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排序方式: 共有233条查询结果,搜索用时 921 毫秒
101.
Hydration of rhyolitic glass during weathering as characterized by IR microspectroscopy 总被引:1,自引:0,他引:1
Tadashi Yokoyama Satoshi Okumura Satoru Nakashima 《Geochimica et cosmochimica acta》2008,72(1):117-125
The mechanism and rate of hydration of rhyolitic glass during weathering were studied. Doubly polished thin sections of two rhyolites with different duration of weathering (Ohsawa lava: 26,000 yr, Awanomikoto lava: 52,000 yr) were prepared. Optical microscope observation showed that altered layers had developed along the glass surfaces. IR spectral line profile analysis was conducted on the glass sections from the surface to the interior for a length of 250 μm and the contents of molecular H2O (H2Om), OH species (OH) and total water (H2Ot) were determined. The diffusion profile of H2Om in Ohsawa lava extends beyond the layer observed by optical microscope. The content of H2Om in the hydrated region is much higher than that of OH species. Thus, the reaction from H2Om to OH appears to be little and H2Om is the dominant water species moving into the glass during weathering. Based on the concentration profiles, the diffusion coefficients of H2Om(DH2Om) and H2Ot(DH2Ot) were determined to be 2.8 × 10−10 and 3.4 × 10−10 μm2 s−1 for Ohsawa lava, and 5.2 × 10−11 and 4.1 × 10−11 μm2 s−1 for Awanomikoto lava, respectively. The obtained DH2Om during weathering are more than 2-3 orders of magnitude larger than the diffusion coefficient at ∼20 °C that is extrapolated from the diffusivity data for >400 °C. This might suggest that the mechanism of water transport is different at weathering conditions and >400 °C. 相似文献
102.
Characterization of Fe(III) (hydr)oxides in soils near the Ichinokawa mine was conducted using X-ray absorption fine structure (XAFS) and Mössbauer spectroscopies, and the structural changes were correlated with the release of As into pore-water. The Eh values decreased monotonically with depth. Iron is mainly present as poorly-ordered Fe(III) (hydr)oxides, such as ferrihydrite, over a wide redox range (from Eh = 360 to −140 mV). Structural details of the short-range order of these Fe(III) (hydr)oxides were examined using Mössbauer spectroscopy by comparing the soil phases with synthesized ferrihydrite samples having varying crystallinities. The crystallinity of the soil Fe (hydr)oxides decreased slightly with depth and Eh. Thus, within the redox range of this soil profile, ferrihydrite dominated, even under very reducing conditions, but the crystalline domain size, and, potentially, particle size, changed with the variation in Eh. In the soil–water system examined here, where As concentration and the As(III)/As(V) ratio in soil water increased with depth, ferrihydrite persisted and maintained or even enhanced its capacity for As retention with increased reducing conditions. Therefore, it is concluded that As release from these soils largely depends on the transformation of As(V) to As(III) rather than reductive dissolution of Fe(III) (hydr)oxide. 相似文献
103.
应用Terra/MODIS卫星数据估算洞庭湖蓄水量的变化 总被引:14,自引:0,他引:14
以洞庭湖为例,利用2002年的美国Terra/MODIS卫星数据,以16天为周期将全年划分为23个时段,分别对湖区水位和蓄水量分布特征和变化规律进行动态监测和综合分析。具体测算方法包括以下4个步骤: (1) 根据湖区特性,将整个洞庭湖分为3个部分:自西向东依此是西洞庭湖 (WDL), 南洞庭湖 (SDL) 和东洞庭湖 (EDL)。这3个部分的蓄水量之和就是整个洞庭湖的总蓄水量。(2) 以水体和陆地的光谱差异为基础,使用Terra/MODIS卫星的NDVI 数据识别并量测湖区水面积。(3) 将湖区水面影像同湖区数字高程模型DEM相叠加,以被监测的湖区水面的平均高度值作为水面高度。水面高度与湖底高度的差即为相应点的水深。(4) 按50 m×50 m网格大小和相应位置的水深的乘积来计算每个水柱体积。最后,将整个湖内的所有水柱的体积值累加便得到洞庭湖的总蓄水量。用上述方法测算的水位和蓄水量与实测资料进行了比较表明,两者具有很好的一致性。 相似文献
104.
Tetsuya Nishikawa Yutaka Hori Satoshi Nagai Kazutaka Miyahara Yukinobu Nakamura Kazuhiro Harada Minoru Tanda Takehiko Manabe Kuninao Tada 《Estuaries and Coasts》2010,33(2):417-427
Long-term monitoring of water quality and phytoplankton was conducted at 19 sampling stations in Harima-Nada, eastern Seto Inland Sea, Japan for 35 years from 1973 to 2007. There were two significant long-term changes, an increase in winter water temperatures of 0.042°C year?1, and a decrease in dissolved inorganic nitrogen (DIN) from about 10 μM in the 1970s to ~5 μM in the late 1990s due to the reduction in nutrient inputs. DIN concentrations and total phytoplankton cell density were both higher during the 1970s to the early 1980s and then exhibited a significant decrease in the mid 1980s and remained relatively constant thereafter. Diatoms were the dominant phytoplankton group (>90%) over the 35-year period, and there was a dramatic shift from Skeletonema dominance (~70%) to Chaetoceros in the mid 1980s. This shift in diatom species may be attributed to differences in the life cycle of Skeletonema and Chaetoceros and the response to the decrease in DIN concentration. 相似文献
105.
Ayumi Asai Takaaki Yokoyama Masumi Shimojo Satoshi Masuda Kazunari Shibata 《Journal of Astrophysics and Astronomy》2006,27(2-3):167-173
We report a detailed examination about the relationship between the evolution of the Hα flare ribbons and the released magnetic
energy during the April 10 2001 flare. In the Hα images, several bright kernels are observed in the flare ribbons. We identified
the conjugated foot-points, by analyzing the lightcurves at each Hα kernels, and showed their connectivities during the flare.
Then, based on the magnetic reconnection model, we calculated quantitatively the released energy by using the photospheric
magnetic field strengths and separation speeds of the Hα flare ribbons. Finally, we examined the downward motions which are
observed at the Hα kernels. We found that the stronger the red-asymmetry tends to be associated with the brighter the Hα kernel. 相似文献
106.
Satoshi Hinata 《Solar physics》1987,109(2):321-333
As the electrical conductivity along the magnetic field in solar atmosphere is large, parallel electric fields have been neglected in most investigations. We will first demonstrate their importance for post-flare loops, and then introduce a model for them which takes into account the effect of parallel electric fields. The electric field calculated from the model is consistent with the electric field observed by Foukal et al. (1983). 相似文献
107.
Terrigenous loading into enclosed water bodies has been blamed for eutrophic conditions marked by massive algal growth and subsequent hypoxia due to decomposition of dead algal cells. This study aims to describe the eutrophication and hypoxia processes in a semi-enclosed water body lying near a big metropolis. Phosphorus mass balance in a small inlet, Ohko Inlet, located at the head of Hiroshima Bay, Japan, was quantified using a numerical model. Dissolved inorganic phosphorous inflow from Kaita Bay next to the inlet was five times higher than that from terrigenous load, which may cause an enhancement of primary production. Therefore, it was concluded that not only the reduction of material load from the land and the suppression of benthic flux are needed, but also reducing the inflow of high phosphorus and oxygen depleted water from Kaita Bay will form a collective alternative measure to remediate the environmental condition of the inlet. 相似文献
108.
Riko Iizuka Hiroyuki Kagi Kazuki Komatsu Daichi Ushijima Satoshi Nakano Asami Sano-Furukawa Takaya Nagai Takehiko Yagi 《Physics and Chemistry of Minerals》2011,38(10):777-785
The pressure responses of portlandite and the isotope effect on the phase transition were investigated at room temperature
from single-crystal Raman and IR spectra and from powder X-ray diffraction using diamond anvil cells under quasi-hydrostatic
conditions in a helium pressure-transmitting medium. Phase transformation and subsequent peak broadening (partial amorphization)
observed from the Raman and IR spectra of Ca(OH)2 occurred at lower pressures than those of Ca(OD)2. In contrast, no isotope effect was found on the volume and axial compressions observed from powder X-ray diffraction patterns.
X-ray diffraction lines attributable to the high-pressure phase remained up to 28.5 GPa, suggesting no total amorphization
in a helium pressure medium within the examined pressure region. These results suggest that the H–D isotope effect is engendered
in the local environment surrounding H(D) atoms. Moreover, the ratio of sample-to-methanol–ethanol pressure medium (i.e.,
packing density) in the sample chamber had a significant effect on the increase in the half widths of the diffraction lines,
even at pressures below the hydrostatic limit of the pressure medium. 相似文献
109.
Tatsuyuki Yamamoto Hideo Akiyoshi Keisuke Yoshikiyo Tetsuya Takahashi Yukiko Tanabe Sakae Kudoh Satoshi Imura Naoyuki Yamamoto 《地学前缘(英文版)》2013,4(6):647-653
A study on the effect of the solar ultra-violet radiation on the human skin fibroblast cells revealed that the production of matrix metalloproteinase-2 was inhibited by the radiation.A CO2 incubator connected by optical fibers to a reflector telescope for collecting the solar light was built at Syowa station by the 49th Japanese Antarctica Research Expedition.The direction of the telescope was continuously controlled by a sun-tracker to follow the movement of the Sun automatically.The intensity of the collected light was monitored by a portable spectrophotometer housed inside.The human skin fibroblast cells were incubated in the CO2 chamber to investigate the effect of the solar radiation at Syowa station and were compared with those reference experiments at a laboratory in Japan.The results showed cell damage by strong UV radiation.The production of matrix metalloproteinase-2 was prompted by the moderate UV-B,but was inhibited by the strong UV-B radiation,as studied under laboratory conditions in Japan.The effect of strong solar radiation at Syowa station involving the radiation of UV-B region was estimated to be of the same extent of the radiation caused by an artificial UV-B light with the intensity more than 50 mJ/cm2. 相似文献
110.
Hirotsugu Minami Akihiro Hachikubo Hirotoshi Sakagami Satoshi Yamashita Yusuke Soramoto Tsuyoshi Kotake Nobuo Takahashi Hitoshi Shoji Tatyana Pogodaeva Oleg Khlystov Andrey Khabuev Lieven Naudts Marc De Batist 《Geo-Marine Letters》2014,34(2-3):241-251
The isotopic and ionic composition of pure gas hydrate (GH) water was examined for GHs recovered in three gravity cores (165–193 cm length) from the Kukuy K-9 mud volcano (MV) in Lake Baikal. A massive GH sample from core St6GC4 (143–165 cm core depth interval) was dissociated progressively over 6 h in a closed glass chamber, and 11 sequentially collected fractions of dissociated GH water analyzed. Their hydrogen and oxygen isotopic compositions, and the concentrations of Cl– and HCO3 – remained essentially constant over time, except that the fraction collected during the first 50 minutes deviated partly from this pattern. Fraction #1 had a substantially higher Cl– concentration, similar to that of pore water sampled immediately above (135–142 cm core depth) the main GH-bearing interval in that core. Like the subsequent fractions, however, the HCO3 – concentration was markedly lower than that of pore water. For the GH water fractions #2 to #11, an essentially constant HCO3 –/Cl– ratio of 305 differed markedly from downcore pore water HCO3 –/Cl– ratios of 63–99. Evidently, contamination of the extracted GH water by ambient pore water probably adhered to the massive GH sample was satisfactorily restricted to the initial phase of GH dissociation. The hydrogen and oxygen isotopic composition of hydrate-forming water was estimated using the measured isotopic composition of extracted GH water combined with known isotopic fractionation factors between GH and GH-forming water. Estimated δD of ?126 to ?133‰ and δ18O of ?15.7 to ?16.7‰ differed partly from the corresponding signatures of ambient pore water (δD of ?123‰, δ18O of ?15.6‰) and of lake bottom water (δD of ?121‰, δ18O of ?15.8‰) at the St6GC4 coring site, suggesting that the GH was not formed from those waters. Observations of breccias in that core point to a possible deep-rooted water source, consistent with published thermal measurements for the neighboring Kukuy K-2 MV. By contrast, the pore waters of core St6GC4 and also of the neighboring cores GC2 and GC3 from the Kukuy K-9 MV show neither isotopic nor ionic evidence of such a source (e.g., elevated sulfate concentration). These findings constrain GH formation to earlier times, but a deep-rooted source of hydrate-forming water remains ambiguous. A possible long-term dampening of key deep-water source signatures deserves further attention, notably in terms of diffusion and/or advection, as well as anaerobic oxidation of methane. 相似文献