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41.
A general analysis of the absorption of the Schumann-Runge bands of molecular oxygen has been made in order to compare the various experimental and theoretical results which have been obtained for an application to the O2 atmospheric absorption and its photodissociation in the mesosphere and stratosphere. The different values of the oscillator strengths deduced from the laboratory absorption spectra and of the predissociation linewidths used for the calculation of the absorption have been compared.Calculations based on a Voight profile of the O2 rotational lines have led to simple formulas for atmospheric applications taking into account that the total photodissociation rate in the stratosphere depends strongly on the absorption of solar radiation in the spectral range of the O2 Herzberg continuum. Specific examples are given. 相似文献
42.
Marcel Nicolet 《Planetary and Space Science》1981,29(9):951-974
A critical analysis has been made of solar irradiance in the spectral region covering wavelengths from 100 nm upwards; the absorption characteristics of molecules of oxygen and ozone have been taken into account with a view to the direct application of the results to atmospheric photochemistry. The absorption of radiation by these molecules results in the photodissociation of both of them in the homosphere, and it also makes possible the penetration of solar radiation from the thermosphere, through the mesosphere and the stratosphere, down to the troposphere.Special attention has been given to each of the following spectral regions: Lyman-alpha radiation at 121.6 nm, the O2 Schumann-Runge continuum at wavelengths less than 175 nm, the O2 Schumann-Runge band system from 200 to 175 nm, and the O2 Herzberg continuum at 242.4 nm. For absorption by ozone, the solar spectrum has been analysed in the following regions: the Hartley band at wavelengths less than 310 nm, the Huggins bands at wavelengths above 310 nm and the visible Chappuis bands. Finally, for the photodissociation of O3, particular attention has been given to the transition region (300–320 nm) in which there is a change-over from the production of the excited atom O(1D) to that of the atom in its ground state O(3p). 相似文献
43.
Yann Hautevelle Raymond Michels Fabrice Malartre Marcel Elie Alain Trouiller 《Applied Geochemistry》2007
The Callovo-Oxfordian claystones located at 500 m depth at Bure (Meuse, France) are currently being investigated by Andra (the French National Radioactive Waste Management Agency) for testing the feasibility of long-term and deep geological nuclear waste disposal. In order to evaluate its potential as a geological barrier, it is very important to study, assess and describe its physico-chemical variability. The molecular biomarker composition of 150 samples of these claystones and their surrounding limestones carry diverse information on the sources of the sedimentary organic matter, the chemistry of the depositional environment, the preservation and diagenesis conditions. It also allows assessing the degree of lateral and vertical variability of the organic matter within these sedimentary series. The abundance of unsaturated biomarkers, the distribution of steroids and hopanoids and CPI values >2 prove the thermal immaturity of the organic matter. The co-occurrence of plankton, bacteria and land plant biomarkers indicate that the organic matter is a mixture of marine and continental contributions. The data also reveal that the organic matter was deposited under oxic and open-sea conditions except for a brief event of photic zone anoxia at the beginning of the Middle Callovian. In the claystones, the geosynthesis of diasterenes is favored to the detriment of the formation of steranes, especially in smectite-rich levels, and the organic matter is rapidly isolated from oxidizing then reducing conditions after the deposition due to the protective effect of clays. On the scale investigated, the claystones are characterized by a unique molecular facies and are thus homogenous from their organic content point of view. Yet, detailed investigation of specific molecular families indicates changes related to major claystone–limestone transitions. The homogeneity of these claystones can be explained by the paleogeographic position of their depositional setting and the plane and sub-horizontal paleotopography on which they were deposited. This study demonstrates the efficiency of organic geochemistry in the assessment of the variability of geological barriers. 相似文献
44.
Ohne Zusammenfassung 相似文献
45.
The mixing properties of Fe3Al2Si3O12-Ca3Al2Si3O12 garnet solid solutions have been studied in the temperature range 850–1100° C. The experimental method involves measuring the composition of garnet in equilibrium with an assemblage in which the activity of the Ca3Al2Si3O12 component is fixed. Experiments on the assemblage garnet solid solution, anorthite, Al2SiO5 polymorph and quartz at known pressure and temperature fix the activity of the Ca3Al2Si3O12 component through the equilibrium: 1 $$\begin{gathered} {\text{3CaAl}}_{\text{2}} {\text{Si}}_{\text{2}} {\text{O}}_{\text{8}} \rightleftarrows {\text{Ca}}_{\text{3}} {\text{Al}}_{\text{2}} {\text{Si}}_{\text{3}} {\text{O}}_{{\text{12}}} \hfill \\ {\text{Anorthite garnet}} \hfill \\ {\text{ + 2Al}}_{\text{2}} {\text{SiO}}_{\text{5}} {\text{ + SiO}}_{\text{2}} \hfill \\ {\text{ sillimanite/kyanite quartz}}{\text{.}} \hfill \\ \end{gathered}$$ This equilibrium, with either sillimanite or kyanite as the aluminosilicate mineral, was used to control \({\text{a}}_{{\text{Ca}}_{\text{3}} {\text{Al}}_{\text{2}} {\text{Si}}_{\text{3}} {\text{O}}_{{\text{12}}} }^{{\text{gt}}} \) . The compositions of the garnet solutions produced were determined by measurement of their unit cell edges. At 1 bar Fe3Al2Si3O12-Ca3Al2Si3O12 garnets exhibit negative deviations from ideality at the Fe-rich end of the series and positive deviations at the calcium end. With increasing pressure the activity coefficients for the Ca3Al2Si3O12 component increase because the partial molar volume of this component is greater than the molar volume of pure grossular. Previous studies indicate that the activity coefficients for the Ca3Al2Si3O12 component also increase with increasing (Mg/Mg+Fe) ratio of the garnet. The region of negative deviation from ideality implies a tendency towards formation of a stable Fe-Ca garnet component. Evidence in support of this conclusion has been found in a natural Fe-rich garnet which was found to contain two different garnet phases of distinctly different compositions. 相似文献
46.
Changes in stream water quality due to logging of the boreal forest in the Montmorency Forest,Québec
Yohann Tremblay Alain N. Rousseau André P. Plamondon Denis Lévesque Marcel Prévost 《水文研究》2009,23(5):764-776
Summer stream water quality was monitored before and following the logging of 50% of the boreal forest within three small watersheds (<50 ha) nested in the ‘Ruisseau des Eaux‐Volées’ Experimental Watershed, Montmorency Forest (Québec, Canada). Logging was conducted in winter, on snow cover according to recommended best management practices (BMPs) to minimize soil disturbance and protect advance growth. A 20‐m forest buffer was maintained along perennial streams. In watershed 7·2, cut‐blocks were located near the stream network and logging was partially allowed within the riparian buffer zone. In watersheds 7·5 and 7·7, logging occurred farther away from the stream network. Observations were also made for watershed 7·3 that collected the runoff from watersheds 7·2 and 7·5, and watershed 7·6, the uproad portion of watershed 7·7. The control watershed 0·2 was contiguous to the impacted watersheds and remained undisturbed. Following clearcutting, changes in summer daily maximum and minimum stream temperatures remained within ± 1 °C while changes in diurnal variation did not decrease by more than 0·5 °C. Concentrations of NO3? greatly increased by up to 6000% and concentrations of K+ increased by up to 300% during the second summer after logging. Smaller increases were observed for Fetotal (up to 71%), specific conductance (up to 26%), and Mg2+ (up to 19%). Post‐logging pH decreased slightly by no more than 7% while PO43? concentration remained relatively constant. Suspended sediment concentrations appeared to increase during post‐logging, but there was not enough pre‐logging data to statistically confirm this result. Logging of moderate intensity and respecting established BMPs may account for the limited changes of water quality parameters and the low exceedances of the criteria for the protection of aquatic life. The proximity of the cutover to the stream network and logging within the riparian zone did not appear to affect water quality. Copyright © 2008 John Wiley & Sons, Ltd. 相似文献
47.
Wave growth in slanting fetch (with wind blowing obliquely off a coast) is investigated with 7 years worth of routine wave measurements in Lake IJssel in The Netherlands and with the SWAN wave model. Two aspects are considered in particular for this case: the validity of the concept of effective fetch and the role of the non-linear four-wave interactions. For slanting and parallel fetch conditions, we found some significant deviations from the effective fetch assumption, leading to 20–35% mismatch in either the peak period Tp or the significant wave height Hm0 respectively. However, the effect of discrepancies between various widely accepted wave growth formulas turned out to be even more important. The wave directions during slanting fetch are significantly ‘steered’ by the coastline, especially in the first kilometre(s) off the coast. The role of the non-linear four-wave interactions is investigated by running the SWAN (version 40.41) wave model with three different quadruplet formulations. Exact quadruplet methods (Xnl) yielded relatively strong wave steering, despite the four-wave interactions being relatively weak. Application of Xnl did not lead to better overall agreement with measurements — improvements for the mean wave period Tm01 were offset by some deterioration for the wave height Hm0. 相似文献
48.
Jean-Alix Barrat Akira Yamaguchi Claire Bollinger Marcel Bohn 《Geochimica et cosmochimica acta》2010,74(21):6218-6231
The eucrites and diogenites are meteorites that probably originate from asteroid 4-Vesta. The upper part of the crust of this body is certainly composed of eucrites which are basaltic or gabbroic rocks. Diogenites are ultramafic cumulates whose relationships with eucritic lithologies are unknown. Here, we show that the orthopyroxenes of some diogenites display very deep negative Eu anomalies (Eu/Eu∗ close to 0.1 or lower). The contamination of the parental magmas of diogenites by melts derived by partial melting of the eucritic crust can satisfactorily explain the range of the Eu anomalies displayed by diogenites. Thus, these anomalies are the first firm indication that parental melts of diogenites have intruded the eucritic crust, and consequently are younger than eucrites. 相似文献
49.
Enhancing the relevance of Shared Socioeconomic Pathways for climate change impacts,adaptation and vulnerability research 总被引:1,自引:1,他引:0
Bas J. van Ruijven Marc A. Levy Arun Agrawal Frank Biermann Joern Birkmann Timothy R. Carter Kristie L. Ebi Matthias Garschagen Bryan Jones Roger Jones Eric Kemp-Benedict Marcel Kok Kasper Kok Maria Carmen Lemos Paul L. Lucas Ben Orlove Shonali Pachauri Tom M. Parris Anand Patwardhan Arthur Petersen Benjamin L. Preston Jesse Ribot Dale S. Rothman Vanessa J. Schweizer 《Climatic change》2014,122(3):481-494
This paper discusses the role and relevance of the shared socioeconomic pathways (SSPs) and the new scenarios that combine SSPs with representative concentration pathways (RCPs) for climate change impacts, adaptation, and vulnerability (IAV) research. It first provides an overview of uses of social–environmental scenarios in IAV studies and identifies the main shortcomings of earlier such scenarios. Second, the paper elaborates on two aspects of the SSPs and new scenarios that would improve their usefulness for IAV studies compared to earlier scenario sets: (i) enhancing their applicability while retaining coherence across spatial scales, and (ii) adding indicators of importance for projecting vulnerability. The paper therefore presents an agenda for future research, recommending that SSPs incorporate not only the standard variables of population and gross domestic product, but also indicators such as income distribution, spatial population, human health and governance. 相似文献
50.
We study a nonlinear mechanism for the excitation of kinetic Alfvén waves (KAWs) by fast magneto-acoustic waves (FWs) in the
solar atmosphere. Our focus is on the excitation of KAWs that have very small wavelengths in the direction perpendicular to
the background magnetic field. Because of their small perpendicular length scales, these waves are very efficient in the energy
exchange with plasmas and other waves. We show that the nonlinear coupling of the energy of the finite-amplitude FWs to the
small-scale KAWs can be much faster than other dissipation mechanisms for fast wave, such as electron viscous damping, Landau
damping, and modulational instability. The nonlinear damping of the FWs due to decay FW = KAW + KAW places a limit on the
amplitude of the magnetic field in the fast waves in the solar corona and solar-wind at the level B/B
0∼10−2. In turn, the nonlinearly excited small-scale KAWs undergo strong dissipation due to resistive or Landau damping and can
provide coronal and solar-wind heating. The transient coronal heating observed by Yohkoh and SOHO may be produced by the kinetic Alfvén waves that are excited by parametric decay of fast waves propagating from
the reconnection sites. 相似文献