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81.
Dissolution and precipitation rates of brucite (Mg(OH)2) were measured at 25°C in a mixed-flow reactor as a function of pH (2.5 to 12), ionic strength (10−4 to 3 M), saturation index (−12 < log Ω < 0.4) and aqueous magnesium concentrations (10−6 to 5·10−4 M). Brucite surface charge and isoelectric point (pHIEP) were determined by surface titrations in a limited residence time reactor and electrophoretic measurements, respectively. The pH of zero charge and pHIEP were close to 11. A two-pK, one site surface speciation model which assumes a constant capacitance of the electric double layer (5 F/m2) and lack of dependence on ionic strength predicts the dominance of >MgOH2+ species at pH < 8 and their progressive replacement by >MgOH° and >MgO− as pH increases to 10-12. Rates are proportional to the square of >MgOH2+ surface concentration at pH from 2.5 to 12. In accord with surface speciation predictions, dissolution rates do not depend on ionic strength at pH 6.5 to 11. Brucite dissolution and precipitation rates at close to equilibrium conditions obeyed TST-derived rate laws. At constant saturation indices, brucite precipitation rates were proportional to the square of >MgOH2+ concentration. The following rate equation, consistent with transition state theory, describes brucite dissolution and precipitation kinetics over a wide range of solution composition and chemical affinity:
82.
The profiles of six photospheric absorption spectral lines (Fei 5250 Å, Fei 5324 Å, Fei 5576 Å, Cai 5590 Å, Cai 6103 Å and Fei 6165 Å), measured in the kernel of a 2N solar flare and in a quiet-Sun area, were compared. The observations were carried out with an echelle spectrograph of the Crimean Astrophysical Observatory. It was shown that, compared to the quiet-Sun profiles, the flare profiles are shallower in the line core and are less steep in the wings. Therefore, measurements of the longitudinal magnetic field made with a magnetograph system which uses the Cai 6103 Å spectral line, can be underestimated by 18–25% in areas of bright H ribbons of a moderate solar flare. Modeling of the solar photosphere performed by using a synthesis method showed that, in a solar flare, the enhanced core emission seems to be related to heating of the photosphere by the flare, whereas the decrease of the slope of the wings was presumably caused by the inhomogeneity of the photospheric magnetic field. 相似文献
83.
Technology innovation and diffusion in “less than ideal” climate policies: An assessment with the WITCH model 总被引:1,自引:1,他引:0
This paper examines the dynamics of innovation in low-carbon energy technologies distinguishing between research and development and technology diffusion as a response to alternative climate policies. We assess the implications of second-best policies that depart from the assumption of immediate and global participation and of full technology availability. The analysis highlights the heterogeneous effects of climate policy on different energy R&D programs and discusses the contribution of important determinants such as carbon price and policy stringency, policy credibility, policy and technological spillovers and absorptive capacity. 相似文献
84.
Gunnar Luderer Valentina Bosetti Michael Jakob Marian Leimbach Jan C. Steckel Henri Waisman Ottmar Edenhofer 《Climatic change》2012,114(1):9-37
This paper synthesizes the results from the model intercomparison exercise among regionalized global energy-economy models conducted in the context of the RECIPE project. The economic adjustment effects of long-term climate policy are investigated based on the cross-comparison of the intertemporal optimization models ReMIND-R and WITCH as well as the recursive dynamic computable general equilibrium model IMACLIM-R. A number of robust findings emerge. If the international community takes immediate action to mitigate climate change, the costs of stabilizing atmospheric CO2 concentrations at 450?ppm (roughly 530?C550?ppm-e) discounted at 3% are estimated to be 1.4% or lower of global consumption over the twenty-first century. Second best settings with either a delay in climate policy or restrictions to the deployment of low-carbon technologies can result in substantial increases of mitigation costs. A delay of global climate policy until 2030 would render the 450?ppm target unachievable. Renewables and CCS are found to be the most critical mitigation technologies, and all models project a rapid switch of investments away from freely emitting energy conversion technologies towards renewables, CCS and nuclear. Concerning end use sectors, the models consistently show an almost full scale decarbonization of the electricity sector by the middle of the twenty-first century, while the decarbonization of non-electric energy demand, in particular in the transport sector remains incomplete in all mitigation scenarios. The results suggest that assumptions about low-carbon alternatives for non-electric energy demand are of key importance for the costs and achievability of very low stabilization scenarios. 相似文献
85.
Climate is simulated for reference and mitigation emissions scenarios from Integrated Assessment Models using the Bern2.5CC
carbon cycle–climate model. Mitigation options encompass all major radiative forcing agents. Temperature change is attributed
to forcings using an impulse–response substitute of Bern2.5CC. The contribution of CO2 to global warming increases over the century in all scenarios. Non-CO2 mitigation measures add to the abatement of global warming. The share of mitigation carried by CO2, however, increases when radiative forcing targets are lowered, and increases after 2000 in all mitigation scenarios. Thus,
non-CO2 mitigation is limited and net CO2 emissions must eventually subside. Mitigation rapidly reduces the sulfate aerosol loading and associated cooling, partly
masking Greenhouse Gas mitigation over the coming decades. A profound effect of mitigation on CO2 concentration, radiative forcing, temperatures and the rate of climate change emerges in the second half of the century. 相似文献
86.
87.
Despite the growing concern about actual on-going climate change, there is little consensus on the scale and timing of actions needed to stabilise the concentrations of greenhouse gases. Many countries are unwilling to implement mitigation strategies, at least in the short term, and no agreement on an ambitious global stabilisation target has yet been reached. It is thus likely that international climate policies will be characterized by a high degree of uncertainty over the stringency of the climate objective, and that some countries might delay their participation to global action. What additional economic costs will this delay in the adoption of mitigation measures imply? What would the optimal short-term strategy be given the uncertainty surrounding the climate policy to come? Is there a hedging strategy that decision makers can adopt to cope with delayed action and uncertain targets? This paper addresses these questions by quantifying the economic implications of delaying mitigation action, and by computing the optimal abatement strategy in the presence of uncertainty about a global stabilisation target (which will be agreed upon in future climate negotiations). Results point to short-term inaction as the key determinant for the economic costs of ambitious climate policies. They also indicate that there is an effective hedging strategy that could minimise the cost of climate policy uncertainty over the global stabilisation target: a short-term moderate climate policy would be a good strategy to reduce the costs of delayed action and to cope with uncertainty about the outcome of future climate negotiations. By contrast, failing to curb emissions in the short term imposes rapidly increasing additional costs of compliance. 相似文献
88.
Vimal Simha David H. Weinberg Romeel Davé Oleg Y. Gnedin Neal Katz Duan Kere 《Monthly notices of the Royal Astronomical Society》2009,399(2):650-662
We examine the accretion and merger histories of central and satellite galaxies in a smoothed particle hydrodynamics (SPH) cosmological simulation that resolves galaxies down to 7 × 109 M⊙ . Most friends-of-friends haloes in the simulation have a distinct central galaxy, typically 2–5 times more massive than the most massive satellite. As expected, satellites have systematically higher assembly redshifts than central galaxies of the same baryonic mass, and satellites in more massive haloes form earlier. However, contrary to the simplest expectations, satellite galaxies continue to accrete gas and convert it to stars; the gas accretion declines steadily over a period of 0.5–1 Gyr after the satellite halo merges with a larger parent halo. Satellites in a cluster mass halo eventually begin to lose baryonic mass. Typically, satellites in our simulation are 0.1–0.2 mag bluer than in models that assume no gas accretion on to satellites after a halo merger. Since z = 1 , 27 per cent of central galaxies (above 3 × 1010 M⊙ ) and 22 per cent of present-day satellite galaxies have merged with a smaller system above a 1:4 mass ratio; about half of the satellite mergers occurred after the galaxy became a satellite and half before. In effect, satellite galaxies can remain 'central' objects of halo substructures, with continuing accretion and mergers, making the transition in assembly histories and physical properties a gradual one. Implementing such a gradual transformation in semi-analytic models would improve their agreement with observed colour distributions of satellite galaxies in groups and with the observed colour dependence of galaxy clustering. 相似文献
89.
Victor G. Kornilov Vladimir M. Lipunov Evgeny S. Gorbovskoy Aleksander A. Belinski Dmitry A. Kuvshinov Natalia V. Tyurina Nikolai I. Shatsky Anatoly V. Sankovich Aleksander V. Krylov Pavel V. Balanutsa Vadim V. Chazov Artem S. Kuznetsov Dmitry S. Zimnuhov Victor A. Senik Andrey G. Tlatov Aleksander V. Parkhomenko Denis V. Dormidontov Vadim V. Krushinsky Ivan S. Zalozhnyh Aleksander A. Popov Sergey A. Yazev Nikolai M. Budnev Kirill I. Ivanov Evgeny N. Konstantinov Oleg A. Gress Oleg V. Chvalaev Vladimir V. Yurkov Yury P. Sergienko Irina P. Kudelina 《Experimental Astronomy》2012,33(1):173-196
Presented paper describes the basic principles and features of the implementation of a robotic network of optical telescopes MASTER, designed to study the prompt (simultaneous with gamma radiation) optical emission of gamma-ray bursts and to perform the sky survey to detect unknown objects and transient phenomena. With joint efforts of Sternberg astronomical institute, High altitude astronomical station of the Pulkovo observatory, Ural state university, Irkutsk state university, Blagoveshchensk pedagogical university, the robotic telescopes MASTER?II near Kislovodsk, Yekaterinburg, Irkutsk and Blagoveshchensk were installed and tested. The network spread over the longitudes is greater than 6?h. A further expansion of the network is considered. 相似文献
90.
Elizabeth R. Stanway Malcolm N. Bremer Valentina Squitieri Laura S. Douglas Matthew D. Lehnert 《Monthly notices of the Royal Astronomical Society》2008,386(1):370-376
We present a survey of bright optical dropout sources in two deep, multiwavelength surveys comprising 11 widely separated fields, aimed at constraining the galaxy luminosity function at z ≈ 7 for sources at 5–10 L * ( z = 6) . Our combined survey area is 225 arcmin2 to a depth of J AB = 24.2 (3σ) and 135 arcmin2 to J = 25.3 (4σ). We find that infrared data longwards of 2 μm are essential for classifying optical dropout sources, and in particular for identifying cool Galactic star contaminants. Our limits on the number density of high-redshift sources are consistent with current estimates of the Lyman break galaxy luminosity function at z = 6 . 相似文献