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1.
Zhaobin Sun Xiaoling Zhang Xiujuan Zhao Xiangao Xia Shiguang Miao Ziming Li Zhigang Cheng Wei Wen Yixi Tang 《Acta Meteorologica Sinica》2018,32(2):288-301
We used simultaneous measurements of surface PM2.5 concentration and vertical profiles of aerosol concentration, temperature, and humidity, together with regional air quality model simulations, to study an episode of aerosol pollution in Beijing from 15 to 19 November 2016. The potential effects of easterly and southerly winds on the surface concentrations and vertical profiles of the PM2.5 pollution were investigated. Favorable easterly winds produced strong upward motion and were able to transport the PM2.5 pollution at the surface to the upper levels of the atmosphere. The amount of surface PM2.5 pollution transported by the easterly winds was determined by the strength and height of the upward motion produced by the easterly winds and the initial height of the upward wind. A greater amount of PM2.5 pollution was transported to upper levels of the atmosphere by upward winds with a lower initial height. The pollutants were diluted by easterly winds from clean ocean air masses. The inversion layer was destroyed by the easterly winds and the surface pollutants and warm air masses were then lifted to the upper levels of the atmosphere, where they re-established a multi-layer inversion. This region of inversion was strengthened by the southerly winds, increasing the severity of pollution. A vortex was produced by southerly winds that led to the convergence of air along the Taihang Mountains. Pollutants were transported from southern–central Hebei Province to Beijing in the boundary layer. Warm advection associated with the southerly winds intensified the inversion produced by the easterly winds and a more stable boundary layer was formed. The layer with high PM2.5 concentration became dee-per with persistent southerly winds of a certain depth. The polluted air masses then rose over the northern Taihang Mountains to the northern mountainous regions of Hebei Province. 相似文献
2.
《大气和海洋科学快报》2023,16(1):100274
China has been frequently suffering from haze pollution in the past several decades. As one of the most emission-intensive regions, the North China Plain (NCP) features severe haze pollution with multiscale variations. Using more than 30 years of visibility measurements and PM2.5 observations, a subseasonal seesaw phenomenon of haze in autumn and early winter over the NCP is revealed in this study. It is found that when September and October are less (more) polluted than the climatology, haze tends to be enhanced (reduced) in November and December. The abrupt turn of anomalous haze is found to be associated with the circulation reversal of regional and large-scale atmospheric circulations. Months with poor air quality exhibit higher relative humidity, lower boundary layer height, lower near-surface wind speed, and southerly anomalies of low-level winds, which are all unfavorable for the vertical and horizontal dispersion and transport of air pollutants, thus leading to enhanced haze pollution over the NCP region on the subseasonal scale. Further exploration indicates that the reversal of circulation patterns is closely connected to the propagation of midlatitude wave trains active on the subseasonal time scale, which is plausibly associated with the East Atlantic/West Russia teleconnection synchronizing with the transition of the North Atlantic SST. The seesaw relation discussed in this paper provides greater insight into the prediction of the multiscale variability of haze, as well as the possibility of efficient short-term mitigation of haze to meet annual air quality targets in North China.摘要中国近几十年来频受雾霾污染问题困扰, 其中华北平原作为排放最密集的区域之一, 常遭遇不同尺度的严重雾霾污染. 本文利用30余年的能见度和颗粒物 (PM2.5) 观测数据, 发现了华北平原地区在秋季和早冬时雾霾污染在次季节尺度上“跷跷板式”反向变化的关系. 研究发现, 当9–10月污染较轻 (重) 时, 11–12月的污染倾向于加重 (减轻) . 这种突然的变化与局地和大尺度环流的反向变化有关. 污染较重的月份常伴随有更高的相对湿度, 更低的边界层高度和近地面风速以及低层的南风异常, 均不利于污染的垂直和水平扩散和传输, 从而导致了次季节尺度上霾污染的加重. 进一步的研究发现环流场的突然转向与在次季节尺度上活跃的中纬度波列的传播密切相关, 而此波列可能主要与大西洋海温转变及引起的EA/WR遥相关型有关. 这一次季节反向变化为霾污染多尺度变率预测提供了新的理解, 同时为华北地区年度空气质量达标的短期目标提供了具有可行性的参考方法. 相似文献
3.
2016年1月我国中东部一次大气污染物传输过程分析 总被引：1，自引：1，他引：0
利用常规气象数据和空气质量模式CAMx对2016年1月15—19日一次冷空气影响下郑州、武汉、南京的大气污染物传输过程进行了分析。观测发现,本次过程中武汉和南京在地面锋线到达后出现明显的PM2.5浓度的快速增长。通过分析发现,两地在1000~950 hPa高度层上偏北风的侵入带来上风向的大气污染物,同时在垂直方向上锋区内的稳定性层结抑制了大气污染物的扩散,两种作用共同导致污染物快速增长。在冷空气主体影响下,尤其是950~900 hPa高度层上弱风区消失后,污染物得到清除。大气污染物的传输作用主要发生在1000~950 hPa高度上。模式PM2.5来源示踪模拟结果表明,武汉(17日夜间至18日)和南京(17日夜间)在本次污染物快速增长过程中区域污染物输入的贡献在51%和58%左右。由于模式对PM2.5传输过程的低估,区域输送贡献率仍存在不确定性。但是,与1月15—19日平均相比, PM2.5的本地贡献明显减少,上风区域贡献明显增加。 相似文献
4.
利用欧洲中期天气预报中心（ECMWF）数值预报产品和动态统计预报方法,对北京、天津、石家庄等14个京津冀重点城市雾霾与空气污染进行定量化的中期预报试验,包括对首要污染物PM2.5浓度和能见度的逐时定量化预报及雾霾现象的客观化判断,并对2015年10月1日-2016年11月10日试验预报效果进行了检验评估。检验结果显示:该方法对北京及周边城市未来10 d逐时和逐日能见度、PM2.5浓度及雾霾现象的预报值与观测值之间具有显著正相关系数、较高的误差减少量和TS评分等,表明基于ECMWF数值预报产品和动态统计预报方法的京津冀雾霾污染中期定量化预报技术整体上具有较高的可靠性、稳定性与预报技巧性。此外,检验指标还显示出该动态统计预报方法对能见度的预报效果要略优于PM2.5浓度预报,同时对霾的预报准确率高于对雾的预报。个例分析显示,该动态统计预报方法能提前5~6 d预报出北京地区典型持续性雾霾污染的发展过程,对持续性雾霾的提前预报预警具有较好的参考意义。 相似文献
5.
PM2.5污染仍然是湖北省冬季大气污染的首要污染类型,且具有明显区域传输特征,重污染过程的空气污染气象条件有别于华北地区,值得关注。采用WRF/Chem不同排放情景下的模拟结果,并结合观测分析,研究了2015年12月—2016年1月湖北省PM2.5重污染过程的气象输送条件及日变化特征,从大尺度输送条件和局地边界层动力作用分析了外来污染物水平传输、悬浮聚集和向下传输的过程,并解释了该地区观测到的午后PM2.5浓度特殊峰值的气象成因。结果表明,湖北重污染爆发以区域传输为主,地面观测PM2.5极值对应10 m风速可达8—10 m/s,边界层0—1 km为较强偏北风输送,污染传输通量极值位于400 m高度附近,为重要传输通道,低空无明显逆温,重污染过程具有“非静稳”边界层气象特征。重污染形成的大尺度输送条件为,长江中下游及北部地区偏北风异常偏强,南部地区风速减缓,使污染物在中游平原堆积,鄂北边界风速越大,越有利污染输送增长。传输性污染主要来自偏北和东北方向的污染源输送,潜在源区贡献主要为途经偏北通道上的豫中、南阳盆地和关中地区,以及途经东北通道上的鲁、皖、苏等部分地区。PM2.5浓度日变化双峰结构的天气成因不同,21—24时（北京时）峰值为静稳性污染,11—14时峰值为传输性污染。污染输送受大气边界层高度影响,日出前大气边界层高度较低,层结稳定并伴有上升运行,使得低空外来输送悬浮聚集在400 m高度附近;日出后随大气边界层高度升高,静稳层结被破坏,在干沉降作用下高浓度PM2.5开始向下传输,并在午后地面形成峰值。 相似文献
6.
Junting Zhong Xiaoye Zhang Yaqiang Wang Junying Sun Yangmei Zhang Jizhi Wang Kaiyan Tan Xiaojing Shen Haochi Che Lu Zhang Zhouxiang Zhang Xuefei Qi Huarong Zhao Sanxue Ren Yang Li 《Acta Meteorologica Sinica》2017,31(5):809-819
Based on observations of urban mass concentration of fine particulate matter smaller than 2.5 μm in diameter (PM2.5), ground meteorological data, vertical measurements of winds, temperature, and relative humidity (RH), and ECMWF reanalysis data, the major changes in the vertical structures of meteorological factors in the boundary layer (BL) during the heavy aerosol pollution episodes (HPEs) that occurred in winter 2016 in the urban Beijing area were analyzed. The HPEs are divided into two stages: the transport of pollutants under prevailing southerly winds, known as the transport stage (TS), and the PM2.5 explosive growth and pollution accumulation period characterized by a temperature inversion with low winds and high RH in the lower BL, known as the cumulative stage (CS). During the TS, a surface high lies south of Beijing, and pollutants are transported northwards. During the CS, a stable BL forms and is characterized by weak winds, temperature inversion, and moisture accumulation. Stable atmospheric stratification featured with light/calm winds and accumulated moisture (RH > 80%) below 250 m at the beginning of the CS is closely associated with the inversion, which is strengthened by the considerable decrease in near-surface air temperature due to the interaction between aerosols and radiation after the aerosol pollution occurs. A significant increase in the PLAM (Parameter Linking Aerosol Pollution and Meteorological Elements) index is found, which is linearly related to PM mass change. During the first 10 h of the CS, the more stable BL contributes approximately 84% of the explosive growth of PM2.5 mass. Additional accumulated near-surface moisture caused by the ground temperature decrease, weak turbulent diffusion, low BL height, and inhibited vertical mixing of water vapor is conducive to the secondary aerosol formation through chemical reactions, including liquid phase and heterogeneous reactions, which further increases the PM2.5 concentration levels. The contribution of these reaction mechanisms to the explosive growth of PM2.5 mass during the early CS and subsequent pollution accumulation requires further investigation. 相似文献
7.
针对2013年1月江苏淮安地区发生的一次连续性雾霾天气过程,分析该天气过程中PM10和PM2.5的质量浓度演变特征、能见度与气象要素之间的关系、中低层环流特征以及污染物来源。结果表明:雾霾期间PM10和PM2.5质量浓度最低值出现在05:00至07:00(北京时间,下同)和13:00至17:00,最高值出现在21:00至23:00,PM10和PM2.5质量浓度并非同时达到极大值;持续变化较小的气压梯度、较低的风速、相对湿度的增大以及PM2.5和PM10质量浓度的增高是雾霾发生发展的必要条件;能见度与气压、相对湿度、PM2.5质量浓度的相关性较好,建立回归方程,对能见度的整体变化趋势拟合效果较好;高空环流形势平稳、中低层的暖平流、持续稳定少动的地面高压场分布为雾霾天气的持续发生发展提供了有利的形势背景;稳定的层结结构、中低层偏东及偏东北方向气团的输送、本地污染源以及严重的空气污染是此次过程中能见度偏低、霾天数较多的主要原因。 相似文献
8.
China has implemented a series of emission reduction policies since 2013, and the concentration of air pollutants has consequently decreased significantly. However, PM2.5 (particulate matter with an aerodynamic diameter less than 2.5 µm) pollution still occurs in China in relation to the interannual variations in meteorological conditions. Considering that El Niño–Southern Oscillation (ENSO) is the strongest signal modulating the interannual variation in the atmosphere–ocean system, in this study the authors investigate the variations in PM2.5 concentrations in four megacity clusters of China during the winter season associated with four individual ENSO events from 2014 to 2021. Results show that the wintertime PM2.5 concentrations in the Beijing–Tianjin–Hebei and Fenwei Plain regions during El Niño years are higher than those during La Niña years, which can be explained by the anomalous southerly (northerly) winds during El Niño (La Niña) favoring PM2.5 accumulation (diffusion). In the Pearl River Delta region, PM2.5 concentrations decrease in El Niño relative to La Niña years owing to the enhanced water vapor flux and precipitation, removing more PM2.5 from the atmosphere. The comprehensive effects of wind and precipitation anomalies lead to the unpredictability of the impacts of ENSO on PM2.5 over the Yangtze River Delta region, which should be analyzed case by case.摘要2013年以来中国实施了一系列减排政策, 大气污染物浓度明显下降, 但由于气象条件的年际变化, 中国PM2.5 (空气动力学直径小于2.5 µm的颗粒物) 污染仍然存在. 厄尔尼诺–南方涛动 (ENSO) 是调节大气–海洋系统年际变化的最强信号. 本文研究了2014–2021年四次ENSO事件期间, 中国四个特大城市群冬季PM2.5浓度的变化. 结果表明, 在京津冀和汾渭平原地区, 由于厄尔尼诺 (拉尼娜) 期间的偏南风 (偏北风) 异常有利于 PM2.5 的积累 (扩散), 冬季PM2.5浓度在厄尔尼诺年高于拉尼娜年. 在珠三角地区, 由于厄尔尼诺冬季水汽通量和降水的增加有利于大气中PM2.5的湿清除, 冬季PM2.5浓度在厄尔尼诺年低于拉尼娜年. 在环流和降水异常的综合作用下, ENSO对长三角地区PM2.5浓度的影响难以预测, 应逐案分析. 相似文献
9.
We present mobile vehicle lidar observations in Tianjin, China during the spring, summer, and winter of 2016. Mobile observations were carried out along the city border road of Tianjin to obtain the vertical distribution characteristics of PM2.5. Hygroscopic growth was not considered since relative humidity was less than 60% during the observation experiments. PM2.5 profile was obtained with the linear regression equation between the particle extinction coefficient and PM2.5 mass concentration. In spring, the vertical distribution of PM2.5 exhibited a hierarchical structure. In addition to a layer of particles that gathered near the ground, a portion of particles floated at 0.6–2.5-km height. In summer and winter, the fine particles basically gathered below 1 km near the ground. In spring and summer, the concentration of fine particles in the south was higher than that in the north because of the influence of south wind. In winter, the distribution of fine particles was opposite to that measured during spring and summer. High concentrations of PM2.5 were observed in the rural areas of North Tianjin with a maximum of 350 μg m–3 on 13 December 2016. It is shown that industrial and ship emissions in spring and summer and coal combustion in winter were the major sources of fine particles that polluted Tianjin. The results provide insights into the mechanisms of haze formation and the effects of meteorological conditions during haze–fog pollution episodes in the Tianjin area. 相似文献
10.
2018年1月,利用颗粒物采样器采集武汉市大气PM2.5样品并进行水溶性无机离子（F-、Cl-、NO3-、SO42-、Na+、NH4+、K+、Mg2+、Ca2+）的分析.结果表明,NO3-、SO42-、NH4+是PM2.5中最主要的3种水溶性无机离子,除Mg2+与Ca2+外,PM2.5与WSⅡs （水溶性无机离子）之间的相关性显著,且移动源贡献占主导地位.阴阳离子平衡表明武汉市冬季灰霾期PM2.5呈中性或弱酸性.通过混合单粒子拉格朗日综合轨迹模式模拟并采用分层聚类得出了4种主要的后向气流轨迹及相应的PM2.5和水溶性离子浓度,结果表明区域传输对此次灰霾期影响较大. 相似文献
11.
北京一次持续性雾霾过程的阶段性特征及影响因子分析 总被引：11，自引：1，他引：10
利用北京地区高时间分辨率观测资料对2009年11月3—8日一次持续性雾霾天气过程中的气象因素和气溶胶演变特征进行了分析。结果表明,该次雾霾过程具有明显的阶段性特征,前期以霾为主,中期发展为雾霾交替,后期随着相对湿度减小再次转换为霾并最终消散。边界层逆温是低能见度过程形成的必要条件,但并不最终决定雾霾低能见度强度。相对湿度和PM2.5浓度是决定能见度大小的两个关键影响因子,对能见度的影响体现出阶段性特征。大部分时段PM2.5浓度是影响能见度的主要因子,当能见度小于1 km时,能见度变化更多受相对湿度影响。不同的情景计算表明,控制PM2.5浓度对于改善本次过程的能见度有重要作用。 相似文献
12.
Yanjun Ma Hujia Zhao Yunsheng Dong Huizheng Che Xiaoxiao Li Ye Hong Xiaolan Li Hongbin Yang Yuche Liu Yangfeng Wang Ningwei Liu Cuiyan Sun 《Acta Meteorologica Sinica》2018,32(2):313-323
This study analyzes and compares aerosol properties and meteorological conditions during two air pollution episodes in 19–22 (E1) and 25–26 (E2) December 2016 in Northeast China. The visibility, particulate matter (PM) mass concentration, and surface meteorological observations were examined, together with the planetary boundary layer (PBL) properties and vertical profiles of aerosol extinction coefficient and volume depolarization ratio that were measured by a ground-based lidar in Shenyang of Liaoning Province, China during December 2016–January 2017. Results suggest that the low PBL height led to poor pollution dilution in E1, while the high PBL accompanied by low visibility in E2 might have been due to cross-regional and vertical air transmission. The PM mass concentration decreased as the PBL height increased in E1 while these two variables were positively correlated in E2. The enhanced winds in E2 diffused the pollutants and contributed largely to the aerosol transport. Strong temperature inversion in E1 resulted in increased PM2.5 and PM10 concentrations, and the winds in E2 favoured the southwesterly transport of aerosols from the North China Plain into the region surrounding Shenyang. The large extinction coefficient was partially attributed to the local pollution under the low PBL with high ground-surface PM mass concentrations in E1, whereas the cross-regional transport of aerosols within a high PBL and the low PM mass concentration near the ground in E2 were associated with severe aerosol extinction at high altitudes. These results may facilitate better understanding of the vertical distribution of aerosol properties during winter pollution events in Northeast China. 相似文献
13.
Inhalable particles (PM10), with aerodynamic equivalent diameters that are generally 10 micrometers or smaller, are basic pollutants in many areas, especially in northern China, and thus the pollution from PM10 inhalable particulate matter is a growing concern for public health. Independent long-term observations are necessary to evaluate the efficacy of PM10 reduction actions. Variations in the PM10 concentration from 2006 to 2017 at an observation station (NJ) in Beijing were recorded and analyzed. The average value ±1 standard deviation of daily mean PM10 concentrations was 138.8 ±96.1 μg m-3 for 1307 days (accounting for 34.7% of the total days), showing PM10 concentration exceeding the National Ambient Air Quality Standard (NAAQS) 24-h average of 150 μg m-3. Particulate concentration depended upon various meteorological conditions as also observed in this work: at low wind speed (<4 m s-1), the concentrations of PM10 revealed a downward trend with -19 μg m-3 per unit of wind speed, but when wind speed rose (>4 m s-1), the values increased by 49 μg m-3 per unit of wind speed. In Beijing, air masses from northwest China, especially from the Gobi Desert and other desert areas, had net contributions to long-range transport of natural dust, enhancing the PM10 concentrations by up to 29%. Overall, PM10 mass concentration showed a significant downward trend with -8.0 μg/m3/yr from 2006 to 2017. Although with higher fluctuations in recorded data, similar downward trends derived from the ) in 2017 still exceeded the NAAQS standard. The results showed that there is still a long way to go to reduce PM10 in Beijing. 相似文献
14.
采用大气辐射传输模式SES2以及2013年1月—2015年10月欧洲中期天气预报中心细网格再分析资料计算了北京地区4个观测站地面接收的短波辐射通量,分析了晴天和云天北京城郊气溶胶对总辐射的定量影响时空变化特征。结果表明:北京城区和近郊区气溶胶对总辐射的影响约为远郊区的2倍,北京南部和西部气溶胶对辐射的影响较大,晴天和云天北京城区和近郊区气溶胶对总辐射的削减值分别为146.23~180.99 W·m-2和202.11~217.02 W·m-2,晴天总辐射削减空间差异较大;秋冬季气溶胶对总辐射的影响明显大于春夏季,北京市观象台秋冬季气溶胶对总辐射的削减作用最大可达60%,较春夏季高10%~20%;北京城郊总辐射和直接辐射削减率与气溶胶光学厚度变化均呈线性关系,近地面PM2.5浓度对辐射的影响不容忽视。 相似文献
15.
利用苏州市2009年6月-2010年5月逐时的能见度、相对湿度、污染物(PM1o、PM2.5、黑碳)浓度和散射系数等资料进行灰霾的判识与统计分析,结果表明:苏州市灰霾日占全年天数的46.6％,雨日和“蓝天”分别占33.2％和21.9％.在苏州所有灰霾日中以轻微灰霾为主,占灰霾曰总数的70.6％,发生中度和重度灰霾的频率较小.灰霾出现频率的日变化规律表明白天出现灰霾的频率比夜间低,在5-8时灰霾出现的频率达到峰值,14-16时灰霾出现的频率最低.灰霾日的污染物浓度远大于非灰霾日,随着灰霾等级增大,黑碳浓度明显增大;除重度灰霾外,PM10和PM2.5浓度也明显增大;散射系数增大. 相似文献
16.
本文利用气体组分及大气气溶胶在线监测系统(MARGA ADI 2080)观测武汉市2018年1月9—26日大气气溶胶中的8种水溶性离子(NH+4、NO-3、SO2-4、Cl-、K+、Ca2+、Na+和Mg2+),结合气象要素数据,使用主成分分析(PCA)、正定矩阵因子分析法(PMF)、HYSPLIT后向轨迹模式、潜在源区贡献(PSCF)和浓度权重轨迹(CWT),对霾污染过程中水溶性离子进行了全面的来源解析,探究了霾不同阶段下来源差异和空间分布特征。结果表明:(1)本次霾污染中的8种水溶性离子和4种污染气体,PCA解析出的源和占比分别为二次源和燃煤源的混合源(41.28%)、工业排放和土壤扬尘混合源(27.73%)和机动车排放源(9.63%),PMF解析出的源和占比分别为燃煤与土壤扬尘混合源(18.57%)、机动车排放源(20.74%)、二次源(18.30%)、光化学污染源(22.24%)和燃煤源(20.15%)。(2)霾在不同阶段下水溶性离子和4种污染气体的来源存在差异,在清洁天和霾消散阶段,光化学的贡献最高,占比分别为31.42%和36.07%;在霾发生阶段燃煤与土壤扬尘源的贡献最高,其贡献为40.94%;在霾发展阶段,最大的控制源为二次源,贡献占比为37.51%。(3)此次武汉市霾污染中PM2.5浓度和NH+4、NO-3和SO2-4的潜在源区为皖豫鄂三省和赣湘鄂三省交界处。霾污染中PM2.5的主要影响范围是武汉市南部和北部省份,NO-3、NH+4和SO2-4的主要影响区域为武汉市东北方向的城市、湖南省和江西省。 相似文献
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综合运用了多元资料（环境空气质量监测资料、地面气象观测资料、L波段雷达探空资料、风廓线雷达探空资料和再分析资料）和多种方法（后向轨迹追踪、聚类分析、潜在源区贡献法和数值模拟）,研究了武汉地区特殊气象条件对重污染过程的影响,揭示了偏东小风所带来的外源污染物对形成严重污染日的贡献.主要研究结论如下：1）后向轨迹追踪分析表明,武汉地区严重污染日气流主要为来自安徽南部（47.5%）的偏东小风,模拟结果也显示偏东气流、偏北气流与局地环流共同作用,在武汉地区形成一个局地涡旋,成为反复污染带,加重了武汉地区的污染程度;2）利用潜在源区贡献法（PSCF）分析发现,武汉市秋冬季的潜在源区主要是安徽、江苏、山东、河南、湖南、江西以及武汉周边地区,因此在冬季大范围污染背景下,跨区域的联防联控（尤其是安徽南部地区）才能有效地减少武汉市秋冬季的重污染日. 相似文献
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利用北京市道面自动气象站、国家级自动气象站等多种观测数据分析北京地区2007—2015年能见度及其主要影响因子, 并挑选两次典型低能见度事件过程进行详细分析。从空间分布看, 北京西北地区能见度明显高于中心城区和东南大部地区。从时间分布看, 北京地区平均能见度最大值出现在5月, 最小值出现在7月; 日间的最低值多出现在06:00(北京时, 下同)左右, 冬季略向后推迟; 最高值多出现在16:00前后, 冬季略有提前。整体而言, 2007—2015年北京地区发生低能见度事件的概率为62.14%, 且发生低能见度的事件集中于1~5 km, 霾事件中干霾、湿霾的发生频率分别为86.13%和13.87%。能见度的主要影响因子为相对湿度、风速和PM2.5浓度。其中, 能见度与风速呈正相关, 与相对湿度和PM2.5浓度呈反相关。需要指出的是, 当相对湿度增加至80%, 能见度受PM2.5浓度的影响程度在下降, 而主要受相对湿度的影响。基于所选个例, 当北京地区出现湿霾事件时, 能见度的恶化程度远高于干霾事件, 且PM2.5浓度需比干霾事件时下降得更低才能有效改善能见度。 相似文献
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面对日益严峻的大气污染形势,针对卫星气溶胶光学厚度（AOD）资料在灰霾数值预报领域的合理有效利用问题,使用WRF-Chem（WRF coupled with Chemistry）大气化学模式以及GSI（Gridpoint Statistical Interpolation）三维变分同化系统,利用MODIS和FY-3A/MERSI AOD资料,对一次灰霾天气过程进行了同化预报试验。试验结果显示,同化卫星AOD资料有效改善了模式初始场,MODIS和MERSI同化试验分别在AOD分析场的中心强度和空间分布各具优势,且对PM2.5和PM10的后续预报改进明显;从统计分析上看,同化试验的预报效果整体上好于控制试验,同化试验中PM2.5和PM10预报值的平均值、中值、平均偏差、均方根误差等指标均明显优于控制试验,且MODIS和MERSI同化试验分别在PM2.5和PM10预报统计结果中体现出了优势;卫星AOD资料同化能明显降低污染事件的空报率和漏报率,提高预报的TS评分和ETS评分。不同卫星AOD资料的差异对分析场中AOD的分布和强度产生了相应影响,进而影响了模式的灰霾预报效果;本次试验中,MODIS和MERSI AOD同化试验分别在PM2.5和PM10预报的评分上表现更佳。结果表明,卫星AOD资料同化对数值预报产生了积极的效果。 相似文献
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Surface ozone (O3) and fine particulate matter (PM2.5) are dominant air pollutants in China. Concentrations of these pollutants can show significant differences between urban and nonurban areas. However, such contrast has never been explored on the country level. This study investigates the spatiotemporal characteristics of urban-to-suburban and urban-to-background difference for O3 (Δ[O3]) and PM2.5 (Δ[PM2.5]) concentrations in China using monitoring data from 1171 urban, 110 suburban, and 15 background sites built by the China National Environmental Monitoring Center (CNEMC). On the annual mean basis, the urban-to-suburban Δ[O3] is ?3.7 ppbv in Beijing–Tianjin–Hebei, 1.0 ppbv in the Yangtze River Delta, ?3.5 ppbv in the Pearl River Delta, and ?3.8 ppbv in the Sichuan Basin. On the contrary, the urban-to-suburban Δ[PM2.5] is 15.8, ?0.3, 3.5 and 2.4 μg m?3 in those areas, respectively. The urban-to-suburban contrast is more significant in winter for both Δ[O3] and Δ[PM2.5]. In eastern China, urban-to-background differences are also moderate during summer, with ?5.1 to 6.8 ppbv for Δ[O3] and ?0.1 to 22.5 μg m?3 for Δ[PM2.5]. However, such contrasts are much larger in winter, with ?22.2 to 5.5 ppbv for Δ[O3] and 3.1 to 82.3 μg m?3 for Δ[PM2.5]. Since the urban region accounts for only 2% of the whole country’s area, the urban-dominant air quality data from the CNEMC network may overestimate winter [PM2.5] but underestimate winter [O3] over the vast domain of China. The study suggests that the CNEMC monitoring data should be used with caution for evaluating chemical models and assessing ecosystem health, which require more data outside urban areas. 相似文献