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1.
Radionuclides are used as tracers of sediments in areas where no plot data or field monitoring data are not available. Caesium-137 can provide important information on both soil loss rates and sediment sources. The 137Cs technique is employed to assess soil erosion rates in forest and grass lands in the Upper Yangtze River Basin, China. The study area includes 6 forestlands and 4 grasslands in 8 counties and cities over the eastern part of the basin. The ^137Cs reference inventories ranged from 620.9 Bq m-2 to 2560.3 Bq m^-2. For the 6 forestlands, the average 137Cs inventory over a field ranges from 960.8 Bq m^-2 to 2560.3 Bq m^-2. The average erosion rate is estimated from the ^137Cs measurements between 0 to 588 t km^-2yr^-1. For the 4 grasslands, the average ^137Cs inventory ranges from 119.0 Bq m2 to 869.7 Bq m^-2. The average rate of erosion from grassland varies from 0 to 4435 t km^-2 yrl. Where the erosion was more severe, the ^137Cs inventory was lower. The results showed that there is no clear relationship between ^137Cs inventory, slope length and slope gradient on uncultivated land. The erosion rates for uncultivated land and cultivated land is compared. The result indicates that the erosion rates on uncultivated land is much lower than those on cultivated slopes and the severity of the soil erosion is closely related to vegetation cover.  相似文献   

2.
A reconnaissance study has been made of the distribution of 238U, 232Th, 40K and 137Cs and geochemical features in soils and sediments samples at various locations in the northwestern coast of Persian Gulf. Activity concentration levels due to radionuclides were measured in 30 soil and sediment samples collected from this region. From the measured spectra, activity concentrations were determined for 40K (range from 146 to 500 Bq kg(-1)), 137Cs (from 5 to 20 Bq kg(-1)), 238U (from 21 to 65 Bq kg(-1)) and 232Th (from 15 to 45 Bq kg(-1)) with lowest limit detection (LLD) of 68, 3.2, 4.3 and 4.3 Bq kg(-1), respectively. The dose rate from ambient air at the soil ranges was between 19 and 58 nGy h(-1) with an average of 37.41+/-9.66 nGy h(-1).  相似文献   

3.
The purpose of this study is to quantify some of the parameters needed to perform near-field modelling of sites in the Kara Sea that were impacted by the disposal of radioactive waste. The parameters of interest are: the distribution coefficients (Kd) for several important radionuclides, the mineralogy of the sediment, and the relationship of Kd to liquid-to-solid ratio. Sediment from the Kara Sea (location: 73 degrees 00'N, 58 degrees 00'E) was sampled from a depth of 287 m on August 23/24, 1992. Analysis of the material included mineralogy, grain size and total organic carbon (TOC). Uptake kinetics were determined for 85Sr, 137Cs, 241Am, 99Tc, 1251, 232U and 210Pb and distribution coefficients (Kd) were determined for these radionuclides using batch type experiments. Sorption isotherms, developed for 137Cs, 85Sr and 99Tc, were linear in each case. Increasing the liquid-to-solid ratio strongly increased uptake of 137Cs and moderately increased uptake of 99Tc. Analysis for anthropogenic radionuclides indicated the presence only of 239/240Pu in the sediment with the highest activity (at the top section of the core) being 0.420 Bq kg(-1). Other anthropogenic radionuclides were below detection limits.  相似文献   

4.
Floodplains comprise geomorphologically important sources and sinks for sediments and associated pollutants, yet the sedimentology of large dryland floodplains is not well understood. Processes occurring on such floodplains are often difficult to observe, and techniques used to investigate smaller perennial floodplains are often not practical in these environments. This study assesses the utility of 137Cs inventory and depth‐profile techniques for determining relative amounts of floodplain sedimentation in the Fitzroy River, northeastern Australia; a 143 000 km2 semi‐arid river system. Caesium‐137 inventories were calculated for floodplain and reference location bulk soil cores collected from four sites. Depth profiles of 137Cs concentration from each floodplain site and a reference location were recorded. The areal density of 137Cs at reference locations ranged from 13 to 978 Bq m–2 (0–1367 Bq m–2 at the 95% confidence interval), and the mean value ± 2 (standard error of the mean) was 436 ± 264 Bq m–2, similar to published data from other Southern Hemisphere locations. Floodplain inventories ranged from 68 to 1142 Bq m–2 (0–1692 Bq m–2 at the 95% confidence interval), essentially falling within the range of reference inventory values, thus preventing calculation of erosion or deposition. Depth‐profiles of 137Cs concentration indicate erosion at one site and over 66 cm of deposition at another since 1954. Analysis of 239+240Pu concentrations in a depositional core substantiated the interpretation made from 137Cs data, and depict a more tightly constrained peak in concentration. Average annual deposition rates range from 0 to 15 mm. The similarity between floodplain and reference bulk inventories does not necessarily indicate a lack of erosion or deposition, due to low 137Cs fallout in the region and associated high measurement uncertainties, and a likely influence of gully and bank eroded sediments with no or limited adsorbed 137Cs. In this low‐fallout environment, detailed depth‐profile data are necessary for investigating sedimentation using 137Cs. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

5.
According to variations of 137Cs and clay contents, 44 flood couplets were identified in a profile of res- ervoir deposit with a vertical length of 28.12 m in the Yuntaishan Gully. Couplet 27 at the middle of the profile had the highest average 137Cs content of 12.65 Bq·kg?1, which indicated the 1963s' deposits, then 137Cs content decreased both downward and upward in the profile. The second top and bottom couplets had average 137Cs contents of 2.15 Bq·kg?1 and 0.92 Bq·kg?1, respectively. By integrated analysis of reservoir construction and management history, variations of 137Cs contents over the profile, sediment yields of flood couplets and rainfall data during the period of 1958-1970, individual storms related to the flood couplets were identified. 44 floods with a total sediment yield of 2.36×104 m3 occurred and flood events in a year varied between 1 and 10 times during the period of 1960-1970. 7-10 flood events occurred during the wet period of 1961-1964 with very wet autumn, while only 1-2 events during the dry period of 1965-1969. Average annual specific sediment yield was 1.29×104 t·km?2·a?1 for the Yuntaishan Gully during the period of 1960-1970, which was slightly higher than 1.11 ×104 t·km?2·a?1 for the Upper Yanhe River Basin above the Ganguyi Hydrological Station and slightly lower than 1.40 ×104 t·km?2·a?1 for the nearby Zhifang Gully during the same period. Annual specific sediment yields for the Yuntaishan Gully were correlated to the wet season's rainfalls well.  相似文献   

6.
The anthropogenic radionuclide 137Cs has been extensively utilized as a tracer of geomorphic processes in the northern hemisphere since its deposition during atmospheric testing of nuclear devices in the 1950s and 1960s. The distribution of bomb‐fallout 137Cs was measured on a sequence of coastal dune sands and soils at Pinery Provincial Park, on the coast of Lake Huron in southern Ontario, Canada. The depth distribution within the stabilized, developed soils inland reflected the relationship between clay content and the adsorption and immobilization of the radionuclide. However, the influence of soil organic matter, silt‐sized particles and vegetation cycling on the profile distribution could not be discounted. Within the geomorphically dynamic dune sands near the coast, there was a significant activity of 137Cs even though the sands were lacking in clay‐sized particles. Within a buried soil on the inland side of a large active dune blowout, the distribution of 137Cs with depth was useful as a stratigraphic marker of the rates of accumulation of sands at that position. Therefore 137Cs may be a useful alternative to erosion pins, sequential air photos and sediment traps in the monitoring of dune destabilization in coastal environments. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献   

7.
Vertical profiles of the activities of 137Cs and 210Pb were measured on floodplain sediment cores and upland soil cores along the Soda Butte Creek and the Yellowstone River to determine floodplain sedimentation rates. The position of mine tailings from a 1950 impoundment failure was used as a stratigraphic marker to estimate the sedimentation rates and to make comparisons with rates provided by radionuclide‐based methods. Mass accumulation (sedimentation) rates calculated from the position of the mine tailings ranged from 0·00 to 0·17 g cm?2 yr?1 and were in good agreement with sedimentation rates calculated from the inventories of 137Cs and 210Pb. Sedimentation rates calculated from the position of the 137Cs peak generally overestimated the sedimentation rates, probably because of increased downward migration of 137Cs caused by the low pH of water moving through the mine tailings or the high permeability of floodplain sediments relative to upland reference soils. This study demonstrates that the 137Cs and 210Pb inventory methods for determining sedimentation rates can be applied to an alpine floodplain where sedimentation events are episodic and where orographic effects on precipitation generate strong downstream gradients in the delivery of atmospheric radionuclides. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

8.
Surface sediment samples in the Laptev Sea have average 137Cs content of 7.1 Bq kg(-1), a value intermediate between that of the western Kara Sea (23 Bq kg(-1) and the East Siberian Sea (4.2 Bq kg-'). Both surface sediment content and sediment inventory of 137Cs in the Laptev Sea sediments show significant variability, and the influence of a variety of environmental factors.137Cs concentrations in the Laptev Sea surface sediments range from 0.8 to 16 Bq kg(-1). There is a marked increase in 137Cs content of surface sediment samples collected near the Lena River delta, and a local enrichment in the 137Cs inventories at these sites is also evident. Fine-grained mixed-layer illite/ smectite rich sediments in the estuary provide effective adsorption sites to fix 137Cs, in spite of desorption processes associated with low salinities in estuarine mixing. The Lena River-Laptev Sea mixing zone is a major site of sea-ice production. River and shelf sediments are incorporated into sea-ice formed in this region (Holmes and Creager, 1974). The irregular 137Cs activity profiles of the Lena River estuary cores indicate disturbance or removal of 137Cs-laden sediments via sea-ice related processes. Lena River and Estuary sediments may have served as a secondary source (i.e. other than direct fallout) of 137Cs in sea-ice. North-east of the Lena River estuary, sediment contains a thin layer of 137Cs-bearing material over an erosion surface. The 137Cs-laden surface layer may be the result of transient deposition of estuarine sediments being delivered by sea-ice or spring floods.  相似文献   

9.
238Pu,239Pu and137Cs in rain and dry fallout and90Sr in rain samples were measured at Woods Hole, Massachusetts, from June 1976 through December 1977. The dry fallout was estimated to be about 7.8% of the total deposition of239Pu and137Cs.239Pu/137Cs ratios, almost constant at about 0.011 in rain or dry fallout, February through December 1977, suggested that fractionation between the refractory and volatile radionuclides is insignificant in stratospheric fallout. This supports the idea of regional homogeneity of radionuclide ratios in fallout.  相似文献   

10.
The radionuclides137Cs,210Pb and7Be have been examined in the alpine Rhoˆne watershed (Switzerland) during a period of two years in order to evaluate their usefulness as tracers of the removal and transport rate of top-soil particles and particle-reactive contaminants of atmospheric origin. The specific activities of the radionuclides in fluvial suspension show a distinct seasonal pattern which depends on the hydrologic regime of the stream and the sources of the suspended matter. Input-output budgets based on the atmospheric deposition and fluvial removal of three radionuclides in the alpine Rhoˆne watershed are used to estimate their erosional residence times. The simplest one box model yields mean residence times of about 800 and 1400 years for137Cs and210Pb, respectively. The removal rate of short-lived7Be suggests that a part of the watershed (0.6–2.3% of the total surface) is exposed to a rapid erosion, in which the mean residence time of the radionuclides is in the range of 1–220 days. This has little influence on the calculated residence time of137Cs but increases the estimated residence time of210Pb in soil to over 1800 years. The use of210Pb-7Be pair in fluvial output may be very helpful in the assessment of the impact of atmospheric pollutants on the water quality in rivers and lakes.  相似文献   

11.
The 137Cs radioactivity of soils was used as a tracer of soil erosion in a catchment in the Netherlands: 143 samples were analysed to map the 137Cs redistribution using geostatistical interpolation methods. Caesium-137 activities on grassland are significantly higher than on arable land. Also, 137Cs activities on waning slopes are higher and activities on steep slopes are lower. The soil erosion estimates, derived from the 137Cs data, are used to validate the USLE erosion model. The recent Chernobyl nuclear accident also contributed to the 137Cs activity. However, the Chernobyl input of 137Cs, with a constant ratio of 1.765:1 to 134Cs, cannot be used as a tracer of soil erosion. Because of the rapid decay of 134Cs, we will not be possible to separate the sources of 137Cs in the near future in areas significantly influenced by Chernobyl fallout and in these areas 137Cs can no longer be used as a soil erosion tracer.  相似文献   

12.
Radon can be used as a naturally occurring tracer for environmental processes. By means of grab-sampling or continuous monitoring of radon concentration, it is possible to assess several types of dynamic phenomena in air and water. We present a review of the use of radon and its progeny at the University of Cantabria. Radon can be an atmospheric dynamics indicator related with air mass interchange near land-sea discontinuities as well as for the study of vertical variations of air parameters (average values of different types of stability: 131–580 Bq m?3). Concerning indoor gas, we present some results obtained at Altamira Cave (Spain): from 222 to 6549 Bq m?3 (Hall) and from 999 to 6697 Bq m?3 (Paintings Room). Finally, variations of radon concentration in soil (0.3 to 9.1 kBq m?3) and underground water (values up to 500 Bq l?1) provide relevant information about different geophysical phenomena.  相似文献   

13.
An estimated 3.5 ± 0.7 × 1015 Bq of 137Cs is thought to have been discharged into the ocean following the melt down at Fukushima Dai-ichi Nuclear Power Plant (F1NPP). While efforts have been made to monitor seafloor radiation levels, the sampling techniques used cannot capture the continuous distribution of radionuclides. In this work, we apply in situ measurement techniques using a towed gamma ray spectrometer to map the continuous distribution of 137Cs on the seafloor within 20 km of the F1NPP. The results reveal the existence of local 137Cs anomalies, with levels of 137Cs an order of magnitude higher than the surrounding seafloors. The sizes of the anomalies mapped in this work range from a few meters to a few hundreds of meters in length, and it is demonstrated that the distribution of these anomalies is strongly influenced by meter scale features of the terrain.  相似文献   

14.
The Cesium-137 technique was used to estimate soil erosion in the Xihanshui River Basin.More than 100 samples were taken from 10 sites and 20 hillslopes with a 10cm diameter hand-operated core driller.Each sample was 60 cm long.The 137Cs activity was analyzed by gamma spectrometry.The simplified mass balance model and the profile distribution model were used to calculate soil erosion and deposition rate.The local 137Cs reference ranged from 1,600 to 2,402 Bq m-2.The data shows an exponential decrease of mass concentration and amount with depth in an undisturbed soil profile.Soil erosion in the river basin is moderate or severe on cultivated land with annual erosion rates of 2,000-6,000 t km-2yr-1.In general,very severe or severe soil erosion occurred at the upper slope sections,moderate or severe soil erosion at the middle section,and moderate or slight soil erosion at the lower slope sections.On the slopes with natural vegetation,consisting of herbaceous and wood species,the erosion rate is much lower or not detectable.On the lower section of slopes with well-developed vegetation however,there was no soil loss,instead deposition occurred at a rate of more than 300 t km-2 yr-1.The slope gradient and vegetation cover affected soil erosion and deposition rates.In general,the rate of soil erosion was proportional to the slope gradient and inversely proportional to the degree of vegetative cover.  相似文献   

15.
The spatial distribution of 137Cs across the landscape and the processes controlling its redistribution are of interest because (i) 137Cs has been widely used to quantify the movement of soil and sediments and (ii) substantial fallout of 137Cs after the Chernobyl accident has led to contamination of foodstuffs in some places. A high‐resolution airborne geophysical radiometric survey of Northern Ireland has provided an opportunity to study the distribution and possible redistribution of 137Cs. The 137Cs activity (recorded at 1·2 million points) is distributed in a series of bands oriented approximately 160° and 115° clockwise from north. Geostatistical analysis of the data shows a strong, short‐range structure (correlation ranges between 0·6 and 8 km) in 137Cs activity across the vast majority of the region; the spatial distribution shows association with a published, coarse‐scale depositional pattern of 137Cs from Chernobyl. Two indices of land form derived from a digital elevation model, namely compound topographic index and the length–slope factor of the Revised Universal Soil Loss Equation, account for only 3% of the variance in 137Cs activity. In contrast, soil type and land cover in combination (including their interaction) account for 20% of the variance. In areas that received moderate fallout from Chernobyl, soil type alone accounts for a substantial proportion of the spatially correlated 137Cs activity. We attribute this to each soil type having a fairly uniform radiocaesium interception potential that differs from those of other soil types and that this potential controls the vertical migration of 137Cs. Over the granitic Mourne Mountains there is a strong spatial cross‐correlation between 137Cs activity and airborne estimates of soil potassium, suggesting that the latter provides a measure of the soil's radiocaesium interception potential; this is probably dominated by the quantity of the mineral illite. Copyright © 2010 John Wiley & Sons, Ltd. and British Geological Survey  相似文献   

16.
The activity concentration of Cesium-137 ((137)Cs) and naturally-occurring Polonium-210 ((210)Po) were measured in the muscle tissue, kidney and liver of Pacific walrus (Odobenus rosmarus divergens) and bearded seal (Erignathus barbatus) collected by native hunters from the Bering Sea during May 1996. The mean (137)Cs concentrations in muscle, liver and kidney of Pacific walrus were 0.07, 0.09 and 0.07 Bq kg(-1) (n=5, wet weight), respectively, and 0.17, 0.10, and 0.17 Bq kg(-1) (n=2, wet weight), respectively, in bearded seal. In general, (137)Cs tissue concentrations are significantly lower than those previously reported for mammals from other regions. By comparison, (210)Po activity concentrations are more variable and appear to be higher level compared with mammal data from other regions. The mean (210)Po concentration in the muscle tissue, liver and kidney of Pacific walrus (n=5, wet weight) were 28.7, 189, and 174 Bq kg(-1), respectively. This compares with (210)Po concentration values (n=2, wet weight) of 27, 207 and 68 Bq kg(-1) measured in the muscle tissue, liver and kidney, of bearded seal, respectively. Estimated concentration factors--as defined by the radionuclide concentration ratio between the target tissue to that in sea water--were two to three orders of magnitude higher for (210)Po that those of (137)Cs. We conclude from radiological dose estimates that ingestion of (137)Cs in foods derived from walrus and seal will pose no threat to human health. This work has important implications for assessment of risks of Alaskan coastal communities concerned about the dumping of nuclear waste in the Russia Arctic.  相似文献   

17.
In recent years, there has been increasing interest in the significance of natural radionuclides, particularly (210)Po, in the marine environment. (210)Po, a naturally occurring alpha emitter, accumulates in marine organisms and reflects differences in their diets. In the literature, there is no data for (210)Po and (210)Pb activity concentrations for fish species on the Turkish coast of Aegean Sea. Therefore, in this study, multiple fish species were collected from six stations seasonally on the Turkish coast of Aegean Sea and were analyzed for their (210)Po and (210)Pb content. The (210)Po and (210)Pb concentrations in the fish samples were found to vary from undetectable levels to 499 ± 44 Bq kg(-1) dry weight (dw) and from 1.0 ± 0.3 Bq kg(-1) to 35 ± 4.0 Bq kg(-1) (dw), respectively. There were no significant differences in the activity concentrations of (210)Po and (210)Pb in fish samples between seasons (ANOVA, P>0.05). The highest dose contribution of (210)Po to humans was calculated to be 10,530 μSv year(-1).  相似文献   

18.
Sedimentation from soil erosion is a critical reservoir watershed management issue. Due to the difficulty of field investigations, empirical formulas are commonly used to estimate the soil erosion rate. However, these estimations are often far from accurate. An effective alternative to estimating soil erosion is to analyze the spatial variation of 137Cs inventory in the soil. 137Cs can be adsorbed by the soil and is widely assumed to change its distribution only when disturbed by rainfall and human activities. Thus, 137Cs distributed in soils can be a useful environmental tracer to estimate soil erosion. In this study, the net soil loss estimate is 108,346 t/yr and the gross erosion and net erosion rates are 10.1 and 9 t/ha yr respectively. The sediment delivery ratio is therefore estimated to be 0.9 based on the two erosion rates. Because of the steep hillsides in the watershed, only 10% of the sediment yield stayed in the deposition sites and 90% was transported to the river as the sediment output. Soil erosion estimates from spatial variations of the 137Cs activity in the Baishi river watershed showed satisfactory accuracy when compared to sediment yield data. Using soil 137Cs concentrations is therefore a feasible method for estimating soil loss or deposition in Taiwan. Data sampling, analysis and result of this approach are given in this paper.  相似文献   

19.
137Cs和241Am在滇池、剑湖沉积孔柱中的蓄积分布及时标意义   总被引：16，自引：2，他引：14  
项亮  吴瑞金  吉磊 《湖泊科学》1996,8(1):27-34
自70年代以来,对湖泊沉积物中核试验散落核素的研究已成为研究现代湖泊沉积过程和沉积年代及沉积速率的一个重要方面,本文通过对分别采自云南省滇池、剑湖的两个沉积孔柱中~(137)Cs和~(241)Am蓄积分布的研究,测定了它们60、70年代以来的沉积速率分别是42.1和28.7mg/(cm~2·a)。研究发现,虽然~(241)Am的含量远低于~(137)Cs,但~(241)Am具有沉积后迁移能力较小,半衰期长等特点,因而随着时间的推移,在未来湖泊现代沉积作用的研究中将会显示出越来越重要的作用。  相似文献   

20.
The state of radioactive pollution of Lake Ladoga has been studied. The purification half-life of lake water from 90Sr was found to be 21.7 year. The ratio of 90Sr storage in lake water volume to its storage in silts (0?C10 cm layer) was 2: 1. Lake water purification from global 137Cs was slower than that from 137Cs originating from Chernobyl emergency emission because of the chronic supplement of global 137Cs reserve by atmospheric fallouts. The behavior of 90Sr, 137Cs, and 239,240Pu in bed soils was in agreement with the geochemical nature of the elements. By the distribution of 239, 240Pu in bed soils, the sedimentation of substances of non-radiation nature was estimated at 0.3 and 0.5 mm/year at denting and flat relief, respectively.  相似文献   

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