems.  相似文献   

7.
The use of isotopic tracers for sediment source apportionment is gaining interest with recent introduction of compound‐specific stable isotope tracers. The method relies on linear mixing of source isotopic tracers, and deconvolution of a sediment mixture initially quantifies the contribution of sources to the mixture's tracer signature. Therefore, a correction to obtain real sediment source proportions is subsequently required. As far as we are aware, all published studies to date have used total isotopic tracer content or a proxy (e.g., soil carbon content) for this post‐unmixing correction. However, as the relationship between the isotopic tracer mixture and the source mixture is different for each isotopic tracer, post‐unmixing corrections cannot be carried out with one single factor. This contribution presents an isotopic tracer model structure—the concentration‐dependent isotope mixing model (CD‐IMM)—to overcome this limitation. Herein, we aim to clarify why the “conventional” approach to converting isotopic tracer proportions to source proportions using a single factor is wrong. In an initial mathematical assessment, error incurred by not using CD‐IMM (NCD‐IMM) in unmixing two sources with two isotopic tracers showed a complex relation as a function of relative tracer contents. Next, three artificial mixtures with different proportions of three soil sources were prepared and deconvoluted using 13C of fatty acids using CD‐IMM and NCD‐IMM. Using NCD‐IMM affected both accuracy (mean average error increased up to a threefold compared with the CD‐IMM output) and precision (interquartile range was up to 2.5 times larger). Finally, as an illustrative example, the proportional source contribution reported in a published study was recalculated using CD‐IMM. This resulted in changes in estimated source proportions and associated uncertainties. Content of isotopic tracers is seldom reported in published work concerning use of isotopic tracers for sediment source partitioning. The magnitude of errors made by miscalculation in former studies is therefore difficult to assess. With this contribution, we hope the community will acknowledge the limitations of prior approaches and use a CD‐IMM in future studies.  相似文献   

8.
In a mountain environment, the transport of coarse material is a key factor for many fields such as geomorphology, ecology, hazard assessment, and reservoir management. Despite this, there have been only a few field investigations of bedload, in particular using multiple monitoring methods. In this sense, attention has frequently focused on the effects of “high magnitude/low frequency floods” rather than on “ordinary events”. This study aims to analyze the sediment dynamics triggered by three high-frequency floods (recurrence interval “RI” between 1.1 and 1.7 yr) that occurred in the Rio Cordon basin during 2014. The flood events were investigated in terms of both sediment mobility and bedload magnitude. The Rio Cordon is an Alpine basin located in northeastern Italy. The catchment has a surface area of 5 km2, ranging between 1763 and 2763 m above sea level. The Rio Cordon flows on an armored streambed layer, with a stable step-pool configuration and large boulders. Since 1986, the basin has been equipped with a permanent station to continuously monitor water discharge and sediment flux. To investigate sediment mobility, 250 PIT-tags were installed in the streambed in 2012. The 2014 floods showed a clear difference in terms of tracer displacement. The near-bankfull events showed equal mobility conditions, with mean travel distance one order of magnitude higher than the below-bankfull event. Furthermore, only the near-bankfull events transported coarse material to the monitoring station. Both events had a peak discharge up to 2.06 m3 s-1, but the bedload transport rates differed by more than one order of magnitude, proving that under the current supply-limited condition, the bedload appears more related to the sediment supply than to the magnitude of the hydrological features. In this sense, the results demonstrated that near-bankfull events can mobilize large amounts of material for long distances, and that floods of apparently similar magnitude may lead to different sediment dynamics, depending on the type and amount of sediment supply.  相似文献   

9.
The pipe microphone has been shown to be an effective means for monitoring bedload transport in mountain streams. It is commonly installed perpendicular to the flow direction on a stable river bed, such as that of a check dam. Acoustic pulses caused by bedload collisions with the pipe are detected by a microphone. However, bedload particles saltating over the pipe remain undetected. To overcome this disadvantage, we installed a horizontal as well as a vertical pipe microphone in the Ashi‐arai‐dani supercritical channel located in the Hodaka mountain range, Japan. The vertical pipe was installed on the wall of the channel and the horizontal pipe was installed on the channel bed. The acoustic response of the horizontal pipe is expected to be larger than that of the vertical pipe, because the bedload concentration decreases with increasing height above the bed. However, at high amplifications, the peak pulse value from the vertical pipe is higher than that from the horizontal pipe. We explain this observation as follows: under high bedload discharge conditions, the pulses of the horizontal pipe are saturated but those of the vertical pipe are not. We proposed a ratio (Rhv) between the pulses detected by these sensors, and applied this ratio for calibrating the contemporaneous pulses detected by a microphone located immediately upstream of a bedload slot sampler. Indeed the Rhv‐corrected pulses correlated well with the bedload discharge calculated from the sampler, supporting our explanation. We conclude that bedload monitoring using concomitant vertical and horizontal pipe microphones can be used to calibrate centrally located pipe microphones when the bedload concentration is approximately homogeneous laterally across the width of the channel cross‐section, and thereby represent bedload discharges more accurately than with only a single pipe microphone. Copyright © 2017 John Wiley & Sons, Ltd.  相似文献   

10.
A continuous record reveals that the incidence of bedload in a coarse-grained river channel changes from flood to flood. Long periods of inactivity encourage the channel bed to consolidate sufficiently so that bedload is largely confined to the recession limb of the next flood-wave. But when floods follow each other closely, the bed material is comparatively loose and offers less resistance to entrainment. In this case, substantial amounts of bedload are generated on the rising limb. This is confirmed by values of bed shear stress or stream power at the threshold of initial motion which can be up to five times the overall mean in the case of isolated floods or those which are the first of the season. This produces a complicated relationship between flow parameters and bedload and explains some of the difficulties in establishing bedload rating curves for coarse-grained channels. Besides this, the threshold of initial motion is shown to occur at levels of bed shear stress three times those at the thresholds of final motion. This adds further confusion to attempts at developing predictive bedload equations and clearly indicates at least one reason why equations currently in use are unsatisfactory. Bedload is shown to be characterized by a series of pulses with a mean periodicity of 1.7 hours. In the absence of migrating bedforms, it is speculated that this well-documented pattern reflects the passage of kinematic waves of particles in a slow-moving traction carpet. The general pattern of bedload, including pulsations, is shown to occur more or less synchronously at different points across the stream channel.  相似文献   

11.
《国际泥沙研究》2021,36(6):723-735
This numerical modeling study (i) assesses the influence of the sediment erosion process on the sediment dynamics and subsequent morphological changes of a mixed-sediment environment, the macrotidal Seine estuary, when non-cohesive particles are dominant within bed mixtures (non-cohesive regime), and (ii) investigates respective contributions of bedload and suspended load in these dynamics. A three dimensional (3D) process-based morphodynamic model was set up and run under realistic forcings (including tide, waves, wind, and river discharge) during a 1-year period. Applying erosion homogeneously to bed sediment in the non-cohesive regime, i.e., average erosion parameters in the erosion law (especially the erodibility parameter, E0), leads to higher resuspension of fine sediment due to the presence of coarser fractions within mixtures, compared to the case of an independent treatment of erosion for each sediment class. This results in more pronounced horizontal sediment flux (two-fold increase for sand, +30% for mud) and erosion/deposition patterns (up to a two-fold increase in erosion over shoals, generally associated with some coarsening of bed sediment). Compared to observed bathymetric changes, more relevant erosion/deposition patterns are derived from the model when independent resuspension fluxes are considered in the non-cohesive regime. These results suggest that this kind of approach may be more relevant when local grain-size distributions become heterogeneous and multimodal for non-cohesive particles. Bedload transport appears to be a non-dominant but significant contributor to the sediment dynamics of the Seine Estuary mouth. The residual bedload flux represents, on average, between 17 and 38% of the suspended sand flux, its contribution generally increasing when bed sediment becomes coarser (can become dominant at specific locations). The average orientation of residual fluxes and erosion/deposition patterns caused by bedload generally follow those resulting from suspended sediment dynamics. Sediment mass budgets cumulated over the simulated year reveal a relative contribution of bedload to total mass budgets around 25% over large erosion areas of shoals, which can even become higher in sedimentation zones. However, bedload-induced dynamics can locally differ from the dynamics related to suspended load, resulting in specific residual transport, erosion/deposition patterns, and changes in seabed nature.  相似文献   

12.
Measurements of annual travel distance (Lb) of bed load sediment at 16 locations in Alaska, the intermountain USA, west coast USA and Scotland are strongly correlated with bankfull channel width (r2 = 0·86, p < 0·001). Travel distance of particles is probably limited by trapping in bars, which have a longitudinal spacing proportional to channel width. Increased abundance of woody debris reduces bar spacing and may reduce Lb. Longer cumulative duration of bed load transporting flows in a year appears to increase Lb. Other predictors of annual travel distance such as stream power per unit length, drainage area and bankfull discharge were less well correlated with Lb (r2 ranging from 0·27 to 0·51). Stream power per unit bed area, basal shear stress and slope were not significantly related to Lb (r2 < 0·05). Most correlations were improved when regressions were limited to data from the west coast USA. Travel distance estimates can be used to help identify reaches that may take longer to recover from large, short‐term increases in sediment supply. Published in 2001 by John Wiley & Sons, Ltd.  相似文献   

13.
Sediment supply (Qs) is often overlooked in modelling studies of landscape evolution, despite sediment playing a key role in the physical processes that drive erosion and sedimentation in river channels. Here, we show the direct impact of the supply of coarse-grained, hard sediment on the geometry of bedrock channels from the Rangitikei River, New Zealand. Channels receiving a coarse bedload sediment supply are systematically (up to an order of magnitude) wider than channels with no bedload sediment input for a given discharge. We also present physical model experiments of a bedrock river channel with a fixed water discharge (1.5 l min−1) under different Qs (between 0 and 20 g l−1) that allow the quantification of the role of sediment in setting the width and slope of channels and the distribution of shear stress within channels. The addition of bedload sediment increases the width, slope and width-to-depth ratio of the channels, and increasing sediment loads promote emerging complexity in channel morphology and shear stress distributions. Channels with low Qs are characterized by simple in-channel morphologies with a uniform distribution of shear stress within the channel while channels with high Qs are characterized by dynamic channels with multiple active threads and a non-uniform distribution of shear stress. We compare bedrock channel geometries from the Rangitikei and the experiments to alluvial channels and demonstrate that the behaviour is similar, with a transition from single-thread and uniform channels to multiple threads occurring when bedload sediment is present. In the experimental bedrock channels, this threshold Qs is when the input sediment supply exceeds the transport capacity of the channel. Caution is required when using the channel geometry to reconstruct past environmental conditions or to invert for tectonic uplift rates, because multiple configurations of channel geometry can exist for a given discharge, solely due to input Qs. © 2020 The Authors. Earth Surface Processes and Landforms published by John Wiley & Sons Ltd  相似文献   

14.
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15.
Analysis of a vertical dipole tracer test in highly fractured rock   总被引：1，自引：0，他引：1  
The results of a vertical dipole tracer experiment performed in highly fractured rocks of the Clare Valley, South Australia, are presented. The injection and withdrawal piezometers were both screened over 3 m and were separated by 6 m (midpoint to midpoint). Due to the long screen length, several fracture sets were intersected, some of which do not connect the two piezometers. Dissolved helium and bromide were injected into the dipole flow field for 75 minutes, followed by an additional 510 minutes of flushing. The breakthrough of helium was retarded relative to bromide, as was expected due to the greater aqueous diffusion coefficient of helium. Also, only -25% of the total mass injected of both tracers was recovered. Modeling of the tracer transport was accomplished using an analytical one-dimensional flow and transport model for flow through a fracture with diffusion into the matrix. The assumptions made include: streamlines connecting the injection and withdrawal point can be modeled as a dipole of equal strength, flow along each streamline is one dimensional, and there is a constant Peclet number for each streamline. In contrast to many other field tracer studies performed in fractured rock, the actual travel length between piezometers was not known. Modeling was accomplished by fitting the characteristics of the tracer breakthrough curves (BTCs), such as arrival times of the peak concentration and the center of mass. The important steps were to determine the fracture aperture (240 microm) based on the parameters that influence the rate of matrix diffusion (this controls the arrival time of the peak concentration); estimating the travel distance (11 m) by fitting the time of arrival of the centers of mass of the tracers; and estimating fracture dispersivity (0.5 m) by fitting the times that the inflection points occurred on the front and back limbs of the BTCs. This method works even though there was dilution in the withdrawal well, the amount of which can be estimated by determining the value that the modeled concentrations need to be reduced to fit the data (approximately 50%). The use of two tracers with different diffusion coefficients was not necessary, but it provides important checks in the modeling process because the apparent retardation between the two tracers is evidence of matrix diffusion and the BTCs of both tracers need to be accurately modeled by the best fit parameters.  相似文献   

16.
Few studies have investigated large reaches of rivers in which multiple sources of groundwater are responsible for maintaining baseflow. This paper builds upon previous work undertaken along the Fitzroy River, one of the largest perennial river systems in north‐western Australia. Synoptic regional‐scale sampling of both river water and groundwater for a suite of environmental tracers (4He, 87Sr/86Sr, 222Rn and major ions), and subsequent modeling of tracer behavior in the river, has enabled definition and quantification of groundwater input from at least three different sources. We show unambiguous evidence of both shallow “local” groundwater, possibly recharged to alluvial aquifers beneath the adjacent floodplain during recent high‐flow events, and old “regional” groundwater introduced via artesian flow from deep confined aquifers. We also invoke hyporheic exchange and either bank return flow or parafluvial flow to account for background 222Rn activities and anomalous chloride trends along river reaches where there is no evidence of the local or regional groundwater inputs. Vertical conductivity sections acquired through an airborne electromagnetic (AEM) survey provide insights to the architecture of the aquifers associated with these sources and general groundwater quality characteristics. These data indicate fresh groundwater from about 300 m below ground preferentially discharging to the river, at locations consistent with those inferred from tracer data. The results demonstrate how sampling rivers for multiple environmental tracers of different types—including stable and radioactive isotopes, dissolved gases and major ions—can significantly improve conceptualization of groundwater—surface water interaction processes, particularly when coupled with geophysical techniques in complex hydrogeological settings.  相似文献   

17.
Using previous results on extended Petri Nets (EPN), we present the relations between various hydrological dynamical systems (HDSys) derived from the water budget. Once the water budget has been implemented, there is a consistent way of getting the equations for backward travel time distributions, for forward response time distributions and for the concentration of a solute or tracer. We show that the water budget has a correspondence of one to many with the backward travel time distributions. In fact, to any one of the water budget equations there correspond as many equations as there are input precipitation events. The backward travel time distributions are related to the response time distributions by Niemi's relationship and, if there are n outputs, by the definition of n − 1 partition functions. These determine what fraction of the water volume injected into the control volume at a specific time tin goes asymptotically to a specific output. Given the backward travel time distributions, the output concentration of a solute or tracer also depends on the input concentration. The paper clarifies the complicated relations described above by taking [Hydrology and Earth System Sciences, 20, 299–328] as an example from literature. Once the appropriate information is presented, it is shown how these HDSys can be solved simultaneously without duplicating calculations. Then, it is also shown that, under the hypothesis of uniform mixing of water ages within each reservoir, these systems can be solved exactly.  相似文献   

18.
Experiments using radioactive tracers in microcosms of 150 l and 13 m3 volumes, which are designed to mimic Narragansett Bay, indicate that Th isotopes are good analogues for studying the removal behavior of “particle-reactive” pollutants such as Am, Pb, Po, Hg and Cr(III) in coastal environments. The removal of Th isotopes and Fe has been found to be closely linked in microcosms and Narragansett Bay. In addition, the settling velocities of tracer microspheres in the experimental tanks were found to be faster in spring and summer than expected from Stokes' law and similar to those of234Th-containing particles in Narragansett Bay [5]. It is concluded that aggregation of particles is important in accelerating the removal of surface-reactive elements during the warm season.  相似文献   

19.
The acidic discharge from Cement Creek, containing elevated concentrations of dissolved metals and sulphate, mixed with the circumneutral‐pH Animas River over a several hundred metre reach (mixing zone) near Silverton, CO, during this study. Differences in concentrations of Ca, Mg, Si, Sr, and SO42? between the creek and the river were sufficiently large for these analytes to be used as natural tracers in the mixing zone. In addition, a sodium chloride (NaCl) tracer was injected into Cement Creek, which provided a Cl? ‘reference’ tracer in the mixing zone. Conservative transport of the dissolved metals and sulphate through the mixing zone was verified by mass balances and by linear mixing plots relative to the injected reference tracer. At each of seven sites in the mixing zone, five samples were collected at evenly spaced increments of the observed across‐channel gradients, as determined by specific conductance. This created sets of samples that adequately covered the ranges of mixtures (mixing ratios, in terms of the fraction of Animas River water, %AR). Concentratis measured in each mixing zone sample and in the upstream Animas River and Cement Creek were used to compute %AR for the reference and natural tracers. Values of %AR from natural tracers generally showed good agreement with values from the reference tracer, but variability in discharge and end‐member concentrations and analytical errors contributed to unexpected outlier values for both injected and natural tracers. The median value (MV) %AR (calculated from all of the tracers) reduced scatter in the mixing plots for the dissolved metals, indicating that the MV estimate reduced the effects of various potential errors that could affect any tracer. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

20.
An important quantity in groundwater protection is the residence time of water in an aquifer. It relates to both the travel time of a pollutant to arrive at a well and the time span required for self-purification of a polluted aquifer after removal of pollutant inputs. Time scales for aquifers can be gained from artificial tracer experiments or from environmental tracer data, the latter offering the only realistic alternative if time scales of years or decades have to be taken into account.

Different tracers show different time scales due to their different transport mechanisms especially in the unsaturated zone. While solute tracers are moved advectively with the seepage water, gas tracers pass the unsaturated zone diffusively through the air phase. Depending on the properties of the unsaturated zone (hydraulic properties, thickness) this difference in behavior can be used to separate the subsurface transport process into the unsaturated and the saturated parts.

In a field study in Germany, SF6 and 3H were used as environmental tracers. Both have a relatively well-known input function. Interpretation of data from observation wells by a box model approach led to spatially and temporally varying residence times. This was an indication that the influence of the unsaturated zone could not be neglected. While the gas tracer SF6 shows only residence times in the saturated zone, the tracer 3H reflects the whole travel time of water including both the unsaturated and saturated zones. Using a one-dimensional plug-flow model for the unsaturated zone combined with a detailed two-dimensional flow and transport model for the saturated zone leads to a holistic and consistent interpretation of the measured tracer concentrations. The observed pattern of old water under thick loess cover and younger water under areas where the fractured basalt aquifer crops out is reproduced after adjusting only two parameters: the effective porosity of the saturated aquifer and the product of field capacity and thickness of the unsaturated zone. While the effective porosity of the saturated zone is adjusted by means of the SF6 data, the field capacity of the loess layer is adjusted by means of the 3H observations. The thickness of the unsaturated zone is deduced from geological and pedological maps. All flow data are obtained from a calibrated flow model, which is based on geological data, observed heads and pumping tests only.

The transport model for the saturated zone was calibrated by fitting the porosity by means of gaseous tracer concentrations (SF6). The combined saturated–unsaturated zone model was then calibrated by fitting the field capacity of the unsaturated zone by means of 3H concentrations. With this model it was possible to verify the observed NO3 concentrations at the drinking water wells and to develop predictions for their future development under various scenarios of fertilizer input reduction in specific areas.  相似文献   


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