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1.
2007年,Ashok等揭示了赤道太平洋区域存在一种三极型分布海表温度异常并称之为厄尔尼诺-Modoki,同时定义了相应的海表温度异常指数EMI（记为IEM）。在此基础上,利用英国哈得来中心逐月海表温度资料、美国NCEP/NCAR月平均再分析数据集、美国国家海洋和大气管理局（NOAA）逐月降水资料（CMAP）,通过在太平洋海表温度异常中扣除厄尔尼诺-Modoki信号后,在Nino1+2区域上定义了东太平洋型海表温度异常指数EPNI（IEPN）。据此,由IEPN和IEM可构成描述热带太平洋海表温度异常变化的一对指数。分析了两个指数相应的海气状态及对海洋性大陆区域气候异常的影响。结果表明,厄尔尼诺-Modoki和东太平洋型海表温度异常及其影响存在显著差异。在北半球夏季,当IEM处于正位相时,热带太平洋海表温度异常呈现“负-正-负”的结构,海洋性大陆大部分区域海表温度异常为负,此时对流层低层太平洋地区辐合,海洋性大陆地区辐散,对流层高层太平洋地区辐散,海洋性大陆地区辐合。对应于辐合辐散中心,存在着自赤道中太平洋分别向赤道东太平洋和海洋性大陆中东部地区的异常垂直环流圈,同时也存在自海洋性大陆西部向印度洋西部的垂直环流。大气在海洋性大陆区域北部加热,南部冷却;在太平洋地区西部加热而东部冷却;在海洋性大陆区域10°N以南降水偏少,而10°N以北降水偏多。当IEPN处于正位相时,热带太平洋海表温度异常呈现“西负东正”分布型,海洋性大陆区域海表温度异常呈现“西正东负”分布,对流层低层海洋性大陆地区辐散中心范围偏大、位置偏东、强度偏强,太平洋地区辐合中心范围偏小、位置偏东,热带环流异常在垂直方向上呈斜压结构,海洋性大陆区域北部大气加热而南部冷却,太平洋地区大气均呈加热正异常,海洋性大陆大部分区域降水均偏少,赤道太平洋降水偏多。以上这些结果有利于深刻理解热带太平洋海表温度异常的特征及其对海洋性大陆区域气候的影响。 相似文献
2.
利用1979-2015年NCEP/NCAR月平均再分析资料、美国国家海洋和大气管理局（NOAA）的月平均降水资料（CMAP）以及英国哈得来中心海表温度月平均资料,采用2009年Kao等定义的中部型ENSO指数,给出了夏季中部型海表温度（SST）异常指数,并分析了中部型ENSO和海洋性大陆（MC）区域气候的联系。结果表明,当夏季中部型海表温度正异常事件发生时,海洋性大陆核心区域（中太平洋）出现显著降水和气温负（正）异常,此时海洋性大陆核心区域有明显的负（正）热源异常,大气受冷却（加热）而下沉（上升）,同时潜热释放之外的非绝热加热表现为负（正）异常,易于导致降水负（正）异常。海洋性大陆区域与中太平洋间主要通过水平环流和垂直环流建立联系。（1）中部型ENSO指数显著正异常时,在对流层低（高）层,海洋性大陆区域和中太平洋间存在由关于赤道的对称气旋性（反气旋性）环流对而形成的直接联系,并使得海洋性大陆区域东部辐散（辐合）偏弱,而海洋性大陆区域西部辐散（辐合）偏强。（2）在垂直剖面上,赤道中太平洋海表温度的正异常和海洋性大陆核心区域的大气异常冷却有利于促使该地区低层赤道西风异常增强并进而利于中部型海表温度正异常的维持,并由此通过反沃克环流圈促进海洋性大陆区域下沉运动增强。此为海洋性大陆与中太平洋间的直接联系,可由皮叶克尼斯机制进行解释。而位于中太平洋与秘鲁地区的异常垂直环流亦可用这一机制进行解释。海洋性大陆与中太平洋的间接联系主要表现在由赤道外低纬和中纬度地区均存在的沿弧形路径上的垂直环流而建立的海洋性大陆与中太平洋地区的联系上。这些弧形垂直剖面上的垂直环流不仅与局地哈得来环流有关,还与热带和中纬度的罗斯贝波动有关。这些结果有利于深刻认识中部型ENSO对海洋性大陆区域气候的影响机理以及与热带外环流异常的联系。 相似文献
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利用1979—2019年Hadley中心的海表温度资料、GPCP的降水资料以及NCEP-DOE的再分析资料等,分析了北半球春季热带南大西洋海表温度异常与北半球夏季亚澳季风区降水异常的联系。研究表明,北半球春季热带南大西洋海表温度异常与随后夏季热带西太平洋到南海（澳大利亚东侧海域到热带东印度洋）地区的降水异常为显著负相关（正相关）关系。北半球春季热带南大西洋的海表温度正异常可以引起热带大西洋和热带太平洋间的异常垂直环流,其中异常上升支（下沉支）位于热带大西洋（热带中太平洋）。热带中太平洋的异常下沉气流和低层辐散气流引起热带中西太平洋低层的异常东风,后者有利于热带中东太平洋海表温度出现负异常。通过Bjerknes正反馈机制,热带中东太平洋海表温度异常从北半球春季到夏季得到发展。热带中东太平洋海表温度负异常激发的Rossby波使得北半球夏季热带西太平洋低层出现一对异常反气旋。此时,850 hPa上热带西太平洋到海洋性大陆地区为显著的异常东风,有利于热带西太平洋到南海（澳大利亚东侧海域到热带东印度洋）地区出现异常的水汽辐散（辐合）,导致该地区降水减少（增加）。 相似文献
4.
夏季印度洋海盆模与MC区域降水异常联系的进一步分析 总被引：1，自引：0，他引：1
利用英国哈德莱中心的逐月海表温度资料及NCEP/NCAR月平均再分析资料等,通过在印度洋海盆模IOBM指数(IIOB)中扣除长期趋势和两类ENSO的同期信号后,得到了修正的IOBM指数(Im IOB),并由此分析了IOBM的变化及与海洋性大陆区域降水异常的联系。结果表明:印度洋IOBM为暖位相时,不同季节的印度洋地区均呈现异常偏暖,但大气是上升还是下沉运动则在印度洋不同季节和不同区域存在很大变化。就夏季而言,印度洋大部分地区存在上升运动,这与海温异常偏暖有关。在北半球夏季,指数Im IOB存在3~5 a的周期变化。当IOBM处于正位相时,印度洋至我国东海地区大范围海温偏暖。MC(Maritime Continent,海洋性大陆)区域西部降水正异常,而MC区域东北部降水为负异常。造成这种降水分布的原因是:当指数为正时,在MC区域的西部对流层低层辐合、高层辐散,上升运动增强,且水汽辐合,而MC区域的东北部对流层低层辐散、高层辐合,上升运动不明显,水汽辐散,不易形成降水。而在对流层低层与西太平洋辐散中心对应,南北半球出现关于赤道对称的反气旋对,赤道印度洋上的异常加热激发东传的Kelvin波,加强东风异常,同时加强了KMC(海洋性大陆的核心区域)之外南北半球热带地区的这对Rossby波型。以上这些结果有利于深刻理解MC降水异常成因及热带海陆气相互作用过程。 相似文献
5.
利用美国国家海洋和大气管理局(NOAA)向外长波辐射(OLR)月平均资料、欧洲中期数值预报中心(ECMWF)ERA-interim月平均再分析资料、全球降水气候中心(GPCC)降水资料及中国气象局国家气象信息中心提供的中国756站逐日观测资料,通过定义一个海洋性大陆区域对流强度指数(IOLR),分析了海洋性大陆区域(Maritime Continent,MC)近35年来11月—次年1月对流活动特征,并揭示了11月—次年1月海洋性大陆区域对流活动强度的年际变化与同期云贵高原降水的联系。结果表明:海洋性大陆区域对流活动除了有逐渐增强的趋势外,还存在3—5 a及8—10 a的振荡周期。当海洋性大陆区域对流活动偏弱(强)时,云贵高原西部降水偏少(多),东部降水偏多(少),高原东西部之间降水分布差异加大(减小)。引起云贵高原降水异常的原因有3个方面:一是在海洋性大陆区域与云贵高原间存在显著的异常垂直环流圈,当下沉(上升)支位于海洋性大陆区域时,上升(下沉)支将位于云贵高原地区。而云贵高原地形可能对云贵高原降水异常在东南部和西北部的差别的产生存在影响;二是海洋性大陆区域在对流层低层的辐散和对流层上层的辐合运动为热带和高原以东地区提供了异常的位涡强迫,直接导致对流层低层南海—孟加拉湾地区异常反气旋和对流层上层位于中国南方的异常气旋性环流的产生;三是由于海洋性大陆区域辐散运动作为位涡制造而激发的位涡扰动的能量从热带地区向云贵高原及其东侧频散并辐合,对云贵高原上空扰动异常的维持起到了重要作用。这些结果有利于深刻理解云贵高原冬季降水异常的形成机理以及为寻找降水异常预测因子提供了有用的线索。 相似文献
6.
利用1963—2013年Hadley中心月平均海表温度资料,以及NCEP/NCAR再分析资料,根据两类厄尔尼诺事件发生时北半球冬季赤道太平洋地区海温异常的不同空间分布特征,即赤道中太平洋CP型和东太平洋EP型海温异常空间分布,从寻找与之相似的空间型角度出发,设计了一组新的海温异常指数I_(CP)和I_(EP)。与以往ENSO指数相比,新指数组I_(CP)和I_(EP)不仅表示了空间上相互独立的海温异常分布,而且在相同的研究时段内,因时间域上相互独立而能更好地表征和区分两类El Ni?o/La Ni?a事件。据此,采用该新指数组探讨了与中部型和东部型海温异常事件相关的热带太平洋的主要海气耦合特征。结果表明,与传统的东部型El Ni?o事件发生时最大暖海温中心位于赤道东太平洋地区不同,中部型El Ni?o事件,异常增暖中心位于赤道中太平洋。中部型时异常Walker环流的上升支向西偏移,异常降水集中于热带中太平洋,不似东部型时异常限定于赤道东太平洋地区。不论哪类事件,海洋性大陆均可受到影响,即CP或EP型El Ni?o发生时,海洋性大陆区域降水偏少。但比较而言,中部型ENSO对海洋性大陆区域的影响更大。 相似文献
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利用美国NOAA卫星观测的SOI(Southern Oscillation Index,南方涛动指数)资料以及NCEP/NCAR、CMAP月平均资料,采用相关分析等方法,研究了南方涛动年际变化与夏季亚澳季风环流及海洋性大陆区域气候异常的联系。结果表明:南方涛动具有显著的年际变化特征,这种年际变化对夏季亚澳季风区及海洋性大陆区域的环流、降水及温度异常有重要影响。当SOI正位相时,赤道以南的澳大利亚东部地区以及西北太平洋海域高层为气旋,低层为反气旋,赤道地区的东部太平洋低层为辐散中心,高层为辐合中心,有利于下沉运动维持;加里曼丹岛附近低层辐合,高层辐散,有利于上升运动维持;海洋性大陆地区降水为显著的正异常,东亚地区降水存在较弱的正异常;海洋性大陆地区以及我国青藏高原到东海一带温度为正异常,孟加拉湾及印度半岛区域温度为负异常。 相似文献
8.
赤道东太平洋海温正异常对西太平洋副高影响的数值模拟研究 总被引：10，自引：0，他引：10
利用LASG九层大气环流谱模式及IAP两层大气环流模式，模拟研究了不同持续时间的赤道东太平洋海表温度正异常(海表温度异常的持续时间分别为1月份，1～2月份，1～4月份及1～8月份，其他月份为气候SST)对西太平洋副高的影响。结果表明，尽管海表温度异常的持续时间不同，但其引起的西太平洋副高的异常演变及其分布却十分相似；同时，季风区的异常降水(进而异常潜热释放)随时间的演变及其分布也存在一定的相似性(对应于不同持续时间的赤道东太平洋的海表温度正异常，5月份印度洋至西太平洋地区都表现出赤道辐合带北移偏晚的特征)；季风区降水的这种变化同西太平副高的异常是一致的，从而揭示出这两种现象有可能存在着某种联系。结果还表明，导致这种大气响应场对赤道东太平洋海表温度异常持续时间不敏感的一个重要原因是大气内部过程的影响:中纬大气的内部Rossby波源维持了热带地区激发的扰动在中高纬的存在，同时大气内部Rossby波源对赤道太平洋地区的海表温度异常持续时间表现出不敏感性，正是由于这种不敏感性才导致了响应场对赤道太平洋地区海表温度异常持续时间的不敏感性。模拟结果还表明，在夏季赤道东太平洋存在海表温度正异常的情况，尽管大气内部动力过程的作用十分重要，但夏季赤道东太平洋海表温度正异常对夏季西太平洋副高的影响却明显存在，因此，基于赤道太平洋地区海表温度异常的夏季西太平洋副高的可预报性受到赤道东太平洋海表温度正异常及大气内部动力过程的双重影响。模式的依赖性研究表明，模拟结果具有一定的普遍性。 相似文献
9.
利用Hadley中心的海表温度资料、全国160站降水资料以及NCEP-DOE AMIP-Ⅱ再分析等资料,运用多种统计分析方法,分析了春季（3—5月）热带大西洋北部海温异常变化特征及其对我国盛夏（7、8月）降水异常的影响。结果表明:春季热带大西洋北部模态是热带大西洋海温异常REOF分解的第一模态,方差贡献率为34.5%。热带大西洋北部海温异常年际变率具有明显的季节差异,其中春季最为显著。春季热带大西洋北部海温异常与我国盛夏华中地区降水异常有显著的正相关关系。进一步分析表明,春季热带大西洋北部的海温正异常可以激发出Rossby波,在热带大西洋西北部和热带东太平洋北部产生异常的气旋式环流,引起上述区域的对流层低层（上层）大气出现异常辐合（辐散）,并通过热带大西洋北部地区和太平洋之间的垂直环流异常,在中太平洋地区对流层低层大气出现异常辐散,有利于西北太平洋地区产生异常反气旋式环流,异常反气旋西北侧的西南气流有利于水汽输送至我国华中地区,使该地区降水偏多。且这种影响可以通过热带大西洋北部海温异常的持续性,从春季一直持续到盛夏。 相似文献
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基于低阶大气环流谱模式，本文设计了太平洋及印度洋4个不同海域的海表温度异常试验，去研究大气环流及降水对热带海表温度异常强迫作用的“同时”性响应。结果表明尽管暖性的海表温度异常均激发出低空辐合及高空辐散，但在不同海域所激发的异常流场却差异甚大。不过降水异常均发生在海表温度异常区及其毗邻处。它在对称的SSTA区的分布一般是非对称的。对水汽收支的分解分析表明，海表温度异常区异常降水的大小主要由异常的低空辐合决定，而异常降水的分布形态则由异常的水汽平流过程所决定。由于异常的低空辐合及异常的水汽平流过程主要发生在海 相似文献
11.
Yanjun Ma Hujia Zhao Yunsheng Dong Huizheng Che Xiaoxiao Li Ye Hong Xiaolan Li Hongbin Yang Yuche Liu Yangfeng Wang Ningwei Liu Cuiyan Sun 《Acta Meteorologica Sinica》2018,32(2):313-323
This study analyzes and compares aerosol properties and meteorological conditions during two air pollution episodes in 19–22 (E1) and 25–26 (E2) December 2016 in Northeast China. The visibility, particulate matter (PM) mass concentration, and surface meteorological observations were examined, together with the planetary boundary layer (PBL) properties and vertical profiles of aerosol extinction coefficient and volume depolarization ratio that were measured by a ground-based lidar in Shenyang of Liaoning Province, China during December 2016–January 2017. Results suggest that the low PBL height led to poor pollution dilution in E1, while the high PBL accompanied by low visibility in E2 might have been due to cross-regional and vertical air transmission. The PM mass concentration decreased as the PBL height increased in E1 while these two variables were positively correlated in E2. The enhanced winds in E2 diffused the pollutants and contributed largely to the aerosol transport. Strong temperature inversion in E1 resulted in increased PM2.5 and PM10 concentrations, and the winds in E2 favoured the southwesterly transport of aerosols from the North China Plain into the region surrounding Shenyang. The large extinction coefficient was partially attributed to the local pollution under the low PBL with high ground-surface PM mass concentrations in E1, whereas the cross-regional transport of aerosols within a high PBL and the low PM mass concentration near the ground in E2 were associated with severe aerosol extinction at high altitudes. These results may facilitate better understanding of the vertical distribution of aerosol properties during winter pollution events in Northeast China. 相似文献
12.
A better knowledge of aerosol properties is of great significance for elucidating the complex mechanisms behind frequently occurring haze pollution events. In this study, we examine the temporal and spatial variations in both PM_1 and its major chemical constituents using three-year field measurements that were collected in six representative regions in China between 2012 and 2014. Our results show that both PM_1 and its chemical compositions varied significantly in space and time, with high PM_1 loadings mainly observed in the winter. By comparing chemical constituents between clean and polluted episodes, we find that the elevated PM_1 mass concentration during pollution events should be largely attributable to significant increases in organic matter(OM) and inorganic aerosols like sulfate, nitrate, and ammonium(SNA),indicative of the critical role of primary emissions and secondary aerosols in elevating PM_1 pollution levels. The ratios of PM_1/PM_(2.5) are found to be generally high in Shanghai and Guangzhou, while relatively low ratios are seen in Xi'an and Chengdu, indicating anthropogenic emissions were more likely to accumulate in forms of finer particles. With respect to the relative importance of chemical components and meteorological factors quantified via statistical modeling practices, we find that primary emissions and secondary aerosols were the two leading factors contributing to PM_1 variations, though meteorological factors also played important roles in regulating the dispersion of atmospheric PM. 相似文献
13.
利用气象模式WRF驱动区域空气质量模式RAQMS,模拟研究了2014年北京地区春季颗粒物及气溶胶化学组分的时空变化,对比分析了沙尘期（3月17日、29日）和霾期（3月25～27日）的天气形势、气象要素和气溶胶化学组分特征,比较了沙尘和人为气溶胶表面非均相化学反应对大气化学成分的影响及相对贡献。结果显示,模式对于气象要素、PM2.5、PM10及其化学组分具有较好的模拟能力,考虑了气溶胶表面非均相化学反应后明显提高了模式对PM2.5及气溶胶化学组分模拟的准确性。沙尘期间,沙尘对PM10质量浓度贡献占主导地位（50.7%）,对PM2.5的贡献与有机气溶胶（OM）和人为排放的一次颗粒物（PPM）相当;霾期间,硝酸盐NO3?（25.6%）和OM（23.6%）对PM2.5的贡献最大,在PM10中NO3?、PPM和OM的贡献相当。沙尘期,粗粒子明显增加,在PM10中所占比例与细粒子相当,为45.5%;霾期,细粒子占主导地位,占PM10质量浓度的85.6%。非均相化学反应使沙尘期间硫酸盐（SO42–）和NO3–浓度分别增加16.9%和83.8%,使霾期间的SO42?和NO3–浓度分别增加14.5%和45.0%。2014年3月,非均相化学反应使北京月均SO2、NO2、O3、SO42?、NH4+和NO3?的浓度分别变化了?2.5%、?5.7%、?3.4%、11.7%、18.6%和58.5%,本文结果表明非均相化学反应对二次无机气溶胶的生成有重要贡献。 相似文献
14.
Roeland Cornelis Jansen Yang Shi Jianmin Chen YunJie Hu Chang Xu Shengmao Hong Jiao Li Min Zhang 《大气科学进展》2014,31(6):1427-1434
This paper explores the role of the secondary inorganic aerosol （SIA） species ammonium,NH4＋,nitrate,NO3-,and sulfate,SO24-,during haze and fog events using hourly mass concentrations of PM2.5 measured at a suburban site in Hangzhou,China.A total of 546 samples were collected between 1 April and 8 May 2012.The samples were analyzed and classified as clear,haze or fog depending on visibility and relative humidity （RH）.The contribution of SIA species to PM2.5 mass increased to ～50％ during haze and fog.The mass contribution of nitrate to PM2.5 increased from 11％ during clear to 20％ during haze episodes.Nitrate mass exceeded sulfate mass during haze,while near equal concentrations were observed during fog episodes.The role of RH on the correlation between concentrations of SIA and visibility was examined,with optimal correlation at 60％-70％ RH.The total acidity during clear,haze and fog periods was 42.38,48.38 and 45.51 nmol m-3,respectively,indicating that sulfate,nitrate and chloride were not neutralized by ammonium during any period.The nitrate to sulfate molar ratio,as a function of the ammonium to sulfate molar ratio,indicated that nitrate formation during fog started at a higher ammonium to sulfate molar ratio compared to clear and haze periods.During haze and fog,the nitrate oxidation ratio increased by a factor of 1.6-1.7,while the sulfur oxidation ratio increased by a factor of 1.2-1.5,indicating that both gaseous NO2 and SO2 were involved in the reduced visibility. 相似文献
15.
N. Galindo J.F. Nicols E. Yubero S. Caballero C. Pastor J. Crespo 《Atmospheric Research》2008,88(3-4):305-313
The present study was carried out between October 2003 and September 2004 at an urban background station near the Mediterranean coast in southeastern Spain. The sulfate and nitrate content was determined in 332 PM10 and PM2.5 daily samples. The results show that the seasonal variation of nitrate measured in PM10 does not correspond with what has been observed at other locations in the Iberian Peninsula, where the minima are reached during the summer months due to decomposition of ammonium nitrate at high temperatures. The recorded levels of PM10 nitrate were slightly higher in summer due to an increase in the concentrations of coarse mode nitrate. On the contrary, both the concentrations and the percentages of nitrate in PM2.5 were lowest from June to September. The sulfate levels in both PM10 and PM2.5 were maxima in summer because the oxidation rate of SO2 increases with solar radiation. An elevated correlation (0.72 < r < 0.92) between the monthly average concentrations and percentages of sulfate and solar radiation has been found. We have also investigated the influence that Saharan dust intrusions and high pollution episodes have upon the sulfate and nitrate concentrations. Both types of events increased NO3− and SO42− levels, particularly the high pollution episodes. 相似文献
16.
To investigate chemical profiles and formation mechanisms of aerosol particles in winter haze events,comprehensive measurements including hourly concentrations of PM2.5 and water-soluble inorganic ions and related gasphase precursors were conducted via an online monitoring system from January to March of 2016 in Shenzhen, a coastal mega-city in south China. In this study, high concentrations of PM2.5, NO2 and lower levels of O3 were observed during haze periods in comparison with clear days(Visibility15 km). The major secondary ionic species were NH+4、NO-3 and SO2-4, which varied significantly on haze and clear days. The ratio of NO-3/SO2-4 in haze days was greater than that on clear days and tended to be larger when air pollution became more serious. At the same time, compared with previous studies, it has been found that the ratio has been increasing gradually in Shenzhen, indicating that the motor vehicle exhaust emissions have a more and more important impact on air quality in Shenzhen. Sulfur oxidation rate(SOR) and nitrogen oxidation rate(NOR) was higher during the haze period than that in clean days, indicating efficient gas to particle conversion. Further analysis shows that high concentrations of sulfate might be explained by aqueous oxidation,but gas-phase reactions might dominate nitrate formation. This study also highlights that wintertime nitrate formation can be an important contributor to aerosol particles, especially during haze periods. 相似文献
17.
Junting Zhong Xiaoye Zhang Yaqiang Wang Junying Sun Yangmei Zhang Jizhi Wang Kaiyan Tan Xiaojing Shen Haochi Che Lu Zhang Zhouxiang Zhang Xuefei Qi Huarong Zhao Sanxue Ren Yang Li 《Acta Meteorologica Sinica》2017,31(5):809-819
Based on observations of urban mass concentration of fine particulate matter smaller than 2.5 μm in diameter (PM2.5), ground meteorological data, vertical measurements of winds, temperature, and relative humidity (RH), and ECMWF reanalysis data, the major changes in the vertical structures of meteorological factors in the boundary layer (BL) during the heavy aerosol pollution episodes (HPEs) that occurred in winter 2016 in the urban Beijing area were analyzed. The HPEs are divided into two stages: the transport of pollutants under prevailing southerly winds, known as the transport stage (TS), and the PM2.5 explosive growth and pollution accumulation period characterized by a temperature inversion with low winds and high RH in the lower BL, known as the cumulative stage (CS). During the TS, a surface high lies south of Beijing, and pollutants are transported northwards. During the CS, a stable BL forms and is characterized by weak winds, temperature inversion, and moisture accumulation. Stable atmospheric stratification featured with light/calm winds and accumulated moisture (RH > 80%) below 250 m at the beginning of the CS is closely associated with the inversion, which is strengthened by the considerable decrease in near-surface air temperature due to the interaction between aerosols and radiation after the aerosol pollution occurs. A significant increase in the PLAM (Parameter Linking Aerosol Pollution and Meteorological Elements) index is found, which is linearly related to PM mass change. During the first 10 h of the CS, the more stable BL contributes approximately 84% of the explosive growth of PM2.5 mass. Additional accumulated near-surface moisture caused by the ground temperature decrease, weak turbulent diffusion, low BL height, and inhibited vertical mixing of water vapor is conducive to the secondary aerosol formation through chemical reactions, including liquid phase and heterogeneous reactions, which further increases the PM2.5 concentration levels. The contribution of these reaction mechanisms to the explosive growth of PM2.5 mass during the early CS and subsequent pollution accumulation requires further investigation. 相似文献
18.
Yu Zheng Huizheng Che Leiku Yang Jing Chen Yaqiang Wang Xiangao Xia Hujia Zhao Hong Wang Deying Wang Ke Gui Linchang An Tianze Sun Jie Yu Xiang Kuang Xin Li Enwei Sun Dapeng Zhao Dongsen Yang Zengyuan Guo Tianliang Zhao Xiaoye Zhang 《Acta Meteorologica Sinica》2017,31(6):1045-1061
The optical and radiative properties of aerosols during a severe haze episode from 15 to 22 December 2016 over Beijing, Shijiazhuang, and Jiaozuo in the North China Plain were analyzed based on the ground-based and satellite data, meteorological observations, and atmospheric environmental monitoring data. The aerosol optical depth at 500 nm was < 0.30 and increased to > 1.4 as the haze pollution developed. The Ångström exponent was > 0.80 for most of the study period. The daily single-scattering albedo was > 0.85 over all of the North China Plain on the most polluted days and was > 0.97 on some particular days. The volumes of fine and coarse mode particles during the haze event were approximately 0.05–0.21 and 0.01–0.43 μm3, respectively—that is, larger than those in the time without haze. The daily absorption aerosol optical depth was about 0.01–0.11 in Beijing, 0.01–0.13 in Shijiazhuang, and 0.01–0.04 in Jiaozuo, and the average absorption Ångström exponent varied between 0.6 and 2.0. The aerosol radiative forcing at the bottom of the atmosphere varied from –23 to –227,–34 to –199, and –29 to –191 W m–2 for the whole haze period, while the aerosol radiative forcing at the top of the atmosphere varied from –4 to –98, –10 to –51, and –21 to –143 W m–2 in Beijing, Shijiazhuang, and Jiaozuo, respectively. Satellite observations showed that smoke, polluted dust, and polluted continental components of aerosols may aggravate air pollution during haze episodes. The analysis of the potential source contribution function and concentration-weighted trajectory showed that the contribution from local emissions and pollutants transport from upstream areas were 190–450 and 100–410 μg m–3, respectively. 相似文献
19.
Frank Drewnick Johannes Schneider Silke S. Hings Nele Hock Kevin Noone Admir Targino Silke Weimer Stephan Borrmann 《Journal of Atmospheric Chemistry》2007,56(1):1-20
The Aerodyne aerosol mass spectrometer (Q-AMS) was coupled with a counterflow virtual impactor (CVI) for the first time to measure cloud droplet residuals of warm tropospheric clouds on Mt. Åreskutan in central Sweden in July 2003. Operating the CVI in different operational modes generated mass concentration and species-resolved mass distribution data for non-refractory species of the ambient, interstitial, and residual aerosol. The ambient aerosol measurements revealed that the aerosol at the site was mainly influenced by long-range transport and regional photochemical generation of nitrate and organic aerosol components. Four different major air masses were identified for the time interval of the experiment. While two air masses that approached the site from northeastern Europe via Finland showed very similar aerosol composition, the other two air masses from polar regions and the British Islands had a significantly different composition. During cloud events the larger aerosol particles were found to be activated into cloud droplets. On a mass basis the activation cut-off diameter was approximately 150 nm for nitrate and organics dominated particles and 200 nm for sulfate dominated particles. Generally nitrate and organics were found to be activated into cloud droplets with higher efficiency than sulfate. While a significant fraction of the nitrate in ambient particles was organic nitrates or nitrogen-containing organic species, the nitrate found in the cloud droplet residuals was mainly ammonium nitrate. After passage of clouds the ambient aerosol size distribution had shifted to smaller particle sizes due to the predominantly activation of larger aerosol particles without a significant change in the relative composition of the ambient aerosol. 相似文献
20.
Field data on the ion composition and mass
concentration of aerosol in the rural (Wingene) and urban (Antwerp)
regions of Belgium and the results of their thermodynamic analysis are
presented. Ammonium nitrate and ammonium sulfate are found to be the
major water-soluble components of aerosol particles. The seasonal
variability of mass concentration, phase state, and ion composition of
aerosol particles is largely determined by variations in temperature and
relative humidity. It is shown that the content of ammonium nitrate and
ammonium sulfate in PM2.5 is close to their thermodynamic
equilibrium concentrations. 相似文献