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21.
Organic matter origin and distribution in suspended particulate materials and surficial sediments from the western Adriatic Sea (Italy) 总被引:5,自引:2,他引:5
T. Tesi S. Miserocchi M.A. Goi L. Langone A. Boldrin M. Turchetto 《Estuarine, Coastal and Shelf Science》2007,73(3-4):431-446
In this study, organic carbon (OC), total nitrogen (TN), stable carbon isotopic (δ13COC) and CuO reaction product compositions were used to identify the sources of organic matter (OM) and to quantify the relative importance of allochthonous and autochthonous contributions to the western Adriatic Sea, Italy. Suspended particulate material (195 samples) and surficial sediments (0–1 cm, 70 samples) from shallow cross-shelf transects were collected in February and May 2003, respectively. Vertical water column profiles were acquired along the same transects. Data include depth, potential temperature, salinity, density and chlorophyll fluorimetry.Along the western Adriatic shelf in the near-shore region, the phytoplankton growth was influenced by dynamics of the buoyant plumes from the Po and Appennine rivers. A small amount of very fine terrigenous material remained suspended within the coastal current and was exported southward along the shelf to the slope. High variability in the bulk composition was detected in the Po prodelta surficial sediments, whereas the western Adriatic shelf, although a larger area, exhibited a narrower range of values.A significant decoupling was observed between suspended particles in the water column and surficial deposits. The organic material collected in the water column was compositionally heterogeneous, with contributions from marine phytoplankton, riverine–estuarine phytoplankton and soil-derived OM. Frequent physical reworking of surficial sediments likely leads to the efficient oxidation of marine OC, resulting in the observed accumulation and preservation of refractory soil-derived OC delivered by the Po and Appennine rivers. 相似文献
22.
Sources and distribution of organic matter in a river-dominated estuary (Winyah Bay, SC, USA) 总被引:12,自引:0,他引:12
Miguel A. Goi Maria J. Teixeira David W. Perkey 《Estuarine, Coastal and Shelf Science》2003,57(5-6):1023-1048
The sources and distribution of organic matter (OM) in surface waters and sediments from Winyah Bay (South Carolina, USA) were investigated using a variety of analytical techniques, including elemental, stable isotope and organic biomarker analyses. Several locations along the estuary salinity gradient were sampled during four different periods of contrasting river discharge and tidal range. The dissolved organic carbon (DOC) concentrations of surface waters ranged from 7 mg l−1 in the lower bay stations closest to the ocean to 20 mg l−1 in the river and upper bay samples. There was a general linear relationship between DOC concentrations and salinity in three of the four sampling periods. In contrast, particulate organic carbon (POC) concentrations were significantly lower (0.1–3 mg l−1) and showed no relationship with salinity. The high molecular weight dissolved OM (HMW DOM) isolated from selected water samples collected along the bay displayed atomic carbon:nitrogen ratios ([C/N]a) and stable carbon isotopic compositions of organic carbon (δ13COC) that ranged from 10 to 30 and from −28 to −25‰, respectively. Combined, such compositions indicate that in most HMW DOM samples, the majority of the OM originates from terrigenous sources, with smaller contributions from riverine and estuarine phytoplankton. In contrast, the [C/N]a ratios of particulate OM (POM) samples varied significantly among the collection periods, ranging from low values of 5 to high values of >20. Overall, the trends in [C/N]a ratios indicated that algal sources of POM were most important during the early and late summer, whereas terrigenous sources dominated in the winter and early spring.In Winyah Bay bottom sediments, the concentrations of the mineral-associated OM were positively correlated with sediment surface area. The [C/N]a ratios and δ13COC compositions of the bulk sedimentary OM ranged from 5 to 45 and from −28 to −23‰, respectively. These compositions were consistent with predominant contributions of terrigenous sources and lesser (but significant) inputs of freshwater, estuarine and marine phytoplankton. The highest terrigenous contents were found in sediments from the river and upper bay sites, with smaller contributions to the lower parts of the estuary. The yields of lignin-derived CuO oxidation products from Winyah Bay sediments indicated that the terrigenous OM in these samples was composed of variable mixtures of relatively fresh vascular plant detritus and moderately altered soil OM. Based on the lignin phenol compositions, most of this material appeared to be derived from angiosperm and gymnosperm vascular plant sources similar to those found in the upland coastal forests in this region. A few samples displayed lignin compositions that suggested a more significant contribution from marsh C3 grasses. However, there was no evidence of inputs of Spartina alterniflora (a C4 grass) remains from the salt marshes that surround the lower sections of Winyah Bay. 相似文献
23.
Jože Kotnik Milena Horvat Emmanuel Tessier Nives Ogrinc Mathilde Monperrus David Amouroux Vesna Fajon Darija Gibičar Suzana Žižek Francesca Sprovieri Nicola Pirrone 《Marine Chemistry》2007
Mercury speciation and its distribution in surface and deep waters of the Mediterranean Sea were studied during two oceanographic cruises on board the Italian research vessel URANIA in summer 2003 and spring 2004 as part of the Med Oceaneor and MERCYMS projects. The study included deep water profiles of dissolved gaseous Hg (DGM), reactive Hg (RHg), total Hg (THg), monomethyl Hg (MeHg) and dimethyl Hg (DMeHg) in open ocean waters. Average concentrations of measured Hg species were characterized by seasonal and spatial variations. Overall average THg concentrations ranged between 0.41 and 2.65 pM (1.32 ± 0.48 pM) and were comparable to those obtained in previous studies of the Mediterranean Sea. A significant fraction of Hg was present as “reactive” Hg (average 0.33 ± 0.32 pM). Dissolved gaseous Hg (DGM), which consists mainly of Hg0, represents a considerable proportion of THg (average 20%, 0.23 ± 0.11 pM). The portion of DGM typically increased towards the bottom, especially in areas with strong tectonic activity (Alboran Sea, Strait of Sicily, Tyrrhenian Sea), indicating its geotectonic origin. No dimethyl Hg was found in surface waters down to the depth of 40 m. Below this depth, its average concentration was 2.67 ± 2.9 fM. Dissolved fractions of total Hg and MeHg were measured in filtered water samples and were 0.68 ± 0.43 pM and 0.29 ± 0.17 pM for THg and MeHg respectively. The fraction of Hg as MeHg was in average 43%, which is relatively high compared to other ocean environments. The concentrations reported in this study are among the lowest found in marine environments and the quality of analytical methods are of key importance. Speciation of Hg in sea water is of crucial importance as THg concentrations alone do not give adequate data for understanding Hg sources and cycling in marine environments. For example, photoinduced transformations are important for the presence of reactive and elemental mercury in the surface layers, biologically mediated reactions are important for the production/degradation of MeHg and DGM in the photic zones of the water column, and the data for DGM in deep sea indicate the natural sources of Hg in geotectonicaly active areas of the Mediterranean Sea. 相似文献
24.
The interstitial water composition (
, alkalinity, Ca2+, Mg2+, Sr2+, Na+, K+) and the cation exchange capacity (CEC) were determined for the muddy sediments of the continental shelf off the Gironde Estuary (France), in the area where the sediment represents the deposit of the muddy suspension of the river. In comparison with seawater concentrations, the pore waters below 10 cm depth, show depletions of
and Ca2+ and below a 30 cm depth show depletions of Mg2+. Inversely, the upper 10 cm an enrichment of Ca2+ concentration, and an increase of K+ concentration to a 40 cm depth. High values of
are observed at the top 4 cm. Alkalinity enrichment is observed along the length of the core. Applying the alkalinity models for the sediment below a 10 cm depth demonstrates generally that calculated alkalinities are higher than the measured ones. Ca2+ dissolution occurs at the first 10 cm and authigenic carbonate precipitation starts beneath that level. Mg2+ depletion is accompanied by bicarbonate loss. This proves that Mg2+ depletion is due to a Mg-silicate reaction. The result of the CEC does not confirm the Mg2+ uptake by clay minerals in exchangeable site, under reducing conditions. Diffusion and bioturbation play an important role in the pore water concentration at the top of the core. 相似文献
25.
S. C. Gonalves J. C. Marques M. A. Pardal M. F. Bouslama M. El Gtari F. Charfi-Cheikhrouha 《Estuarine, Coastal and Shelf Science》2003,58(4):901-916
The biology, population dynamics, and production of Talorchestia brito were studied at two sandy beaches located on the Atlantic (Portugal) and on the Mediterranean (Tunisia) coasts, respectively. The seasonal variation in abundance and the overall densities were similar in both populations. Reproduction occurred from February to September in the Atlantic, and from March to early November in the Mediterranean. The sex ratio was male biased in the Atlantic, and female biased in the Mediterranean. Based on data from the Atlantic population, both abundance and the proportion of reproductive females were positively correlated with temperature, while the proportion of juveniles in the population was positively correlated with temperature and sediment moisture. On average, individuals from the Atlantic were larger than the ones from the Mediterranean. Life span was estimated at six to nine months in the Atlantic, and five to eight months in the Mediterranean. Talorchestia brito was shown to be a semiannual species, with iteroparous females producing two broods per year, and exhibited a bivoltine life cycle. The minimum age required for males' and females' sexual differentiation and for female sexual maturation was shorter in the Mediterranean. Growth production (P) was estimated at 0.19 g m−2 y−1 ash free dry weight (AFDW; 4.3 kJ m−2 y−1) in the Atlantic population, and 0.217 g m−2 y−1 AFDW (4.9 kJ m−2 y−1) in the Mediterranean one. Elimination production (E) was estimated at 0.35 g m−2 y−1 AFDW (7.9 kJ m−2 y−1) in the Atlantic, and 0.28 g m−2 y−1 AFDW (6.3 kJ m−2 y−1) in the Mediterranean. The average annual biomass (
) (standing stock) was estimated at 0.032 g m−2 in the Atlantic beach, and 0.029 g m−2 in the Mediterranean one, resulting, respectively, in
ratios of 5.9 and 7.5 and
ratios of 10.8 and 9.6. Like other talitrids, T. brito exhibited geographic variation in morphometrical characteristics, sex ratio, growth rates, life span, and reproduction period, with the Atlantic population presenting a slower life history. 相似文献
26.
Several areas of erosion and accretion were observed along the Burullus-Gamasa beach. The accreted sands are coarser and less sorted than the eroded ones. Differentiation between them could be achieved on the basis of their grain-size fractions, shape of grain-size distribution curves and statistical grain-size parameter relationships. 相似文献
27.
28.
Telli-Karakoç F Ruddock PJ Bird DJ Hewer A Van Schanke A Phillips DH Peters LD 《Marine environmental research》2002,54(3-5):511-515
Juvenile turbot (Scophthalmus maximus) were injected intraperitoneally with either corn oil or 5 mg/kg benzo[a]pyrene (BaP) dissolved in corn oil and sampled I and 3 days after injection. After 1 day, no elevation of 7-ethoxyresorufin O-deethylase (EROD) activity was observed, however bile metabolites (BaP-7,8 dihydrodiol representing 70% of the total metabolites) and a single hepatic DNA adduct spot (0.47 adducts/10(8) nucleotides) identified by 32P-postlabelling were formed. No BaP metabolites or DNA adducts were observed in either control or carrier control fish. Fish sampled after 3 days reported 5-fold higher (P < 0.05) levels of EROD activity, a shift in the bile metabolite profile towards BaP phenol formation (1OH and 30H BaP comprising up to 60% of total metabolites detected) and the formation of two adduct spots (0.86 and 0.71 adducts/10(8) nucleotides). These results show that BaP can be metabolised and form hydrophobic DNA adducts in turbot without EROD elevation. Following EROD elevation, a shift in the profile of both BaP metabolites and BaP metabolite-DNA interactions occurs indicative of other oxidative processes. 相似文献
29.
François M. Costard 《Earth, Moon, and Planets》1989,45(3):265-290
In order to quantify the spatial distribution of volatiles on Mars, 2600 fluidized ejecta craters have been systematically measured, classified and mapped over the planet Mars, using 1 : 2 M scale USGS photomosaics. The latitudinal distribution of ejecta craters reveals that flower ejecta deposits (Type 1), together with low mobility ejecta, are frequently observed in the equatorial region and on ridged plains. Rampart craters (Type 2), with high mobility ejecta, occur at mid latitudes and exhibit a spatial relationship with polygonal patterns and pseudocrater areas. The increase of ejecta mobility with latitude attests for a concentration of volatiles at high latitudes. Statistical analysis shows that cratered uplands and ridged plains contain less volatile material near the surface than the underlying materials. In Chryse Planitia and Utopia Planitia the statistical study and the spatial relationships between polygonally fractured patterns, pseudocraters and the great number of high mobility ejecta deposits suggest the presence of a water-rich alluvial deposit close to the surface near the mouth of Chryse and Elysium channels. This result explains, on a more quantitative basis, the idea that fractured patterns were preferentially developed in a volatile-rich sedimentary deposits. The behaviour of volatiles, at 41 S, 257 W near Reull Vallis, exhibits a strong anomaly, with the presence of an abnormally volatile rich layer close to the surface. 相似文献
30.
Atίla Özgüç 《Solar physics》1989,123(2):381-383
After re-examination of data presented by Verma (1984), some misuse of solar parameteres published in Solar Geophysical Data is presented. Consequently some conclusions made by Verma (1984, 1986) on about the longitudinal distribution of cool solar surges based on these misuses are discussed. 相似文献