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141.
David Orejana Carlos Villaseca Pablo Valverde-Vaquero Elena A. Belousova Richard A. Armstrong 《International Journal of Earth Sciences》2012,101(7):1789-1815
The Spanish Central System (SCS) batholith, located in the Central Iberian Zone, is one of the largest masses of granite in the European Variscan Belt. This batholith is a composite unit of late- and post-kinematic granitoids dominated by S- and I-type series granite, with subordinate leucogranite and granodiorite. Zircon trace element contents, from two representative S-type and three I-type granitoids from the eastern portion of the SCS batholith, indicate a heterogeneous composition due to magma differentiation and co-crystallisation of other trace element-rich accessory phases. In situ, U–Pb dating of these zircons by SHRIMP and LA-ICP-MS shows 479–462-Ma inherited zircon ages in the I-type intrusions, indicating the involvement of an Ordovician metaigneous protolith, while the S-type intrusions exclusively contain Cadomian and older zircon ages. The zircon crystallisation ages show that these granites have been emplaced at ca. 300?Ma with a time span between 303?±?3?Ma and 298?±?3?Ma. Precise dating by CA-ID-TIMS reveals a pulse at 305.7?±?0.4?Ma and confirms the major pulse at 300.7?±?0.6?Ma. These ages match the Permo-Carboniferous age for granulite-facies metamorphism of the lower crust under the SCS batholith and coincide with a widespread granitic event throughout the Southern Variscides. Ti-in zircon thermometry indicates temperatures between 844 and 784°C for both the S- and I-type granites, reinforcing the hypothesis that these granites are derived from deep crustal sources. 相似文献
142.
Non‐Metabolic Uptake of Al3+ by Dead Leaves of Rubus ulmifolius: Comparison With Metabolic Bioaccumulation Data
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143.
The vertical distribution of macrobenthic fauna, heavy metals, and other physico‐chemical and biological characteristics of the sediments were studied in three sediment layers (0–7, 8–14, 15–21 cm) at seven stations in the Ubatuba region, north coast of São Paulo State, Brazil at several temporal and spatial scales. Six stations were located in the inner bay near the riverine run‐off, and one was outside the bay, distant from the riverine influence. The samples were collected four times in 1 year, on a seasonal basis. Sediments were basis comprised predominantly of very fine sand and the vertical distribution of grain size was uniform to a depth of 21 cm in all stations. Higher values of total organic matter, organic carbon, sulphur, heavy metals and phaeopigments were recorded at the inner Ubatuba Bay stations, probably due to the riverine influence. C/N ratios indicated a mixed origin of organic matter with a major contribution of terrestrial material in the inner stations. The vertical distribution of heavy metals showed a slight decline with sediment depth in the inner stations, indicating the present contribution. Most of the macrofauna was found at the surface sediment layer. Biological data showed that in the inner stations of Ubatuba Bay, which are under the influence of urban sewage and are moderately polluted, the fauna was distributed more superficially within the substrate than in St. 7, which is located in the external portion of the bay distant from sewage inputs. The environmental quality of the sites studied varied little throughout the year, at least in relation to the variables considered here. Temporal variation in the vertical distribution of benthic fauna was not evident in the four sampling surveys analysed. Only minor changes in the vertical distribution of the total fauna were detected in the seasonal scale, with the organisms located less deep within the sediment column in summer, indicating some influence of the tourism impact and/or rainy season. 相似文献
144.
145.
146.
Pablo A. Lara-Martín Eduardo González-Mazo Mira Petrovic Damià Barceló Bruce J. Brownawell 《Marine pollution bulletin》2014
This work deals with the environmental distribution of nonionic surfactants (nonylphenol and alcohol ethoxylates), their metabolites (NP, nonylphenol; NPEC, nonylphenol ethoxycarboxylates; and PEG, polyethylene glycols) and a selection of 64 pharmaceuticals in the Long Island Sound (LIS) Estuary which receives important sewage discharges from New York City (NYC). Most target compounds were efficiently removed (>95%) in one wastewater treatment plant monitored, with the exception of NPEC and some specific drugs (e.g., hydrochlorothiazide). Concentrations of surfactants (1.4–4.5 μg L−1) and pharmaceuticals (0.1–0.3 μg L−1) in seawater were influenced by tides and sampling depth, consistent with salinity differences. Surfactants levels in suspended solids samples were higher than 1 μg g−1, whereas only most hydrophobic or positively charged pharmaceuticals could be found (e.g., tamoxifen, clarithromycin). Maximum levels of target compounds in LIS sediments (PEG at highest concentrations, 2.8 μg g−1) were measured nearest NYC, sharply decreasing with distance from major sewage inputs. 相似文献
147.
Lateglacial and Holocene palaeohydrology in the western Mediterranean region: The Lake Estanya record (NE Spain) 总被引:3,自引:0,他引:3
Mario Morelln Blas Valero-Garcs Teresa Vegas-Vilarrúbia Penlope Gonzlez-Sampriz
scar Romero Antonio Delgado-Huertas Pilar Mata Ana Moreno Mayte Rico Juan Pablo Corella 《Quaternary Science Reviews》2009,28(25-26):2582-2599
The multi-proxy analysis of sediment cores recovered in karstic Lake Estanya (42°02′ N, 0°32′ E; 670 m a. s. l., NE Spain), located in the transitional area between the humid Pyrenees and the semi-arid Central Ebro Basin, provides the first high-resolution, continuous sedimentary record in the region, extending back the last 21 000 years. The integration of sedimentary facies, elemental and isotopical geochemistry and biogenic silica, together with a robust age model based on 17 AMS radiocarbon dates, enables precise reconstruction of the main hydrological and environmental changes in the region during the last deglaciation.Arid conditions, represented by shallow lake levels, predominantly saline waters and reduced organic productivity occurred throughout the last glacial maximum (21–18 cal kyrs BP) and the lateglacial, reaching their maximum intensity during the period 18–14.5 cal kyrs BP (including Heinrich event 1) and the Younger Dryas (12.9–11.6 cal kyrs BP). Less saline conditions characterized the 14.5–12.6 cal kyrs BP period, suggesting higher effective moisture during the Bölling/Allerød. The onset of more humid conditions started at 9.4 cal kyrs, indicating a delayed hydrological response to the onset of the Holocene which is also documented in several sites of the Mediterranean Basin. Higher, although fluctuating, Holocene lake levels were punctuated by a mid Holocene arid period between 4.8 and 4.0 cal kyrs BP. A major lake-level rise occurred at 1.2 cal kyrs BP, conducive to the establishment of conditions similar to the present and interrupted by a last major water level drop, occurring around 800 cal yrs BP, which coincides with the Medieval Climate Anomaly.The main hydrological stages in Lake Estanya are in phase with most Western Mediterranean and North Atlantic continental and marine records, but our results also show similarities with other Iberian and northern African reconstructions, emphasizing peculiarities of palaeohydrological evolution of the Iberian Peninsula during the last deglaciation. 相似文献
148.
Claude Robin Pablo Samaniego Jean-Luc Le Pennec Michel Fornari Patricia Mothes Johannes van der Plicht 《Bulletin of Volcanology》2010,72(9):1109-1129
Fieldwork, radiometric (40Ar/39Ar and 14C) ages and whole-rock geochemistry allow a reconstruction of eruptive stages at the active, mainly dacitic, Pichincha Volcanic
Complex (PVC), whose eruptions have repeatedly threatened Quito, most recently from 1999 to 2001. After the emplacement of
basal lavas dated at ∼1100 to 900 ka, the eruptive activity of the old Rucu Pichincha volcano lasted from ∼850 ka to ∼150 ka
before present (BP) and resulted in a 15 × 20 km-wide edifice, which comprises three main building stages: (1) A lower stratocone
(Lower Rucu, ∼160 km3 in volume) developed from ∼850 to 600 ka; (2) This edifice was capped by a steeper-sided and less voluminous cone (the Upper
Rucu, 40–50 km3), the history of which started 450–430 ka ago and ended around 250 ka with a sector collapse; (3) A smaller (8–10 km3) but more explosive edifice grew in the avalanche amphitheatre and ended Rucu Pichincha's history about 150 ka ago. The Guagua
Pichincha volcano (GGP) was developed from 60 ka on the western flank of Rucu with four growth stages separated by major catastrophic
events. (1) From ∼60 to 47 ka, a basal effusive stratocone developed, terminating with a large ash-and-pumice flow event.
(2) This basal volcano was followed by a long-lasting dome building stage and related explosive episodes, the latter occurring
between 28–30 and 22–23 ka. These first two stages formed the main GGP (∼30 km3), a large part of which was removed by a major collapse 11 ka BP. (3) Sustained explosive activity and viscous lava extrusions
gave rise to a new edifice, Toaza (4–5 km3 in volume), which in turn collapsed around 4 ka BP. (4) The ensuing amphitheatre was partly filled by the ∼1-km3 Cristal dome, which is the historically active centre of the Pichincha complex. The average output rate for the whole PVC
is 0.29 km3/ka. Nevertheless, the chronostratigraphic resolution we obtained for Lower Rucu Pichincha and for the two main edifices of
Guagua Pichincha (main GGP and Toaza), leads to eruptive rates of 0.60–0.65 km3/ka during these construction stages. These output rates are compared to those of other mainly dacitic volcanoes from continental
arcs. Our study also supports an overall SiO2 and large-ion lithophile elements enrichment as the PVC develops. In particular, distinctive geochemical signatures indicate
the involvement of a new magma batch at the transition between Rucu and Guagua. At the GGP, the same phenomenon occurs at
each major collapse event marking the onset of the ensuing magmatic stage. Since the 11-ka-BP collapse event, this magmatic
behaviour has led to increasingly explosive activity. Four explosive cycles of between 100 and 200 years long have taken place
at the Cristal dome in the past 3.7 ka, and repose intervals between these cycles have tended to decrease with time. As a
consequence, we suggest that the 1999–2001 eruptive period may have initiated a new eruptive cycle that might pose a future
hazard to Quito (∼2 million inhabitants). 相似文献
149.
150.
Roberto Oyarzun Paloma Cubas Pablo Higueras Javier Lillo Willians Llanos 《Environmental Geology》2009,58(4):761-777
The Rodalquilar mineral deposits (SE Spain) were formed in Miocene time in relation to caldera volcanic episodes and dome
emplacement phenomena. Two types of ore deposits are recognized: (1) the El Cinto epithermal, Au–As high sulphidation vein
and breccia type; and (2) peripheral low sulphidation epithermal Pb–Zn–Cu–(Au) veins. The first metallurgical plants for gold
extraction were set up in the 1920s and used amalgamation. Cyanide leaching began in the 1930s and the operations lasted until
the mid 1960s. The latter left a huge pile of ~900,000–1,250,000 m3 of abandoned As-rich tailings adjacent to the town of Rodalquilar. A frustrated initiative to reactivate the El Cinto mines
took place in the late 1980s and left a heap leaching pile of ~120,000 m3. Adverse mineralogical and structural conditions favoured metal and metalloid dispersion from the ore bodies into soils and
sediments, whereas mining and metallurgical operations considerably aggravated contamination. We present geochemical data
for soils, tailings and wild plant species. Compared to world and local baselines, both the tailings and soils of Rodalquilar
are highly enriched in As (mean concentrations of 950 and 180 μg g−1, respectively). Regarding plants, only the concentrations of As, Bi and Sb in Asparagus horridus, Launaea arborescens, Salsola genistoides, and Stipa tenacissima are above the local baselines. Bioaccumulation factors in these species are generally lower in the tailings, which may be
related to an exclusion strategy for metal tolerance. The statistical analysis of geochemical data from soils and plants allows
recognition of two well-differentiated clusters of elements (As–Bi–Sb–Se–Sn–Te and Cd–Cu–Hg–Pb–Zn), which ultimately reflect
the strong chemical influence of both El Cinto and peripheral deposits mineral assemblages. 相似文献