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1.
The absorption of anthropogenic CO2 and atmospheric deposition of acidity can both contribute to the acidification of the global ocean. Rainfall pH measurements and chemical compositions monitored on the island of Bermuda since 1980, and a long-term seawater CO2 time-series (1983–2005) in the subtropical North Atlantic Ocean near Bermuda were used to evaluate the influence of acidic deposition on the acidification of oligotrophic waters of the North Atlantic Ocean and coastal waters of the coral reef ecosystem of Bermuda. Since the early 1980's, the average annual wet deposition of acidity at Bermuda was 15 ± 14 mmol m− 2 year− 1, while surface seawater pH decreased by 0.0017 ± 0.0001 pH units each year. The gradual acidification of subtropical gyre waters was primarily due to uptake of anthropogenic CO2. We estimate that direct atmospheric acid deposition contributed 2% to the acidification of surface waters in the subtropical North Atlantic Ocean, although this value likely represents an upper limit. Acidifying deposition had negligible influence on seawater CO2 chemistry of the Bermuda coral reef, with no evident impact on hard coral calcification. 相似文献
2.
The study of aerosols and rainwater presented here demonstrates that episodic atmospheric deposition events associated with southeasterly flow are quantitatively significant for large areas of the North Atlantic Ocean. This paper considers aluminium and manganese, with predominantly crustal sources, and lead and zinc, which are mobilised into the atmosphere primarily through anthropogenic activity. High levels of all trace metals are associated with southeasterly flow from Europe as the air passes over heavily populated and industrialised regions before reaching the northeast Atlantic Ocean. Fluxes calculated using the 1% HNO3 acid soluble metal concentration show that, although the climatological norm for this area is westerly flow, short-lived southeasterly transport events dominate the input of trace metals to this ocean region. This material may be toxic to phytoplankton or may be represent a new source of nutrients to the biological community. A significant decrease in atmospheric lead levels in polluted air is seen between June 1996 and May 1997, reflecting the decrease in use of leaded fuels in Europe. Comparing atmospheric flux values to sediment trap metal fluxes shows that the atmosphere represents the dominant source of zinc to the deep ocean, whereas an additional, non-atmospheric, manganese source this required, perhaps from mobilisation of sedimentary material from the continental shelf or long range advection of manganese rich Saharan material. 相似文献
3.
A data base of 111 filter-collected marine atmospheric particulates is used to describe the distribution of lead over the North and South Atlantic, the Mediterranean Sea, the Red Sea, the Gulf of Aden and the northern and central Arabian Sea. The distribution of atmospheric Pb is assessed in terms of enrichment factor diagrams, and it is shown that over the marine regions studied in both the Northern and Southern Hemispheres the distribution of Pb in the atmosphere is controlled by the mixing of a background component, or components, with crustal material within certain concentration limits. For the Northern Hemisphere samples used in the investigation there is a reasonably well-defined Pb concentration minimum of ～ 0.6 ng m?3 of air; however, this will be severely decreased in more remote Northern Hemisphere marine regions. Geometric average Pb atmospheric concentrations vary from one marine region to another, ranging from ～ 0.98 ng m?3 of air for the South Atlantic westerlies to ～ 15 ng m?3 of air in the North Atlantic westerlies; although the latter reduces to ～ 7 ng m?3 of air when ‘polluted’ samples are excluded. Lead sea-surface deposition fluxes are calculated on the basis of two deposition velocities (0.25 and 1 cm s?1), the largest flux (220 ng Pb cm?2 yr?1) being found for the westerlies over the eastern margins of the North Atlantic. The distribution of lead over the North Atlantic is assessed in terms of the global lead budget and it is estimated that a maximum of ～ 24% of the total ‘natural’ lead injected annually into the World atmosphere, and ～ 3.5% of the anthropogenic lead injected annually into the Northern Hemisphere atmosphere, are deposited over the North Atlantic sea surface. 相似文献
4.
At present, in most oceans the lead (Pb) biogeochemical cycling has been disturbed by anthropogenic Pb through atmospheric input. The Pb concentrations in the upper water positively correlate with atmospheric input fluxes of Pb. The North Pacific is affected greatly by atmospheric substances via long-range transport from eastern Asia, especially from Mainland China. Mainland China may export considerable amounts of pollutants into the seas via rivers and the atmosphere owing to its recent fast growth in industry and economy. The East China Sea lies in an important geographical position--a transit between Mainland China and the western North Pacific. However, no data are available for seawater concentrations of Pb, a representative element with anthropogenic origin. In this work seawater samples from both 5 and 30-50 m water layers of 15 stations occupied over a cyclonic eddy in the southern East China Sea were analyzed for particulate Pb (PPb) and dissolved Pb (DPb). The Mean concentration of DPb (approximately 128 ng/l) in the southern East China Sea upper waters (< or = 50 m) is approximately several times higher than those in the Pacific; the high DPb concentrations in the southern East China Sea waters correspond to much higher atmospheric supplies of Pb to the East China Sea. Thus, this study partly fills the 'data gap' of the marginal seas. Also, it indicates that the East China Sea may be considerably contaminated by deposited polluted aerosols. Spatial distributions of DPb in the surface water show a tendency of increasing concentrations with distance offshore, that depends on the magnitudes of atmospheric Pb inputs and on particle scavenging processes. In contrast to DPb, spatial distributions of PPb basically display an 'omega'-like picture and a tendency of decreasing concentrations with distance offshore. These are related to riverine and scavenging sources and to the drive by the eddy. Additionally, the residence times of DPb in the surface water were estimated to be about 2 years, agreeing well with the reported data. 相似文献
5.
The ecosystem model ERSEM II has been used to hindcast the development of the ecosystem of the North Sea during the years 1955 to 1993. The simulation was driven by the box-aggregated output from a general circulation model of the North Sea of corresponding duration; radiation, river inputs, atmospheric input and boundary conditions at the borders to the Atlantic Ocean and to the Baltic Sea were applied as realistically as possible. The general features of the eutrophication process are reproduced in the hindcast: the coastal areas show strong changes in nutrient concentrations in the hindcast as well as in the observations. Eutrophication not only shows up in the nutrient concentrations, but also in primary production. The simulated spatial distributions of phosphate, nitrate and primary production compare well with the observed ones. In addition, the hindcast simulates considerable trend-like changes of the nutrients in the southern part of the North Sea, where the nutrients are transported from the continental coastal strip to the southern central North Sea. The line from the river Humber to southern Norway separates the region of noticeable anthropogenic influence of riverine and atmospheric input from the northern area, which is mainly influenced by the Atlantic nutrient inflow. The observed annual cycles in the central and northern North Sea are quite well reproduced by the hindcast. The comparison of the hindcast with the long-term observations at two sites in the continental coastal zone of the North Sea shows that the long-term behaviour of phosphate, nitrate and silicate is simulated well. Primary production is increased in summers during the main period of eutrophication, 1975 to 1989, in the hindcast and in the observations. The flagellates at Helgoland, however, experience much more pronounced annual cycles with much less interannual variability in the hindcast than in the observations. 相似文献
6.
1Introduction Sulfurisoneofthemostimportantelements whosebiogeochemicalcyclesarepivotaltotheatmo- sphericenvironmentandtotheclimaticchanges.The predominant,stablechemicalspeciesofsulfurinthe atmosphereissulfuricacidorsulfatewhichunderor- dinaryconditionsexistsmainlyinsmallaerosolparti- cles(Chinetal.,1996;Kerminenetal.,2000;Restadet al.,1998).Sulfuricacidorsulfate-dominatedaerosols areubiquitousintheloweratmosphere.Inthemarine boundarylayer(MBL),non-sea-saltsulfuricacidorsulfate(nss-SO42-)… 相似文献
7.
生物活性铁(Fe)进入生物地球化学循环中能够调节碳循环,影响海洋初级生产力,间接影响全球气候变化。决定Fe生物可利用度的关键因子是可溶Fe含量,其中大气气溶胶的长距离传输是上层海洋获取生物可利用Fe的重要来源。近年来,对气溶胶中的Fe及溶解度的研究取得了重要进展,包括对不同区域Fe质量浓度和溶解度的观测以及对Fe溶解度影响因素的讨论。基于以上研究成果,汇总了近二十年全球部分陆地和海洋站点观测所得的不同粒径气溶胶颗粒物中的Fe质量浓度及其溶解度数据;重点介绍了气溶胶沉降入海洋前影响Fe溶解度的主要因素,包括Fe的来源、大气物理过程以及大气化学和传输混合过程等,并就各影响因素间的关联及相对重要性展开讨论;对未来气溶胶Fe的研究方向和方法提出建议。 相似文献
8.
北欧海作为连接北冰洋和北大西洋的重要海域,其由热效应产生的辐合场值得关注。本文利用NECP/NCAR的速度势函数(Velocity Potential,VP)数据表征北欧海辐合辐散场,发现在秋冬季北欧海上空大气低层存在一个独立的辐合区域。经验正交函数分解结果表明,北欧海上空的VP显示出除了表征北极涛动的全区一致型模态外,还表现出一个东西向辐合辐散反位相的东西振荡型模态。该模态与一支连接北大西洋涛动(NAO)和欧亚遥相关(EU)的复合型大气遥相关波列有关,北欧海表层潜热和感热异常加热通过影响低空大气的异常辐合辐散,与北大西洋偶极子型海温异常加热共同作用,加强了NAO异常环流;同时高空急流波导作用加强了从北欧海到东亚的EU波列,使得位于NAO和EU之间的北欧海成为连接NAO和EU大气遥相关波列的“中继站”,进而通过这种复合型大气遥相关波列将北大西洋与东亚大气环流联系起来,形成对东亚地区天气气候的远程影响。 相似文献
9.
Atlantic multidecadal oscillation and its manifestations in the Atlantic-European region 总被引：2，自引：0，他引：2
A. B. Polonskii 《Physical Oceanography》2008,18(4):227-236
We present a brief survey of the works devoted to the investigation of the Atlantic Multidecadal Oscillation, i.e., of the
quasiperiodic variations of sea-surface temperature in the North Atlantic with typical time scales of 50–100 yr. This oscillation
is a manifestation of the natural variability in the ocean-atmosphere system. The characteristic scale of the Atlantic Multidecadal
Oscillation is determined by the speed of the meridional oceanic circulation in the North Atlantic. The analyzed oscillation
affects various climatic characteristics: air temperature, river discharge in the European and North-American regions, the
number and intensity of tropical cyclones in the Atlantic Ocean, and the parameters of mid-latitude cyclones and anticyclones
in the Atlantic-European region. The main mechanism by which the Atlantic Multidecadal Oscillation affects the climatic characteristics
of the regions neighboring with the North Atlantic is the atmospheric response to the thermal anomalies in the ocean leading
to a shift of the centers of atmospheric action and to the changes in the intensity and predominant directions of propagation
of atmospheric cyclones and anticyclones. By using the results of long-term instrumental observations carried out in Eastern
Europe and the data array of reconstructed temperature in the Alpine region, it is shown that the Atlantic Multidecadal Oscillation
is responsible for a significant part of low-frequency variations of temperature in Europe. This fact confirms the potential
predictability of the regional atmospheric manifestations of the Atlantic Multidecadal Oscillation on the decadal-scale.
Translated from Morskoi Gidrofizicheskii Zhurnal, No. 4, pp. 69–79, July–August, 2008. 相似文献
10.
北大西洋秋季“三极子”海温结构对冬季大气环流场的影响 总被引：1，自引：0，他引：1
利用NCEP再分析资料、Hadley中心的海表面温度(SST)资料等,从北大西洋秋季海表面温度异常(SSTA)变化入手,对其影响后期冬季大气环流场的机制进行了分析。研究结果如下:(1)北大西洋SST异常与大气环流异常之间存在着相互作用;(2)秋季北大西洋SSTA具有较好的持续性,"正负正"海温异常空间分布导致12月巴伦支海上空500hPa位势高度异常偏高;(3)异常环流形势对应的海表面风异常场(SSWA)通过阶段性风-蒸发-SST异常反馈机制(WES机制)利于海温异常分布的持续及对上空异常大气环流的反馈;(4)三极子海温结构中负异常海温自10月份开始有自西向东的移动,风作用下蒸发加大,伴随上升运动自欧洲西部爱尔兰群岛出现自西向东移动的降水正异常区,潜热释放有利于冬季巴伦支海上空的异常高压脊发展。研究表明,北大西洋秋季SSTA通过阶段性海气相互作用机制影响海洋温度分布和大气环流异常,对后期冬季中国东北部的气候变化产生影响。 相似文献
11.
Concentrations of dissolved Ni, Cu, Zn, Cd and Pb were measured in water samples collected during a cruise with R.V Pelagia (29-6/14-7-1993) in the northern North Sea and N.E. Atlantic Ocean. At least six depths (0–90 m) were sampled with modified Go-Flo samplers from a rubber zodiac. In the study area, the first 25 m were well mixed and stratification occurred below this depth. The local bloom of Emiliania huxleyi hardly affected the trace metals concentration, except for some removal of Cd as seen from its correlation with nitrate. The mean dissolved concentrations were for Ni (3.66 nM), Cu (1.61 nM), Zn (4.5 nM), Cd (48 pM) and Pb (108 pM). These concentrations are among the lowest reported for the North Sea and are of similar magnitude to those found in the eastern North Atlantic at the same latitude. Zn was the only exception with values 10 times higher compared to those in the Atlantic Ocean, suggesting external inputs, mainly atmospheric and possibly from surrounding land masses. The observed ratio Zn:Cd in the North Sea and estuaries is in between the high ratio 600–900 for continental sources and the low ratio 5–10 for oceanic waters. Latter low ratio is consistent with the 21-fold stronger inorganic complexation of Cd in seawater which, in combination with the preferential biological uptake of Zn, may lead to the observed about hundredfold fractionation of Zn versus Cd in the marine system. Other processes may play a role but would need further investigation. The dissolved Pb values tend to be lower than found before in the North Sea, indicating decreasing inventories due to reduced anthropogenic emissions. 相似文献
12.
The study focuses on investigating significant wave height, including both mean and extreme values, in the North Atlantic in winter during the period from 1979 to 2010. We perform a 32-year wind wave hindcast for the North Atlantic using a spectral ocean wave model (WaveWatch III) and a high-resolution nonhydrostatic atmospheric model (WRF-ARW), which provides the wind forcing function. Analysis of the 32-year hindcast of wave characteristics in the North Atlantic reveals stronger mean and extreme waves simulated with high resolution modeling systems and identifies significant downward trends in the mean significant wave height in the subpolar North Atlantic. Such trends were not found in the wave characteristics from ERA-Interim reanalysis. At the same time, the 32-year hindcast did not confirm the statistically significance of strong positive trends in the central Atlantic diagnosed by ERA-Interim reanalysis; differences between the reanalysis and hindcast are discussed. 相似文献
13.
A. M. Macdonald M. O. Baringer R. Wanninkhof K. Lee D. W. R. Wallace 《Deep Sea Research Part II: Topical Studies in Oceanography》2003,50(22-26):3041
In January and February 1998, when an unprecedented fourth repetition of the zonal hydrographic transect at 24.5°N in the Atlantic was undertaken, carbon measurements were obtained for the second time in less than a decade. The field of total carbon along this section is compared to that provided by 1992 cruise which followed a similar path (albeit in a different season). Consistent with the increase in atmospheric carbon levels, an increase in anthropogenic carbon concentrations of 8±3 μmolkg−1 was found in the surface layers. Using an inverse analysis to determine estimates of absolute velocity, the flux of inorganic carbon across 24.5° is estimated to be −0.74±0.91 and −1.31±0.99 PgCyr−1 southward in 1998 and 1992, respectively. Estimates of total inorganic carbon flux depend strongly upon the estimated mass transport, particularly of the Deep Western Boundary Current. The 1998 estimate reduces the large regional divergence in the meridional carbon transport suggested by previous studies and brings into question the idea that the tropical Atlantic constantly outgasses carbon, while the subpolar Atlantic sequesters it. Uncertainty in the carbon transports themselves, dominated by the uncertainty in the total mass transport estimates, are a hindrance to determining the “true” picture.The flux of anthropogenic carbon (CANTH) across the two transects is estimated as northward at 0.20±0.08 and 0.17±0.06 PgCyr−1 for the 1998 and 1992 sections, respectively. The net transport of CANTH across 24.5°N is strongly affected by the difference in concentrations between the northward flowing shallow Florida Current and the mass balancing, interior return flow. The net northward transport of CANTH is opposite the net flow of total carbon and suggests, as has been found by others, that the pre-industrial southward transport of carbon within the Atlantic was stronger than it is today. Combining these flux results with estimates of atmospheric and riverine inorganic carbon input, it is determined that today's oceanic carbon system differs from the pre-industrial system in that today there is an uptake of anthropogenic carbon to the south that is advected northward and stored within the North Atlantic basin. 相似文献
14.
Marine aerosols in the western North Pacific were collected using a cascade impactor. Size-separated aerosols were analyzed for organic carbon, alkanes and polycyclic aromatic hydrocarbons (PAH). The results showed that the rate of decrease of the atmospheric concentrations of these organic components with increase in distance from Japan as well as from the coast of the Eurasian Continent was in the order PAHalkanes>organic carbon. The bulk of all these organic components occurred in the smallest size fraction of particles (<1m). Analysis of the alkanes and PAH indicated that the hydrocarbons in aerosols in Japanese coastal marine areas are primarily derived from terrestrial anthropogenic sources which also contribute to a lesser extent to aerosols in marine areas about 1,000 km off the coast of Japan. In remote marine areas the hydrocarbons on small particles (<1m) have principally a natural terrestrial origin while those on larger particles are marine in origin. 相似文献
15.
M. S. Artamonova D. P. Gubanova M. A. Iordanskii V. A. Lebedev L. O. Maksimenkov V. M. Minashkin Y. I. Obvintsev O. G. Chketiani 《Izvestiya Atmospheric and Oceanic Physics》2016,52(8):769-783
Variations in the surface aerosol over the arid steppe zone of Southern Russia have been measured. The parameters of atmospheric aerosol (mass concentration, both dispersed and elemental compositions) and meteorological parameters were measured in Tsimlaynsk raion (Rostov oblast). The chemical composition of aerosol particles in the atmospheric surface layer has been determined, and the coefficients of enrichment of elements with respect to clarkes in the Earth’s crust have been calculated. It is shown that, in summer, arid aerosols are transported from both alkaline and sandy soils of Kalmykia to the air basin over the observation zone. Aerosol particles in the surface air layer over this region have been found to contain the products of combustion of oil, coal, and ethylized fuel. These combustion products make a small contribution to the total mass concentration of atmospheric aerosol; however, they are most hazardous to the health of people because of their sizes and heavy-metal contents. A high concentration of submicron sulfur-containing aerosol particles of chemocondensation nature has been recorded. Sources of aerosol of both natural and anthropogenic origins in southern Russia are discussed. 相似文献
16.
The results of simulating global ocean circulation and its interannual variability in 1948–2007 using INM RAS ocean general circulation model INMOM (Institute of Numerical Mathematics Ocean Model) are presented. One of the INMOM versions is also used for the Black Sea dynamics simulation. The CORE datasets were used to set realistic atmospheric forcing. Sea ice area decrease by 2007 was reproduced in the Arctic Ocean that is in good agreement with observations. The interdecadal climatic variability was revealed with significant decrease of Atlantic thermohaline circulation (ATHC) and meridional heat transport (MHT) in North Atlantic (NA) since the late 1990’s. MHT presents decrease of heat transport from NA to the atmosphere since the mid-1990’s. Therefore the negative feedback is revealed in the Earth climate system that leads to reducing of climate warming caused primarily by anthropogenic factor for the last decades. Long-term variability (60 years) of ATHC is revealed as well which influences NA thermal state with 10 year delay. The assumption is argued that this mechanism can make a contribution in the ATHC own long-term variability. 相似文献
17.
Structure of temperature variability in the high latitudes of the Northern Hemisphere 总被引：1，自引：0，他引：1
V. A. Semenov 《Izvestiya Atmospheric and Oceanic Physics》2007,43(6):687-695
The spatial structure of surface air temperature (SAT) anomalies in the extratropical latitudes of the Northern Hemisphere (NH) during the 20th century is studied from the data obtained over the period 1892–1999. The expansion of the mean (over the winter and summer periods) SAT anomalies into empirical orthogonal functions (EOFs) is used for analysis. It is shown that variations in the mean air temperature in the Arctic region (within the latitudes 60°–90°N) during both the winter and summer periods can be described with a high accuracy by two spatial orthogonal modes of variability. For the winter period, these are the EOF related to the leading mode of variability of large-scale atmospheric circulation in the NH, the North Atlantic Oscillation, and the spatially localized (in the Arctic) EOF, which describes the Arctic warming of the mid-20th century. The expansion coefficient of this EOF does not correlate with the indices of atmospheric circulation and is hypothetically related to variations in the area of the Arctic ice cover that are due to long-period variations in the influx of oceanic heat from the Atlantic. On the whole, a significantly weaker relation to the atmospheric circulation is characteristic of the summer period. The first leading variability mode describes a positive temperature trend of the past decades, which is hypothetically related to global warming, while the second leading EOF describes a long-period oscillation. On the whole, the results of analysis suggest a significant effect of natural climatic variability on air-temperature anomalies in the NH high latitudes and possible difficulties in isolating an anthropogenic component of climate changes. 相似文献
18.
《Deep Sea Research Part I: Oceanographic Research Papers》2002,49(3):539-554
A simple one-dimensional model, validated with observations from ship of opportunity programs, was run at different locations in the North and South Atlantic gyres to produce seasonal partial pressure of CO2 (pCO2)–sea surface temperature (SST) relationships. The pCO2–SST relationships obtained at different locations in the North Atlantic gyre can be approximated by two regression lines, one from February to July and another from August to January. An algorithm including SST, latitude, longitude and atmospheric pCO2 was constructed for each period. The robustness of these relationships was tested along several transects in the North Atlantic gyre and found to be in good agreement with the observations. The same approach was used in the South Atlantic gyre, but more observations are required in this region. In both gyres, the pCO2–SST relationships are close to 4%/°C, which is higher than the pCO2–SST relationships deduced from a CO2 climatology. 相似文献
19.
Jan E. Vermaat Abigail McQuatters-Gollop Marieke A. Eleveld Alison J. Gilbert 《Estuarine, Coastal and Shelf Science》2008
Comprehensive, aggregate nutrient budgets were established for two compartments of the North Sea, the shallow coastal and deeper open regions, and for three different periods, representing pre-eutrophication (∼1950), eutrophication (∼1990) and contemporary (∼2000) phases. The aim was to quantify the major budget components, to identify their sources of variability, to specify the anthropogenic components, and to draw implications for past and future policy. For all three periods, open North Sea budgets were dominated (75%) by fluxes from and to the North-East Atlantic; sediment exchange was of secondary importance (18%). For the coastal North Sea, fluxes during the eutrophication period were dominated by sediment exchange (49% of all inputs), followed by exchange with the open sea (21%), and anthropogenic inputs (19%). Between 1950 and 1990, N-loading of coastal waters increased by a factor of 1.62 and P-loading by 1.45. These loads declined after 1990. Interannual variability in Atlantic inflow was found to correspond to a variability of 11% in nutrient load to the open North Sea. Area-specific external loads of both the open and coastal North Sea were below Vollenweider-type critical loads when expressed relative to depth and flushing. External area-specific load of the coastal North Sea has declined since 1990 from 1.8 to about 1.4 g P m−2 y−1 in 2000, which is close to the estimate of 1.3 for 1950. N-load declined less, leading to an increase in N/P ratio. 相似文献
20.
Oceanology - The article presents the results of a study of black carbon concentrations in the atmospheric boundary layer over the Baltic and North seas, the North Atlantic, and Norwegian, Barents,... 相似文献