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1.
Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases.  相似文献   

2.
This study estimates direct radiative forcing by tropospheric ozone and all aerosols between the years 1850 and 2000, using the new IPCC AR5 (the Intergovernmental Panel on Climate Change Fifth Assessment Report) emissions inventories and a fully coupled chemistry-aerosol general circulation model. As compared to the previous Global Emissions Inventory Activity (GEIA) data, that have been commonly used for forcing estimates since 1990, the IPCC AR5 emissions inventories report lower anthropogenic emissions of organic carbon and black carbon aerosols and higher sulfur and NOx emissions. The simulated global and annual mean burdens of sulfate, nitrate, black carbon (BC), primary organic aerosol (POA), secondary organic aerosol (SOA), and ozone were 0.79, 0.35, 0.05, 0.49, 0.34, and 269 Tg, respectively, in the year 1850, and 1.90, 0.90, 0.11, 0.71, 0.32, and 377 Tg, respectively, in the year 2000. The estimated annual mean top of the atmosphere (TOA) direct radiative forcing of all anthropogenic aerosols based on the AR5 emissions inventories is -0.60 W m^-2 on a global mean basis from 1850 to 2000. However, this is -2.40 W m-2 when forcing values are averaged over eastern China (18-45°N and 95-125°E). The value for tropospheric ozone is 0.17 W m^-1 on a global mean basis and 0.24 W m^-2 over eastern China. Forcing values indicate that the climatic effect of aerosols over eastern China is much more significant than the globally averaged effect.  相似文献   

3.
In May 2008, ScienceWatch.com named Advances in Atmospheric Sciences a Rising Star among Geosciences journals. According to Essential Science IndicatorsSM from Thomson Reuters, the journal's cur-rent citation record includes 764 papers cited a total of 1,658 times between January 1, 1998 and February 29 2008.  相似文献   

4.
A case of hailstorm process occurring on 24 June 2006 in northwestern China was studied using satellite retrieval methodology. The particle effective radius (re) in the cloud tops was calculated by the reflectance in the 3.7μm channel, and cloud-top microphysical properties were vividly represented using the RGB visual multispectral classification scheme. The microphysical zones of clouds and the processes of hail formation and development are inferred using the relations of cloud-top temperature (T) versus re for the tops of convective clouds. The results show that particle effective radius was smaller near the cloud base of hailstorm. There was a deep zone of diffusional droplet growth at the low level where the particles grew slowly with height, and there existed an evident area of small ice particles in the cloud top, suggesting the existence of a strong updraft in the clouds. The low glaciated temperature indicated a great depth from the cloud base to the glaciation height, which provided a deep layer of supercooled water for hail growth.  相似文献   

5.
孙源隆  石广玉 《大气科学》2011,35(2):350-360
本文提出了一种利用可见光与近红外大气窗区内的0.5μm和0.85μm双通道的组合,通过观测地气系统的反射辐射从卫星上遥感陆面上空气溶胶的方法.模拟试验发现,对于不同类型的气溶胶,随着气溶胶光学厚度的逐渐增大,0.5μm和0.85μm双通道的反射辐亮度的差值和比值呈现出明显不同的变化趋势,据此便可以识别出气溶胶的类型,并...  相似文献   

6.
大气气溶胶的卫星遥感及其在气候和环境研究中的应用   总被引:2,自引:1,他引:1  
卫星遥感可以获得全球范围的大气气溶胶光学特性,目前国内外已有多颗卫星观测能够提供气溶胶特性的资料。本文综述性介绍国内外卫星遥感气溶胶特性方面的研究进展和成果,并讨论了卫星遥感资料在气候和环境研究领域中的应用。主要内容包括:极轨/静止卫星平台搭载的被动遥感传感器及其反演气溶胶特性的方法;星载激光雷达获取气溶胶光学特性的方法;国内外正在研发的新一代卫星主、被动气溶胶遥感探测器;卫星气溶胶产品在气溶胶辐射强迫、气候效应、大尺度污染输送、区域空气质量监测等研究中的应用。  相似文献   

7.
The Stratospheric Aerosol and Gas Experiment (SAGE) II aerosol extinction profiles at 1020 nm were used to study the distribution characteristics of stratospheric aerosols during the volcanically quiescent period of 1998-2004. The stratospheric aerosol distributions exhibited hemispheric asymmetry between the Northern Hemisphere (NH) and the Southern Hemisphere (SH). In the lower stratosphere below 20 km, the zonal averaged aerosol optical depths in the NH were higher than those of the corresponding SH; whereas at higher altitudes above 20 km, the optical depths in the SH-- except the equatorial region--were higher than those of the NH. At 0-10°N and 10-20°N, the stratospheric aerosol optical depth (SAOD) exhibited larger values in boreal winter and lower values in the spring and summer; at 0-10°S and 10-20°S, the SAOD presented small seasonal variations. At 30-40°N, the SAOD presented larger values in the boreal fall and winter and lower values in the spring and summer; while at 30-40°S, the SAOD exhibited larger values in the austral winter and early spring and lower values in the summer and fall. These characteristics can mainly be attributed to the seasonal cycle of the dynamic transport, and the effects of the buildup and breakdown of the polar vortex. At 50-60°S, the SAOD exhibited extremely high values during austral winter associated with the Antarctic polar vortex boundary; at 50-60°N, the SAOD also exhibited larger values during the boreal winter, but it was much less obvious than that of its southern counterpart.  相似文献   

8.
本文应用WRF-Chem(Weather Research and Forecasting—Chemistry)模式研究中国东部地区气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)在天气尺度下的辐射强迫和对地面气温的影响。5个无明显降水时间段(2006年8月23~25日、2008年11月10~12日、2008年12月16~18日、2009年1月15~17日和2009年4月27~29日)的模拟显示,气溶胶浓度呈现显著的白天低,夜间高的日变化特征,且北方区域(29.8°~42.6°N,110.2°~120.3°E)平均PM2.5近地面浓度(40~80 μg m-3)高于南方区域(22.3°~29.9°N,109.7°~120.2°E,30~47 μg m-3)。气溶胶对地面2 m温度(地面气温)有明显的降温效果,在早上08:00(北京时,下同)和下午17:00左右最为显著,最高可降低约0.2~1 K,同时气溶胶的参与改善了模式对地面气温的模拟。本文还通过对2006年8月23~25日一次个例的模拟,定量分析了气溶胶及其部分组分(硫酸盐、硝酸盐和黑碳气溶胶)的总天气效应(直接效应+间接效应)、直接效应和间接效应分别对到达地面的短波辐射和地面气温的影响。北方区域平均气溶胶直接效应所造成的短波辐射强迫要高于南方区域,分别为-11.3 W m-2和-5.8 W m-2,导致地面气温分别降低了0.074 K和0.039 K。南方区域平均气溶胶间接效应所产的短波辐射强迫高于北方区域,分别为-14.4 W m-2和-12.4 W m-2,引起的地面气温的改变分别为-0.094 K和-0.035 K。对于气溶胶组分,硫酸盐气溶胶的直接效应和间接效应的作用相当,其总效应在北方和南方区域平均短波辐射强迫分别为-7.0 W m-2和-10.5 W m-2,对地面气温的影响为-0.062 K和-0.074 K,而硝酸盐气溶胶的作用略小。黑碳气溶胶使得北方和南方区域平均到达地表的太阳短波辐射分别减少了6.5 W m-2和5.8 W m-2,而地表气温则分别增加了0.053 K和0.017 K,相比于间接效应,黑碳气溶胶的直接效应的影响更加显著。  相似文献   

9.
The sub-monthly evolution of the interannual variations of absorbing aerosols and related hydrometeorology over South Asia in the pre-monsoon period is investigated from the analysis of pentad-resolution observational datasets.It is shown that pre-monsoon (late April–early May) variations are characterized by increased aerosols, reduced cloudiness and precipitation, and increased downward shortwave radiation. Lead-lag regressions indicate the significant influence of synoptic scale advection (and related vertical motion) in simultaneously shaping the aerosol distribution and associated significant hydroclimate (precipitation, cloudiness, surface shortwave radiation, and 2-m air temperature) over the Indo-Gangetic Plain.The above findings can be interpreted as a manifestation of the aerosol “semi-direct” effect if one is not mindful of the prevailing circulation anomalies and their concurrent impact on aerosol and hydroclimate. The complex interplay among aerosols, dynamics and precipitation also shows the challenge of extracting the aerosol impact from an observational analysis. Finally, the analysis points to the pitfalls of a columnar, circulation-blind framework in investigating aerosol–monsoon interactions, a concern of relevance in analyses of the impact of long-term aerosol trends, as well.  相似文献   

10.
利用地面细颗粒物(PM2.5)浓度和气象常规观测资料、地基 AERONET观测资料、GFED生物质燃烧排放清单和大气化学—天气耦合模式WRF-Chem,模拟研究了华北地区2014年10月气象要素和大气污染物的时空演变,重点关注北京10月7~11日的一次重霾事件及其天气形势、边界层气象特征、输送路径、PM2.5及其化学成分浓度变化等特征,以及秸秆燃烧对华北和北京地区细颗粒物浓度和地面短波辐射的影响。与观测资料的对比结果显示,模式可以很好地模拟北京地区地面气象要素和PM2.5质量浓度,考虑秸秆燃烧排放源可以明显改进北京PM2.5浓度模拟的准确性,但在重度污染情况下,模式总体上低估气溶胶光学厚度和高估地面短波辐射。10月7~11日北京地区重霾事件主要是不利气象条件下人为污染物累积和区域输送造成,也受到华北地区南部秸秆燃烧的影响。河南北部、河北南部和山东西部大面积秸秆燃烧释放的气态污染物和颗粒物在南风的作用下输送至北京,秸秆燃烧对北京地区地面PM2.5、有机碳(OC)、硝酸盐、铵盐、硫酸盐和黑碳(BC)的平均贡献率分别为24.6%、36.8%、23.2%、22.6%、7.1%和19.8%,秸秆燃烧产生的气溶胶可以导致北京地面平均短波辐射最大减小超过20 W m-2,约占总气溶胶导致地表短波辐射变化的24%。  相似文献   

11.
Cloud radiative kernels were built by BCC_RAD(Beijing Climate Center radiative transfer model) radiative transfer code. Then, short-term cloud feedback and its mechanisms in East Asia(0.5°S-60.5°N, 69.5°-150.5°E) were analyzed quantitatively using the kernels combined with MODIS satellite data from July 2002 to June 2018. According to the surface and monsoon types, four subregions in East Asia—the Tibetan Plateau, northwest, temperate monsoon(TM), and subtropical monsoon(SM)—were selected. The average longwave, shortwave, and net cloud feedbacks in East Asia are-0.68 ± 1.20, 1.34 ± 1.08, and 0.66 ± 0.40 W m~(-2) K~(-1)(±2σ), respectively, among which the net feedback is dominated by the positive shortwave feedback. Positive feedback in SM is the strongest of all subregions, mainly due to the contributions of nimbostratus and stratus. In East Asia, short-term feedback in spring is primarily caused by marine stratus in SM, in summer is primarily driven by deep convective cloud in TM, in autumn is mainly caused by land nimbostratus in SM, and in winter is mainly driven by land stratus in SM. Cloud feedback in East Asia is chiefly driven by decreases in mid-level and low cloud fraction owing to the changes in relative humidity, and a decrease in low cloud optical thickness due to the changes in cloud water content.  相似文献   

12.
不同污染条件下气溶胶对短波辐射通量影响的模拟研究   总被引:1,自引:0,他引:1  
将高光谱分辨率的气溶胶光学参数化方案应用于高精度的辐射传输模式BCC_RAD(974带)中,研究不同污染状况下气溶胶在地表与近地层大气中造成的直接辐射强迫与辐射强迫效率。发现气溶胶在地表产生的直接辐射强迫为负,在近地层大气中产生的直接辐射强迫为正,且随气溶胶浓度的升高变大,说明大气气溶胶的含量越高,单位气溶胶光学厚度产生的直接辐射强迫越大。将短波划分为3个波段:紫外、可见光和近红外,发现在紫外、可见光和近红外波段中,不同污染状况下气溶胶在地表造成的直接辐射强迫范围分别为:-1.36—-13.66、-3.03—-32.41和-2.74—-28.62 W/m2,在近地层大气中产生的直接辐射强迫范围分别为0.44—4.26、0.99—9.80和0.93—8.87 W/m2。通过进一步对比自然和人为气溶胶的影响,发现人为气溶胶在地表和大气层顶产生的负直接辐射强迫以及对整层和近地面大气造成的正直接辐射强迫均大于自然气溶胶的影响,且上述两种排放源的气溶胶对整层大气辐射收支的影响主要集中在800 hPa高度以下的大气中。按照地表直接辐射强迫大小来分析不同种类气溶胶的影响,结果为硫酸盐>有机碳>黑碳>海盐>沙尘;按照近地层大气直接辐射强迫大小排序则为黑碳>有机碳>沙尘>海盐>硫酸盐。最后,通过分析散射型气溶胶与吸收型气溶胶对辐射通量的影响,还探究了大气中散射与吸收过程的异同。   相似文献   

13.
Characterization of aerosols is required to reduce uncertainties in satellite retrievals of global aerosols and for modeling the effects of these aerosols on climate.Aerosols in the North China Plain(NCP) are complex,which provides a good opportunity to study key aerosol optical properties for various aerosol types.A cluster analysis of key optical properties obtained from Aerosol Robotic Network(AERONET) data in Beijing and Xianghe during 2001-11 was performed to identify dominant aerosol types and their associated optical properties.Five dominant aerosol types were identified.The results show that the urban/industrial aerosol of moderate absorption was dominant in the region and that this type varied little with season.Urban/industrial aerosol of weak absorption was the next most common type and mainly occurs in summer,followed by that strong aerosols occurring mainly in winter.All were predominantly fine mode particles.Mineral dust(MD) and polluted dust(PD) occurred mainly in spring,followed by winter,and their absorption decreased with wavelength.In addition,aerosol dynamics and optical parameters such as refractive index and asymmetry factor were examined.Results show that the size of coarse mode particles decreased with AOD indicating the domination of external mixing between aerosols.  相似文献   

14.
Simultaneous measurements on physical, chemical and optical properties of aerosols over a tropical semi-arid location, Agra in north India, were undertaken during December 2004. The average concentration of total suspended particulates (TSP) increased by about 1.4 times during intense foggy/hazy days. Concentrations of SO4 2−, NO3 , NH4 + and Black Carbon (BC) aerosols increased by 4, 2, 3.5 and 1.7 times, respectively during that period. Aerosols were acidic during intense foggy/hazy days but the fog water showed alkaline nature, mainly due to the neutralizing capacity of NH4 aerosols. Trajectory analyses showed that air masses were predominantly from NW direction, which might be responsible for transport of BC from distant and surrounding local sources. Diurnal variation of BC on all days showed a morning and an evening peak that were related to domestic cooking and vehicular emissions, apart from boundary layer changes. OPAC (Optical properties of aerosols and clouds) model was used to compute the optical properties of aerosols. Both OPAC-derived and observed aerosol optical depth (AOD) values showed spectral variation with high loadings in the short wavelengths (<1 μm). AOD value at 0.5 μm wavelength was significantly high during intense foggy/hazy days (1.22) than during clear sky or less foggy/hazy days (0.63). OPAC-derived Single scattering albedo (SSA) was 0.84 during the observational period, indicating significant contribution of absorbing aerosols. However, the BC mass fraction to TSP increased by only 1% during intense foggy/hazy days and thereby did not show any impact on SSA during that period. A large increase was observed in the shortwave (SW) atmospheric (ATM) forcing during intense foggy/hazy days (+75.8 W/m2) than that during clear sky or less foggy/hazy days (+38 W/m2), mainly due to increase in absorbing aerosols. Whereas SW forcing at surface (SUF) increased from −40 W/m2 during clear sky or less foggy/hazy days to −76 W/m2 during intense foggy/hazy days, mainly due to the scattering aerosols like SO4 2-.  相似文献   

15.
Aerosol optical properties and direct radiative effects on surface irradiance were examined using seven years(2006–2012)of Cimel sunphotometer data collected at Panyu—the main atmospheric composition monitoring station in the Pearl River Delta(PRD) region of China. During the dry season(October to February), mean values of the aerosol optical depth(AOD)at 550 nm, the ?ngstr?m exponent, and the single scattering albedo at 440 nm(SSA) were 0.54, 1.33 and 0.87, respectively.About 90% of aerosols were dominated by fine-mode strongly absorbing particles. The size distribution was bimodal, with fine-mode particles dominating. The fine mode showed a peak at a radius of 0.12 μm in February and October(~0.10μm~3μm~(-2)). The mean diurnal shortwave direct radiative forcing at the surface, inside the atmosphere(FATM), and at the top of the atmosphere, was-33.4 ± 7.0, 26.1 ± 5.6 and-7.3 ± 2.7 W m~(-2), respectively. The corresponding mean values of aerosol direct shortwave radiative forcing per AOD were-60.0 ± 7.8, 47.3 ± 8.3 and-12.8 ± 3.1 W m~(-2), respectively. Moreover,during the study period, FATMshowed a significant decreasing trend(p 0.01) and SSA increased from 0.87 in 2006 to 0.91 in 2012, suggesting a decreasing trend of absorbing particles being released into the atmosphere. Optical properties and radiative impacts of the absorbing particles can be used to improve the accuracy of inversion algorithms for satellite-based aerosol retrievals in the PRD region and to better constrain the climate effect of aerosols in climate models.  相似文献   

16.
彭杰  张华 《大气科学学报》2015,38(4):465-472
结合Cloud Sat对云的主动观测和MODIS(MODerate-Resolution Imaging Spectroradiometer)对气溶胶的被动反演,研究了典型站点气溶胶对云的宏观、微观和辐射特性的影响。结果表明,气溶胶对大陆性和海洋性站点的云均有显著影响。1)随气溶胶光学厚度(Aerosol Optical Depth,AOD)增加,水汽含量较弱站点的低层(高层)云量呈减小(增加)趋势,而水汽条件较强站点的各层云量均增大,且具有较高(较低)云顶的云层发生概率在各个站点都呈增加(减小)趋势。2)AOD的增大导致各站点云滴和冰晶粒子的有效半径均减小、大气层顶的短波和长波云辐射强迫均增强、短波云辐射强迫绝对值的加强更显著、长波云辐射强迫增加的幅度相对更大。3)气象要素在AOD大(小)值情况下的变化表明,大尺度动力条件并不能解释云的上述特性随AOD的显著改变。  相似文献   

17.
Lee  Wei-Liang  Liou  K. N.  He  Cenlin  Liang  Hsin-Chien  Wang  Tai-Chi  Li  Qinbin  Liu  Zhenxin  Yue  Qing 《Theoretical and Applied Climatology》2017,129(3-4):1373-1382

We investigate the snow albedo variation in spring over the southern Tibetan Plateau induced by the deposition of light-absorbing aerosols using remote sensing data from moderate resolution imaging spectroradiometer (MODIS) aboard Terra satellite during 2001–2012. We have selected pixels with 100 % snow cover for the entire period in March and April to avoid albedo contamination by other types of land surfaces. A model simulation using GEOS-Chem shows that aerosol optical depth (AOD) is a good indicator for black carbon and dust deposition on snow over the southern Tibetan Plateau. The monthly means of satellite-retrieved land surface temperature (LST) and AOD over 100 % snow-covered pixels during the 12 years are used in multiple linear regression analysis to derive the empirical relationship between snow albedo and these variables. Along with the LST effect, AOD is shown to be an important factor contributing to snow albedo reduction. We illustrate through statistical analysis that a 1-K increase in LST and a 0.1 increase in AOD indicate decreases in snow albedo by 0.75 and 2.1 % in the southern Tibetan Plateau, corresponding to local shortwave radiative forcing of 1.5 and 4.2 W m−2, respectively.

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18.
This study is based on ground-based measurements of downward surface shortwave irradiance (SW), columnar water vapour (wv), and aerosol optical depth (τ) obtained at Thule Air Base (Greenland) in 2007–2010, together with MODIS observations of the surface shortwave albedo (A). Radiative transfer model calculations are used in combination with measurements to separate the radiative effect of A (ΔSWA), wv (ΔSWwv), and aerosols (ΔSWτ) in modulating SW in cloud-free conditions. The shortwave radiation at the surface is mainly affected by water vapour absorption, which produces a reduction of SW as low as ?100 Wm?2 (?18%). The seasonal change of A produces an increase of SW by up to +25 Wm?2 (+4.5%). The annual mean radiative effect is estimated to be ?(21–22) Wm?2 for wv, and +(2–3) Wm?2 for A. An increase by +0.065 cm in the annual mean wv, to which corresponds an absolute increase in ΔSWwv by 0.93 Wm?2 (4.3%), has been observed to occur between 2007 and 2010. In the same period, the annual mean A has decreased by ?0.027, with a corresponding decrease in ΔSWA by 0.41 Wm?2 (?14.9%). Atmospheric aerosols produce a reduction of SW as low as ?32 Wm?2 (?6.7%). The instantaneous aerosol radiative forcing (RFτ) reaches values of ?28 Wm?2 and shows a strong dependency on surface albedo. The derived radiative forcing efficiency (FEτ) for solar zenith angles between 55° and 70° is estimated to be (?120.6 ± 4.3) for 0.1 < A < 0.2, and (?41.2 ± 1.6) Wm?2 for 0.5 < A < 0.6.  相似文献   

19.
Chinese FengYun-2C(FY-2C) satellite data were combined into the Local Analysis and Prediction System(LAPS) model to obtain three-dimensional cloud parameters and rain content. These parameters analyzed by LAPS were used to initialize the Global/Regional Assimilation and Prediction System model(GRAPES) in China to predict precipitation in a rainstorm case in the country. Three prediction experiments were conducted and were used to investigate the impacts of FY-2C satellite data on cloud analysis of LAPS and on short range precipitation forecasts. In the first experiment, the initial cloud fields was zero value. In the second, the initial cloud fields were cloud liquid water, cloud ice, and rain content derived from LAPS without combining the satellite data. In the third experiment, the initial cloud fields were cloud liquid water, cloud ice, and rain content derived from LAPS including satellite data. The results indicated that the FY-2C satellite data combination in LAPS can show more realistic cloud distributions, and the model simulation for precipitation in 1–6 h had certain improvements over that when satellite data and complex cloud analysis were not applied.  相似文献   

20.
The climatic effects of the atmospheric boundary aerosols are studied by the use of a three-dimensional climatemodel.Simulated results show that the climate states both at the surface and in the atmosphere change remarkably whenthe aerosols with different optical thicknesses and properties are introduced into the atmospheric boundary layer of themodel.The aerosols absorb and scatter the solar shortwave radiation,therefore,they reduce the solar energy reachingthe ground surface and decrease the surface and the soil temperatures.The temperature in the boundary layer increasesbecause of the supplementary absorption of radiation by the boundary aerosols.In the atmosphere,the temperatures atall isobaric surfaces rise up except for the 100 hPa level.The atmospheric temperatures below the 500 hPa level aredirectly influenced by the boundary aerosols,while the atmospheric temperatures above the 500 hPa level are influencedby the heating due to convective condensation and the changes in the vertical motion field.Cyclonic differential circula-tions appear over the desert areas at the low levels,and anticyclonic differential circulations exist at the upper levels inthe horizontal flow fields.The vertical motions change in correspondence with the differential circulations.The changesin precipitation are directly related to that of vertical motions.The mechanisms of climate effects of the boundaryaerosols are also discussed in this paper.  相似文献   

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