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11.
Magnesium isotope systematics of the lithologically varied Moselle river basin, France 总被引:2,自引:0,他引:2
Agnès Brenot Christophe Cloquet Nathalie Vigier Jean Carignan Christian France-Lanord 《Geochimica et cosmochimica acta》2008,72(20):5070-5089
Magnesium and strontium isotope signatures were determined during different seasons for the main rivers of the Moselle basin, northeastern France. This small basin is remarkable for its well-constrained and varied lithology on a small distance scale, and this is reflected in river water Sr isotope compositions. Upstream, where the Moselle River drains silicate rocks of the Vosges mountains, waters are characterized by relatively high 87Sr/86Sr ratios (0.7128-0.7174). In contrast, downstream of the city of Epinal where the Moselle River flows through carbonates and evaporites of the Lorraine plateau, 87Sr/86Sr ratios are lower, down to 0.70824.Magnesium in river waters draining silicates is systematically depleted in heavy isotopes (δ26Mg values range from −1.2 to −0.7‰) relative to the value presently estimated for the continental crust and a local diorite (−0.5‰). In comparison, δ26Mg values measured in soil samples are higher (∼0.0‰). This suggests that Mg isotope fractionation occurs during mineral leaching and/or formation of secondary clay minerals. On the Lorraine plateau, tributaries draining marls, carbonates and evaporites are characterized by low Ca/Mg (1.5-3.2) and low Ca/Sr (80-400) when compared to local carbonate rocks (Ca/Mg = 29-59; Ca/Sr = 370-2200), similar to other rivers draining carbonates. The most likely cause of the Mg and Sr excesses in these rivers is early thermodynamic saturation of groundwater with calcite relative to magnesite and strontianite as groundwater chemistry progressively evolves in the aquifer. δ26Mg of the dissolved phases of tributaries draining mainly carbonates and evaporites are relatively low and constant throughout the year (from −1.4‰ to −1.6‰ and from −1.2‰ to −1.4‰, respectively), within the range defined for the underlying rocks. Downstream of Epinal, the compositions of the Moselle River samples in a δ26Mg vs. 87Sr/86Sr diagram can be explained by mixing curves between silicate, carbonate and evaporite waters, with a significant contribution from the Vosgian silicate lithologies (>70%). Temporal co-variation between δ26Mg and 87Sr/86Sr for the Moselle River throughout year is also observed, and is consistent with a higher contribution from the Vosges mountains in winter, in terms of runoff and dissolved element flux. Overall, this study shows that Mg isotopes measured in waters, rocks and soils, coupled with other tracers such as Sr isotopes, could be used to better constrain riverine Mg sources, particularly if analytical uncertainties in Mg isotope measurements can be improved in order to perform more precise quantifications. 相似文献
12.
Philippe E. Raison Regis Jardin Daniel Bouëxière Rudy J. M. Konings Thorsten Geisler Claudiu C. Pavel Jean Rebizant Karin Popa 《Physics and Chemistry of Minerals》2008,35(10):603-609
The crystallographic structures of the synthetic cheralite, CaTh(PO4)2, and its homolog CaNp(PO4)2 have been investigated by X-ray diffraction at room temperature. Rietveld analyses showed that both compounds crystallize in the monoclinic system and are isostructural to monazite LnPO4 (Ln = La to Gd). The space group is P21/n (I.T. = 14) with Z = 2. The refined lattice parameters of CaTh(PO4)2 are a = 6.7085(8) Å, b = 6.9160(6) Å, c = 6.4152(6) Å, and β = 103.71(1)° with best fit parameters R wp = 4.87%, R p = 3.69% and R B = 3.99%. For CaNp(PO4)2, we obtained a = 6.6509(5) Å, b = 6.8390(3) Å, c = 6.3537(8) Å, and β = 104.12(6)° and R wp = 6.74%, R p = 5.23%, and R B = 6.05%. The results indicate significant distortions of bond length and angles of the PO4 tetrahedra in CaTh(PO4)2 and to a lesser extent in CaNp(PO4)2. The structural distortions were confirmed by Raman spectroscopy of CaTh(PO4)2. A comparison with the isostructural compounds LnPO4 (Ln = Ce and Sm) confirmed that the substitution of the large rare earth trivalent cations with Ca2+ and Th4+ introduces a distortion of the PO4 tetrahedra. 相似文献
13.
We test the hypothesis that flexural isostatic compensation of the mass removed by enhanced Quaternary erosion is responsible for uplift of the Western European Alps and their forelands. We use two well‐preserved and well‐dated (1.8 Ma) abandonment surfaces of foreland basin remnants in SE France (the Chambaran and Valensole plateaux) as passive benchmarks for tilting of the foreland. Estimating their initial slope from morphometric scaling relationships, we determine bulk post‐depositional tilting of 0.5–0.8% for these surfaces. The calculated isostatic response of the Alpine lithosphere to erosional unloading, using the method recently proposed by Champagnac et al. [Geology 35 (2007) 195–198] , yields a predicted tilting of 0.3–0.4% in the considered areas, explaining approximately half of the determined post‐depositional tilting. Such long‐term deformation being insensitive to cyclic loading/unloading because of glaciations, we suspect the other half to be related to as yet undetermined long‐wavelength and long‐lived tectonic process(es). 相似文献
14.
Methods are described for the complexometric determination of calcium and magnesium in seawater, using an amalgamated silver electrode for end-point detection. In the presence of a small amount of mercury(II)-chelonate, the amalgamated silver electrode serves as a pM indicator during the complexometric titration, the Hg complex being stronger than Ca, Mg and Sr complexes. Calcium is determined by titration with EGTA, calcium+magnesium+strontium by titration with EDTA and magnesium is obtained by difference. Average values of 0.02120 (standard deviation 0.00004) for Ca:Cl‰ and 0.06671 (standard deviation 0.00014) for Mg:Cl‰ were obtained for samples from tropical North Atlantic Ocean. 相似文献
15.
16.
Jean Pierre Baudin 《Marine environmental research》1982,7(3):227-233
Uptake of 65Zn by Gammarus aequicauda results in a concentration factor of approximately 50 and it is characterised by a maximal accumulation level attained as early as the third day of the experiment. After ingestion by the gammarids of twenty contaminated meals which are distributed over a 45-day period, a transfer of 65Zn between the food and the consumer can be observed but there is no sign of the biomagnification phenomenon. The retention rate of the radionuclide is only about 1·5% and the 65Zn concentration in the gammarids remains markedly inferior to that of the ingested food.The elimination of the 65Zn fixed directly from water takes place according to an exponential model which corresponds to the existence of three biological half-lives of the radionuclide, . The excretion of 65Zn accumulated from food is a simple exponential phenomenon which corresponds to only one biological half-life of approximately 17 days. 相似文献
17.
Abstract. Boonea (= Odostomia) impressa is a common ectoparasite of oysters. In the laboratory, small oysters (Crassostrea virginica) parasitized by natural densities of B. impressa produced 75 % less new shell than unparasitized oysters. Shell deposition rates of previously parasitized oysters increased significantly after all B. impressa were removed. Thus, the decrease in growth rate, although significant, apparently was not permanent. B. impressa preferentially parasitized small, living oysters (≤2.5cm) in the field, even though a higher percentage of large, living oysters (>2.5cm) was available. The snails maintained an aggregated distribution on the oyster reef. The number of B. impressa per oyster clump was positively correlated with the number of living oysters per clump, however some clumps with few or no living oysters had many B. impressa. Thus, food availability only partially explained the pattern of distribution. B. impressa was very mobile. About 50 % of the population moved in one week. Reproduction occurred throughout the year with a peak period in May. Recruitment was greatest in July, however new recruits were observed throughout the year. The reduction in growth rate of parasitized oysters, the snaiľs propensity towards parasitizing small oysters and the snail's tendency to be contagiously distributed suggests that B. impressa potentially exerts a significant influence on the population structure and health of oyster populations. 相似文献
18.
Lina Li Jean Guenzennec Peter Nichols Pierre Henry Miki Yanagibayashi Chiaki Kato 《Journal of Oceanography》1999,55(5):635-642
Dense populations of bivalves, primarily Calyptogena sp., were observed at cold seeps of the Nankai Trough. Bacterial input to the sediment was estimated through determination of phospholipid ester-linked fatty acid (PLFA) and DNA profiles. Results indicated a bacterial biomass of 109 cells (g dry wt)-1 while individual fatty acid profiles revealed a predominance of monounsaturated fatty acids, mainly 18:1 isomers. The presence of these fatty acids can be interpreted to reflect a response to low temperature and a predominance of psychrophilic bacteria. DNA fragments encoding bacterial ribosomal RNA small-subunit sequences (16S rDNA) were amplified by the polymerase chain reaction method using DNA extracted directly from the sediment samples. From the sequencing results, at least 19 kinds of bacterial 16S rDNAs related to mostly the Proteobacteria and a few gram-positive bacteria were identified. These results suggest that the bacterial community in the Nankai Trough sediments consists of mainly bacteria belonging to the Proteobacteria , , and subdivisions. Bacteria belonging to the and subdivisions, which are known to include epibiont and sulfate reducing bacteria, respectively, were mostly detected in the sediment obtained from inside the area of the Calyptogena community, and the -Proteobacteria may function to supply reduced sulfur to bacterial endosymbionts of Calyptogena. 相似文献
19.
The Côte d’Ivoire–Ghana transform margin is bounded to the south by a prominent marginal ridge. ODP Leg 159 shipboard analyses on sediments from four sites document three distinct transform margin sedimentary and tectonic stages of evolution: (1)?an intracontinental stage of transform faulting recorded in deformed lacustrine to marine siliciclastic sequences; (2)?a marginal ridge uplift stage, recorded by shallow water limestones, appears coeval with the passing of a hot, oceanic spreading center just south of the sediment wedge; and (3)?cool ing subsidence of the transform margin recorded in bathyal to abyssal sediments emphasizes a passive margin stage. These results are consistent with previously published models of evolution. 相似文献
20.
Nabil Sultan Pierre Cochonat Jean Fran ois Bourillet Florence Cayocca 《Marine Georesources & Geotechnology》2001,19(2):107-133
This article presents a methodology developed to evaluate the instability of submarine slopes that extend over a large area. Special attention was paid to (1) the complex geometry (bathymetry) and the expanse of the slope, (2) the heterogeneity of the sediment, and (3) the distribution of the pore pressure. The safety factor was considered as a spatially varying quantity. The General Formulation (GLE, Fredlund and Krahn 1977), which fully satisfies equilibrium conditions, was used for evaluating the stability of the marine slope. The submarine slope failure, which occurred on 16 October 1979 during the construction of the new Nice airport, was studied in order to test the developed model. Geotechnical parameters were taken from experimental tests carried out by IFREMER on 19 cores extracted at different depths (from 27 m to 1300 m) (Cochonat, Bourillet, and Savoye, 1993; Mulder et al., 1994). Many scenarios were proposed in order to explain the cause of the Nice slope failure (Habib, 1994). In this article, two of those scenarios were tested. Simulation results are presented and discussed. 相似文献