首页 | 本学科首页   官方微博 | 高级检索  
相似文献
 共查询到20条相似文献,搜索用时 62 毫秒
1.
白洋淀沉积物氮磷赋存特征及其内源负荷   总被引:11,自引:2,他引:9  
杜奕衡  刘成  陈开宁  古小治  黄蔚  韦众 《湖泊科学》2018,30(6):1537-1551
白洋淀环境整治对区域生态文明建设具有重要意义,然而,目前对加剧白洋淀富营养化的内源氮、磷污染负荷依然缺乏系统的研究.本研究以野外调研和室内培养实验相结合形式,在白洋淀主要水域内采集原位柱状沉积物样品,详细地研究了白洋淀沉积物中氮、磷赋存形态、间隙水中氮、磷剖面特征以及沉积物-水界面氮、磷交换特征.结果表明,白洋淀沉积物总氮、总磷含量分别为1230.8~9559.0 mg/kg(均值2379.5 mg/kg)和344.4~915.4 mg/kg(均值608.4 mg/kg),氮、磷累积污染量大.沉积物中铵态氮赋存量大(3.2~175.8 mg/kg),由此导致间隙水中铵态氮浓度较高,最高达到28.8 mg/L.沉积物磷形态以Ca-P和Fe-P为主,分别占总量的38.3%~76.1%和3.98%~18.0%,间隙水中磷酸盐浓度已接近甚至高于国内外典型富营养湖区.间隙水中高浓度的铵态氮和磷酸盐导致沉积物-水界面氮、磷交换通量较高,铵态氮平均释放和扩散通量分别为106.37和12.42 mg/(m2·d);磷酸盐平均释放和扩散通量分别为15.06和2.33 mg/(m2·d),沉积物内源氮、磷污染负荷较高,已严重威胁到白洋淀水环境质量,迫切需要整治.其中,北部河口区域以及中部府河入湖区和人口密集活动区沉积物氮、磷内源负荷尤为突出,应成为白洋淀沉积物内源污染整治的关键区域.  相似文献   

2.
东巢湖沉积物水界面氮、磷、氧迁移特征及意义   总被引:2,自引:0,他引:2  
以东巢湖近城市湖湾沉积物为研究对象,在沉积物氮、磷营养盐分析的基础上,采用沉积物柱状芯样静态释放模拟法定量评估研究区域沉积物—水界面氨氮、溶解性活性磷酸盐营养盐释放潜力,利用微电极非损伤测定技术获得沉积物—水微界面溶解氧(DO)剖面分布及微界面DO消耗和扩散特征.结果表明:东巢湖近城市湖湾沉积物氮、磷污染物蓄积量较高,受TN、TP污染程度较重.沉积物内源氨氮、磷酸盐释放明显,平均释放速率分别达到32.44 mg/(m~2·d)和1.25mg/(m~2·d),区域内沉积物已成为水柱中氮、磷营养盐的污染源.研究区域上覆水体处于好氧状态,沉积物—水微界面平均DO穿透深度(OPD)达到5.3 mm,平均DO扩散通量为4.56 mmol/(m~2·d),表现出良好的DO扩散能力.沉积物内源氨氮和磷酸盐释放能力与表层沉积物TN/TP物质含量及沉积物—水微界面DO穿透深度有关,在沉积物氮、磷污染较重的情况下,DO穿透深度越低越有利于氮、磷污染物从沉积物向上覆水体释放.  相似文献   

3.
采集柱状芯样,室内静态模拟不同温度下太湖沉积物铵态氮释放.结果表明,经面积加权,5℃、15℃和25℃下氮的交换速率分别为-16.0±17.6mg/穴m2·d雪、12.6±6.9mg/穴m2·d雪和34.1±20.8mg/穴m2·d雪,不同湖区其释放速率差异极大.受外源污染影响较大的水域,氮释放量随温度的升高而增加;受死亡残体沉降和分解影响明显的草藻型湖区,氮的年释放通量较大.全太湖沉积物-水界面NH4 -N的年净通量为9960.3±4960.0t,其中成汇的通量值约为-911±637.9t/a,大部分泥区在一年中至少经过了一次的源-汇转换过程.  相似文献   

4.
湖泊底泥疏浚环境效应:II.内源氮释放控制作用   总被引:2,自引:0,他引:2  
通过为期一年的疏浚模拟试验,在试验室培养疏浚与对照柱样研究了底泥疏浚对内源氮释放的控制效果.研究结果发现,疏浚表层30cm能够有效的消减沉积物中有机质含量与孔隙水中NH4^+含量.在一年的试验周期内,疏浚和对照柱沉积物-水界面的NH4’通量分别为5.3至18.6mg/(m2·d)与-9.4至67.5mg/(m2·d),疏浚柱沉积物-水界面的Nm+通量总体上低于未疏浚对照的通量,尤其是在温度较高的月份,从2006年5-12月疏浚柱沉积物-水界面NH4^+释放通量显著低于未疏浚对照柱,疏浚沉积物的NH4^+的释放潜力低于未疏浚对照沉积物.研究结果表明,在外源得到有效控制的前提下,底泥疏浚是消减研究区内源氮负荷有效的技术手段.  相似文献   

5.
好氧和厌氧条件对霞浦湖沉积物-水界面氮磷交换的影响   总被引:55,自引:4,他引:55  
在实验室控制条件下,研究了日本霞浦湾和湖心区底泥中形态氮磷,在好氧和厌氧条件下水土界面交换量变化及差异,结果表明;好氧条件下,NO^-3-N,NO^-2-N,NH^+4,-N,和PO^3-4-P均有释放作用产生,量值多数较小,DTN和DTP则净释放作用接近零;厌氧条件下,NO^-3-N和NO^-2-N呈负释放状态,NH^+4-N和PO^3-4-P的释放速率是好氧条件下的2-8倍。  相似文献   

6.
太湖梅梁湾沉积物-水界面氮迁移特征初步研究   总被引:36,自引:7,他引:29  
用乙炔为抑制剂,气相色谱法测定了1997年夏季太湖梅梁湾口沉积物-水界面的反硝化率和N2O的自然排放率,太湖梅梁湾沉积物的反硝化率为1.4-5.6μmolN2/(m^2.h),N2O的复原斐和率为0.08-0.66μmolN2/(m^2.h),探讨了沉积物-水界面NO^-3的交换动态。指出沉积物内硝化-反硝化作用是太湖湖泊生态系统氮循环过程中一个重要的环节。在湖泊水土界面氮交换中,沉积物是具有吸收  相似文献   

7.
太湖水体中胶体磷含量初探   总被引:34,自引:3,他引:34  
室内静态模拟不同温度下太湖15个湖区柱状沉积物磷酸根释放,分析了相应表层沉积物形态磷,以及梅梁湾间隙水中相关离子Al(Ⅲ)、Fe(Ⅱ)、Ca(Ⅱ)和PO43-含量的季节变化.研究表明,受陆源影响较大的泥区通常是太湖内源磷的稳定源;而在开敞度较大的湖区,由于表层沉积物胶体的物化吸附,使得温度对底泥磷释放的影响作用减弱,并易产生磷的“内汇”现象;在梅梁湾区成汇区,还加上春夏季藻类的局部超负荷需磷这一控制因素,从而使得太湖大部分泥区在一年中至少发生一次源-汇转换过程.化学热力学分析揭示,Al-P较之Fe-P和Ca-P更易在界面发生溶解可能是太湖表层沉积物Al-P与PO43-P释放速率呈显著相关(r=0.3858>r1-0.01,n=45)的内在原因.虽然沉积物中Fe-P有较高的释磷潜力,但浅水湖所营造的沉积物表层氧化层和广泛覆盖的无机胶体及粘土矿物的强吸附介质,可能是抑制沉积物中Fe-P释放成为优势的主要因素.估算太湖沉积物-水界面磷的净通量为899.4±573.6 t/a,约占太湖磷入湖量的1/4-1/2,其中成汇通量约为-91.2±42.4 t/a.  相似文献   

8.
太湖底泥及其间隙水中氮磷垂直分布及相互关系分析   总被引:97,自引:16,他引:81  
范成新  杨龙元  张路 《湖泊科学》2000,12(4):359-366
对太湖主要湖区柱状样底泥的总氮、总磷含量及其间隙水铵态氮(NH^+4-N)、磷酸根磷(PO^3-4-P)和二价铁Fe(II)含量进行了分析,并对底泥和间隙水中相应物质含量进行了比较,结果表明:太湖近表层10cm内底泥TN、TP赋存含量较之下层高12%-20%左右,间隙水中PO^3+4-P和NH^+4-N含量随浓度增加而大致呈上升趋势,表层未见高浓度层存在,各湖区底泥间隙水中PO^3+4-P和NH^  相似文献   

9.
福建山仔水库不同季节表层沉积物内源磷负荷分析   总被引:4,自引:0,他引:4  
对山仔水库沉积物各形态磷的季节性特征以及夏、冬季磷释放速率进行研究.结果表明,该水库表层沉积物含有较丰富的磷,4个季节各采样点表层沉积物总磷含量范围为(521.23±7.60)~(1255.54±11.03)μg/g,夏季各采样断面中总磷含量及各形态磷含量均高于其他季节.表层沉积物磷以无机磷为主,且主要赋存形态为铁/铝结合态磷.活性较大的铁/铝结合态磷和有机磷占总磷量的77%~90%.柱状样模拟实验结果表明:夏季溶解性磷释放平均速率范围在1.66~2.49 mg/(m2·d),冬季溶解性磷释放平均速率范围为0.69~1.29 mg/(m2·d),夏季各采样点表层沉积物磷释放速率约为冬季的2倍.由于水温分层,夏季沉积物释放的溶解性磷主要滞留在上覆层,但夏季暴雨天气可能导致水温分层破坏,沉积物释放的溶解性磷对水体将产生重要影响;冬季由于水温分层破坏导致上、下水层混合,沉积物释放的溶解性磷被带到上层,对上覆水体水质的影响不容忽视.  相似文献   

10.
藏南沉错钻孔沉积物金属元素分布特征及其与粒度的关系   总被引:4,自引:1,他引:3  
王君波  朱立平 《湖泊科学》2008,20(6):715-722
从沉积物磷的化学形态特征、沉积物-水界面的环境条件和水库的水文参数等角度探讨了山仔水库沉积物磷对上覆水体的磷浓度贡献,并从沉积物间隙水与水体垂向溶解性磷的浓度梯度估算对水体磷浓度的贡献大小.结果表明:山仔水库沉积物具有大的释放磷的潜力,沉积物间隙水和水体之间存在着明显的溶解性磷的浓度梯度,沉积物的溶解性磷释放通量在0.0420—0.167μg/(cm^2·d))之间,沉积物磷对水体营养贡献大小在0.7%-6%之间,其中秋冬季节沉积物磷对水体的贡献大于春夏季节,当外源减少时,沉积物磷负荷在一定时间内将成为水库营养状态的重要贡献因子。  相似文献   

11.
12.
正Director:Shangfu Kuang,China Vice-directors:Chunhong Hu,China Duihu Ning,China Guangquan Liu,China The International Research and Training Center on Erosion and Sedimentation(IRTCES)was jointly set up by the Government of China and UNESCO on July 21,1984.It aims at the promotion of international exchange of knowledge and cooperation in the studies of erosion and  相似文献   

13.
14.
15.
16.
正SCIENCE CHINA Earth Sciences,an academic journal cosponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China,and published by Science China Press and Springer,is committed to publishing high-quality,original results in both basic and applied research.  相似文献   

17.
Feedback mechanisms, which operate upstream through drawdown and backwater effects and downstream through sediment discharge are responsible for channel evolution. By combining these mechanisms with channel processes it euables a dynamic process-response model to be developed to simulate the initial evolution of straight gravel-bed channels. When erosion commences on a land surface, sediment entrained in the headwater reach by hydraulic action is selectively transported, deposited and reworked. This produces a damped oscillation between degradation and aggradation as the channel and valley respond to spatial and temporal variations in sediment calibre and hydraulic conditions. The initial cut and fill phases are responsible for valley incision and floodplain development while secondary and subsequent activity can produce river terraces. Eventually sediment entrainment in the headwaters declines as slopes are reduced. Subsequent channel evolution is relatively insignificant because it is dependent on local weathering activity producing material that can be transported on declining slopes. Therefore landforms produced during the initial phase of development, when local weathering was non-limiting, dominate the landscape.  相似文献   

18.
Based on relocating the Jiujiang-Ruichang earthquake sequence which occurred on November 26, 2005 in Jiangxi Province with the double-difference (DD) algorithm and master event technique, the paper discusses the focal mechanism of the main shock (MsS.7) and the probable seismo-tectonics. The precise relocation results indicate that the average horizontal error is 0.31kin in a EW direction and 0.40kin in a NS direction, and the average depth error is 0.48kin. The focal depths vary from 8kin to 14kin, with the predominant distribution at 10kin - 12kin. The epicenter of the main shock is relocated to be 29.69^oN, 115.74^oE and the focal depth is about 10.Skin. Combining the predominant distribution of the earthquake sequence, the focal mechanism of the main shock and the tectonic conditions of N-E- and NW-strike faults growth in the seismic region, we infer that the main shock of the earthquake sequence was caused by a NW striking buried fault in the Rnichang basin. The nature of seismic faults needs to be further explored.  相似文献   

19.
Abstract

The western reservoirs represent the principal groundwater system in Morocco. Demographic, industrial and agricultural developments during the last decade have markedly altered groundwater quality. The Mamora coastal aquifer system is among the Atlantic systems which are most heavily threatened by pollution. Agricultural and industrial activities, and rapid urban growth contribute to the pollution of the groundwater. Contamination transport is facilitated by a high permeability of the aquifer formations. In order to assess the actual groundwater quality of the Mamora aquifer and to understand the influence of the factors generating the pollution, an extensive multidisciplinary research programme is in progress, with hydrochemistry and microbiology playing essential roles. The present paper concerns the spatial distribution of physico-chemical parameters in the groundwater, subjected to domestic, industrial and agricultural pollution. Fifty-seven samples were analysed for several parameters (Ca2+, Mg2+, Na+, K+, Cl?, SO4 2?, HCO3 ?, NO3 ?, pH, electrical conductivity and temperature). The microbiological analysis of 143 samples reveals the presence of four kinds of indicator bacteria in the groundwater resources: faecal Streptococci, faecal coliform, Escherichia coli and Clostridium. The physico-chemical results and bacteriological monitoring show that the nitrate and bacteria concentrations exceed the maximum admissible levels, notably around pumping stations in the sectors of Sidi Taibi, Sidi Ahmed Taleb and Aïn Sbaâ. Contamination is generated by uncontrolled anthropogenic activities and accentuated by the high intrinsic vulnerability of the aquifer system. Several parameters appeared to exceed admissibility standards. Measures are recommended to prevent groundwater pollution in the region.  相似文献   

20.
正SCIENCE CHINA Earth Sciences,an academic journal cosponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China,and published by Science China Press and Springer,is committed to publishing high-quality,original results in both basic and applied research.  相似文献   

设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司  京ICP备09084417号