On the absolute determination of the deflections of the plumb-line     

F. Andersson 《Journal of Geodesy》1971,45(3):335-340

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Thallium isotope composition of the upper continental crust and rivers—An investigation of the continental sources of dissolved marine thallium     

Sune G. Nielsen  Mark Rehkämper  Per Andersson  Peter W. Swarzenski  Detlef Günther 《Geochimica et cosmochimica acta》2005,69(8):2007-2019

The thallium (Tl) concentrations and isotope compositions of various river and estuarine waters, suspended riverine particulates and loess have been determined. These data are used to evaluate whether weathering reactions are associated with significant Tl isotope fractionation and to estimate the average Tl isotope composition of the upper continental crust as well as the mean Tl concentration and isotope composition of river water. Such parameters provide key constraints on the dissolved Tl fluxes to the oceans from rivers and mineral aerosols.The Tl isotope data for loess and suspended riverine detritus are relatively uniform with a mean of ε²⁰⁵Tl = −2.0 ± 0.3 (ε²⁰⁵Tl represents the deviation of the ²⁰⁵Tl/²⁰³Tl isotope ratio of a sample from NIST SRM 997 Tl in parts per 10⁴). For waters from four major and eight smaller rivers, the majority were found to have Tl concentrations between 1 and 7 ng/kg. Most have Tl isotope compositions very similar (within ±1.5 ε²⁰⁵Tl) to that deduced for the upper continental crust, which indicates that no significant Tl isotope fractionation occurs during weathering. Based on these results, it is estimated that rivers have a mean natural Tl concentration and isotope composition of 6 ± 4 ng/kg and ε²⁰⁵Tl = −2.5 ± 1.0, respectively.In the Amazon estuary, both additions and losses of Tl were observed, and these correlate with variations in Fe and Mn contents. The changes in Tl concentrations have much lower amplitudes, however, and are not associated with significant Tl isotope effects. In the Kalix estuary, the Tl concentrations and isotope compositions can be explained by two-component mixing between river water and a high-salinity end member that is enriched in Tl relative to seawater. These results indicate that Tl can display variable behavior in estuarine systems but large additions and losses of Tl were not observed in the present study.  相似文献   

The Moon: A Taylor perspective   总被引：1，自引：0，他引：1  

S. Ross Taylor  G. Jeffrey Taylor  L. August Taylor 《Geochimica et cosmochimica acta》2006,70(24):5904-5918

We address several current lunar problems. The data suggest that the Moon likely possesses an Fe-rich metallic core a few percent of lunar volume, although definitive proof is lacking. Refractory elements appear to be enriched relative both to the composition of the primordial solar nebula (CI) and the Earth. Very volatile elements appear to be depleted uniformly at high levels. We adopt the single-impact hypothesis for lunar origin, which formed a high-temperature silicate vapor disk, mostly of metal-poor silicate material from an impactor (Theia) that was already depleted in volatiles. We speculate that the curious lunar bulk-composition resulted from condensation from high-temperature vapor at around a few Earth radii. This could produce an enriched refractory-element composition that cut off below 1000 K, producing a uniform depletion in very volatile elements.  相似文献   

Modelling of uranium and neptunium chemistry in a deep rock environment     

Iréne Lundén  Karin Andersson  Gunnar Skarnemark 《Aquatic Geochemistry》1996,2(4):345-358

According to the present concept for final storage of spent nuclear fuel in Sweden, the spent fuel, encapsulated in copper or copper/steel canisters, will be placed in tunnels in a deep rock formation. The canisters will be surrounded by compacted bentonite clay acting as a buffer material. In connection with a safety analysis of such a storage facility, the total solubility of certain elements (e.g., uranium) as well as the transport properties (e.g., retardation due to sorption on mineral surfaces) of the long-lived radionuclides released from the canister have to be predicted or measured. The chemical conditions, governing the solubility and speciation of trace elements encountered in and around the repository depend on interactions between the ground water and the engineering materials in the repository and a production of oxidants due to radiolysis in the spent fuel. In the present study the speciation and solubility of uranium and neptunium in a bentonite-ground water system and in ground waters with compositions measured at a site at äspö, SE Sweden, have been calculated. The calculations have been carried out using a recent version of the geochemical computer code PHREEQE and the database HATCHES 5.0. Predictions of the uranium and neptunium concentrations in the ground water in the vicinity of a damaged high level waste repository have also been performed. The uranium concentration in the water in the bentonite barrier is predicted to be of the same order of magnitude or lower than that found in some granitic ground waters. For neptunium the calculations are uncertain due to the small amount of experimentally determined thermodynamic data and few verifications under the conditions (pH - Eh - carbonate concentration) considered. The predicted concentrations (ca 10^–12 m, corresponds to ca 0.006 Bq/l) may be regarded as high, considering the high toxicity of neptunium and its long half-life.  相似文献   

Levels and patterns of polychlorinated dibenzo-p-dioxins, dibenzofurans and biphenyls in surface sediments from the western Baltic Sea (Arkona Basin) and the Oder River estuarine system     

D. Dannenberger  R. Andersson  C. Rappe 《Marine pollution bulletin》1997,34(12):1016-1024

Surface sediment samples were collected from the western Baltic Sea (Arkona Basin) and the Oder River estuarine system in May and August 1995 and analysed for polychlorinated dibenzo-p-dioxins, dibenzofurans and biphenyls. Contents of PCDF (sum) and PCDD (sum) varied from 2.5 to 820.0 pg g⁻¹ dw and from 12.7 to 2991.0 pg g⁻¹ dw, respectively. PCB contents (sum of 23 congeners) ranged between < 130.0 and 16267.0 pg g⁻¹ dw. Only slight variations in PCDF/D and PCB contents on dry weight basis were found between the Oder River estuarine system and the open Baltic Sea. TOC-normalization of the data showed an approximately homogen PCDF/D distribution in the study area. The distribution pattern for PCDF/D and PCB may be attributed to high sediment dynamics combined with transport processes from the temporary sedimentation basin (Oderhaff) to the deeper parts of the Baltic Sea.  相似文献   

Modelling the dynamics of superfluid neutron stars     

N. Andersson 《Astrophysics and Space Science》2007,308(1-4):395-402

In this brief summary I describe our recent work on superfluid neutron star dynamics. I review results on shear viscosity, hyperon bulk viscosity, vortex mediated mutual friction and the modelling of multifluid systems in general. For each problem I provide a set of questions that need to be addressed by future work.  相似文献   

Colloidal rare earth elements in a boreal river: Changing sources and distributions during the spring flood     

Karen Andersson  David Turner  Björn Stolpe  Johan Ingri 《Geochimica et cosmochimica acta》2006,70(13):3261-3274

Variations in the physico-chemical speciation of the rare earth elements (REE) have been investigated in a subarctic boreal river during an intense spring flood event using prefiltered (<100 μm) samples, cross-flow (ultra)filtration (CFF), flow field-flow fractionation (FlFFF), and diffusive gradients in thin films (DGT). This combination of techniques has provided new information regarding the release and transport of the REE in river water. The colloidal material can be described in terms of two fractions dominated by carbon and iron, respectively. These two fractions, termed colloidal carrier phases, showed significant temporal changes in concentration and size distribution. Before the spring flood, colloidal carbon concentrations were low, the colloids being dominated by relatively large iron colloids. Colloidal concentrations increased sharply during the spring flood, with smaller carbon colloids dominating. Following the spring flood, colloidal concentrations decreased again, smaller carbon colloids still dominating. The REE are transported mainly in the particulate and colloidal phases. Before the spring flood, the REE composition of all measured fractions was similar to local till. During the spring flood, the REE concentrations in the colloidal and particulate fractions increased. The increase was most marked for the lighter REE, which therefore showed a strong enrichment when normalized to local till. Following the spring flood, the REE concentrations decreased again and reverted to a distribution similar to local till. These changes in the concentration and distributions of carbon iron and REE are interpreted in terms of changing hydrological flow paths in soil and bedrock which occur during the spring flood.  相似文献   

A search for millimeter-wave emission from HCN and other molecules in Comet Bradfield (1979l)     

L. Ekelund  W.M. Irvine  Ch. Andersson  F.P. Schloerb  S.E. Robinson 《Icarus》1981,47(3):431-433

Millimeter-wave emission from HCN, CS, CH₃OH, and two unidentified lines (previously observed in Comet Kohoutek (1973 XII)) was sought and not detected from Comet Bradfield (1979l) after perihelion passage. Limits on column densities and production rates are derived. In the case of HCN, the production rate is less than that reported for Comet Kohoutek, even after scaling relative to the observed OH emission from each comet.  相似文献   

Seasonal changes in the distribution and exchange of inorganic nitrogen between sediment and water in the Northern Baltic (Gulf of Bothnia)     

David B. Nedwell  Sven-Eric Hall  Agneta Andersson  Åke F. Hagström  E.Börje Lindström 《Estuarine, Coastal and Shelf Science》1983,17(2):169-179

The concentration profiles of nitrate plus nitrite, ammonium, and redox potential in sediment and water column were determined in late winter and summer at a sampling site off Norrbyn, northern Sweden, in the Gulf of Bothnia. The sediment had an oxidized surface layer during winter and spring, and nitrification occurred. Nitrate but not ammonium was present in the water column at this time. During summer a layer of planktonic detritus was deposited onto the sediment and led to its deoxygenation and reduction. Ammonium was then the predominant form of inorganic nitrogen in the water column.Laboratory experiments confirmed that nitrification in the surface layer of sediment prevented ammonium export during winter. Enhanced temperature or organic detritus deoxygenated the surface sediment and inhibited nitrification, and export of ammonium from the sediment increased. Although nitrification was important in determining the flow of nitrogen in the sediment it accounted for at most only 5% of the total oxygen uptake by the sediment.  相似文献   

Precipitation and evaporation budgets over the Baltic Proper: observations and modelling     

Ann-Sofi Smedman  Sven-Erik Gryning  Karl Bumke  Ulf H  gstr  m  Anna Rutgersson  Ekaterina Batchvarova  Gerhard Peters  Barbara Hennemuth  Bengt Tammelin  Reijo Hyv  nen  Anders Omstedt  Daniel Michelson  Tage Andersson  Marco Clemens 《Journal of Atmospheric & Ocean Science》2005,10(3):163-191

Precipitation and evaporation budgets over the Baltic Sea were studied in a concerted project called PEP in BALTEX (Pilot study of Evaporation and Precipitation in the Baltic Sea), combining extensive field measurements and modelling efforts. Eddy-correlation-measurements of turbulent heat flux were made on a semi-continuous basis for a 12 month period at four well-exposed coastal sites in the Baltic Proper (the main basin of the Baltic Sea). Precipitation was measured at land-based sites with standard gauges and on four merchant ships travelling between Germany and Finland with the aid of specially designed ship rain gauges (SRGs). The evaporation and precipitation regime of the Baltic Sea was modelled for a 12 month period by applying a wide range of numerical models: the operational atmospheric High Resolution Limited Area Model (HIRLAM, Swedish and Finnish versions), the German atmospheric REgional-scale MOdel, REMO, the operational German Europe Model (only precipitation), the oceanographic model PROBE-Baltic, and two models that use interpolation of ground-based data, the Swedish MESAN model of SMHI and a German model of IFM-GEOMAR Kiel. Modelled precipitation was compared with SRG measurements on board the ships. A reasonable correlation was obtained, but the regional-scale models and MESAN gave some 20% higher precipitation over the sea than is measured. Bulk parameterisation schemes for evaporation were evaluated against measurements. A constant value of C_HN and C_EN with wind speed, underestimated large fluxes of both sensible and latent heat flux. The limited area models do not resolve the influence of the height of the marine boundary layer in coastal zones and the entrainment (on the surface fluxes), which may explain the observed low correlations between modelled and measured latent heat fluxes. Estimates of evaporation, E, and precipitation, P, for the entire Baltic Proper were made with several models for a 12 month period. While the annual variation was well represented by all predictions, there are still important differences in the annual means. Evaporation ranges from 509 to 625 mm year^-1 and precipitation between 624 and 805 mm year^-1 for this particular 12 month period. Taking the results of model verification from the present study into account, the best estimate of P-E is about 100 ± 50 mm for this particular 12 month period. But the annual mean of P-E varies considerably from year to year. This is reflected in simulations with the PROBE-Baltic model for an 18 year period, which gave 95 mm year^-1 for the 12 month period studied here and 32 mm year^-1 as an average for 18 years.  相似文献