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131.
Mohamad R. Soltanian Mohammad A. Amooie David R. Cole Thomas H. Darrah David E. Graham Susan M. Pfiffner Tommy J. Phelps Joachim Moortgat 《Ground water》2018,56(2):176-186
In the context of geological carbon sequestration (GCS), carbon dioxide (CO2) is often injected into deep formations saturated with a brine that may contain dissolved light hydrocarbons, such as methane (CH4). In this multicomponent multiphase displacement process, CO2 competes with CH4 in terms of dissolution, and CH4 tends to exsolve from the aqueous into a gaseous phase. Because CH4 has a lower viscosity than injected CO2, CH4 is swept up into a ‘bank’ of CH4‐rich gas ahead of the CO2 displacement front. On the one hand, this may provide a useful tracer signal of an approaching CO2 front. On the other hand, the emergence of gaseous CH4 is undesirable because it poses a leakage risk of a far more potent greenhouse gas than CO2 if the cap rock is compromised. Open fractures or faults and wells could result in CH4 contamination of overlying groundwater aquifers as well as surface emissions. We investigate this process through detailed numerical simulations for a large‐scale GCS pilot project (near Cranfield, Mississippi) for which a rich set of field data is available. An accurate cubic‐plus‐association equation‐of‐state is used to describe the non‐linear phase behavior of multiphase brine‐CH4‐CO2 mixtures, and breakthrough curves in two observation wells are used to constrain transport processes. Both field data and simulations indeed show the development of an extensive plume of CH4‐rich (up to 90 mol%) gas as a consequence of CO2 injection, with important implications for the risk assessment of future GCS projects. 相似文献
132.
Kristina Hippe Tiemen Gordijn Vincenzo Picotti Irka Hajdas John D. Jansen Marcus Christl Christof Vockenhuber Colin Maden Naki Akçar Susan Ivy-Ochs 《地球表面变化过程与地形》2019,44(3):766-780
Determining sediment transfer times is key to understanding source-to-sink dynamics and the transmission of environmental signals through the fluvial system. Previous work on the Bolivian Altiplano applied the in situ cosmogenic 14C-10Be-chronometer to river sands and proposed sediment storage times of ~10–20 kyr in four catchments southeast of Lake Titicaca. However, the fidelity of those results hinges upon isotopic steady-state within sediment supplied from the source area. With the aim of independently quantifying sediment storage times and testing the 14C-10Be steady-state assumption, we dated sediment storage units within one of the previously investigated catchments using radiocarbon dating, cosmogenic 10Be-26Al isochron burial dating, and 10Be-26Al depth-profile dating. Palaeosurfaces appear to preserve remnants of a former fluvial system, which has undergone drainage reversal, reduction in catchment area, and local isostatic uplift since ~2.8 Ma. From alluvium mantling the palaeosurfaces we gained a deposition age of ~580 ka, while lower down fluvial terraces yielded ≤34 ka, and floodplains ~3–1 ka. Owing to restricted channel connectivity with the terraces and palaeosurfaces, the main source of channel sediment is via reworking of the late Holocene floodplain. Yet modelling a set of feasible scenarios reveals that floodplain storage and burial depth are incompatible with the 14C-10Be disequilibrium measured in the channel. Instead we propose that the 14C-10Be offset results from: (i) non-uniform erosion whereby deep gullies supply hillslope-derived debris; and/or (ii) holocene landscape transience associated with climate or human impact. The reliability of the 14C-10Be chronometer vitally depends upon careful evaluation of sources of isotopic disequilibrium in a wide range of depositional and erosional landforms in the landscape. © 2018 John Wiley & Sons, Ltd. 相似文献
133.
During a series of substorm events on November 12 2004, the Neutral Atom Detector Unit(NUADU) flying onboard the TC-2 spacecraft observed, close to perigee, bright low-altitude Energetic Neutral Atom(ENA) emissions from both north and south poles. Through utilizing high temporal and spatial resolution data inversion techniques we present here a global view the associated processes of energetic ion deposition and injection at the uniquely high temporal resolution of a few minutes. It is demonstrated that the ENA emissions observed came mainly from the, low-altitude, high magnetic latitude polar region. Since precipitating ions follow magnetic field lines and have more chance to produce ENA emissions through charge exchange there.Therefore, the employment of a low-orbit satellite to record at high temporal and spatial resolution ENA image data is inferred to be the best way to monitor those dynamic ring current variations that occur during geomagnetic activity. 相似文献
134.
Anne Claude Naki Akçar Susan Ivy-Ochs Fritz Schlunegger Philippe Rentzel Christine Pümpin Dmitry Tikhomirov Peter W. Kubik Christof Vockenhuber Andreas Dehnert Meinert Rahn Christian Schlüchter 《Swiss Journal of Geoscience》2017,110(3):793-809
The Quaternary stratigraphy of the Alpine Foreland consists of distinct terrace levels, which have been assigned to four morphostratigraphic units: Höhere (Higher) Deckenschotter, Tiefere (Lower) Deckenschotter, Hochterrasse (High Terrace) and Niederterrasse (Lower Terrace). Here, we focus on the terrace gravels at Hohle Gasse, SSE of Pratteln near Basel, which are mapped as Tiefere Deckenschotter. Petrographic and morphometric data established from clasts allowed to infer the transport mechanisms and sources of the gravels. Sedimentological analyses indicate that the gravels were transported by a braided river and deposited in a distal glaciofluvial setting. In addition, it can be shown that the majority of the clasts display multiple reworking and only a minority maintained a distinct glaciofluvial shape. Cosmogenic multi-isotope dating using 10Be and 36Cl allowed direct dating of the sediments at the study site. A depth-profile age of \(2 70_{ - 1 90}^{ + 8 30}\) ka for 10Be was achieved for the deposits at Hohle Gasse. Unfortunately, no age could be modelled from the 36Cl concentrations as the blank correction was too high. Furthermore, this age proves that the studied terrace level should be assigned to the morphostratigraphic unit Hochterrasse. 相似文献
135.
William D. Robertson James W. Roy Susan J. Brown Dale R. Van Stempvoort Greg Bickerton 《Ground water》2014,52(1):63-70
Monitoring of a well‐defined septic system groundwater plume and groundwater discharging to two urban streams located in southern Ontario, Canada, provided evidence of natural attenuation of background low level (ng/L) perchlorate (ClO4?) under denitrifying conditions in the field. The septic system site at Long Point contains ClO4? from a mix of waste water, atmospheric deposition, and periodic use of fireworks, while the nitrate plume indicates active denitrification. Plume nitrate (NO3?‐N) concentrations of up to 103 mg/L declined with depth and downgradient of the tile bed due to denitrification and anammox activity, and the plume was almost completely denitrified beyond 35 m from the tile bed. The ClO4? natural attenuation occurs at the site only when NO3?‐N concentrations are <0.3 mg/L, after which ClO4? concentrations decline abruptly from 187 ± 202 to 11 ± 15 ng/L. A similar pattern between NO3?‐N and ClO4? was found in groundwater discharging to the two urban streams. These findings suggest that natural attenuation (i.e., biodegradation) of ClO4? may be commonplace in denitrified aquifers with appropriate electron donors present, and thus, should be considered as a remediation option for ClO4? contaminated groundwater. 相似文献
136.
Trenton T Cladouhos Susan Petty Yini Nordin Michael Moore Kyla Grasso Matt Uddenberg Michael W Swyer 《地下水科学与工程》2014,2(3):1-7
The Newberry Volcano EGS Demonstration in central Oregon tests recent technological advances designed to reduce the cost of power generated by EGS in a hot, dry well (NWG 55-29) drilled in 2008. An EGS reservoir was created by injecting large volumes of cold water, causing existing fractures to slip in shear (known as hydroshearing) generating the seismic waves that can be used to map fracture location and size. At the Newberry Demonstration the final injectivity ranged between 1.4 and 1.7 L/s/MPa a ~6x improvement over the initial injectivity of the well. The injectivity improvement and seismic analysis indicate that previously impermeable fractures were enhanced during the NWG 55-29 stimulation. 相似文献
137.
Yousif K. Kharaka James J. Thordsen Susan D. Hovorka H. Seay Nance David R. Cole Tommy J. Phelps Kevin G. Knauss 《Applied Geochemistry》2009
Sedimentary basins in general, and deep saline aquifers in particular, are being investigated as possible repositories for large volumes of anthropogenic CO2 that must be sequestered to mitigate global warming and related climate changes. To investigate the potential for the long-term storage of CO2 in such aquifers, 1600 t of CO2 were injected at 1500 m depth into a 24-m-thick “C” sandstone unit of the Frio Formation, a regional aquifer in the US Gulf Coast. Fluid samples obtained before CO2 injection from the injection well and an observation well 30 m updip showed a Na–Ca–Cl type brine with ∼93,000 mg/L TDS at saturation with CH4 at reservoir conditions; gas analyses showed that CH4 comprised ∼95% of dissolved gas, but CO2 was low at 0.3%. Following CO2 breakthrough, 51 h after injection, samples showed sharp drops in pH (6.5–5.7), pronounced increases in alkalinity (100–3000 mg/L as HCO3) and in Fe (30–1100 mg/L), a slug of very high DOC values, and significant shifts in the isotopic compositions of H2O, DIC, and CH4. These data, coupled with geochemical modeling, indicate corrosion of pipe and well casing as well as rapid dissolution of minerals, especially calcite and iron oxyhydroxides, both caused by lowered pH (initially ∼3.0 at subsurface conditions) of the brine in contact with supercritical CO2. 相似文献
138.
In 1902, the Florida red mangrove, Rhizophora mangle L., was introduced to the island of Molokai, Hawaii, and has since colonized nearly 25% of the south coast shoreline. By classifying three kinds of remote sensing imagery, we compared abilities to detect invasive mangrove distributions and to discriminate mangroves from surrounding terrestrial vegetation. Using three analytical techniques, we compared mangrove mapping accuracy for various sensor-technique combinations. ANOVA of accuracy assessments demonstrated significant differences among techniques, but no significant differences among the three sensors. We summarize advantages and disadvantages of each sensor and technique for mapping mangrove distributions in tropical coastal environments. 相似文献
139.
We describe the development and application of a management procedure (decision rule) that resulted in a voluntary reduction in the commercial catch of spiny rock lobster (Jasus edwardsii) in the lower east coast of North Island of New Zealand. The management procedure was developed from an accepted assessment of the CRA 4 (Wellington‐Hawke's Bay) fishery, which used an integrated length‐based assessment model fitted to commercial fishery catch‐per‐unit‐effort (CPUE) biomass indices, commercial length‐frequency data, and tag‐recapture data. The assessment model had been Bayesian, and used the joint posterior distribution of parameters to predict the effect of 384 alternative harvest control rules on the future size of the CRA 4 stock. The harvest control rules all used CPUE as their input, and generated annual changes in catch, which were then simulated by the population dynamics of the operating model. Uncertainty was added to evaluations through observation error, added to the simulated CPUE observations, and stochastic serial auto‐correlation variation in recruitment. We describe how this management procedure was used to effect a voluntary reduction in catch to address the problem of a rapidly declining population. 相似文献
140.