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Estimates of greenhouse gas evasion from rivers have been refined over the past decades to constrain their role in global carbon cycle processes. However, despite 55% of the human population living in urban areas, urban rivers have had limited attention. We monitored carbon dynamics in an urbanized river (River Kelvin, 331 km2, UK) to explore the drivers of dissolved carbon lateral and vertical export. Over a 2-year sampling period, riverine methane (CH4) and carbon dioxide (CO2) concentrations were consistently oversaturated with respect to atmospheric equilibria, leading to continual degassing to the atmosphere. Carbon stable isotopic compositions (δ13C) indicated that terrestrially derived carbon comprised most of the riverine CH4 and dissolved CO2 (CO2*) load while dissolved inorganic carbon (DIC) from groundwater was the main form of riverine DIC. The dynamics of CH4, CO2*, and DIC in the river were primarily hydrology-controlled, that is, [CH4] and [CO2*] both increased with elevated discharge, total [DIC] decreased with elevated discharge while the proportion of biologically derived DIC increased with increasing discharge. The concentration of dissolved organic carbon (DOC) showed a weak relationship with river hydrology in summer and autumn and was likely influenced by the combined sewer overflows. Carbon emission to the atmosphere is estimated to be 3.10 ± 0.61 kg C·m−2·yr−1 normalized to water surface area, with more than 99% emitted as CO2. Annual carbon loss to the coastal estuary is approximately 4.69 ± 0.70 Gg C yr−1, with annual DIC export approximately double that of DOC. Per unit area, the River Kelvin was a smaller carbon source to the atmosphere than natural rivers/streams but shows elevated fluxes of DIC and DOC under comparable conditions. This research illustrates the role urban systems may have on riverine carbon dynamics and demonstrates the potential tight link between urbanization and riverine carbon export. 相似文献
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155.
酸洗法测定海洋沉积物有机碳和无机碳含量的致命缺陷 总被引:2,自引:0,他引:2
Organic and inorganic carbon contents of marine sediments are important to reconstruct marine productivity,global carbon cycle, and climate change. A proper method to separate and determine organic and inorganic carbons is thus of great necessity. Although the best method is still disputable, the acid leaching method is widely used in many laboratories because of its ease-of-use and high accuracy. The results of the elemental analysis of sediment trap samples reveal that organic and inorganic carbon contents cannot be obtained using the acid leaching method, causing an infinitely amplified error when the carbon content of the decarbonated sample is 12%±1% according to a mathematical derivation. Acid fumigation and gasometric methods are used for comparison, which indicates that other methods can avoid this problem in organic carbon analysis. For the first time, this study uncovers the pitfalls of the acid leaching method, which limits the implication in practical laboratory measurement, and recommends alternative solutions of organic/inorganic carbon determination in marine sediments. 相似文献
156.
Łydżba Dariusz Różański Adrian Sevostianov Igor Stefaniuk Damian 《Acta Geotechnica》2022,17(11):5059-5072
Acta Geotechnica - We evaluate thermal conductivity of the skeleton of porous sandstone from the measurements of the effective thermal conductivities of dry and saturated specimens provided by... 相似文献
157.
Microstructural evidence for a disequilibrium condensation origin for hibonite‐spinel inclusions in the ALHA77307 CO3.0 chondrite 下载免费PDF全文
Jangmi Han Adrian J. Brearley Lindsay P. Keller 《Meteoritics & planetary science》2015,50(12):2121-2136
Two hibonite‐spinel inclusions (CAIs 03 and 08) in the ALHA77307 CO3.0 chondrite have been characterized in detail using the focused ion beam sample preparation technique combined with transmission electron microscopy. These hibonite‐spinel inclusions are irregularly shaped and porous objects and consist of randomly oriented hibonite laths enclosed by aggregates of spinel with fine‐grained perovskite inclusions finally surrounded by a partial rim of diopside. Melilite is an extremely rare phase in this type of CAI and occurs only in one inclusion (CAI 03) as interstitial grains between hibonite laths and on the exterior of the inclusion. The overall petrologic and mineralogical observations suggest that the hibonite‐spinel inclusions represent high‐temperature condensates from a cooling nebular gas. The textural relationships indicate that hibonite is the first phase to condense, followed by perovskite, spinel, and diopside. Texturally, melilite condensation appears to have occurred after spinel, suggesting that the condensation conditions were far from equilibrium. The crystallographic orientation relationships between hibonite and spinel provide evidence of epitaxial nucleation and growth of spinel on hibonite surfaces, which may have lowered the activation energy for spinel nucleation compared with that of melilite and consequently inhibited melilite condensation. Hibonite contains abundant stacking defects along the (001) plane consisting of different ratios of the spinel and Ca‐containing blocks within the ideal hexagonal hibonite structure. This modification of the stacking sequence is likely the result of accommodation of excess Al in the gas into hibonite due to incomplete condensation of corundum from a cooling gas under disequilibrium conditions. We therefore conclude that these two hibonite‐spinel inclusions in ALHA77307 formed by high‐temperature condensation under disequilibrium conditions. 相似文献
158.
Satellite laser ranging to GPS and GLONASS 总被引:5,自引:4,他引:1
159.
GOCE: assessment of GPS-only gravity field determination 总被引:2,自引:1,他引:1
160.
The synchronization between the orbital motion and axial rotation of the two component stars of a binary system is reviewed.
Some previous published papers are mentioned and the general conclusion is outlined: If we shall use a rotating coordinate
system synchronous with one of the two stellar axial rotations, it is not possible to obtain a Jacobi integral and the Roche
geometry cannot be further analyzed. In addition, a theoretical approach is summarized in order to use the axial rotations
of the two component stars, even if the constants of the stellar structure (k2)1, (k2)2must be taken into consideration. So it is found that if the stellar angular velocities are higher than the corresponding
Keplerian angular velocity (ωi≫ ωk, i=
), the problem of the rotational effect could be of practical consideration. Finally, a theoretical relationship between the
two constants (k2)1and (k2)2of the stellar structure is established. 相似文献