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Pascal Richet 《Geochimica et cosmochimica acta》1984,48(3):471-483
With the configurational entropy theory of relaxation processes of Adam and Gibbs (1965), one predicts that the viscosity depends on temperature according to log , where Sconf is the configurational entropy of the liquid. Thermochemical calculations of Sconf performed for some mineral compositions show the importance of non-configurational contributions to the entropy differences between amorphous and crystalline phases. Except for the case of SiO2, the available thermodynamic data indicate that the above equation for viscosity accounts quantitatively for the experimentally determined temperature dependence of the viscosity of silicate melts. The Adam and Gibbs theory also provides a simple rationale for the non linear variation of the logarithmic viscosity with composition in mixed alkali silicate liquids at low temperatures, the minimum of viscosity resulting from the contribution of the entropy of mixing to Sconf. 相似文献
35.
Equations are developed for calculating the density of aluminosilicate liquids as a function of composition and temperature. The mean molar volume at reference temperature Tr, is given by , where the summation is taken over all oxide components except A12O3, X stands for mole fraction, terms are constants derived independently from an analysis of volume-composition relations in alumina-free silicate liquids, and is the composition-dependent apparent partial molar volume of Al2O3. The thermal expansion coefficient of aluminosilicate liquids is given by , where terms are constants independent of temperature and composition, and is a composition-dependent term representing the effect of Al2O3 on the thermal expansion. Parameters necessary to calculate the volume of silicate liquids at any temperature T according to V(T) = Vrexp[α(T-Tr)], where Tr = 1400°C have been evaluated by least-square analysis of selected density measurements in aluminosilicate melts. Mean molar volumes of aluminosilicate liquids calculated according to the model equation conform to experimentally measured volumes with a root mean square difference of 0.28 and an average absolute difference of 0.90% for 248 experimental observations. The compositional dependence of is discussed in terms of several possible interpretations of the structural role of Al3+ in aluminosilicate melts. 相似文献
36.
Thermochemistry and melting properties of basalt 总被引:1,自引:0,他引:1
M. A. Bouhifd P. Besson P. Courtial C. Gérardin A. Navrotsky P. Richet 《Contributions to Mineralogy and Petrology》2007,153(6):689-698
The heat capacities of the liquid, glassy and crystalline phases of an alkali basalt have been determined from relative enthalpies
measured between 400 and 1,800 K. Values given by available models of calculation generally agree to within 2% of these results.
As derived from the new data and the enthalpy of vitrification measured at 973 K by oxide-melt drop solution calorimetry for
the same sample, the enthalpy of fusion of this basalt increases from 15.4 kJ/mol at 1,000 K to 33.6 kJ/mol at 1,800 K. Comparisons
between the enthalpies of fusion of basalt and model compositions confirm the small magnitude of the enthalpy of mixing between
the molten mineral components of the liquids. Minor variations in the chemical composition have only a small effect in the
heat capacity and the enthalpy of melting of basalt. The enthalpies of formation at 298 K from the oxides of the crystallized
and glass phases of this alkali basalt are −112.2 and −98.5 kJ/mol, respectively, for a gram formula weight based on one mole
of oxide components. 相似文献
37.
Vincent Jomelli & Pascal Bertran 《Geografiska Annaler: Series A, Physical Geography》2001,83(1-2):15-28
We analyse the morphology and sedimentology of 25 dirty snow avalanche deposits in the French Alps. The deposits typically have either a snow-ball structure or a massive structure with sliding planes. The snow balls show a longitudinal and a vertical sorting that reflects a sieve effect, similar to that observed in other rapid inertial granular flows. The massive type results from snow compaction when the avalanche is channelled by a gully or when it reaches the distal part of the scree. Velocity decrease and compaction limit the deformation to a zone at the base of the snow mass and cause the formation of distinctive sliding planes. These appear as smooth recrystallised surfaces due to local melt from frictional heating. The flow can be assimilated to a frictional granular flow. No systematic variation of size and shape of the rock debris has been observed along the profiles in both types of deposit. The distribution of rock debris and its fabric suggest that the clasts are transported passively and do not undergo any sorting during displacement. Snow melt after avalanching causes a redistribution of rock debris particularly when the snow thickness is important. This redistribution does not generate new sedimentological characteristics such as enhanced sorting or fabric. 相似文献
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Fluid composition and evolution in coesite-bearing rocks (Dora-Maira massif,Western Alps): implications for element recycling during subduction 总被引:10,自引:0,他引:10
Pascal Philippot Pierre Chevallier Christian Chopin Jean Dubessy 《Contributions to Mineralogy and Petrology》1995,121(1):29-44
Fluid inclusions and F, Cl concentration of hydrous minerals were analysed in the coesite-pyrope quartzite, the interlayered jadeite quartzite and their country-rock gneiss from the Dora-Maira massif using a combination of microthermometry, Raman spectrometry, synchrotron X-ray microfiuorescence and electron microprobe analysis. Three populations of fluid inclusions were recognized texturally and can be related to distinct metamorphic stages. A low-salinity aqueous fluid occurs in the retrogressed country gneiss and as late secondary inclusions in jadeite quartzite and chloritized pyrope. An earlier secondary population is found in matrix quartz of the jadeite- and pyro-pe-quartzites. This population can be related to the early decompression and so to incipient breakdown of garnet into phlogopite-bearing assemblages. The inclusion fluid is highly saline (up to 84 wt% equivalent NaCl) and contains Na, Ca, Fe, Cu and Zn as major cations. In pyrope quartzite, additional K was found in these brines, which locally coexist with CO2-rich inclusions. The oldest fluid inclusions are preserved in kyanite grains included in fresh pyrope and in pyrope itself. In pyrope, all inclusions have decrepitated and contain magnesite, an Mg-phosphate, sheet-silicate(s), a chloride and an opaque phase, with no fluid preser ved. In contrast, the kyanite inclusions in pyrope preserve primary H2O-CO2 low-salinity fluid inclusions, probably owing to the low compressibility of the kyanite inclusions and host garnet. In spite of in-situ re-equilibration, these inclusions can be interpreted as relics of the dehydration fluid that attended pyrope growth. These correlations between textural and chemical fluid inclusion data and metamorphic stages are consistent with the fluid composition calculated from the halogen content of different generations of phlogopite and biotite. The preservation of different fluid compositions, both in time and space, is evidence for local control and possibly origin of the fluids, in agreement with isotopic data. These results, in particular the absence of CO2 in the jadeite quartzite, are best interpreted in terms of a fluid-melt system evolution. With increasing metamorphism, partitioning of H2O, Na, Ca, Fe and heavy metals into melt (jadeite quartzite) and Mg, Na/K, F, CO2 and P(?) into a residual aqueous fluid can account for depletion in Na, Ca and Fe of the pyrope quartzite. During the retrograde path, a H 2 O rose as melt crystallized, generating the two populations of hypersaline and water-rich fluids that were highly reactive to pyrope. The process of fluid-melt interaction envisioned here coupled with models of melt extraction in subduction zones provides an attractive opportunity for the instantaneous ( < 1 Ma) and selective transport of elements between a downgoing slab and the overlying mantle wedge. 相似文献