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1.
Releases of halocarbons into the atmosphere over the last 50 years are among the factors that have contributed to changes in the Earth’s climate since pre-industrial times. Their individual and collective potential to contribute directly to surface climate change is usually gauged through calculation of their radiative efficiency, radiative forcing, and/or Global Warming Potential (GWP). For those halocarbons that contain chlorine and bromine, indirect effects on temperature via ozone layer depletion represent another way in which these gases affect climate. Further, halocarbons can also affect the temperature in the stratosphere. In this paper, we use a narrow-band radiative transfer model together with a range of climate models to examine the role of these gases on atmospheric temperatures in the stratosphere and troposphere. We evaluate in detail the halocarbon contributions to temperature changes at the tropical tropopause, and find that they have contributed a significant warming of ~0.4 K over the last 50 years, dominating the effect of the other well-mixed greenhouse gases at these levels. The fact that observed tropical temperatures have not warmed strongly suggests that other mechanisms may be countering this effect. In a climate model this warming of the tropopause layer is found to lead to a 6% smaller climate sensitivity for halocarbons on a globally averaged basis, compared to that for carbon dioxide changes. Using recent observations together with scenarios we also assess their past and predicted future direct and indirect roles on the evolution of surface temperature. We find that the indirect effect of stratospheric ozone depletion could have offset up to approximately half of the predicted past increases in surface temperature that would otherwise have occurred as a result of the direct effect of halocarbons. However, as ozone will likely recover in the next few decades, a slightly faster rate of warming should be expected from the net effect of halocarbons, and we find that together halocarbons could bring forward next century’s expected warming by ~20 years if future emissions projections are realized. In both the troposphere and stratosphere CFC-12 contributes most to the past temperature changes and the emissions projection considered suggest that HFC-134a could contribute most of the warming over the coming century.  相似文献   

2.
The global three-dimensional Lagrangian chemistry-transport model STOCHEM has been used to follow the changes in the tropospheric distributions of the two major radiatively-active trace gases, methane and tropospheric ozone, following the emission of pulses of the short-lived tropospheric ozone precursor species, methane, carbon monoxide, NOx and hydrogen. The radiative impacts of NOx emissionswere dependent on the location chosen for the emission pulse, whether at the surface or in the upper troposphere or whether in the northern or southern hemispheres. Global warming potentials were derived for each of the short-lived tropospheric ozone precursor species by integrating the methane and tropospheric ozone responses over a 100 year time horizon. Indirect radiative forcing due to methane and tropospheric ozone changes appear to be significant for all of the tropospheric ozone precursor species studied. Whereas the radiative forcing from methane changes is likely to be dominated by methane emissions, that from tropospheric ozone changes is controlled by all the tropospheric ozone precursor gases, particularly NOxemissions. The indirect radiative forcing impacts of tropospheric ozone changes may be large enough such that ozone precursors should be considered in the basket of trace gases through which policy-makers aim to combat global climate change.  相似文献   

3.
A global two-dimensional (altitude-latitude) chemistry transport model is used to follow the changes in the tropospheric distribution of the two major radiatively active trace gases, methane and ozone, following step changes to the sustained emissions of the short-lived trace gases methane, carbon monoxide and non-methane hydrocarbons. The radiative impacts were dependent on the latitude chosen for the applied change in emissions. Step change global warming potentials (GWPs) were derived for a range of short-lived trace gases to describe their time-integrated radiative forcing impacts for unit emissions relative to that of carbon dioxide. The GWPs show that the tropospheric chemistry of the hydrocarbons can produce significant indirect radiative impacts through changing the tropospheric distributions of hydroxyl radicals, methane and ozone. For aircraft, the indirect radiative forcing impact of the NO x emissions appears to be greater than that from their carbon dioxide emissions. Quantitative results from this two-dimensional model study must, however, be viewed against the known inadequacies of zonally-averaged models and their poor representation of many important tropospheric processes.  相似文献   

4.
The effect of anthropogenic emissions from China on global burdens of ozone, sulphate, organic carbon (OC) and black carbon (BC) aerosols is examined, using the three-dimensional chemistry transport model Oslo CTM2. Two model simulations were performed, the first with global present-day emissions and the second with the anthropogenic emissions from China set to their pre-industrial levels. The global radiative forcing for these species is then calculated. Industrial emissions from China are found to account for a 4–5% increase in the global burden of OC aerosol, the change in secondary organic aerosol being slightly less than that of primary organic aerosol. A 10% increase in the global sulphate aerosol burden is calculated, and the increase in BC is 23%. The global radiative forcing of aerosols from China was calculated to be −62, −3.7, −13 and 89 mW m−2, for sulphate, secondary organic, primary organic and BC aerosols, respectively. The increase in ozone causes a forcing of 77 mW m−2.  相似文献   

5.
The radiative impact of greenhouse gases in warming the Earth varies significantly, depending on whether one considers the forcing at the tropopause or at the surface. Compared to the former, the surface forcing for some greenhouse gases is reduced by the interference of water vapour. Hence, we calculate alternative surface global warming potentials (SGWPs) that are derived from the surface forcing radiation of greenhouse gases for potential use in surface radiative energy balance models (SREBMs). For gases with a large water vapour overlap, the SGWPs are typically 30% smaller than current GWPs; for gases with relatively little overlap, the SGWPs are larger by more than 33%. These results may be used in conjunction with SREBMs as an additional means of calculating climate change, and may lead to an altered emissions budget compared to that outlined by the current Kyoto agreement.  相似文献   

6.
Understanding the historical and future response of the global climate system to anthropogenic emissions of radiatively active atmospheric constituents has become a timely and compelling concern. At present, however, there are uncertainties in: the total radiative forcing associated with changes in the chemical composition of the atmosphere; the effective forcing applied to the climate system resulting from a (temporary) reduction via ocean-heat uptake; and the strength of the climate feedbacks that subsequently modify this forcing. Here a set of analyses derived from atmospheric general circulation model simulations are used to estimate the effective and total radiative forcing of the observed climate system due to anthropogenic emissions over the last 50 years of the twentieth century. They are also used to estimate the sensitivity of the observed climate system to these emissions, as well as the expected change in global surface temperatures once the climate system returns to radiative equilibrium. Results indicate that estimates of the effective radiative forcing and total radiative forcing associated with historical anthropogenic emissions differ across models. In addition estimates of the historical sensitivity of the climate to these emissions differ across models. However, results suggest that the variations in climate sensitivity and total climate forcing are not independent, and that the two vary inversely with respect to one another. As such, expected equilibrium temperature changes, which are given by the product of the total radiative forcing and the climate sensitivity, are relatively constant between models, particularly in comparison to results in which the total radiative forcing is assumed constant. Implications of these results for projected future climate forcings and subsequent responses are also discussed.  相似文献   

7.
Temperature trends in the upper stratosphere are investigated using satellite measurements from Stratospheric Sounding Unit(SSU) outputs and simulations from chemistry–climate models(CCMs) and the Coupled Model Intercomparison Project Phase 6(CMIP6). Observational evidence shows a lack of cooling in the Antarctic, in contrast to strong cooling at other latitudes, during austral winter over 1979–97. Analysis of CCM simulations for a longer period of1961–97 also shows a significant contrast in the...  相似文献   

8.
We test for causality between radiative forcing and temperature using multivariate time series models and Granger causality tests that are robust to the non-stationary (trending) nature of global climate data. We find that both natural and anthropogenic forcings cause temperature change and also that temperature causes greenhouse gas concentration changes. Although the effects of greenhouse gases and volcanic forcing are robust across model specifications, we cannot detect any effect of black carbon on temperature, the effect of changes in solar irradiance is weak, and the effect of anthropogenic sulfate aerosols may be only around half that usually attributed to them.  相似文献   

9.
RCP4.5: a pathway for stabilization of radiative forcing by 2100   总被引：3，自引：2，他引：1  
Representative Concentration Pathway (RCP) 4.5 is a scenario that stabilizes radiative forcing at 4.5?W?m?2 in the year 2100 without ever exceeding that value. Simulated with the Global Change Assessment Model (GCAM), RCP4.5 includes long-term, global emissions of greenhouse gases, short-lived species, and land-use-land-cover in a global economic framework. RCP4.5 was updated from earlier GCAM scenarios to incorporate historical emissions and land cover information common to the RCP process and follows a cost-minimizing pathway to reach the target radiative forcing. The imperative to limit emissions in order to reach this target drives changes in the energy system, including shifts to electricity, to lower emissions energy technologies and to the deployment of carbon capture and geologic storage technology. In addition, the RCP4.5 emissions price also applies to land use emissions; as a result, forest lands expand from their present day extent. The simulated future emissions and land use were downscaled from the regional simulation to a grid to facilitate transfer to climate models. While there are many alternative pathways to achieve a radiative forcing level of 4.5?W?m?2, the application of the RCP4.5 provides a common platform for climate models to explore the climate system response to stabilizing the anthropogenic components of radiative forcing.  相似文献   

10.
Increasing greenhouse gases and likely ozone recovery will be the two most important factors influencing changes in stratospheric temperatures in the 21st century. The radiative effect of increasing greenhouse gases will cause cooling in the stratosphere, while ozone recovery will lead to stratospheric warming. To investigate how stratospheric temperatures change under the two opposite forcings in the 21st century, we use observed ozone and reanalysis data as well as simulation results from four coupled oceanic and atmo- spheric general circulation models （GISS-ER, GFDL-CM20, NCAR-CCSM3, and UKMO-HadCM3） used in the IPCC （Intergovernment Panel for Climate Change） Fourth Assessment Report （AR4）. Observational analysis shows that total column ozone and lower stratospheric temperatures all show increasing in the past 10 years, while middle stratospheric temperatures demonstrate cooling. IPCC AR4 simulations show that greenhouse forcing alone will lead to stratospheric cooling. However, with forcing of both increasing greenhouse gases and ozone recovery, the middle stratosphere will be cooled, while the lower stratosphere will be warmed. Warming magnitudes vary from one model to another. UKMO-HadCM3 generates relatively strong warming for all three greenhouse scenarios, and warming extends to 40 hPa. GFDL-CM20 and NCAR-CCSM3 produce weak warming, and warming mainly exists at lower levels, below about 60 hPa. In addition, we also discuss the effect of temperature changes on ozone recovery.  相似文献   

11.
 The potential of aircraft-induced ozone changes to force a substantial climate impact is investigated by means of simulations with an atmospheric general circulation model, coupled to a mixed layer ocean model. We present results from several numerical experiments that are based on ozone change patterns for 1992 aviation and on a future scenario for the year 2015. In both cases, the climate signal is statistically significant. The strength of the ozone impact is of comparable magnitude to that arising from aircraft CO2 emissions, thus meaning a non-negligible contribution to the total climate effect of aviation emissions. There are indications of a characteristic signature of the aircraft ozone related temperature response pattern, distinctly different from that associated with the increase of well-mixed greenhouse gases. Likewise, the climate sensitivity to non-uniform ozone changes including a strong concentration perturbation at the tropopause may be higher than the climate sensitivity to uniform changes of a greenhouse gas. In a hierarchy of experiments, for which the spatial structure of an aircraft-related ozone perturbation was left fixed, while the amplitude of the perturbation was artificially increased, the climate signal depends in a non-linear way on the radiative forcing. Received: 10 September 1998 / Accepted: 4 May 1999  相似文献   

12.
Anthropogenic aerosols play an important role in the atmospheric energy balance. Anthropogenic aerosol optical depth (AOD) and its accompanying shortwave radiative forcing (RF) are usually simulated by nu- merical models. Recently, with the development of space-borne instruments and sophisticated retrieval algorithms, it has become possible to estimate aerosol radiative forcing based on satellite observations. In this study, we have estimated shortwave direct radiative forcing due to anthropogenic aerosols over oceans in all-sky conditions by combining clouds and the Single Scanner Footprint data of the Clouds and Earth’s Radiant Energy System (CERES/SSF) experiment, which provide measurements of upward shortwave fluxes at the top of atmosphere, with Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol and cloud products. We found that globally averaged aerosol radiative forcing over oceans in the clear-sky conditions and all-sky conditions were -1.03±0.48 W m-2 and -0.34 ±0.16 W m-2, respectively. Direct radiative forcing by anthropogenic aerosols shows large regional and seasonal variations. In some regions and in particular seasons, the magnitude of direct forcing by anthropogenic aerosols can be comparable to the forcing of greenhouse gases. However, it shows that aerosols caused the cooling effect, rather than warming effect from global scale, which is different from greenhouse gases.  相似文献   

13.
We summarize an on-line coupled meteorological–emissions–photochemical modelling system that allows feedback from air-quality/chemistry to meteorology via radiative forcing. We focus on the radiative-forcing impacts (direct effects) of ozone. We present an application of the coupled modelling system to the episode of 23–31 July 1998 in Portland, Oregon, U.S.A. Results suggest that the inclusion of radiative-forcing feedback produces small but accountable impacts. For this region and episode, stand-alone radiative transfer simulations, i.e., evaluating the effects of radiative forcing independently of changes in meteorology or emissions, suggest that a change of 1 ppb in ground-level ozone is approximately equivalent to a change of 0.017 W m−2 in radiative forcing. In on-line, coupled, three-dimensional simulations, where the meteorological dependencies are accounted for, domain-wide peak ozone concentrations were higher by 2–4 ppb (relative to a simulated peak of 119.4 ppb) when including the effects of radiative-forcing feedback. A scenario of 10% reduction in anthropogenic emissions produced slightly larger decreases in ozone, an additional 1 ppb in local-peak reductions, relative to scenarios without feedback.  相似文献   

14.
温室气体和硫酸盐气溶胶的辐射强迫作用   总被引：5，自引：4，他引：5  
对GOALS4 .0海 陆 气耦合模式的相关部分进行了改进 ,主要改进包括温室气体的扩充和硫酸盐气溶胶“显式”方案的引入 ,并引入 2 0世纪温室气体的实际浓度变化以及硫循环模式模拟的硫酸盐气溶胶的三维全球浓度分布 ,模拟了温室气体和硫酸盐气溶胶造成的辐射强迫的空间分布和时间变化。全球平均的温室气体和硫酸盐气溶胶的辐射强迫分别为 2 .17W /m2 和 - 0 .2 9W /m2 ;温室气体造成的辐射强迫在空间上呈现明显的纬向结构 ,最大值 (大于 2 .5W/m2 )和最小值 (小于 1W /m2 )分别位于副热带和两极地区 ,在北半球主要工业区硫酸盐气溶胶的辐射强迫绝对值接近温室气体的辐射强迫值 (大于 - 2 .0W /m2 )。  相似文献   

15.
Continuous emissions of anthropogenic greenhouse gases(GHGs) and aerosols in the last 160 years have resulted in an increasing trend of global mean surface temperatures(GMSTs). Due to interactions with natural variability,rates of the combined anthropogenically and naturally induced warming trends are characterized by significant slowdowns and speedups on decadal timescales. Here, by analyzing observed and model-simulated data, we investigate how the duration of these episodes will change with different strengths of GHG and aerosol forcing. We found that the duration of warming slowdowns can be more than 30 yr with a slower rate of anthropogenic emissions but would shorten to about 5 yr with a higher one. This duration reduction depends on both the magnitude of the climate response to anthropogenic forcing and the strength of the internal variability. Moreover, the warming slowdowns can still occur even towards the end of this century under high emissions scenarios but with significantly shortened duration.  相似文献   

16.
水文循环过程受气候变化与人类活动的共同作用,区分气候内部自然变率与人类活动作用于水循环贡献对于增加气候变化的理解非常重要。本研究利用近期发展的考虑地下水取用水与灌溉影响的全球陆气耦合模式进行数值模拟,基于最优指纹法分析探讨中国东部季风区黄河、淮河、海河、珠江、长江、松花江流域水循环变化(地表温度、降水、径流、蒸散发)及归因。结果表明:大部分流域的地表温度年际变化在1965~2005年间检测到包括温室气体气溶胶人为排放、臭氧与土地利用变化产生的外强迫效应,显示在长期对于地表温度起主要作用的可能为上述强迫;1965~2005年降水年际变化仅在淮河及长江下游检测到上述强迫效应,且在长江下游效应占主导。在1965~1984年间,地表温度的年际变化在海河流域检测到由于地下水取水灌溉产生的外强迫效应,并且该效应占主导。在1982~2005年径流年际变化中,在淮河、长江下游及黄河下游处检测到了由于温室气体排放、气溶胶人为排放、臭氧变化及土地利用变化等产生的外强迫效应但无法有效分离,显示该信号在这些地区可能不为主导效应;1982~2005年间的蒸散发年际变化在珠江、长江下游同样检测到了上述强迫效应,并且该效应在长江下游占主导效应。  相似文献   

17.
Climate policies must consider radiative forcing from Kyoto greenhouse gases, as well as other forcing constituents, such as aerosols and tropospheric ozone that result from air pollutants. Non-Kyoto forcing constituents contribute negative, as well as positive forcing, and overall increases in total forcing result in increases in global average temperature. Non-Kyoto forcing modeling is a relatively new component of climate management scenarios. This paper describes and assesses current non-Kyoto radiative forcing modeling within five integrated assessment models. The study finds negative forcing from aerosols masking (offsetting) approximately 25 % of positive forcing in the near-term in reference non-climate policy projections. However, masking is projected to decline rapidly to 5–10 % by 2100 with increasing Kyoto emissions and assumed reductions in air pollution—with the later declining to as much as 50 % and 80 % below today’s levels by 2050 and 2100 respectively. Together they imply declining importance of non-Kyoto forcing over time. There are however significant uncertainties and large differences across models in projected non-Kyoto emissions and forcing. A look into the modeling reveals differences in base conditions, relationships between Kyoto and non-Kyoto emissions, pollution control assumptions, and other fundamental modeling. In addition, under climate policy scenarios, we find air pollution and resulting non-Kyoto forcing reduced to levels below those produced by air pollution policies alone—e.g., China sulfur emissions fall an additional 45–85 % by 2050. None of the models actively manage non-Kyoto forcing for climate implications. Nonetheless, non-Kyoto forcing may be influencing mitigation results, including allowable carbon dioxide emissions, and further evaluation is merited.  相似文献   

18.
Sulfur hexafluoride (SF6), perfluoromethane (CF4) and perfluoroethane (C2F6) are strong greenhouse gases with long (>1000 year) atmospheric residence times. We derive emission factors for the major anthropogenic sources and project future emissions for 5 regions and the world. Although firms in many industrialized countries are already limiting emissions, without further policy intervention global emissions will rise 150% (CF4 and C2F6) and 210% (SF6) between 1990 and 2050; radiative forcing will increase 0.026 W m-2. Full application of available low-cost and costless policies in industrialized nations would cut that radiative forcing by one-quarter. Increased forcing due to these gases is small (<2%) relative to other gases but permanent on the timescale of human civilization. We also quantify plausible manipulations to governmental data that will be used to determine compliance with the 1997 Kyoto Protocol, which includes commitments for industrialized countries to regulate these and other greenhouse gases. More complete and transparent data are urgently needed. West European nations, for example, can cut their emissions of these gases by half by 2010 simply by manipulating emission factors within the current bounds of uncertainty.  相似文献   

19.
 The concept of radiative forcing has been extensively used as an indicator of the potential importance of climate change mechanisms. It allows a first order estimate of the global-mean surface temperature change; and it is possible to compare forcings from different mechanisms, on the assumption that similar global-mean forcings produce similar global-mean surface temperature changes. This study illustrates two circumstances where simple models show that the conventional definition of radiative forcing needs refining. These problems arise mainly with the calculation of forcing due to stratospheric ozone depletion. The first part uses simple arguments to produce an alternative definition of radiative forcing, using a time-dependent stratospheric adjustment method, which can give different forcings from those calculated using the standard definition. A seasonally varying ozone depletion can produce a quite different seasonal evolution of forcing than fixed dynamical heating arguments would suggest. This is especially true of an idealised and extreme “Antarctic ozone hole” type scenario where a sudden loss of ozone is followed by a sudden recovery. However, for observed ozone changes the annually averaged forcing is usually within 5% of the forcing calculated using the fixed dynamical heating approximation. Another problem with the accepted view of radiative forcing arises from the definition of the tropopause considered in the second part of this study. For a correct radiative forcing estimate the “tropopause” needs to separate the atmosphere into regions with a purely radiative response and those with a radiative-convective response. From radiative-convective model results it is found that radiative equilibrium conditions persist for several kilometres below the tropopause (the tropopause being defined as where the lapse rate reaches 2 K km-1). This region needs to be included in stratospheric adjustment calculations for an accurate calculation of forcing, as it is only the region between the surface and the top of the convection that can be considered as a single, forced, system. Including temperature changes in this region has a very large effect on stratospheric ozone forcing estimates, and can reduce the magnitude of the forcing by more than a factor of two. Although these experiments are performed using simple climate models, the results are of equal importance for the analysis of forcing-response relationships using general circulation models. Received: 25 October 1996/Accepted: 14 April 1997  相似文献   

20.
硫酸盐和烟尘气溶胶辐射特性及辐射强迫的模拟估算   总被引：21，自引：6，他引：21       下载免费PDF全文
张立盛  石广玉 《大气科学》2001,25(2):231-242
利用已有的硫酸盐和烟尘气溶胶折射指数资料，精确计算了这两种气溶胶从太阳短波到红外谱段的辐射特性。然后，在LLNL化学输送模式(CTM)模拟的硫酸盐和烟尘气溶胶资料及改进的气溶胶参数化基础上，在国内首次用GCM估算了这两种气溶胶引起的全球辐射强迫。结果表明:(1)西欧是全球最大的硫酸盐辐射强迫中心，最大值出现在夏季，达-5.0W/m2；(2)烟尘强迫的最大中心出现在夏季的南美和非洲中南部，为4.0W/m2；(3)南半球大陆人为气溶胶的强迫不容忽视；(4)某些地区人为气溶胶的强迫在量值上可与CO2等温室气体引起的强迫相比拟。  相似文献   

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