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1.
Paolo Laj Andrea I. Flossmann Wolfram Wobrock Sandro Fuzzi Giordano Orsi Loretta Ricci Stephan Mertes Alfons Schwarzenbck Jost Heintzenberg Harry Ten Brink 《Atmospheric Research》2001,58(4):256
We investigated the partitioning of trace substances during the phase transition from supercooled to mixed-phase cloud induced by artificial seeding. Simultaneous determination of the concentrations of H2O2, NH3 and black carbon (BC) in both condensed and interstitial phases with high time resolution showed that the three species undergo different behaviour in the presence of a mixture of ice crystals and supercooled droplets. Both H2O2 and NH3 are efficiently scavenged by growing ice crystals, whereas BC stayed predominantly in the interstitial phase. In addition, the scavenging of H2O2 is driven by co-condensation with water vapour onto ice crystals while NH3 uptake into the ice phase is more efficient than co-condensation alone. The high solubility of NH4+ in the ice could explain this result. Finally, it appears that the H2O2–SO2 reaction is very slow in the ice phase with respect to the liquid phase. Our results are directly applicable for clouds undergoing limited riming. 相似文献
2.
在可压缩三维冷云数值模式里对冰晶繁生过程进行了参数化,显式考虑了过冷滴冻结破裂和Hallett-Mossop两个繁生机制,并对冰晶浓度进行了订正。对暖底孤立积云的模拟实例表明繁生作用对对流系统宏观特征没有显著改变,地面总降水略有增加,最大雨强增大且时间提前。繁生过程的主要作用是改变了云的微物理结构特征,使云中冰化时间提早,冰化程度大大加强,引起云上部增暖并抬高云顶。在所考虑的两个繁生机制中,冻结破裂繁生机制是引起微物理结构发生变化的主要过程。还对各冰相微物理过程的相对作用进行了分析。 相似文献
3.
Prof. K. N. Liou J. L. Lee S. C. Ou Q. Fu Y. Takano 《Meteorology and Atmospheric Physics》1991,46(1-2):41-50
Summary Parameterization programs for cloud microphyscs and radiative transfer involving ice clouds have been developed in terms of the mean effective size and ice water path. The mean effective size appears to be adequate in representing the ice crystal size distribution for radiative parameterizations. For a given ice water path, smaller mean effective sizes reflect more solar radiation, emit more IR radiation and enhance net radiative heating/cooling at the cloud top and bottom than larger sizes. The presence of small ice crystals may generate steeper lapse rates in clouds. A 3-D global cloud model that prescribes the horizontal wind fields in a 24 hour period is used to investigate the sensitivity of the mean effective size of ice crystals on the simulation of radiative heating, temperature, cloud cover and ice water content. A variation in the mean effective size from 75 to 50 m in a 24 hour prediction on simulation generates more cooling above the high cloud top and a decrease of temperature. These results lead to an increase of high cloud cover in some latitudes by as much as 4% and, at the same time, a decrease of middle cloud cover by 3–4% in latitudes between 60°S and 60°N.With 7 Figures 相似文献
4.
Two-moment bulk stratiform cloud microphysics in the grid-point atmospheric model of IAP LASG (GAMIL) 总被引：1，自引：0，他引：1
A two-moment bulk stratiform microphysics scheme, including recently developed physically-based droplet activation/ice nucleation parameterizations has been implemented into the Grid-point Atmospheric Model of IAP LASG (GAMIL) as an effort to enhance the model’s capability to simulate aerosol indirect effects. Unlike the previous one-moment cloud microphysics scheme, the new scheme produces a reasonable representation of cloud particle size and number concentration. This scheme captures the observed spatial variations in cloud droplet number concentrations. Simulated ice crystal number concentrations in cirrus clouds qualitatively agree with in situ observations. The longwave and shortwave cloud forcings are in better agreement with observations. Sensitivity tests show that the column cloud droplet number concentrations calculated from two different droplet activation parameterizations are similar. However, ice crystal number concentration in mixed-phased clouds is sensitive to different heterogeneous ice nucleation formulations. The simulation with high ice crystal number concentration in mixed-phase clouds has less liquid water path and weaker cloud forcing. Furthermore, ice crystal number concentration in cirrus clouds is sensitive to different ice nucleation parameterizations. Sensitivity tests also suggest that the impact of pre-existing ice crystals on homogeneous freezing in old clouds should be taken into account. 相似文献
5.
Andr Ehrlich Manfred Wendisch Eike Bierwirth Andreas Herber Alfons Schwarzenbck 《Atmospheric Research》2008,88(3-4):266-276
Based on 1-year cloud measurements with radar and microwave radiometer broadband solar radiative transfer simulations were performed to quantify the impact of different ice crystal shapes of Arctic mixed-phase clouds on their radiative properties (reflectance, transmittance and absorptance). The ice crystal shape effects were investigated as a function of microphysical cloud properties (ice volume fraction fi, ice and liquid water content IWC and LWC, mean particle diameter DmI and DmW of ice/water particle number size distributions, NSDs).The required NSDs were statistically derived from radar data. The NSD was composed of a liquid and a solid mode defined by LWC, DmW (water mode) and IWC, DmI (ice mode). It was found that the ratio of DmI and DmW determines the magnitude of the shape effect. For mixed-phase clouds with DmI ≤ 27 μm a significant shape effect was obtained. The shape effect was almost insensitive with regard to the solar zenith angle, but highly sensitive to the ice volume fraction of the mixed-phase cloud. For mixed-phase clouds containing small ice crystals (DmI ≤ 27 μm) and high ice volume fractions (fi > 0.5) crystal shape is crucial. The largest shape effects were observed assuming aggregates and columns. If the IWC was conserved the shape effect reaches values up to 0.23 in cloud reflectance and transmittance. If the ice mode NSD was kept constant only a small shape effect was quantified (≤ 0.04). 相似文献
6.
The paper focuses on the redistribution of aerosol particles (APs) during the artificial nucleation and subsequent growth of ice crystals in a supercooled cloud. A significant number of the supercooled cloud droplets during icing periods (seeding agents: C3H8, CO2) did not freeze as was presumed prior to the experiment but instead evaporated. The net mass flux of water vapour from the evaporating droplets to the nucleating ice crystals (Bergeron–Findeisen mechanism) led to the release of residual particles that simultaneously appeared in the interstitial phase. The strong decrease of the droplet residuals confirms the nucleation of ice particles on seeding germs without natural aerosol particles serving as ice nuclei. As the number of residual particles during the seedings did not drop to zero, other processes such as heterogeneous ice nucleation, spontaneous freezing, entrainment of supercooled droplets and diffusion to the created particle-free ice germs must have contributed to the experimental findings. During the icing periods, residual mass concentrations in the condensed phase dropped by a factor of 1.1–6.7, as compared to the unperturbed supercooled cloud. As the Bergeron–Findeisen process also occurs without artificial seeding in the atmosphere, this study demonstrated that the hydrometeors in mixed-phase clouds might be much cleaner than anticipated for the simple freezing process of supercooled droplets in tropospheric mid latitude clouds. 相似文献
7.
华北秋季一次低槽冷锋积层混合云宏微物理特征与催化响应分析 总被引：2，自引：0，他引：2
利用2013年10月13日机载粒子测量系统（PMS）在张家口涞源地区对积层混合云中上部进行的增雨探测数据,分析了云的垂直微物理结构、云区的可播性和作业前后液态云粒子、冰晶及降水粒子的微物理变化。结果表明,此次降水性积层混合云的垂直结构由冷、暖两层云配置,云层发展厚实,冷云区云粒子浓度平均为62 cm-3,液态水含量最大0.05 g/m3;2DC和2DP探测的冰晶及降水粒子平均浓度分别为1.9和2.2 L-1;暖云内云粒子数浓度集中在300 cm-3左右,液态水含量约0.1 g/m3。探测区域云粒子数浓度的水平分布不均匀。利用云内过冷水含量和冰晶浓度等参数判断,该降水性积层混合云的播撒作业层具有强可播性。对比作业前后云中粒子浓度及平均直径发现,云粒子在作业前时段内的平均浓度为31 cm-3,远高于作业后平均浓度（17.6 cm-3）;但平均直径变化不大。作业后冰晶粒子通过贝吉龙过程消耗过冷水长大,浓度由之前的0.86 L-1增至4.27 L-1,平均直径也增至550 μm。冰晶粒子逐渐长大形成降水,降水粒子浓度也相应有所升高,谱明显变宽。 相似文献
8.
J. Rosinski 《Atmospheric Research》1991,26(6)
Some cloud condensation nuclei (CCN) constitute a reservoir of latent ice-forming nuclei (IFN) active by condensation-followed-by-freezing and by sorption. Evaporated droplets occasionally left aerosol particles that acted as sorption IFN at temperatures as high as −5°C and water vapor supersaturation over ice of 0.2%. The newly formed aerosol particles (residues of evaporated droplets) are all mixed particles. The discovery of IFN produced from CCN promotes new insights into the process of ice formation in clouds; in an evaporating parcel of a cloud the rate of formation of ice particles will be enhanced by continuous production of IFN. Aerosol particles left behind after evaporation of a cloud may provide a source of IFN for formation of some of the cirrus clouds. 相似文献
9.
The potential effects of ice microphysics involving ice crystal size distribution and ice water path (IWP) on climatic temperature perturbations are investigated by using a one-dimensional radiative-turbulent climate model. We define a mean effective size, denoting the width of ice crystals weighted by the geometric cross section area, to represent ice crystal size distribution. Based on aircraft measurements, both the mean effective size and IWP are related to temperature and may be parameterized as functions of temperature. The radiative properties of cirrus clouds are further parameterized in terms of these two basic cloud physics parameters. Using CO2 doubling as the radiative forcing, feedbacks among temperature, the mean effective size and IWP, and the radiative properties of clouds are analyzed from the model results. We show that overall, a positive feedback associated with ice microphysics and the coupled radiative transfer is produced by temperature increase. 相似文献
10.
Measurements of natural ice nuclei were made in winter continental airmasses with a continuous flow thermal gradient diffusion chamber (described in a separate paper). Over the range of temperatures −7°C to −20°C, the concentration of ice nuclei was closely related to ice supersaturation (SSi) for humidities both below and above water saturation. Measurements below water saturation were interpreted as deposition nuclei with average concentrations (per liter) approximately 0.32 SSi(%)0.81. Measurements were made up to 5% above water saturation and activated both deposition and condensation-freezing nuclei. The average concentration of condensation-freezing nuclei was 0.25 e−0.15 T(°C). Sample residence time in the chamber was probably too small to detect contact nuclei, unless the nucleating aerosols are extremely small. There was large variability in nucleus concentrations, as much as two orders of magnitude at −15°C. Comparisons are made between these ice nuclei measurements and aircraft observations of ice crystal concentrations in winter orographic clouds. 相似文献
11.
青海秋季对流云降水及催化过程数值模拟研究 总被引：5，自引：3，他引：5
利用CAMS三维对流云模式和青海省河南县秋季外场试验取得的资料，对自然云的发展演变过程进行了数值模拟试验。进一步就催化时间、催化剂量对增雨效果的影响进行了数值试验。结果表明，该地区秋季对流云降水主要为冷云降水，冰晶是霰产生的主要来源，冰霰自动转化是霰产生的最主要方式，冰晶与霰的碰并又促进了霰的进一步增长，霰是云中过冷水消耗的主要因素。人工播撒催化剂应在冰核活化过程大量开始以前进行，以达到增加冰晶浓度，消耗过冷云水，从而增加降水的目的。 相似文献
12.
利用2013～2016年的Aqua MODIS卫星和CloudSat卫星的二级产品资料,对发生在京津冀地区夏季的降水冰云和非降水冰云进行了统计。基于此,对比分析了两类冰云的云类型,研究了二者在云特征参数、云层数及垂直结构上的差异,并且探究了二者在不同通道下云特征参数的相对大小。结果表明:1）京津冀地区的降水冰云以深对流云和雨层云为主,分别占48.63%和34.65%,而非降水冰云以高层云和卷云为主,分别占55.62%和31.58%。2）降水冰云和非降水冰云的平均云顶温度、云顶高度、光学厚度、积分云水总量、有效粒子半径分别为230.99 K、10.90 km、53.26、937.98 g/m2、31.45
13.
14.
利用红外高光谱探测仪（Infrared Atmospheric Sounding Interferometer,IASI）在二氧化碳吸收带的长短波红外通道对云反应程度的不同来探测云。依据不同通道的权重函数峰值高度和云不敏感层高度将IASI长短波红外通道进行配对,成功配对的长短波红外通道晴空亮温之间建立线性回归模型,即通过长波红外通道亮温可以线性回归得到配对的短波通道亮温,将短波通道的晴空回归亮温和观测亮温之差定义为云指数。权重函数峰值高度位于383 hPa的云指数空间分布和云成分为冰的空间分布较为一致,尤其在赤道和低纬度地区。权重函数峰值高度位于790 hPa的云指数空间分布和低云云顶气压也有较好的一致性。 相似文献
15.
Wolfram Wobrock Andrea I. Flossmann Marie Monier Jean-Marc Pichon Laurent Cortez Jean-Franois Fournol Alfons Schwarzenbck Stephan Mertes Jost Heintzenberg Paolo Laj Giordano Orsi Loretta Ricci Sandro Fuzzi Harry Ten Brink Piet Jongejan Ren Otjes 《Atmospheric Research》2001,58(4):7907
The second field campaign of the Cloud Ice Mountain Experiment (CIME) project took place in February 1998 on the mountain Puy de Dôme in the centre of France. The content of residual aerosol particles, of H2O2 and NH3 in cloud droplets was evaluated by evaporating the drops larger than 5 μm in a Counterflow Virtual Impactor (CVI) and by measuring the residual particle concentration and the released gas content. The same trace species were studied behind a round jet impactor for the complementary interstitial aerosol particles smaller than 5 μm diameter. In a second step of experiments, the ambient supercooled cloud was converted to a mixed phase cloud by seeding the cloud with ice particles by the gas release from pressurised gas bottles. A comparison between the physical and chemical characteristics of liquid drops and ice particles allows a study of the fate of the trace constituents during the presence of ice crystals in the cloud.In the present paper, an overview is given of the CIME 98 experiment and the instrumentation deployed. The meteorological situation during the experiment was analysed with the help of a cloud scale model. The microphysics processes and the behaviour of the scavenged aerosol particles before and during seeding are analysed with the detailed microphysical model ExMix. The simulation results agreed well with the observations and confirmed the assumption that the Bergeron–Findeisen process was dominating during seeding and was influencing the partitioning of aerosol particles between drops and ice crystals. The results of the CIME 98 experiment give an insight on microphysical changes, redistribution of aerosol particles and cloud chemistry during the Bergeron–Findeisen process when acting also in natural clouds. 相似文献
16.
THE MICROPHYSICAL STRUCTURE OF SNOW CLOUDS AND THE GROWTH PROCESS OF SNOW PARTICLES IN WINTER IN XINJIANG 
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下载免费PDF全文 The microphysical structure of snow clouds and the growth process of snow crystals were observed by means of instrumented aircraft,weather radar,snow crystal observations etc.in Urumqi region during the winter of 1982.The analysis of three cases show that about 70% of snow mass growth is produced in the lower layer below 2000 m under the cold front,and that the concentration of ice crystals is as high as 60 L-1 and the supercooled water is absent in lower clouds.We may infer that the deposition of ice crystals and the aggregation of snow crystals are important processes for the snow development.The microphysical structure of the snow band near the front aloft and its characteristics as a seeder cloud are also described in this paper. 相似文献
17.
18.
I. P. Mazin 《Atmospheric Research》1995,35(2-4)
A large data set of the total (liquid and ice) cloud water content in continental stratiform clouds of middle latitudes was collected in the Cloud Physics Laboratory (CPL) of the Central Aerological Observatory (CAO). The total flight length in clouds was over 100,000 km. On the basis of these data, the cumulative frequencies of TCWC occurrences F(w) were found and parameterized by log-normal distributions which parameters depend on temperature. In the temperature interval from 0°C to −40°C the empirical values of F(w) deviate of no more than 5% from the parameterized ones.The new data, with a better probe detecting threshold, lead to a noticeable increase of the cases with small values of cloud water content and correspondingly, decrease of cloud water content characteristic values comparing with the values previously obtained by many authors. The difference increased with decreasing temperature. 相似文献
19.
《Atmospheric Research》2005,73(1-2):131-148
The effect of pollution-derived sulphuric acid aerosols on wintertime arctic lower atmospheric ice crystals is investigated. These anthropogenic aerosols differ from natural background aerosols by their number concentration, strong solubility and reduced homogeneous freezing temperature when internally mixed with other compounds. Furthermore, observations suggest that the ice-forming nuclei concentration is reduced by one to four orders of magnitude when the sulphuric acid aerosol concentration is high.Simulations performed using a column model and analysis of observed data for the period of 1991–1994 at Alert (82° 30'N, 62°20'W) are used to assess the changes of the boundary layer cloud characteristics by sulphuric acid aerosols and the potential effect on arctic climate. Results show that aerosol acidification leads to depletion of the ice crystal number concentration and an increase of its mean size. As a result, low-level precipitating ice crystals occur more frequently than ice fog and thick nonprecipitating clouds during high concentration of pollution-derived aerosols. This result is in agreement with observations that indicate an increase by more than 50% of the frequency of precipitating ice crystals when the weight proportion of sulphuric acid is greater than its mean value of 20% of the total aerosol mass. Consequently, the ice crystal size increases and number decreases, and the sedimentation flux of ice crystals and the dehydration rate of the lower troposphere are accelerated in the presence of high sulphuric acid aerosol concentration. As a result, the infrared radiation flux reaching the surface and the greenhouse effect are decreased. This process is referred to as the dehydration–greenhouse feedback. One-dimensional simulation for Alert during the period of 1991 to 1994 shows that a negative cloud radiative forcing of −9 W m−2 may occur locally as a result of the enhanced dehydration rate produced by the aerosol acidity. 相似文献
20.
Summary Crystal size and optical depth of optically thin cirrus clouds and contrails over the North Sea and Adriatic Sea on the 18th of October 1989 are retrieved by comparison of NOAA AVHRR/2 brightness temperatures of channel 4 (9.97 µm–11.56 µm) and channel 5 (11.075 µm–12.76 µm) with one dimensional radiative transfer calculations. Measured brightness temperatures in all three infrared channels and their differences show higher values for contrails than for cirrus. The radiative properties of young contrails are consistent only, if smaller crystal size than those given for natural cirrus are adopted for the calculations. However, there is a continuous transition in radiative parameters between clouds classified as natural cirrus or contrails. For the test areas ice clouds are classified with respect to optical depth and mean crystal size. Finally infrared fluxes and heating rates in the spectral range 4 µm–40 µm are calculated for an atmosphere with a 500 m thick contrail or cirrus uncinus. At given ice content a far stronger atmospheric warming is found for a contrail with relatively small ice crystals: up to 80 K/day at cloud base for an ice content of 0.05 gm–3 compared to 10 K/day for a cirrus uncinus with large crystals.With 11 Figures 相似文献