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1860年以来博斯腾湖碳沉积过程演变 总被引：1，自引：1，他引：0
选取博斯腾湖3个不同点位岩芯，在210Pb和137Cs年代序列基础上，利用沉积物中的各理化指标，分析了该湖碳沉积的时空变化特征，结合各指标的相关性、沉积速率、C/N、同位素特征等，探讨了该湖1860年以来碳沉积环境的变化过程，为干旱区湖泊碳埋藏研究提供了依据.结果表明：1860-1910年，沉积速率相对较小，受人类活动影响较小，磁化率、中值粒径、总无机碳（TIC）较为稳定，总有机碳（TOC）含量相对较低，此时该湖有较多陆源有机质的输入；1910-1950年，湖泊西部浅水域沉积速率明显高于东部深水区，西北湖区水域有大量外源物质的输入，而湖泊初级生产力较低，内源贡献相对较小；1950-1980年，全湖TOC、TIC含量均呈现升高的趋势，尤其是西北近黄水沟水域升高最快，湖泊内源贡献在增加，陆源组分的输入相对前一阶段要少；1980-2002年，沉积速率快速升高，尤其湖泊东部水域最为明显，TOC含量均呈现升高的趋势，湖泊西部水域初级生产力要高于东部深水区，湖面蒸发较强，气候比较温暖；2002年以来，全湖沉积速率相对较高，外源有机质贡献较小.过去150年博斯腾湖沉积物碳累积速率整体上呈现出升高的趋势，尤其是近50年来快速升高，东部湖区碳累积速率比西部湖区高. 相似文献
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大布苏湖地貌——沉积类型与湖泊演化 总被引：2，自引：1，他引：2
大布苏湖地处松嫩平原南部，是一个封闭的构造断湖，湖区山貌类型复杂，沉积环境独具特色，根据地形面的分层和特征，结合^14C测年，确定大布苏湖形成于晚更新世晚期，湖泊形成的早期，曾经历了深湖的发育阶段，全新世以来，湖面波动式下降，并有两次规模较大的扩张和收缩时期，形成了两个完整的湖进、湖退沉积旋回、晚全新世以来，气候干燥，风力作用活跃，湖面明显萎缩，形成我国东部地区极为罕见的盐湖。 相似文献
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近50年来内蒙古查干淖尔湖水量变化及其成因分析 总被引：1，自引：1，他引：0
内蒙古查干淖尔湖是位于季风边缘区干旱与半干旱过渡带的封闭湖泊,对气候变化响应极为敏感.利用1958-2010年的查干淖尔湖21期遥感影像以及湖泊流域1955-2010年的3个气象站点和1个水文站点的气温、降水、蒸发和径流等数据,分析查干淖尔湖近50余年的湖泊水量、面积/水位波动及其原因.结果表明,近50年来在区域气候暖干化的背景下,查干淖尔湖不断萎缩,流域生态环境退化.1958-2010年湖泊容积以2×106m3/a的速度锐减66.9%(从124.1×106m3降到41.1×106m3),湖泊面积缩小73.3%(从105.3 km2降到28.1 km2),平均缩减速度为1.8 km2/a;流域年均气温上升了2.5℃,年降水量下降了36.6 mm.湖泊水量与流域气温和蒸发量显著负相关.查干淖尔湖分为东西两部分,中间由天然堤坝相连,东湖在水闸的人为控制下水位波动范围不超过1 m.西湖水位波动则相对剧烈,湖面下降7.6 m,于2002年彻底干涸,湖盆裸露,已成为盐尘暴、沙尘暴源地. 相似文献
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对位于大兴安岭中北段四方山天池全新世以来湖泊沉积物中正构烷烃的分布特征及其单体碳同位素组成进行了讨论分析.结果表明,正构烷烃碳数分布范围为nC_(17)~nC_(33),绝大多数样品具有单峰型的分布特征,少数样品呈现双峰型分布特征,单峰型以nC_(27)为主峰,双峰型分布中前峰群以nC_(21)为主峰、后峰群以nC_(27)为主峰;短链正构烷烃(nC_(21))奇偶优势不明显,中链(n C23~n C25)和长链正构烷烃(nC_(27))具有明显的奇碳优势;正构烷烃的分布特征揭示四方山天池湖泊沉积物中的有机质来源于陆生植物和水生植物的共同输入,并以陆生植物贡献为主.全新世以来,四方山天池湖泊沉积物中长链正构烷烃单体碳同位素值(δ~(13)C_(27~31))逐渐偏负,与太阳辐射的变化表现出明显的一致性,表明在轨道尺度上该区域的有效湿度的逐渐增加主要受太阳辐射的控制,湖泊水位的变化则既受到西太平洋副热带高压和鄂霍次克海高压相对位置的影响,又受到东南季风和东北季风势力强弱的制约.根据多种气候代用指标的变化,全新世以来四方山天池湖泊环境及其区域气候演化可以划分为5个阶段:(1)11.2-8.0 ka BP:区域有效湿度较低,陆生C_3植物中木本植物比例略有增加,湖泊水位频繁波动,湖泊初级生产力下降,湖泊营养状态发生贫化;(2)8.0-6.4 ka BP:区域有效湿度增加,陆生C_3植物中草本植物比例略有增大,湖泊水面收缩、水位下降,湖泊初级生产力变化不大,湖泊营养状态较为稳定;(3)6.4-3.4 ka BP:区域有效湿度比上一阶段更高,陆生C_3植物中木本植物扩张,草本植物比例相对收缩,湖泊水位上升、水面扩大,湖泊初级生产力增加,湖泊营养状态发生好转;(4)3.4-2.4 ka BP:区域有效降水量继续增加,陆生C_3植物中草本植物比例升高,湖泊水位下降、水面收缩,湖泊初级生产力下降,湖泊营养状态发生贫化;(5)2.4-0.9 ka BP:区域有效湿度较高,陆生C_3植物中木本植物逐渐增加,湖泊水位上升、水面扩张,湖泊初级生产力增加,湖泊营养状态有所好转.四方山天池湖泊沉积物所记录的全新世以来区域气候环境演化历史,既与中国东北地区其他高分辨率气候记录有较好的一致性,也存在着差异性,表现出独有的区域气候特征. 相似文献
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区域增温和大气氮沉降作用已成为高山湖泊面临的重要环境胁迫,已有高山湖泊生物群落响应的长期模式研究主要集中于藻类而缺乏更高营养级生物(如浮游动物)的系统调查。本研究选择滇西北地区深水型的高山湖泊沃迪错开展沉积物调查,通过多指标分析(总氮、总磷、叶绿素a、氮稳定同位素等)并结合区域气候重建记录,识别近两百年来该湖泊及流域环境的变化历史,进一步利用枝角类群落指标(物种组成、生物量等)定量评价了湖泊生物群落的响应模式与驱动因子。结果表明,湖泊营养水平(如总氮浓度)和初级生产力(叶绿素a浓度等)在过去近两百年总体呈上升趋势。相关分析显示,大气氮沉降和流域外源输入是影响总氮上升的主要因素,同时区域增温和营养盐富集促进了湖泊初级生产力的不断上升。自1960s以来区域升温明显,湖泊营养水平和叶绿素a浓度呈现加速上升的趋势。钻孔中枝角类群落以浮游属种(Daphnia longispina等)为优势种,在1900AD以前D.longispina相对丰度较为稳定(40.83%±8.02%),之后出现下降趋势且在1948—1965年间明显下降,之后再次明显上升并成为主要优势种。排序分析显示,气温、叶绿素a和总... 相似文献
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湖泊沉积有机碳同位素与环境变化的研究进展 总被引：20，自引：2，他引：20
湖泊沉积有机质稳定碳同位素（δ^13Corg)在区域气候与环境变化方面的应用近年来发展迅速，成果令人瞩目，保存在各类湖泊岩芯中的δ^13Corg记录揭示了晚更新世以来大气CO2浓度的变化、湖泊水位波动、湖区生态与植被的变迁以及气温变化等重要环境信息，由于造成δ^13Corg值变化的影响因素较多，确定个湖与环境变化有关的主导因素时常有赖于其它证据的帮助，诸如地球化学、古湖沼学、孢粉学、分子同位素地层学等等，前人通过研究来自不同类型湖泊、具不同曲线形态特征的δ^13Corg记录，提出了多种环境解释模型，本文对此作了归纳和评述。鉴别和澄清湖泊沉积有机质的源物质以及有机物源随环境变化而发生过的变化，是研究δ^13Corg记录环境意义至关重要的基础性工作，由于有机质含量、碳氮比值、氢指数、生物残留物鉴别等常能提供有关有关湖泊有机质来源、产率、成岩作用等方面的有用信息，这方面的研究结果应该尽可能一并提供，以利于恰当地应用现有的环境解释模型，或者建立个湖新模型，单体生物标志化合物鉴别通常也能为区分湖积有机质中陆生、水生、细菌生等不同碳的来源提供有用信息，特定化合物同位素分析技术近年来成功地应用于建立单体生物标志化合物碳同位素地层学，为湖积有机碳同位素在生态环境演变研究方面的应用提供了思路，我国许多湖泊的湖底沉积岩芯尚未钻取，那些对过去全球变化研究有价值的δ^13Corg记录有待我们去获取和研究。 相似文献
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陕西红碱淖近百年来环境变化的湖泊沉积记录 总被引：14，自引：1，他引：14
本文通过岩性、粒度、磁化率、有机碳、化学元素的多指标综合分析,对陕西红碱淖近百年以来的环境演化进行了探讨。红碱淖于1927年后开始成湖,以较低的磁化率值、低湖泊生产力和较高的Fe/Mn比值为特征;1952-1960年,为短暂湖泊快速扩张时期,在沉积物中表现为粘粒含量一度下降、各元素浓度明显被稀释;自1960年以来,岩性和指标特征反映了该湖演化为稳定的深湖环境。湖泊的形成和扩张与区域降水量的增加有关,而50年代后期以来湖面的迅速扩大同时得益于人类滩地疏导导致的入湖水量增加。人类活动也引起了近40年来湖泊生产力的提高和沉积物-水界面氧系统的变化。此外,钻孔粒度特征较好地分辨出20世纪30年代末至40年代3次强沙尘暴事件。 相似文献
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湖泊沉积通量蕴含了流域降水量及人类活动的丰富信息.依据太白湖沉积岩芯210Pb定结果及CRS模式,建立了近百年来的沉积年代序列,对比分析了不同时期沉积通量变化与流域降水量及人类活动的关系.1900-1920、1928、1937-1942、1953-1954年沉积通量较高的四个时段,分别对应于夏季降水较多的1900-1920、1931、1938-1939、1954年,沉积通量增加主要与夏季降水量偏多,被带入湖泊的泥沙量增加有关.1958-1963年,太白湖流域上游兴建三座水库,对洪水及入湖泥沙起到了调蓄作用,自此之后,太白湖的平均沉积通量减小,降水量已不再是影响沉积通量的主导因素;1958-1970年沉积通量较高,主要是太白湖围垦导致的入湖泥沙量的增加及湖泊面积减小所致;1983-1993年沉积通量的增加则反映了农业生产方式由集体转为个体生产模式后,耕作业的快速发展所导致的水土流失的加重.研究结果证明,采用210Pb强度及CRS模式所建立的太白湖近百年来的沉积年代标尺精度较高(误差小于4年),太白湖沉积环境稳定,可采用其沉积指标进行流域及湖泊环境演化重建. 相似文献
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《Limnologica》2014
Human activities in Lake Fuxian and its catchment have caused environmental changes that are preserved in the geochemical records of lake sediments. Human activities responsible for the environmental changes include agriculture, mining, industrial development, and fishery management. To elucidate human impacts on this deep water body during the past several decades, two short sediment cores were collected from the lake, dated by 137Cs, and analyzed for several geochemical variables (total organic carbon (TOC), total nitrogen (TN), δ13C and heavy metals). The multi-proxy geochemical and isotopic evidence can be used to divide the limnological record into a 3-part history. Although increasing inputs of chromium (Cr) had begun as early as the 1950s, human activities, including heavy metal contamination, apparently had little effect on lacustrine production, as δ13C, TOC, TN and TOC/TN were relatively constant until the 1980s. Mining and industry have generated large amounts of heavy metal elements such as Zn, Pb and Cd that have been deposited into the lake since the 1980s, increasing to their highest concentrations over the last decades. Zn, Pb and Cd probably were released by industrial processes such as the manufacture of cement. Cr concentrations increased at site FB, but declined at site FZ, most likely due to the closer proximity of site FB to the source of metal production. From the middle of the 1980s, the decreased δ13C, and increased TOC, TN and TOC/TN suggest a broad change in lake ecology. In the 1980s, a new fish species was introduced into Lake Fuxian and fish yields increased quickly, which may mark the beginning of a change in ecosystem structure. 相似文献
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武汉典型湖泊沉积物中重金属累积特征及其环境风险 总被引：20，自引：1，他引：19
采集武汉市8个典型湖泊的表层沉积物,分析11种重金属的含量及其不同形态组成,研究了不同湖泊金属元素的富集与污染程度,探讨了沉积物中重金属的污染来源及其潜在生态风险,结果表明,沉积物中重金属Cd累积最严重,Zn和Hg也发生明显累积,龙阳湖污染较重,南太子湖和墨水湖污染中等,其它湖泊污染总体较轻.沉积物性质对重金属累积的影响不显著,城市工业活动强烈影响着重金属的分布,不同重金属的形态分布差异较大,Cd生物可利用态含量最高,其次为Mn、Zn、Co、Cu和Pb;而Sb和Hg以残留态占绝对优势,生态风险较小,相关分析和主成分分析表明,化石燃料燃烧、金属冶炼等是武汉市湖泊沉积物中重金属来源的主要贡献者,同时岩石风化等地球化学过程也影响着重金属的污染. 相似文献
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Maija Jylhä-Ollila Hanne Laine-Kaulio Jos Schilder Paula Niinikoski-Fuβwinkel Timo Kekäläinen Janne Jänis Harri Koivusalo 《Ground water》2021,59(5):644-657
Managed aquifer recharge (MAR) provides means to remove natural organic matter (NOM) from surface waters. Recent studies have explored the degree of NOM removal in groundwater. In this study, we further elaborate the NOM removal at a lakeside natural bank infiltration site that functions as a surrogate for MAR. Our objective was to quantify the carbon budget in the aquifer based on concentration measurements of dissolved (in)organic carbon, and the molecular changes in NOM using Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS). According to the carbon budget, only 25% of the dissolved carbon entering the aquifer was organic, and it predominantly originated from lake water. Of the inorganic majority, on average 40% was produced in the vadose zone above the groundwater table, 31% in the lake bank, 22% in the aquifer as a result of degrading organic matter of lake water, and 7% in the lake. Seasonal concentration variations suggested that the lake bank was the main carbon source in the summer, increasing the carbon concentration of infiltrating lake water, that is, 3.0 mg/L to 7.9 mg/L. FT-ICR MS results showed 4960 to 5330 individual compounds in lake and groundwater. NOM removal in the aquifer was selective: the relative abundance of oxygen-containing species decreased from 75 to 31%, while the relative abundance of sulfur-containing species increased from 15 to 57%. The average molecular weights of both species remained unchanged. The study highlighted the role of lake bank processes and sulfur-containing species in groundwater quality. 相似文献
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Skadar Lake,the largest lake on the Balkan Peninsula,is famous for a wide range of endemic and rare,or even endangered plant and animal species.Different anthropogenic pressures have,however,influenced the fragile equilibria of the lake ecosystem,with metal pollution as one of the primary concerns.Therefore,this study investigated spatial distribution of metal pollutants in the water and sediment phase of Skadar Lake,and anthropogenic and environmental factors affecting this distribution.A sieving analysis showed that sediment in Skadar Lake is mainly distributed in the three smallest fractions（colloid,clay and silt）.Eleven metals were analyzed in the lake surface and bottom water,and only six of them were detected：potassium,magnesium,calcium,nickel,aluminum and manganese.They were all present at low concentrations.In contrast,sediments contained elevated levels of some metals with concentrations between 28.1-126.8 mg kg~（-1） for Ni,23.6-79.2 mg kg~（-1） for Cr,9.2-36.9 mg kg~（-1） for Cu,199-878 mg kg~（-1） for Mn and 9.6-23.1 g kg~（-1） for Fe.Nickel exceeded consensus-based guidelines for safety towards freshwater dwelling organisms.The organic matter content of the sediment fluctuated between 4.7 and 21.5%.No correlations were found between metal concentrations,organic matter and sediment particle size fractions,suggesting that the latter are not the main factors controlling metal accumulation in Skadar Lake. 相似文献
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湖泊沉积物碳库作为湖泊生态系统的重要组成部分,对湖泊碳循环起重要作用,而蓝藻水华衰亡过程对湖泊碳库稳定性影响研究较少本研究采集太湖蓝藻、湖水、沉积物样品,建立蓝藻水沉积物室内模拟实验系统,分析蓝藻水华衰亡过程中沉积物碳库易氧化有机碳(EOC)、惰性有机碳(ROC)、微生物量碳(MBC)、轻组有机碳(LFOC)和重组有机碳(HFOC)的变化规律,探究蓝藻水华衰亡过程对湖泊碳库稳定性的影响结果表明,蓝藻水华衰亡前期(1～9天),ROC缓慢下降,EOC和LFOC快速下降,MBC有所增加;衰亡中期(10～45天),沉积物TOC和ROC含量升高;衰亡末期(46～63天),HFOC和ROC等稳定有机碳进入一个从缓慢分解逐渐趋于稳定的阶段周期性的蓝藻水华暴发、衰亡和湖泊稳定性有机碳的日渐累积,最终会对沉积物碳库有机碳组分及其稳定造成显著影响. 相似文献
16.
Variation characteristics of heavy metals and nutrients in the core sediments of Taihu Lake and their pollution history 总被引：4，自引：2，他引：4
The sedimentary environment change, trophic evolution and heavy metals pollution history of the northern Taihu Lake in the last 100 years are studied according to the sedimentary geo-chemical proxies of the core sediments, such as grain size, nutrients, heavy metals, diatom, etc. The nutrients in the sediments depended mainly on the lake internal circulation and the heavy metals were from natural geogenic sources before the 1920s, which were not influenced by human activities generally, and grain size was one of the key factors influencing heavy metals content in the sediments. The alternation of manner and strength of human activities in Taihu Lake catchment before and after the 1920s made the lake sediments coarser, and hence heavy metals and TP content decreased contrasted with that before the 1920s. TP content in sediments and water increased from the 1950s to late 1970s due to anthropogenic pollutants discharge, and the lake belonging to mesotrophic state. TN and TOC content and C/N ratio increased due to the increasing external pollutants into Taihu Lake by human activities, TP content also increased obviously in water and sediments, and the diatom association was dominated by eutrophic species since the late 1970s, indicating the eutrophication state of Taihu Lake in this period. Meanwhile the increasing in heavy metals content, such as Cu, Mn, Ni, Pb and Zn, and their proportion of valid fractions in the sediments indicates that they all result from human pollutants since the late 1970s. The heavy metals in the surface sediments have certain potential biological toxicity due to the higher SEM/AVS ratio. 相似文献
17.
XIAO Huayun & LIU Congqiang The Key Laboratory of Environmental Geochemistry Institute of Geochemistry Chinese Academy of Sciences Guiyang China 《中国科学D辑(英文版)》2004,47(9)
Withtheintensificationofhumanindustrialandagriculturalactivities,theinputofindustrialnitrogen,includinginorganicandorganicnitrogen,intothelakesystemwilldrasticallyincrease.Afterfindingitswayintolakes,terrestrialorganicnitrogenwillsettledowntogetherwithlakehydrogenousorganicnitrogen,experiencedegradationandfinallybecomelakeinteriornitrogen.Studieshaveshownthatthecontentsoforganicnitrogenarerelativelyhighinlacustrinesediments,andthedegradationoforganicmattermaybringaboutmoreNO3-totheupper-levelw… 相似文献