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1.
In the present reported study, the vertical distributions of local atmospheric refractivity were retrieved from ground- based GPS observations at low elevation angles. An improved optimization method was implemented at altitudes of 0-10 km to search for a best-fit refractivity profile that resulted in atmospheric delays most similar to the delays calculated from the observations. A ray-tracing model was used to simulate neutral atmospheric delays corresponding to a given refractivity profile. We initially performed a ＂theoretical retrieval＂, in which no observation data were involved, to verify the optimization method. A statistical relative error of this ＂theoretical retrieval＂ （-2% to 2%） indicated that such a retrieval is effective. In a practical retrieval, observations were obtained using a dual-frequency GPS receiver, and its initial value was provided by CIRA86aQ_UoG data. The statistical relative errors of the practical retrieval range from -3% to 5% were compared with co-located radiosonde measurements, Results clearly revealed diurnal variations in local refractivity prc,files, The results also suggest that the general vertical distribution of refractivity can be derived with a high temporal resolution. However, further study is needed to describe the vertical refractivity gradient clearly. 相似文献
2.
利用1996年3月-2003年6月部分时段拉萨、西宁、北京3个站的臭氧探空资料验证了GOME（Global Ozone Monitoring Experiment）卫星臭氧廓线及对流层臭氧柱总量。对比结果表明:在对流层中下层,拉萨和西宁两地GOME与探空的平均偏差小于5%,北京地区平均偏差小于10%;在对流层上层/平流层下层,拉萨和西宁平均偏差小于10%,北京小于20%;在平流层中上层3个站的平均偏差均小于5%。在对流层上层/平流层下层区域,GOME与臭氧探空的平均偏差在北京明显高于拉萨和西宁。3个地区对流层柱总量的平均偏差都在10%以内,表明该资料可用于研究我国对流层臭氧总量的变化规律。同时段的GOME最低层（0~2.5km）月平均臭氧浓度对比结果显示,GOME结果同地面臭氧观测值有很好的相关性,GOME臭氧浓度反映了拉萨、瓦里关、临安地面臭氧浓度的主要变化特征。 相似文献
3.
In this study, the TOMS/SBUV (Total Ozone Mapping Spectrometer/Solar Backscatter Ultraviolet Radiometer) data and SAGE (Stratospheric Aerosol and Gas Experiment) II data were employed to calculate the monthly total zonal ozone deviations over the Tibetan Plateau and the 150?C50-hPa zonal ozone variations. The results show that there is a significant correlation between the two, with a correlation coefficient of 0.977. From 150 to 50 hPa, the ozone valley over the Tibetan Plateau (OVTP) becomes the strongest based on the SAGE II data, and the South Asian high (SAH) is the most active according to the 40-yr reanalysis data of the European Centre for Medium-Range Weather Forecasts (ERA40), so a correlation between the SAH and the OVTP may exist. The WACCM3 (Whole Atmosphere Community Climate Model version 3) simulation results show that both SAH and OVTP could still present within 150?C50 hPa with reduced strength even when the height of the Tibetan Plateau was cut down to 1500 m. It is also shown that the seasonal variation of SAH would result in a matched seasonal variation of the OVTP, which suggests a meaningful effect of SAH on the OVTP. Meanwhile, it is found that the atmospheric circulation would impose different effects on the OVTP, depending on the SAH??s evolution stages and movement directions. At 150?C50 hPa, as the SAH approaches the plateau, the SAH zonal (meridional) transport would make the OVTP deeper (shallower), while the vertical transport of ozone produces a deeper (shallower) OVTP at the lower (higher) level; the combined dynamic effects lead to a weakened OVTP. When the SAH stabilizes over the plateau, the zonal (meridional) transport results in a shallower (deeper) OVTP while the vertical transport would create a deeper (shallower) OVTP at the middle (bottom and top) levels; the combined dynamic effects produce a deeper OVTP. As the SAH retreats from the plateau, the OVTP becomes deeper (shallower) under the zonal (meridional) effect or shallower under the vertical effect; the combined dynamic effects contribute to a deeper (shallower) OVTP at the middle (bottom and top) levels. The SAH would have a weak effect on the OVTP over the plateau when positioned over the tropical Pacific. 相似文献
4.
北京冬季低层大气O3垂直分布观测结果的研究 总被引：17，自引：7，他引：17
给出了2001年2月26～28日在北京市方庄小区用系留气艇观测大气边界层O3垂直分布的结果.结合相关资料,对边界层O3的变化机制进行了初步分析.研究表明,冬季边界层O3主要受边界层气象条件、尤其是逆温层的影响比较大.在逆温层以下O3都维持极低值分布,超过仪器所能观测的最低极限.在逆温层向自由大气过渡的高度区域,O3浓度明显的梯度变化与风速垂直切变有关.观测还表明冬季城市市区大量排放的氮氧化物、水汽参与的化学反应是影响边界层O3变化的重要因素. 相似文献
5.
Long-term record of global distribution of ozone during 1979 to 2001, from Total Ozone Mapping Spectrometer (TOMS), over a tropical urban environment has been analyzed and compared with ground measurements. Increase in atmospheric UV-absorbing aerosol loading has been observed after 1991. TOMS columnar ozone during 1979 to 2001 suggested a clear Gaussian pattern of minimum concentration in winter months and maximum in summer months. TOMS ozone showed good correlation with the ground measured columnar ozone during winter months and negative correlation with Sunburning Ultraviolet (SUV) (280–370 nm), UVA and aerosol optical depth (AOD). 相似文献
6.
Based on the Stratospheric Aerosol and Gas Experiment (SAGE) II and the Halogen Occultation Experiment (HALOE) ozone profiles and the Total Ozone Mapping Spectrometer (TOMS) total ozone data sets, an empirical model for estimating the vertical distribution of stratospheric ozone over China is proposed. By using this model, the vertical distribution of stratospheric (16–50 km) ozone can be estimated according to latitude, month and total ozone. Comparisons are made between the modeled ozone profiles and the ... 相似文献
7.
国产GPSO3与芬兰Vaisala臭氧探空仪的比对试验 总被引：10，自引：0，他引：10
臭氧探空仪是一种主要而又直接的探测大气臭氧垂直分布的技术手段。为了了解国产GPSO3臭氧探空仪的测量精度、灵敏度和可靠性．我们开展了与芬兰Vaisala ECC臭氧探空仪的系列平行比对试验,包括实验室臭氧传感器比对测试．室外地面臭氧传感器比对测试,低压环境下进气柱塞泵(效)比对测试和臭氧探空施放比对试验。测试结果分析表明,国产GPSO3臭氧探空仪的主要指标性能与国际通用的Vaisala臭氧探空仪的相当。 相似文献
8.
该文介绍了中国科学院大气物理研究所（简称IAP）研制的电化学浓度电池（ECC）型臭氧（O3）探空仪基本性能测试和2013年上半年室外比对观测结果。结果表明:ECC的背景电流（Ibg）在0.1 μA以下或更低;测量O3的响应时间为21~26 s;NO2（SO2）使O3测值偏高（低）;抽气泵低压泵效系数（Cef）在100 hPa高度以下为1.0左右,在该高度以上上升,10 hPa达到1.17±0.10,5 hPa达到1.28±0.16,性能略低于同类进口产品（1.055以下）。国产和进口仪器在气象探空或抽气泵等部件上具有良好兼容性;两者所测O3垂直分布廓线总体一致。IAP O3探空仪O3总量与Brewer光谱仪测值比值为0.9~1.1;Cef和Ibg订正有效降低了IAP O3探空仪在平流层低层与进口仪器测值的差别,这一订正对O3柱浓度在平流层和对流层的贡献分别为约15 DU和4~6 DU;在对流层,IAP O3探空仪测值与进口仪器间的绝对差别稳定且低于0.5 mPa;而平流层受泵效影响较明显。因此,建议IAP O3探空仪提高其Cef的稳定性,参与国际比对测试,国产气象探空平台数据接收处理增加必要的滤波技术以降低平流层探测数据（包括O3）的振荡。 相似文献
9.
10.
In this paper we present first-time measurements of ozone profiles from a high altitude station in Quito, Ecuador (0.19°S, 78.4°W, and 2391 masl) taken from June 2014 to September 2015. We interpret ozone observations in the troposphere, tropopause, and stratosphere through a zonal comparison with data from stations in the Atlantic and Pacific (Natal and San Cristobal from the SHADOZ network). Tropospheric ozone concentrations above the Andes are lower than ozone over San Cristobal and Natal for similar time periods. Ozone variability and pollution layers are also reduced in the troposphere above the Andes. We explain these differences in terms of reduced contributions from the boundary layer and from horizontal transport. In the tropical tropopause layer, ozone is well-mixed up to near the cold point tropopause level. In this regard, our profiles do not show constraints to deep mixing above 14 km, as has been consistently observed at other tropical stations. Total column ozone and stratospheric column ozone are comparable among the three sites. However, the contribution of tropospheric column ozone to total column ozone is significantly lower above the Andes. Our comparisons provide a connection between observations from tropical stations in equatorial South America separated by the wide continental mass. Identified differences in ozone throughout the atmospheric column demonstrate the global benefit of having an ozone sounding station at the equatorial Andes in support of global monitoring networks. 相似文献
11.
I. IntroductionOzone p1ays a very 1mportant ro1e in globa1 climate change. This is particularly true inthe stratosphere, where ultra--v1olet solar radiation is strongly absorbed by ozone, leading tosubstantlal change in the earths atmospheric thermal, physical and chemical structure. Al-though the troposphere contains only about l0% of the total atmospheric ozone, the varia-tlon of tropospheric ozone may have more significant cllmatic effect than stratospheric ozoneon the earth's surface temP… 相似文献
12.
ＴｈｅＣａｐａｂｉｌｉｔｙｏｆＡｔｍｏｓｐｈｅｒｉｃＰｒｏｆｉｌｅＲｅｔｒｉｅｖａｌｆｒｏｍＳａｔｅｌｌｉｔｅＨｉｇｈＲｅｓｏｌｕｔｉｏｎＩｎｆｒａｒｅｄＳｏｕｎｄｅｒＲａｄｉａｎｃｅｓＬｉＪｕｎ（李俊）（Ｃｏｏｐｅｒａｔｉｖｅｉｎｓｔｉｔｕｔｅｆｏ... 相似文献
13.
A two-step method is employed in this study to retrieve vertical ozone profiles using scattered measure- ments from the limb of the atmosphere. The combination of the Differential Optical Absorption Spectroscopy (DOAS) and the Multiplicative Algebraic Reconstruction Technique (MART) is proposed. First, the limb radiance, measured over a range of tangent heights, is processed using the DOAS technique to recover the effective column densities of atmospheric ozone. Second, these effective column densities along the lines of sight (LOSs) are inverted using the MART coupled with a forward model SCIATRAN (radiative transfer model for SCIAMACHY) to derive the ozone profiles. This method is applied to Optical Spectrograph and Infra Red Imager System (OSIRIS) radiance, using the wavelength windows 571-617 nm. Vertical ozone profiles between 10 and 48 km are derived with a vertical resolution of 1 km. The results illustrate a good agreement with the cloud-free coincident SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) ozone measurements, with deviations less than ± 10% ( ± 5% for altitudes from 17 to 47 km). Furthermore, sensitivities of retrieved ozone to aerosol, cloud parameters and NO 2 concentration are also investigated. 相似文献
14.
北极臭氧垂直分布和天气尺度变化的观测研究 总被引：2，自引：0，他引：2
北极地区臭氧对北极气候和环境系统起着重要作用。研究其分布和变化有助于了解北极的气候和环境及其对全球气候系统的影响,有助于气候和环境变化的数值预报。中国北极科学探测1999在北冰洋楚可奇海域成功的进行了大气臭氧观测。通过在中国“雪龙”号破冰船甲板上（于1999年8月18-24日在75°N,160°W附近处）释放大气臭氧探空仪获得了高分辨率的大气垂直结构和臭氧分布资料,可以进行大气尺度的大气臭氧变化研究。分析大气监测资料、TOMS臭氧总量资料和NCEP大气环流资料表明,大气臭氧总量随着对流层顶的低一高一低变化呈高一低一高的变化过程。研究还表明,大气柱的臭氧总量与13公里以下的大气臭氧含量关系密切,而在约20公里处的大气臭氧浓度最大值的变化与整个气柱臭氧的关系不大。500 hPa天气形势图上一个弱一强一弱的西南天气型造成的弱臭氧平流可能是这次臭氧变化的主要原因。 相似文献
15.
Profile data from simultaneous sodar and tethered balloon measurements have been analyzed with respect to the complex structure of the atmospheric boundary layer in the Upper Rhine Valley. Special attention was focused on ozone concentration profiles measured with a novel lightweight ozone sensor at the balloon. In general, good agreement was found between the signature of the ozone concentration profiles and special features of the backscattered sound intensity profiles. This allows reliable estimation of the mixing height from the sodar data even in a complex stable ABL, except for very shallow mixing layers (below about 75 m), which could not be detected by the sodar. 相似文献
16.
WU Xuebao LI Jun ZHANG Fengying ZHAN Wenjian ZHU Yuanjing 《Acta Meteorologica Sinica》2004,18(2):129-140
The Advanced TIROS-N Operational Vertical Sounder(ATOVS) measurements are used to generate the atmospheric parameters,such as temperature and moisture profiles,under both clear and cloudy situations.This paper describes briefly the nonlinear iterative physical retrieval method.By using this retrieval scheme,an experiment has been carried out to retrieve the moisture profiles from ATOVS measurements on the NOAA-16 satellite for July of 2002.ATOVS profile retrieval results are evaluated by root mean square(RMS) differences with respect to RAdiosonde OBservation(RAOB) profiles.The accuracy of the retrieval is about 15%-23% for the relative humidity profile in this study. 相似文献
17.
A Tibetan ozone low was found in the 1990s after the Antarctic ozone hole.Whether this ozone low has been recovering from the beginning of the 2000s following the global ozone recovery is an intriguing topic.With the most recent merged TOMS/SBUV(Total Ozone Mapping Spectrometer/Solar Backscatter Ultra Violet) ozone data,the Tibetan ozone low and its long-term variation during 1979-2010 are analyzed using a statistical regression model that includes the seasonal cycle,solar cycle,quasi-biennial oscillation(QBO),ENSO signal,and trends.The results show that the Tibetan ozone low maintains and may become more severe on average during 1979-2010,compared with its mean state in the periods before 2000,possibly caused by the stronger downward trend of total ozone concentration over the Tibet.Compared with the ozone variation over the non-Tibetan region along the same latitudes,the Tibetan ozone has a larger downward trend during 1979-2010,with a maximum value of-0.40±0.10 DU yr 1 in January,which suggests the strengthening of the Tibetan ozone low in contrast to the recovery of global ozone.Regression analyses show that the QBO signal plays an important role in determining the total ozone variation over the Tibet.In addition,the long-term ozone variation over the Tibetan region is largely affected by the thermal-dynamical proxies such as the lower stratospheric temperature,with its contribution reaching around 10% of the total ozone change,which is greatly different from that over the non-Tibetan region. 相似文献
18.
Ozone vertical column densities (VCDs) were retrieved by Zenith Scattered Light-Differential Optical Absorption Spectroscopy (ZSL-DOAS) from January 2017 to February 2020 over Fildes Peninsula, West Antarctica (62.22°S, 58.96°W). Each year, ozone VCDs started to decline around July with a comparable gradient around 1.4 Dobson Units (DU) per day, then dropped to their lowest levels in September and October, when ozone holes appeared (less than 220 DU). Daily mean values of retrieved ozone VCDs were compared with Ozone Monitoring Instrument (OMI) and Global Ozone Monitoring Experiment 2 (GOME-2) satellite observations and the Modern-Era Retrospective analysis for Research and Applications Version 2 (MERRA-2) reanalysis dataset, with correlation coefficients (R2) of 0.86, 0.94, and 0.90, respectively. To better understand the causes of ozone depletion, the retrieved ozone VCDs, temperature, and potential vorticity (PV) at certain altitudes were analyzed. The profiles of ozone and PV were positively correlated during their fluctuations, which indicates that the polar vortex has a strong influence on stratospheric ozone depletion during Antarctic spring. Located at the edge of polar vortex, the observed data will provide a basis for further analysis and prediction of the inter-annual variations of stratospheric ozone in the future. 相似文献
19.
Sensitivity Studies for Monitoring Tropospheric Ozone from Space Using the Ultraviolet,Visible,and Polarization Bands 
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下载免费PDF全文 The authors analyzed the retrieval sensitivity of tropospheric ozone using simulated the Global Ozone Monitoring Experiment-2 （GOME-2） measurements. The retrieval sensitivity was evaluated by the degree of free- dom for signal （DFS）. The combination of the ultraviolet （UV）, UV polarization （UVPOL）, and visible （VIS） bands enhances DFS of tropospheric ozone and improves the vertical resolution of the retrieved ozone profile. UVPOL reduces the dependence on solar zenith angle, mainly in- creases the sensitivity in upper troposphere. Polarization increased the DFS by 20% on the eastern side of the GOME-2 orbit, with little improvement on the western side because the increase in DFS due to polarization is depend- ent on the relative azimuth angle. The inclusion of the visi- ble band reduces significantly the dependence on viewing geometry, and mainly increases the DFS in the lower tro- posphere （0-6 kin） by a factor of two. It was possible to retrieve several independent pieces of tropospheric ozone information from GOME-2 UV/UVPOL/VIS measure- ments, especially in the lower troposphere. 相似文献
20.
Joonsuk Lee Won Jun Choi Deok Rae Kim Seung-Yeon Kim Chang-Keun Song Jun Suk Hong Youdeog Hong Sukjo Lee 《Asia-Pacific Journal of Atmospheric Sciences》2013,49(3):271-278
Surface erythemal UV radiation is mainly affected by total column ozone, aerosols, clouds, and solar zenith angle. The effect of ozone on the surface UV radiation has been explored many times in the previous studies due to the decrease of ozone layer. In this study, we calculated the effect of aerosols on the surface UV radiation as well as that of ozone using data acquired from Ozone Monitoring Instrument (OMI). First, ozone, aerosol optical depth (AOD), and surface erythemal UVB radiation measured from satellite are compared with those from ground measurements. The results showed that the comparison for ozone was good with r 2 of 0.92. For aerosol, there was difference between satellite measurements and surface measurements due to the insufficient information on aerosol in the retrieval algorithm. The r 2 for surface erythemal UV radiation was high (～0.94) but satellite measurements showed about 30% larger values than surface measurements on average by not considering the effect of absorbing aerosols in the retrieval process from satellite measurements. Radiative amplification factor (RAF) is used to access the effect of ozone and aerosol quantitatively. RAF for ozone was 0.97～1.49 with solar zenith angle. To evaluate the effect of aerosol on the surface UV radiation, only clear-sky pixel data were used and solar zenith angle and total column amount of ozone were fixed. Also, RAF for aerosol was assessed according to the single scattering albedo (SSA) of aerosols. The results showed that RAF for aerosol with smaller SSA (< 0.90) was larger than that for with larger SSA (> 0.90). The RAF for aerosol was 0.09～0.22 for the given conditions which was relatively small compared to that for ozone. However, considering the fact that aerosol optical depth can change largely in time and space while the total column amount of ozone does not change very much, it needs to include the effect of aerosol to predict the variations of surface UV radiation more correctly. 相似文献