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41.
Stefano Pini Maria Franca Brigatti Marco Affronte Daniele Malferrari Augusto Marcelli 《Physics and Chemistry of Minerals》2012,39(8):665-674
This contribution is finalized at the discussion of the magnetic structure of two samples, belonging to phlogopite–annite [sample TK, chemical composition IV(Si2.76Al1.24) VI(Al0.64Mg0.72 $ {\text{Fe}}_{1.45}^{2 + } $ Mn0.03Ti0.15) (K0.96Na0.05) O10.67 (OH)1.31 Cl0.02] and polylithionite–siderophyllite joints [sample PPB, chemical composition IV(Si3.14Al0.86)VI(Al0.75Mg0.01 $ {\text{Fe}}_{1.03}^{2 + } $ $ {\text{Fe}}_{1.03}^{3 + } $ Mn0.01Ti0.01Li1.09) (K0.99Na0.01) O10.00 (OH)0.65F1.35]. Samples differ for Fe ordering in octahedral sites, Fe2+/(Fe2+?+?Fe3+) ratio, octahedral composition, defining a different environment around Fe cations, and layer symmetry. Spin-glass behavior was detected for both samples, as evidenced by the dependency of the temperature giving the peak in the susceptibility curve from the frequency of the applied alternating current magnetic field. The crystal chemical features are associated to the different temperature at which the maximum in magnetic susceptibility is observed: 6?K in TK, where Fe is disordered in all octahedral sites, and 8?K in PPB sample, showing a smaller and more regular coordination polyhedron for Fe, which is ordered in the trans-site and in one of the two cis-sites. 相似文献
42.
43.
Rodrigo de Freitas Lagoon, located in the Rio de Janeiro City, receives several types of polluted discharges. The knowledge of the sediment microfauna correlated with heavy metal and organic matter concentrations could supply important data about the conditions of the lagoon. The benthic foraminiferal assemblage presented larger diversity and more abundant samples in the lagoon entrance than in the inner area. The Ammonia tepida - Elphidiumexcavatum foraminiferal assemblage is characterized by dwarf, corroded and weak organisms. Agglutinated species were found only near the entrance. Low abundance values and sterility of five samples in the inner area (north/northeast) can be caused by high levels of heavy metals and organic matter. A. tepida shows negative correlation with increasing heavy metals values. PAHs and coprostanol high indexes, and the absence or low presence of microfauna in samples around the lagoon margin confirm illegal flows from gas stations and domestic sewage. 相似文献
44.
Paganelli D Forni G Marchini A Mazziotti C Occhipinti-Ambrogi A 《Marine pollution bulletin》2011,62(8):1725-256
According to the European Water Framework Directive, the ecological status (ES) of a water body is determined by comparing observation data with undisturbed Reference Conditions (RCs). Defining RCs is crucial when evaluating the ES of a water body as it strongly affects the final outcome of any index application. Identifying RCs by observing real sites is not feasible in many marine environments, such as the Emilia-Romagna coast (Italy, N-Adriatic Sea). We used a statistical approach on a large dataset to derive RCs for the application of the benthic index M-AMBI in this area. We then applied M-AMBI to samples collected along a gradient of presumed environmental disturbance. The results put 14.8% of the Emilia-Romagna samples in “High” ES, 60.2% in “Good”, 23.0% in “Moderate” and 2.0% in “Poor”, showing a spatial gradient of improving quality. These results are in agreement with the extensive ecological knowledge available for this area. 相似文献
45.
Daniele L. Pinti Catherine Béland-Otis Alain Tremblay Chris M. Hall Jean-Yves Lavoie 《Geochimica et cosmochimica acta》2011,75(15):4228-4243
Brines in Cambrian sandstones and Ordovician dolostones of the St-Lawrence Lowlands at Bécancour, Québec, Canada were sampled for analysis of all stable noble gases in order to trace their origin and migration path, in addition to quantifying their residence time. Major ion chemistry indicates that the brines are of Na-Ca-Cl type, possibly derived from halite dissolution. 87Sr/86Sr ratios and Ca excess indicate prolonged interactions with silicate rocks of the Proterozoic Grenville basement or the Cambrian Potsdam sandstone. The brines constrain a 2-3% contribution of mantle 3He and large amounts of nucleogenic 21Ne∗ and 38Ar∗ and radiogenic 4He and 40Ar∗. 4He/40Ar∗ and 21Ne∗/40Ar∗ ratios, corrected for mass fractionation during incomplete brine degassing, are identical to their production ratios in rocks. The source of salinity (halite dissolution), plus the occurrence of large amounts of 40Ar∗ in brines constrain the residence time of Bécancour brines as being older than the Cretaceous. Evaporites in the St-Lawrence Lowlands likely existed only during Devonian-Silurian time. Brines might result from infiltration of Devonian water leaching halite, penetrating into or below the deeper Cambrian-Ordovician aquifers. During the Devonian, the basin reached temperatures higher than 250 °C, allowing for thermal maturation of local gas-prone source rocks (Utica shales) and possibly facilitating the release of radiogenic 40Ar∗ into the brines. The last thermal event that could have facilitated the liberation of 40Ar∗ into fluids and contributed to mantle 3He is the Cretaceous Monteregian Hills magmatic episode. For residence times younger than the Cretaceous, it is difficult to find an appropriate source of salinity and of nucleogenic/radiogenic gases to the Bécancour brines. 相似文献
46.
Francesco Di Benedetto Daniele Borrini Andrea Caneschi Gabriele Fornaciai Massimo Innocenti Alessandro Lavacchi Carlo Andrea Massa Giordano Montegrossi Werner Oberhauser Luca A. Pardi Maurizio Romanelli 《Physics and Chemistry of Minerals》2011,38(6):483-490
An extensive characterisation of the magnetic properties of synthetic powders of kuramite, with formal composition Cu3SnS4, was performed. Powders were investigated through superconducting quantum interference device (SQUID) magnetometry, electron paramagnetic resonance (EPR) spectroscopy, X-ray powder diffraction (XRPD), scanning and transmission electron microscopies (SEM and TEM) and microanalysis. SEM and TEM reveal the presence of nanodimensioned particles. XRPD clearly shows that Cu3SnS4 crystallised in a cubic sphalerite-type structural model, in spite of the stannite-type tetragonal structure described for the natural phase. This difference arises from a full random distribution of cations. Synthetic kuramite nanopowders exhibit a marked paramagnetism, originated by the presence of Cu(II), definitely assessed by EPR measurements. Moreover, the overall magnetic behaviour of the sample cannot be simply ascribed to diluted paramagnetism, and this suggests the presence of strong superexchange interactions among Cu(II) ions even at room temperature. The main consequences of these results are the definitive assessment of the chemical formula Cu(I)2Cu(II)SnS4 and of a random distribution of Cu(II), Cu(I) and Sn(IV) ions within the available tetrahedral sites. 相似文献
47.
RésuménLa découverte, dans le Nord des Marches (Italie), de nouveaux gisements de Poissons Cyprinodontidae appartenant à l’espèce Aphanius crassicaudus (AGASSIZ), conduit à réexaminer, à la lumière des données lithostratigraphiques, la signification géodynamique des ichthyofaunes messiniennes de ce secteur de l’Apennin. Après avoir précisé la position stratigraphique et la répartition paléogéographique des gisements étudiés, les auteurs montrent que le développement des faunes à Aphanius crassicaudus (AGASSIZ) dans les eaux saumâtres du domaine continental n’implique pas la disparition corrélative du milieu marin. En effet, certains genres marins sont parfois présents à côté de cette espèce, comme c’est le cas dans le gisement de Pésaro. Les auteurs contestent en outre l’interprétation selon laquelle le fait qu’aucune ichthyofaune marine ne soit connue dans le Messinien supérieur d’Italie puisse suffire à conclure que la Méditerranée était asséchée pendant le dépôt de la « Formation à colombacci » 相似文献
48.
Giovanna Daniele 《Geodinamica Acta》2013,26(5):313-333
AbstractThis work deals with the Cretaceous-Tertiary Helminthoid flysch successions of the Emilian Apennines and related basal complexes (Mt. Caio, Val Baganza, Solignano, Mt. Venere-Monghidoro and Mt. Cassio Units): it is based on an integrated approach which included stratigraphic, petrographic and structural observations. Detailed stratigraphic sections measured in the various successions evidenced the specific features of the different flysch formations. The main framework composition analysis of the arenites pointed out a partly ‘oceanic’ alimentation for the Mt. Caio Flysch Fm; the Mt. Venere-Monghidoro, and Mt. Cassio Flysch Fms have been alimented exclusively by a terrigenous detritus mainly derived from continental basement source areas. The heavy mineral assemblage of the Mt. Caio Flysch Fm is characterized by picotite, that of the Mt. Venere-Monghidoro, Solignano and Mt. Cassio Flysch Fms commonly contains straurolite, garnet and chloritoid, generally considered to be typical products of the Adriatic continental margin. The calcareous nannofossils biostratigraphy indicated that the flysch sedimentation started during the Late Campanian and ended between the Paleocene (Mt. Cassio Flysch Fm and Mt. Venere-Monghidoro Fms) and the Middle Eocene (Mt. Caio Flysch Fm). We propose a schematic paleogeographic restoration for the External Ligurian Domain which implies a more internal position for the Mt. Caio succession and a more external one for the Mt. Venere-Monghidoro and Mt. Cassio successions. The Helminthoid flyschs sedimented after and during deformation and subduction phases in perched and fore-arc basins partly overlying the marginal part of the Adriatic plate. The External Ligurian nappes’ stacking consists, in the study area, from the bottom, of the following units: Caio Unit, Val Baganza Ophiolitic Unit, Monghidoro Unit, Cassio Unit. This pile of thrust-nappes, sealed by the Epiligurian succession, has been already realized before Late Eocene. In our opinion it was generated by a frontal west-verging frontal accretion process (offscraping), which let the flysch successions remain, in this phase, quite undeformed. This westverging thrusting phase, starting from the Middle-Late Eocene, has been followed by an important folding event which generated striking hectometric and kilometric ‘Apenninic’ reverse folds, sometimes associated with NE-verging thrust surfaces. The Oligocene and post-Oligocene evolution is characterized by a block-translation of the Ligurian staking over the Subligurian, Tuscan and Umbrian Domains, associated with a new generation of minor thrusts and thrust related Apenninic folds. © 2000 Éditions scientifiques et médicales Elsevier SAS 相似文献
49.
Daniele Norbiato Marco Borga Ralf Merz Günther Blschl Alberto Carton 《Journal of Hydrology》2009,375(3-4):312-325
Analyses of event runoff coefficients provide essential insight on catchment response, particularly if a range of catchments and a range of events are compared by a single indicator. In this study we examine the effect of climate, geology, land use, flood types and initial soil moisture conditions on the distribution functions of the event runoff coefficients for a set of 14 mountainous catchments located in the eastern Italian Alps, ranging in size from 7.3 to 608.4 km2. Runoff coefficients were computed from hourly precipitation, runoff data and estimates of snowmelt. A total of 535 events were analysed over the period 1989–2004. We classified each basin using a “permeability index” which was inferred from a geologic map and ranged from “low” to “high permeability”. A continuous soil moisture accounting model was applied to each catchment to classify ‘wet’ and ‘dry’ initial soil moisture conditions. The results indicate that the spatial distribution of runoff coefficients is highly correlated with mean annual precipitation, with the mean runoff coefficient increasing with mean annual precipitation. Geology, through the ‘permeability index’, is another important control on runoff coefficients for catchments with mean annual precipitation less than 1200 mm. Land use, as indexed by the SCS curve number, influences runoff coefficient distribution to a lesser degree. An analysis of the runoff coefficients by flood type indicates that runoff coefficients increase with event snowmelt. Results show that there exists an intermediate region of subsurface water storage capacity, as indexed by a flow–duration curve-based index, which maximises the impact of initial wetness conditions on the runoff coefficient. This means that the difference between runoff coefficients characterised by wet and dry initial conditions is negligible both for basins with very large storage capacity and for basins with small storage capacity. For basins with intermediate storage capacities, the impact of the initial wetness conditions may be relatively large. 相似文献
50.
Physical processes contributing to the water mass transformation of the Indonesian Throughflow 总被引:1,自引:1,他引:0
Ariane Koch-Larrouy Gurvan Madec Daniele Iudicone Agus Atmadipoera Robert Molcard 《Ocean Dynamics》2008,58(3-4):275-288
The properties of the waters that move from the Pacific to the Indian Ocean via passages in the Indonesian archipelago are observed to vary with along-flow-path distance. We study an ocean model of the Indonesian Seas with reference to the observed water property distributions and diagnose the mechanisms and magnitude of the water mass transformations using a thermodynamical methodology. This model includes a key parameterization of mixing due to baroclinic tidal dissipation and simulates realistic water property distributions in all of the seas within the archipelago. A combination of air–sea forcing and mixing is found to significantly change the character of the Indonesian Throughflow (ITF). Around 6 Sv (approximately 1/3 the model net ITF transport) of the flow leaves the Indonesian Seas with reduced density. Mixing transforms both the intermediate depth waters (transforming 4.3 Sv to lighter density) and the surface waters (made denser despite the buoyancy input by air–sea exchange, net transformation?=?2 Sv). The intermediate transformation to lighter waters suggests that the Indonesian transformation contributes significantly to the upwelling of cold water in the global conveyor belt. The mixing induced by the wind is not driving the transformation. In contrast, the baroclinic tides have a major role in this transformation. In particular, they are the only source of energy acting on the thermocline and are responsible for creating the homostad thermocline water, a characteristic of the Indonesian outflow water. Furthermore, they cool the sea surface temperature by between 0.6 and 1.5°C, and thus allow the ocean to absorb more heat from the atmosphere. The additional heat imprints its characteristics into the thermocline. The Indonesian Seas cannot only be seen as a region of water mass transformation (in the sense of only transforming water masses in its interior) but also as a region of water mass formation (as it modifies the heat flux and induced more buoyancy flux). This analysis is complemented with a series of companion numerical experiments using different representations of the mixing and advection schemes. All the different schemes diagnose a lack of significant lateral mixing in the transformation. 相似文献