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1.
鄂尔多斯盆地JX井延长组砂岩固碳潜力分析 总被引：1，自引：1，他引：0
神华集团在我国CO2地下埋藏的潜在目标区(鄂尔多斯盆地)实施的CO2注入工程仍存在有关其注入层之上泥岩盖层安全性方面的争议.通过对与神华集团CO2注入井相邻且钻遇地层系统、岩石组合一致的JX井三叠系延长组(位于注入层之上)的研究预测一旦CO2透过盖层后的再续固碳能力.研究层位岩屑样品类型主要为长石砂岩和岩屑长石砂岩,其次为岩屑砂岩和岩屑石英砂岩;其物源区岩石类型主要为长英质火山岩、其次为中性火山岩及少量富含石英的沉积岩,具中性斜长岩成分特征;其上段(466~534 m)及下段(666~958 m)砂岩母岩受到弱-中等化学蚀变,并可能经历了再旋回过程;中段(534~666 m)砂岩母岩未受化学蚀变影响,并可能为第一次旋回沉积物.作为潜在的CO2再续固碳场所,延长组砂岩具有实现CO2矿物圈闭的物质条件及形成片钠铝石、方解石、铁白云石和菱铁矿等固碳矿物的潜力. 相似文献
2.
东濮凹陷上古生界石千峰组发育一套厚度较大且具有勘探潜力的河流-湖泊相致密砂岩。采用岩心观察、薄片鉴定、扫描电镜、阴极发光、X衍射全岩及黏土矿物分析等技术手段,对东濮凹陷上古生界石千峰组致密砂岩储层的岩石学特征、物性特征和成岩作用进行了分析。结果表明:储层岩石类型主要为岩屑长石砂岩和长石岩屑砂岩;孔隙度2%~10%,渗透率(0~1)10-3m2,整体上表现出特低孔超低渗特点;成岩作用主要为压实、压溶、胶结、溶蚀和交代作用。样品古地温、镜质体反射率(Ro,%)和X衍射黏土矿物分析结果进一步证实研究区石千峰组砂岩储层属于中成岩阶段A期。 相似文献
3.
海拉尔盆地乌尔逊凹陷南屯组与松辽盆地孤店CO2气田泉头组发育大量含片钠铝石砂岩。通过偏光显微镜、扫描电镜、茜素红-S染色、X射线衍射、电子探针与INCA能谱分析等,对含片钠铝石砂岩的骨架碎屑组分、胶结物与自生矿物、成岩共生序列等岩石学特征进行了系统研究。研究表明,含片钠铝石砂岩的岩石类型为长石砂岩和岩屑长石砂岩,粒度以细粒、细-中粒为主,分选差-中等。砂岩中胶结物主要为次生加大石英、自生石英、片钠铝石、铁白云石和粘土矿物。其中,片钠铝石最高可达砂岩总体积的22％在砂岩中或以放射状、束状、菊花状、杂乱毛发状、毛球状、板状等集合体充填孔隙,或呈束状和板状交代长石和岩屑。电子探针与INCA能谱综合分析表明,片钠铝石主要由Na、Al、O、C等组成。在含片钠铝石砂岩中,成岩共生序列依次为粘土矿物包壳-次生加大石英、自生石英、自生高岭石-油气充注-CO2充注-片钠铝石-铁白云石。其中,CO2注入前形成的自生矿物组合主要为次生加大石英、自生石英和自生高岭石,CO2注入后形成的自生矿物组合主要为片钠铝石和铁白云石。 相似文献
4.
海拉尔盆地乌尔逊凹陷南屯组与松辽盆地孤店CO2气田泉头组发育大量含片钠铝石砂岩.通过偏光显微镜、扫描电镜、茜素红-S染色、X射线衍射、电子探针与INCA能谱分析等,对含片钠铝石砂岩的骨架碎屑组分、胶结物与自生矿物、成岩共生序列等岩石学特征进行了系统研究.研究表明,含片钠铝石砂岩的岩石类型为长石砂岩和岩屑长石砂岩,粒度以细粒、细-中粒为主,分选差-中等.砂岩中胶结物主要为次生加大石英、自生石英、片钠铝石、铁白云石和牯土矿物.其中,片钠铝石最高可达砂岩总体积的22%,在砂岩中或以放射状、束状、菊花状、杂乱毛发状、毛球状、板状等集合体充填孔隙,或呈束状和板状交代长石和岩屑.电子探针与INCA能谱综合分析表明,片钠铝石主要由Na、AI、O、C等组成.在含片钠铝石砂岩中,成岩共生序列依次为牯土矿物包壳-次生加大石英、自生石英、自生高岭石-油气充注-CO2充注-片钠铝石-铁白云石.其中,CO2注入前形成的自生矿物组合主要为次生加大石英、自生石英和自生高岭石,C02注入后形成的自生矿物组合主要为片钠铝石和铁白云石. 相似文献
5.
CO2的地质封存技术是减少CO2向大气排放的一种有效方法。矿物封存由于储存时间长,安全性高,对CO2地质封存至关重要。本文以鄂尔多斯盆地石盒子组地层为例,利用模拟软件TOUGHREACT研究了CO2注入后,各矿物的溶解和沉淀机理,确定固碳矿物和CO2的矿物封存量;通过改变绿泥石和长石类矿物的初始含量,研究原生矿物组分对CO2矿物封存潜力的影响。结果表明,以石英、长石为主的砂岩储集层中,长石类、绿泥石和高岭石是主要的溶解矿物,铁白云石是主要的固碳矿物,原生矿物中绿泥石和长石类矿物对CO2的矿物封存量影响很大,绿泥石和长石类矿物的体积分数增加,CO2的矿物封存量也增加。 相似文献
6.
鄂尔多斯盆地马家滩地区石盒子组是天然气的重点勘探层位。对马家滩地区石盒子组的岩石学特征和成岩作用研究表明,石盒子组的储层岩石类型主要为石英砂岩、岩屑石英砂岩,少量的长石岩屑砂岩。储层砂岩的成岩作用类型主要有压实和压溶、石英次生加大、胶结、溶解。根据成岩作用特征,建立了研究区储层砂岩的成岩共生序列: 自生伊利石--自生绿泥石--石英次生加大--高岭石--方解石。鄂尔多斯盆地作为中国CO2 地下埋藏的潜在目标区,开展CO2 可能埋藏层段的岩石学特征和成岩作用研究,可为CO2 地质储存的数值模拟研究提供岩石学信息。 相似文献
7.
基于野外地质露头观察、岩心描述、薄片鉴定和地球化学等分析测试资料的综合分析,对鄂尔多斯盆地及周缘地区上二叠统石千峰组沉积岩石类型、沉积构造、沉积相类型及沉积体系空间展布等方面开展研究。结果表明,石千峰组主要发育冲积平原、三角洲平原、三角洲前缘、浅湖和南部海陆过渡的潟湖、沙坝等沉积环境,石千峰期,古气候干燥炎热,沉积古地形相对平缓,物源供给充足,形成了一套紫红色、棕红色泥岩和浅灰色中粗粒长石岩屑砂岩、岩屑长石砂岩、长石砂岩为主的地层。盆地北部三角洲规模大,以辫状河道发育沉积特征为主,砂体厚度大、横向分布稳定,而盆地南部三角洲规模相对较小。石千峰期,海水可能多次入侵盆地南部麟游-韩城-乡宁一带,发育海相夹层和沙坝沉积,一定程度上影响了南部的沉积环境和砂体展布。 相似文献
8.
含片钠铝石砂岩是一种含片钠铝石自生矿物的砂岩，一般为富含长石的砂岩，与片钠铝石稳定共生的自生矿物主要为铁白云石、菱铁矿等碳酸盐矿物。砂岩中片钠铝石的含量变化较大，其存在与否不受砂岩结构的制约。含片钠铝石砂岩往往分布在断裂和岩浆岩体附近，既可以作为CO2气储层，又可以作为油气储层。含片钠铝石砂岩是一种具有特殊地质意义的砂岩，表现为：①含片钠铝石砂岩记录了深、浅部层圈之间及烃源岩—储层之间的物质转移；②在含油CO2气藏和油藏中，含片钠铝石砂岩记录了CO2与油气双重充注，其中含油CO2气藏中的含片钠铝石砂岩记录了CO2充注驱油现象；③含片钠铝石砂岩是进行CO2地下储存研究的理想的天然实验室。 相似文献
9.
基于野外地质露头观察、岩心描述、薄片鉴定和地球化学等分析测试资料的综合分析,对鄂尔多斯盆地及周缘地区上二叠统石千峰组沉积岩石类型、沉积构造、沉积相类型及沉积体系空间展布等方面开展研究。结果表明,石千峰组主要发育冲积平原、三角洲平原、三角洲前缘、浅湖和南部海陆过渡的潟湖、沙坝等沉积环境,石千峰期,古气候干燥炎热,沉积古地形相对平缓,物源供给充足,形成了一套紫红色、棕红色泥岩和浅灰色中粗粒长石岩屑砂岩、岩屑长石砂岩、长石砂岩为主的地层。盆地北部三角洲规模大,以辫状河道发育沉积特征为主,砂体厚度大、横向分布稳定,而盆地南部三角洲规模相对较小。石千峰期,海水可能多次入侵盆地南部麟游—韩城—乡宁一带,发育海相夹层和沙坝沉积,一定程度上影响了南部的沉积环境和砂体展布。 相似文献
10.
二氧化碳地质封存(CO2geological sequestration,CGS)是一种直接、高效的减少大气中CO2含量的方式。本文以鄂尔多斯盆地CGS示范工程场地刘家沟组实测数据为基础,利用数值模拟方法,研究储集层岩石初始矿物组分变化对CO2矿物封存能力的影响。结果表明,在长石为主的砂岩储集层中,绿泥石、方解石和长石类矿物是主要的溶解矿物,铁白云石是主要的固碳矿物,初始矿物中钾长石、方解石含量变化对矿物封存量的影响极小,奥长石含量对矿物封存量有一定程度的影响,而绿泥石初始含量显著影响矿物封存量。 相似文献
11.
塔里木盆地西北地区苏盖特布拉克组发育一套潮坪相沉积,是该层系油气勘探的主要目标。基于什艾日克剖面、奇格布拉克剖面、肖尔布拉克剖面的地质测量,采用薄片鉴定、阴极发光、扫描电镜、流体包裹体测温及黏土矿物X衍射等分析手段开展海相碎屑岩成岩作用和成岩演化研究,为塔里木盆地苏盖特布拉克组进一步开展油气勘探部署和甜点储层预测提供地质依据。结果表明：（1）研究区苏盖特布拉克组发育潮坪沉积环境的砂体,砂岩类型以岩屑石英砂岩、岩屑砂岩为主,偶见长石岩屑砂岩,成分成熟度和结构成熟度中等;（2）苏盖特布拉克组砂岩经历了压实（溶）作用、胶结作用、溶蚀作用及交代作用等成岩作用,压实作用是造成储层致密的直接原因,钙质胶结和硅质胶结是储层致密化的根本因素;（3）苏盖特布拉克组砂岩的成岩演化阶段已达到中成岩B期,成岩演化序列为：压实作用/自生黏土矿物（绿泥石）环边—第一期长石、岩屑溶蚀作用—第一期硅质胶结—第一期泥微晶方解石胶结/压溶作用/黏土矿物的伊利化—第二次硅质胶结/第二期铁方解石胶结—钙质胶结物溶蚀。据此建立的成岩演化模式为塔里木盆地超深层致密砂岩中甜点储层预测提供可靠的地质依据。 相似文献
12.
神府解家堡区构造上位于鄂尔多斯盆地东缘晋西挠褶带,上古生界自下而上发育本1段、太2段、山2段和千5段等多套致密砂岩储集层.储层岩石类型以石英砂岩、岩屑石英砂岩、长石石英砂岩、岩屑砂岩和长石岩屑砂岩为主,自下而上储层石英含量呈递减、岩屑和长石含量呈递增趋势.储集空间类型以粒间溶孔、粒内溶孔、晶间孔和微裂缝为主,储层最大孔隙半径总体偏小,孔隙中值半径较小,排驱压力中等,储层孔隙以小孔—微孔为主.本溪组海相障壁—潮坪沉积、太原组浅水三角洲沉积、山西组三角洲沉积和石千峰组陆相辫状河沉积演化序列下,岩石成分成熟度和结构成熟度自下而上降低,储层空间展布呈层多而薄、砂—泥—煤岩交互特征.成岩作用类型以压实、胶结、溶蚀作用为主,局部发育高岭石化和微裂缝.以沉积相带、岩石类型和成岩作用类型作为3个控制端元,以孔隙度和渗透率为标准,上古生界致密砂岩储层可划分为4个大类和10个亚类,优势相和强溶蚀、弱胶结作用下的Ⅰ类储层孔隙度大于8%,渗透率大于0.5 mD,是最优质储层. 相似文献
13.
Yuyu Wan Shanghai Du Guangyu Lin Fengjun Zhang Tianfu Xu 《Environmental Earth Sciences》2017,76(1):43
This study focused on typical injection layers of deep saline aquifers in the Shiqianfeng Formation used in the Carbon Capture and Sequestration Demonstration Projects in the Ordos Basin, Northwest China. The study employed experiments and numerical simulations to investigate the mechanism of CO2 mineral sequestration in these deep saline aquifers. The experimental results showed that the dissolved minerals are plagioclase, hematite, illite–smectite mixed layer clay and illite, whereas the precipitated minerals are quartz (at 55, and 70 °C) and kaolinite (at 70 °C). There are rare carbonate mineral precipitations at the experimental time scale, while the precipitation of quartz as a product of the dissolution of silicate minerals and some intermediate minerals rich in K and Mg that transform to clay minerals, reveals the possibility of carbonate precipitation at the longer time scale. These results are consistent with some results previously reported in the literature. We calibrated the kinetic parameters of mineral dissolution and precipitation by these experimental results and then simulated the CO2 mineral sequestration under deep saline aquifer conditions. The simulation results showed that the dissolved minerals are albite, anorthite and minor hematite, whereas the precipitated minerals are calcite, kaolinite and smectite at 55 and 70 °C. The geochemical reaction of illite is more complex. At 55 °C, illite is dissolved at the relatively lag time and transformed to dawsonite; at 70 °C, illite is precipitated in the early reaction period and then transformed to kaolinite. Based on this research, sequestrated CO2 minerals, which are mainly related to the temperature of deep saline aquifers in Shiqianfeng Fm., are calcite and dawsonite at lower temperature, and calcite at higher temperature. The simulation results also establish that calcite could precipitate over a time scale of thousands of years, and the higher the temperature the sooner such a process would occur due to increased reaction rates. These characteristics are conducive, not only to the earlier occurrence of mineral sequestration, but also increase the sequestration capacity of the same mineral components. For a sequestration period of 10,000 years, we determined that the mineral sequestration capacity is 0.786 kg/m3 at 55 °C, and 2.180 kg/m3 at 70 °C. Furthermore, the occurrence of mineral sequestration indirectly increases the solubility of CO2 in the early reaction period, but this decreases with the increase in temperature. 相似文献
14.
In CO2 geological storage (CGS) context, the evolution of the caprock sealing capacity has received increasing attention, particularly on a geological time span (thousands of years). At this time scale, geochemical reactions may enhance or weaken the caprock quality. It is widely recognized that, for the reservoir, geological heterogeneities affect the concentration and spatial distribution of CO2, and then affect the extent of gas–water–rock interactions, which in turn alters the hydrogeological properties of the reservoir. However, much less attention of these effects has been paid to the caprock. In this study, we presented and applied a novel approach to evaluate the effects of permeability and porosity heterogeneities on the alteration of minerals, the associated evolution of the caprock sealing efficiency and the containment of supercritical CO2 (scCO2) within the caprock. Even though this is a generic study, several conditions and parameters such as pressure, permeability, and mineral composition, were extracted from a caprock layer of the Shiqianfeng Formation in the Ordos Basin demonstration site in China. For the sake of simplification, a 2-dimensional model was designed to represent the caprock domain. We firstly generated an appropriate heterogeneous random field of permeability with the average permeability taken from the uppermost mudstone layer of the Shiqianfeng Formation, and then the heterogeneity in porosity was incorporated using a joint normal distribution method based on the available data. Homogeneous mineral compositions of the reservoir and caprock were used in all simulations. Simulations of three cases were performed, including a homogeneous case, a case with only permeability heterogeneity and a case with both permeability and porosity heterogeneities. The results demonstrate dramatic influences of permeability and porosity heterogeneities on the migration of scCO2 within the caprock, the alteration of minerals, and therefore the evolution of the caprock sealing quality. Specific to the data used in this study, hydrogeological heterogeneities facilitated the overall penetration of scCO2 within the caprock and promoted the alteration of minerals, thereby weakening the caprock sealing efficiency over the simulation time. 相似文献
15.
沉积物源分析是认识盆山演化的重要途径。了解四川盆地西南缘上二叠统宣威组物源,对于重建晚二叠世扬子克拉通周缘演化具有重要意义。本文对峨眉山地区宣威组顶部泥岩、砂岩开展了岩石学和全岩地球化学分析,进行了物源、沉积环境和构造背景的研究。宣威组泥岩主要成分为黏土矿物,SiO2含量(平均49.42%)中等;砂岩成分大部分为火山岩屑,含有少量石英及长石,具中等的SiO2含量(平均44.12%),属于杂砂岩系列。泥岩与砂岩均具有轻稀土元素富集、重稀土元素较右倾的稀土元素配分型式,微量元素相对大陆上地壳富集高场强元素(如Nb、Zr),亏损大离子亲石元素(如Sr、Ba)。根据地球化学分析结果结合已发表的扬子克拉通周缘二叠系沉积岩数据,认为上二叠统宣威组顶部沉积岩物源区经历了强烈的化学风化作用,沉积古环境为富氧的淡水沉积环境;宣威组顶部沉积物物源不仅来自于近源搬运的峨眉山高Ti玄武岩,还接受了扬子克拉通的补给,扬子克拉通西缘晚二叠世时期是活动大陆边缘沉积。 相似文献
16.
In order to evaluate the extent of CO2–water–rock interactions in geological formations for C sequestration, three batch experiments were conducted on alkali feldspars–CO2–brine interactions at 150–200 °C and 300 bars. The elevated temperatures were necessary to accelerate the reactions to facilitate attainable laboratory measurements. Temporal evolution of fluid chemistry was monitored by major element analysis of in situ fluid samples. SEM, TEM and XRD analysis of reaction products showed extensive dissolution features (etch pits, channels, kinks and steps) on feldspars and precipitation of secondary minerals (boehmite, kaolinite, muscovite and paragonite) on feldspar surfaces. Therefore, these experiments have generated both solution chemistry and secondary mineral identity. The experimental results show that partial equilibrium was not attained between secondary minerals and aqueous solutions for the feldspar hydrolysis batch systems. Evidence came from both solution chemistry (supersaturation of the secondary minerals during the entire experimental duration) and metastable co-existence of secondary minerals. The slow precipitation of secondary minerals results in a negative feedback in the dissolution–precipitation loop, reducing the overall feldspar dissolution rates by orders of magnitude. Furthermore, the experimental data indicate the form of rate laws greatly influence the steady state rates under which feldspar dissolution took place. Negligence of both the mitigating effects of secondary mineral precipitation and the sigmoidal shape of rate–ΔGr relationship can overestimate the extent of feldspar dissolution during CO2 storage. Finally, the literature on feldspar dissolution in CO2-charged systems has been reviewed. The data available are insufficient and new experiments are urgently needed to establish a database on feldspar dissolution mechanism, rates and rate laws, as well as secondary mineral information at CO2 storage conditions. 相似文献