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1.
The characteristics of atmospheric aerosols in the Golmud desert over the Tibetan (Qinghai-Xizang) Plateau are investigated using the measurements made during the QXPMEX-79.Using spectroscopic observations at the surface and satellite data,the aerosol optical depth is calculated,from which the aerosol size distribution is worked out by means of an inversion method.The effects of vertical distribution of aerosols on irradiance and heating rate profiles are investigated using radiation models in conjunction with the assumption of three idealized aerosol profiles.The effect of aerosols on solar irradiance at the surface is also investigated and the results are compared with the observations.It is shown that the solar irradiance can be reduced by up to 100 W m-2 in the presence of aerosols,and the heating rate can be increased by 1 Kd-1. 相似文献
2.
Francisco P. J. Valero Thomas P. Ackerman Warren J. Y. Gore 《Journal of Atmospheric Chemistry》1989,9(1-3):225-244
The interaction of the Aretic winter aerosol (Arctic haze) with solar radiation produces changes in the radiation field that result in the enhancement of scattering and absorption processes which alter the energy balance and solar energy distribution in the Arctic atmosphere-surface system. During the second Arctic Gas and Aerosols Sampling Project (AGASP II) field experiment, we measured radiation parameters using the NOAA WP-3D research aircraft as a platform. State-of-the-art instrumentation was used to measure in situ the absorption of solar radiation by the Arctic atmosphere during severe haze events. Simultaneously with the absorption measurements, we determined optical depths, and total, direct, and scattered radiation fields. All optical measurements were made at spectral bands centered at 412, 500, 675, and 778 nm and with a bandpass of 10 nm. With this selection of spectral regions we concentrated on the measurement of the radiative effects of the aerosol excluding most of the contributions by the gaseous components of the atmosphere. An additional measurement performed during these experiments was the determination of total solar spectrum fluxes. The experimentally determined parameters were used to define an aerosol model that was employed to deduce the absorption by the aerosols over the full solar spectrum and to calculate atmospheric heating rate profiles. The analyses summarized above allowed us to deduce the magnitude of the change in some important parameters. For example, we found changes in instantaneous heating rate of up to about 0.6 K/day. Besides the increased absorption (30 to 40%) and scattering of radiation by the atmosphere, the haze reduces the surface absorption of solar energy by 6 to 10% and the effective planetary albedo over ice surfaces by 3 to 6%. The vertical distribution of the absorbing aerosol is inferred from the flux measurements. Values for the specific absorption of carbon are found to be around 6 m2/g for externally mixed aerosol and about 11.7 m2/g for internally mixed aerosol. A complete study of the radiative effects of the Arctic haze should include infrared measurements and calculations as well as physics of the ice, snow, and water surfaces. 相似文献
3.
The aerosol optical depth of the atmospheric boundary layer was determined both from direct solar irradiance measurements and from vertical extrapolation of ground-based nephelometry, during a period with cloudless skies and high aerosol mass loadings in the Netherlands. The vertical profile of the aerosol was obtained from lidar measurements. From humidity controlled nephelometry at the ground and humidity profiles from soundings, the scattering aerosol extinction as a function of height was assessed. Integration of the extinction over the aerosol layer gave the aerosol optical depth of the atmospheric boundary layer. This optical depth at the narrow band of the nephelometer was translated to a spectrally integrated value, assuming an Angstrom wavelength exponent of 1.5, a typical value for The Netherlands.It was found that scattering by the boundary layer aerosol contributed on average 80% to the total atmospheric aerosol optical depth. The uncertainty in this value is estimated to be of the order of 13%. Ammonium nitrate dominated the light scattering. This is an anthropogenic aerosol component.The radiative forcing caused by the light scattering of the anthropogenic aerosol was calculated assuming an upward scattered fraction of 0.3. An average value of − 12 W m −2 was found (with an estimated uncertainty of 20%). This corresponds to an absolute increase in the planetary albedo of 0.03, which is equivalent to a 15% increase in the local planetary albedo of 0.2. 相似文献
4.
U. Feister 《Journal of Atmospheric Chemistry》1994,19(3):289-315
Solar ultraviolet radiation at the surface has been measured at Potsdam on cloudless days by spectrometer OL 752/10. The measurements are compared with broad-band filter measurements and with model calculations using a modified version of Green's model, which is independent of the measurements. Input data to the model such as atmospheric ozone and aerosol optical thicknesses were measured by a Dobson and Brewer spectrophotometer as well as a Linke Feussner pyrheliometer, respectively. Differences between the model and the measurements are discussed in terms of uncertainties in the calibration and errors of instruments as well as uncertainties in the model calculations including the errors of input data. It is demonstrated that different chemically and biologically effective radiances can be determined from only one set of measured spectral irradiance components, i.e. global radiation and diffuse downward and upward directed radiation. Examples of diurnal variations of the photochemical production of ozone and hydroxyl radicals as determined from spectral irradiance measurements and measured concentrations of relevant trace gases are given.It is shown from the measured irradiance that relations between different effects of radiation to the biosphere depend on solar zenith angle, and to a certain extent also on atmospheric ozone. This has to be taken into account when adverse effects of changing UV radiation are evaluated. Radiation Amplification Factors derived from measurements correspond to those determined from model calculations. 相似文献
5.
The aerosol optical depth of the atmosphere obtained from spectral sun photometer measurements and the integral optical depth determined from standard actinometric observations of direct solar radiation are the parameters of the optical state of the atmosphere. The quantitative estimates of the integral transparency and aerosol optical depth of the atmosphere in Antarctica are presented, their long-term variability over the entire period of observations is analyzed. The comparison of obtained data with the estimates for other natural regions and conditions revealed that during the periods without the impact of volcanic eruptions, the levels of atmospheric aerosol turbidity in Antarctica over the recent decades are minimal on the planet and can be considered as global background characteristics. 相似文献
6.
K. V. S. Badarinath Shailesh Kumar Kharol V. Krishna Prasad Anu Rani Sharma E. U. B. Reddi H. D. Kambezidis D. G. Kaskaoutis 《Journal of Atmospheric Chemistry》2008,59(3):219-236
Measurements of total ozone column and solar UV radiation under different atmospheric conditions are needed to define variations
of both UV and ozone and to study the impact of ozone depletion at the Earth’s surface. In this study, spectral and broadband
measurements of UV-B irradiance were obtained along with total ozone observations and aerosol optical depth measurements in
the tropical urban region of Hyderabad, south India. We specifically used an Ultra-Violet Multifilter Rotating Shadow band
Radiometer (UVMFR-SR), to measure UV irradiance in time and space. To assess the aerosol and O3 effects on ground-reaching UV irradiance, we used measurements from a Microtops II sun photometer in addition to the Tropospheric
Ultraviolet Visible radiation (TUV) model. We also assessed the Defense Meteorological Satellite Program – Operational Line
Scanner (DMSP-OLS) night time satellite data for inferring biomass burning fires during the study period. Results clearly
suggested a negative correlation between the DMSP-OLS satellite derived fire count data and UVMFR-SR data suggesting that
aerosols from biomass burning are directly attenuating UV irradiance in the study region. Also, correlation analysis between
UV index and ozone measurements from sun photometer and TOMS-Ozone Mapping Instrument (OMI) indicated a clear decrease in
ground reaching UV-B irradiance during higher ozone conditions. The higher levels are attributed to photochemical production
of O3 during the oxidation of trace gases emitted from biomass burning. Results also suggested a relatively high attenuation in
UV irradiance (~6% higher) from smoke particles than dust. We also found a relatively good agreement between the modeled (TUV)
and measured UV irradiance spectra for different atmospheric conditions. Our results highlight the factors affecting UV irradiance
in a tropical urban environment, south India. 相似文献
7.
8.
以较为精确的大气辐射传输模式为基础,研制出晴天地表总辐射和净辐射瞬时值的计算方案。与以往的经验计算方法不同,该方案将辐射传输带模式的思路引入地面太阳辐射计算,并尽可能将大气中吸收和散射物质对太阳辐射的影响考虑进去,从而使该方法具有较好的精确性和普适性。在此基础上采用了Kokhanovsky等人提出的大气气溶胶反射率和透过率参数化方案,使得气溶胶对地面总辐射和净辐射的影响得到较好的处理。采用的自变量都是数值预报模式或卫星观测能提供的气象要素,因此该方案即可用于数值预报模式或陆面过程模式计算地表辐射平衡,又可以利用卫星观测或再分析资料估算地面太阳能资源分布。利用美国能源部三个大气辐射观测站点2005年全年的观测资料及欧洲宇航局提供的卫星反演气溶胶资料对计算方案进行了检验。结果表明,该方法十分精确,所有点的平均相对误差都小于6%,误差的均方差都小于0.3 W•m-2。 相似文献
9.
Aircraft observations of solar radiative fluxes (including the downward diffuse component) made in cloud-free conditions in the lowest 8 km of the atmosphere, have been interpreted using simultaneous measurements of aerosol characteristics. Measured flux profiles have been compared with those derived from a two-stream model of radiative transfer which can incorporate both gaseous and aerosol effects. In one of the four cases examined, sufficient aerosol data were available to estimate the radiative properties of the aerosol which could then be included in the model calculations. The findings are shown to be broadly consistent with the observations when a realistic aerosol refractive index is used. The measurement of the downward diffuse radiation enabled the radiative properties of the aerosol to be calculated directly from the flux measurements. In particular, the average single-scattering albedo of aerosol within the boundary layer in continental air masses was estimated to be about 0.7.The implications of having a highly absorbing aerosol present within the boundary layer are also considered. In one case a heating rate of about 5 K day-1 was observed across the aerosol layer, which suggests that on occasions, aerosol heating will be a significant term in the heat budget for the boundary layer. 相似文献
10.
Joonsuk Lee Won Jun Choi Deok Rae Kim Seung-Yeon Kim Chang-Keun Song Jun Suk Hong Youdeog Hong Sukjo Lee 《Asia-Pacific Journal of Atmospheric Sciences》2013,49(3):271-278
Surface erythemal UV radiation is mainly affected by total column ozone, aerosols, clouds, and solar zenith angle. The effect of ozone on the surface UV radiation has been explored many times in the previous studies due to the decrease of ozone layer. In this study, we calculated the effect of aerosols on the surface UV radiation as well as that of ozone using data acquired from Ozone Monitoring Instrument (OMI). First, ozone, aerosol optical depth (AOD), and surface erythemal UVB radiation measured from satellite are compared with those from ground measurements. The results showed that the comparison for ozone was good with r 2 of 0.92. For aerosol, there was difference between satellite measurements and surface measurements due to the insufficient information on aerosol in the retrieval algorithm. The r 2 for surface erythemal UV radiation was high (～0.94) but satellite measurements showed about 30% larger values than surface measurements on average by not considering the effect of absorbing aerosols in the retrieval process from satellite measurements. Radiative amplification factor (RAF) is used to access the effect of ozone and aerosol quantitatively. RAF for ozone was 0.97～1.49 with solar zenith angle. To evaluate the effect of aerosol on the surface UV radiation, only clear-sky pixel data were used and solar zenith angle and total column amount of ozone were fixed. Also, RAF for aerosol was assessed according to the single scattering albedo (SSA) of aerosols. The results showed that RAF for aerosol with smaller SSA (< 0.90) was larger than that for with larger SSA (> 0.90). The RAF for aerosol was 0.09～0.22 for the given conditions which was relatively small compared to that for ozone. However, considering the fact that aerosol optical depth can change largely in time and space while the total column amount of ozone does not change very much, it needs to include the effect of aerosol to predict the variations of surface UV radiation more correctly. 相似文献
11.
Broadband solar irradiance data obtained in the spectral range 400–940 nm at Kwangju, South Korea from 1999–2000 have been analyzed to investigate the effects of cloud cover and atmospheric optical depth on solar radiation components. Results from measurements indicate that the percentage of direct and diffuse horizontal components of solar irradiance depend largely on total optical depth (TOD) and cloud cover. During summer and spring, the percentages of diffuse solar irradiance relative to the global irradiance were 5.0% and 4.9% as compared to 2.2% and 3.0% during winter and autumn. The diffuse solar irradiance is higher than the direct in spring and summer by 24.2%, and 40.6%, respectively, which may largely be attributed to the attenuation (scattering) of radiation by heavy dust pollution and large cloud amount. In cloud-free conditions with cloud cover ≤2/10, the fraction of the direct and diffuse components were 66.0% and 34.0%, respectively, with a mean daily global irradiance value of 7.92±2.91 MJ m−2 day−1. However, under cloudy conditions (with cloud cover ≥8/10), the diffuse and direct fractions were 97.9% and 2.2% of the global component, respectively. The annual mean TOD under cloudless conditions (cloud cover≤2/10) yields 0.74±0.33 and increased to as much as 3.15±0.67 under cloudy conditions with cloud amount ≥8/10. An empirical formula is derived for estimating the diffuse and direct components of horizontal solar irradiance by considering the total atmospheric optical depth (TOD). Results from statistical models are shown for the estimation of solar irradiance components as a function of TOD with sufficient accuracy as indicated by low standard error for each solar zenith angle (SZA). 相似文献
12.
Global and net solar radiation profiles were measured by traversing sensors at four heights in a square-sown plot and a row plot of field corn on four relatively cloudless days in August 1972. The fluxes and their vertical distributions are discussed. A numerical model of the short-wave radiation fluxes in a canopy is presented. Using leaf area index and fixed leaf radiative properties, calculated values of radiation are within 10% of measurements in most instances. The performance under predominantly beam or diffuse radiation is similar and model values of crop albedo compare well with values calculated from radiation measurements above the crops. 相似文献
13.
A simple form of solar radiation model was analysed for cloudless days for Goose, Nfld., Port Hardy, B.C., and Edmonton, Alta. Performance for daily values of total solar radiation was satisfactory; however, data for Goose indicated that the model over‐and under‐estimated the direct and diffuse components of solar radiation, respectively. Modifications, including solving for an aerosol parameter k and substituting 0.6 forward scattering instead of the more commonly used 0.5, improved model performance for direct and diffuse radiation. 相似文献
14.
我国的大气透明状况 总被引：4，自引：1，他引：4
根据全国65个甲种日射站自建站起至1978年9:30,12:30,15:30各时次直接辐射的观测资料,计算了大气透明系数。为了便于各地间的比较和绘制全国分布图,所有各时次的资料都统一订正到M=2的情况下,计算中太阳常数取值S_0=1.98卡厘米~(-2)分~(-1)。 就我国的具体情况而论,地势对大气透明度的影响最为显著,直接的结果是:高原为透明度高值区,盆地为低值区。 分析了影响大气透明度的两个重要因子——水汽和气溶胶的分布特点,以及它们之间的比例关系。水汽对辐射的吸收系根据探空资料求得的整层大气的含水量按Mugge和Muller的公式计算的。 相似文献
15.
Aerosol modulation of atmospheric and surface solar heating over the tropical Indian Ocean 总被引：1，自引：0，他引：1
I. A. PODGORNY W. CONANT V. RAMANATHAN S. K. SATHEESH 《Tellus. Series B, Chemical and physical meteorology》2000,52(3):947-958
The major finding of this study is that aerosols over the tropical Indian Ocean enhance clear sky atmospheric solar heating significantly and decrease the surface solar heating by even a larger amount. The results presented here are based on aerosol chemical, microphysical, and optical and radiometric data collected at the island of Kaashidhoo (4.97°N, 73.47°E) during February and March of 1998, as part of the first field phase of the Indian Ocean experiment (INDOEX). The aerosol optical properties were integrated with a multiple scattering Monte Carlo radiative transfer model which was validated at the surface with broadband flux measurements and at the top of the atmosphere (TOA) with the clouds and earth's radiant energy system (CERES) radiation budget measurements. We consider both externally and internally mixed aerosol models with very little difference between the two models in the estimated forcing. For the February–March period, the aerosols increase the monthly mean clear sky atmospheric solar heating by about 12 W/m2 (about 15% of the total atmospheric solar heating) and decrease the sea surface clear sky solar heating by about 16 W/m2 with a daily range from 5 to 23 W/m2 . The net aerosol forcing at the top of the atmosphere is about −4 W/m2 with a daily range from −2 to −6 W/m2 . Although the soot contributes only about 10% to the aerosol optical thickness, it contributes more than 50% to the aerosol induced atmospheric solar heating. The fundamental conclusion of this study is that anthropogenic aerosols over the tropical Indian Ocean are altering the clear sky radiation budget of the atmosphere and surface in a major manner. 相似文献
16.
17.
北京地区大气气溶胶光学特性监测研究 总被引：23，自引：1，他引：23
该文依据气溶胶光学厚度测量原理,利用CE318太阳光度计,于2000年7月～2001年7月期间对北京地区大气气溶胶光学厚度进行观测试验,计算得到约50天的气溶胶光学厚度和Junge参数等大气光学特性数据,给出了北京地区气溶胶光学特性分布特征.计算统计得到北京城区晴空条件下的Junge参数为3
15、2001年3月份沙尘天气状况下急剧下降为2.28,而北京郊区顺义县的测量结果介于二者之间为2.65.分析表明,由试验获得的气溶胶光学特性数据对于分析和监测北京地区大气污染、改善北京地区空气质量具有一定的意义. 相似文献
18.
The actinometric system installed aboard the Yak-42D "Roshydromet" research aircraft is presented. It is designed to study radiation processes in the troposphere. The system is based on standard Kipp&Zonen actinometric instruments for measuring solar, thermal, and ultraviolet radiation fluxes as well as on specially developed radiation models with high-precision methods for solving radiative transfer equations (Monte Carlo, k-distribution, and line-by-line calculations). The combination of actinometric measurements and detailed simulation of radiative transfer in the atmosphere allows examining the radiation balance components throughout the troposphere using in situ measurements at the aircraft location. Some results of studying radiation fluxes obtained during the flights over the Arctic region of the Russian Federation are presented. The data of measurements carried out using the presented system are useful for validating radiation codes utilized in general atmospheric circulation models and for processing satellite remote sensing data. 相似文献
19.
STEPHAN BORRMANN REAS THOMAS VLADIMIR RUDAKOV VLADIMIR YUSHKOV BORIS LEPUCHOV TERRY DESHLER NIKOLAI VINNICHENKO VYACHESLAV KHATTATOV LEOPOLDO STEFANUTTI 《Tellus. Series B, Chemical and physical meteorology》2000,52(4):1088-1103
In‐situ aerosol measurements were performed in the northern hemispheric stratosphere up to altitudes of 21 km between 13 November 1996 and 14 January 1997, inside and outside of the polar vortex during the Airborne Polar Experiment (APE) field campaign. These are measurements of particle size distributions with a laser optical particle counter of the FSSP‐300 type operated during 9 flights on the Russian M‐55 high‐altitude research aircraft Geophysika. For specific flights, the FSSP‐300 measurements are compared with balloon‐borne data (launched from Kiruna, Sweden). It was found that the stratospheric aerosol content reached levels well below the background concentrations measured by the NASA operated ER‐2 in 1988/89 in the northern hemisphere. During the APE campaign, no PSC particle formation was observed at flight altitudes although the temperatures were below the NAT condensation point during one flight. The measured correlations between ozone and aerosol give an indication of the subsidence inside the 1996/97 polar vortex. Despite the lower aerosol content in the winter 1996/97 compared to the 1989 background, the heterogeneous reactivity of the aerosol (as calculated from the measured data with additional model input) is comparable. This is due to the dependency of the reactive uptake coefficients on the atmospheric water vapor content. Under the described assumptions the reaction rates on the background aerosol are significantly smaller than for competing gas phase chlorine activation, as can be expected for stratospheric background conditions especially inside the polar vortex. 相似文献
20.
干旱地区大气与地表特征对辐射加热场的影响 总被引：1，自引：0，他引：1
本文利用美国犹他大学气象系的辐射和云参数化模式，对ＨＥＩＦＥ期间张掖地区１９９１年春、夏、秋、冬四季资料进行了计算，讨论了晴天条件下的大气状况态地表反射率与地表比辐射率等因子对地气系统的太阳辐射收支以及短波加热率与长波冷却率分布的影响；揭示了不同季节的整层大气反射、透过与吸收特征，分析了大气中各主要吸收成分对加热率与冷却率的贡献，同时就辐射模式的垂直分辨率对加热率与冷却率的影响亦作了讨论。 相似文献