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Fifteen organic and three inorganic compounds were tested for methane (CH4) evolution under simulated martian conditions of 6.9 mbar; UVC (200-280 nm) flux of 4 W m−2; 20 °C; simulated optical depth of 0.1; and a Mars gas composition of CO2 (95.3%), N2 (2.7%), Ar (1.7%), O2 (0.13%), and water vapor (0.03%). All three inorganic compounds (i.e., NaCl, CaCO3, graphite) failed to evolve methane at the minimum detection level 0.5 ppm, or above. In contrast, all organic compounds evolved methane when exposed to UV irradiation under simulated martian conditions. The polycyclic aromatic hydrocarbon, pyrene, released the most methane per unit of time at 0.175 nmol CH4 g−1 h−1, and a spectral reflectance target material used for the MER rovers and Phoenix lander released the least methane at 0.00065 nmol CH4 cm−2 h−1. Methane was also released from UV-killed bacterial endospores of Bacillus subtilis. Although all organic compounds evolved methane when irradiated with UV photons under martian conditions, the concentrations of residual organics, biogenic signature molecules, and dead microbial cells should be relatively low on the exterior surfaces of the MSL rover, and, thus, not significant sources of methane contamination. In contrast, kapton tape was found to evolve methane at the rate of 0.00165 nmol CH4 cm−2 h−1 (16.5 nmol m−2 h−1) under the UV and martian conditions tested. Although the evolution of methane from kapton tape was found to decline over time, the large amount of kapton tape used on the MSL rover (lower bound estimated at 3 m2) is likely to create a significant source of terrestrial methane contamination during the early part of the mission. 相似文献
175.
Ming CHEN Christian KOEBERL Wansheng XIAO Xiande XIE Dayong TAN 《Meteoritics & planetary science》2011,46(5):729-736
Abstract– The 1.8 km‐diameter Xiuyan crater is an impact structure in northeastern China, exposed in a Proterozoic metamorphic rock complex. The major rocks of the crater are composed of granulite, hornblendite, gneiss, tremolite marble, and marble. The bottom at the center of the crater covers about 100 m thick lacustrine sediments underlain by 188 m thick crater‐fill breccia. A layer of polymict breccia composed of clasts of granulite, gneiss, hornblendite, and fragments of glass as well as clastic matrix, occurs near the base, in the depth interval from 260 to 295 m. An investigation in quartz from the polymict breccia in the crater‐fill units reveals abundant planar deformation features (PDFs). Quartz with multiple sets of PDFs is found in clasts of granulite that consist of mainly quartz and feldspar, and in fine‐grained matrix of the impact‐produced polymict breccia. A universal stage was used to measure the orientation of PDFs in 70 grains of quartz from five thin sections made from the clasts of granulite of polymict breccia recovered at the depth of 290 m. Forty‐four percent of the quartz grains contain three sets of PDFs, and another 40% contain two sets of PDFs. The most abundant PDFs are rhombohedron forms of , , and with frequency of 33.5, 22.3, and 9.6%, respectively. A predominant PDF form of in quartz suggests a shock pressure >20 GPa. The occurrence of PDFs in quartz from the polymict breccia provides crucial evidence for shock metamorphism of target rocks and confirms the impact origin of this crater, which thus appears to be the first confirmed impact crater in China. 相似文献
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177.
Ansgar GRESHAKE Christian KOEBERL Jrg FRITZ W. Uwe REIMOLD 《Meteoritics & planetary science》2010,45(6):973-989
Abstract– Dark streaks and different types of inclusions in Libyan Desert Glass (LDG) collected from the LDG strewn field in Egypt were investigated. Rare transparent spherules enclosed in the glassy matrix are characterized by concentric cracks, irregular internal cracks, intense twinning, and considerable amounts of Ti and Al. Raman spectra show that the spherules are α‐cristobalite. Their occurrence together with lechatelierite indicates quick heating of the source rock to at least 1550 °C, followed by rapid quenching leading to crystallization of β‐cristobalite, which upon cooling inverted into α‐cristobalite. Brownish inclusions are irregularly shaped, elongated objects with smooth contacts to the surrounding glass. They contain small roundish to elliptical droplets, and a few larger angular grains, which compositionally and according to their Raman spectra most closely resemble low‐Ca, Al‐rich orthopyroxene. Composition and texture of the orthopyroxene suggest that the brownish inclusions formed by incomplete melting of an Al‐rich orthopyroxene bearing precursor, e.g., mafic phases present in desert surface sands or also of orthopyroxene‐bearing granulite dykes in the LDG target. Experimental data on Ca‐poor enstatite also support that the inclusions were heated to about 1550 °C. Analyses of dark streaks in LDG reveal high abundances of Al, Ti, Mn, Cr, Fe, and Ni and a pronounced correlation between the abundances of Cr, Mn, Fe, and Ni. As the Fe/Ni, Mn/Ni, and Cr/Ni ratios are all clearly nonchondritic, the source of this material is most likely terrestrial and the dark streaks studied here represent a different type of schlieren compared to those which contain a meteoritic component. These findings suggest LDG formation during a short high‐temperature event. Melting of Al‐rich orthopyroxene bearing target material seems to suggest an asteroid impact rather than a near‐surface airburst. 相似文献
178.
Latent heat polynyas are regions generating strong ice formation, convection and extensive water mass formation. Here we report on the effects of these processes on resuspension of sediments and subsequent methane release from the seafloor and on the resulting excess methane concentration in surface water on a polar shelf during winter. The study is based on measurements of concentration and δ13C values of methane, water temperature, salinity, light transmission and sea ice data collected in March 2003 in Storfjorden, southern Svalbard. In winter, strong and persistent northeasterly winds create polynyas in eastern Storfjorden and cause ice formation. The resulting brine-enriched water cascades from the Storfjordbanken into the central depression thereby enhancing the turbulence near the seafloor. A distinct benthic nepheloid layer was observed reflecting the resuspension of sediments by the cascading dense bottom water. High concentrations of 13C-depleted methane suggest submarine discharge of methane with the resuspended sediments. As the source of the submarine methane, we propose recent bacterial methanogenesis near the sediment surface because of extremely high accumulation rates of organic carbon in Storfjorden. Convective mixing transports newly released methane from the bottom to the sea surface. This eventually results in an excess concentration in surface water with respect to the atmospheric equilibrium, and a sea-air flux of methane during periods of open water. When a new ice cover is formed, methane becomes trapped in the water column and subsequently oxidized. Thus, the residual methane is strongly enriched in 13C in relation to the δ13CCH4 signature of atmospheric methane. Our results show that latent heat polynyas may induce a direct pathway for biogases like methane from sediments to the atmosphere through coupling of biogeochemical and oceanographic processes. Extrapolating these processes to all Arctic ocean polynyas, we estimate a transfer of CH4 between 0.005 and 0.02 Tg yr−1. This is not a large contribution but the fluxes from the polynyas are 20–200 times larger than the ocean average and the methane evasion process in polynyas is certainly one that can be altered under climate change. 相似文献
179.
Ocean/ice interaction at the base of deep-drafted Antarctic ice shelves modifies the physical properties of inflowing shelf
waters to become Ice Shelf Water (ISW). In contrast to the conditions at the atmosphere/ocean interface, the increased hydrostatic
pressure at the glacial base causes gases embedded in the ice to dissolve completely after being released by melting. Helium
and neon, with an extremely low solubility, are saturated in glacial meltwater by more than 1000%. At the continental slope
in front of the large Antarctic caverns, ISW mixes with ambient waters to form different precursors of Antarctic Bottom Water.
A regional ocean circulation model, which uses an explicit formulation of the ocean/ice shelf interaction to describe for
the first time the input of noble gases to the Southern Ocean, is presented. The results reveal a long-term variability of
the basal mass loss solely controlled by the interaction between waters of the continental shelf and the ice shelf cavern.
Modeled helium and neon supersaturations from the Filchner–Ronne Ice Shelf front show a “low-pass” filtering of the inflowing
signal due to cavern processes. On circumpolar scales, the simulated helium and neon distributions allow us to quantify the
ISW contribution to bottom water, which spreads with the coastal current connecting the major formation sites in Ross and
Weddell Seas.
相似文献
Christian B. RodehackeEmail: |
180.
Christian Timm Kaj Hoernle Reinhard Werner Folkmar Hauff Paul van den Bogaard James White Nick Mortimer Dieter Garbe-Schönberg 《Earth》2010,98(1-2):38-64
In order to constrain better the distribution, age, geochemistry and origin of widespread Cenozoic intraplate volcanism on Zealandia, the New Zealand micro-continent, we report new 40Ar/39Ar and geochemical (major and trace element and Sr–Nd–Hf–Pb isotope) data from offshore (Chatham Rise, Campbell and Challenger Plateaus) and onland (North, South, Auckland, Campbell, Chatham and Antipodes Islands of New Zealand) volcanism on Zealandia. The samples include nephelinite, basanite through phonolite, alkali basalt through trachyte/rhyolite, and minor tholeiite and basaltic andesite, all of which have ocean island basalt (OIB)-type trace element signatures and which range in age from 64.8 to 0.17 Ma. Isotope ratios show a wide range in composition (87Sr/86Sr = 0.7027–0.7050, 143Nd/144Nd = 0.5128–0.5131, 177Hf/176Hf = 0.2829–0.2831, 206Pb/204Pb = 18.62–20.67, 207Pb/204Pb = 15.54–15.72 and 208Pb/204Pb = 38.27–40.34) with samples plotting between mid-ocean-ridge basalts (MORB) and Cretaceous New Zealand intraplate volcanic rocks.Major characteristics of Zealandia's Cenozoic volcanism include longevity, irregular distribution and lack of age progressions in the direction of plate motion, or indeed any systematic temporal or spatial geochemical variations. We believe that these characteristics can be best explained in the context of lithospheric detachment, which causes upwelling and melting of the upper asthenospheric mantle and portions of the removed lithosphere. We propose that a large-scale seismic low-velocity anomaly, that stretches from beneath West Antarctica to Zealandia at a depth of > 600 km may represent a geochemical reservoir that has been in existence since the Cretaceous, and has been supplying the upper mantle beneath Zealandia with HIMU-type plume material throughout the Cenozoic. In addition, the sources of the Cenozoic intraplate volcanism may be at least partially derived through melting of locally detached Zealandia lower lithosphere. 相似文献