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61.
Implications for behavior of volatile elements during impacts—Zinc and copper systematics in sediments from the Ries impact structure and central European tektites
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Zuzana Rodovská Tomáš Magna Karel Žák Chizu Kato Paul S. Savage Frédéric Moynier Roman Skála Josef Ježek 《Meteoritics & planetary science》2017,52(10):2178-2192
Moldavites are tektites genetically related to the Ries impact structure, located in Central Europe, but the source materials and the processes related to the chemical fractionation of moldavites are not fully constrained. To further understand moldavite genesis, the Cu and Zn abundances and isotope compositions were measured in a suite of tektites from four different substrewn fields (South Bohemia, Moravia, Cheb Basin, Lusatia) and chemically diverse sediments from the surroundings of the Ries impact structure. Moldavites are slightly depleted in Zn (~10–20%) and distinctly depleted in Cu (>90%) relative to supposed sedimentary precursors. Moreover, the moldavites show a wide range in δ66Zn values between 1.7 and 3.7‰ (relative to JMC 3‐0749 Lyon) and δ65Cu values between 1.6 and 12.5‰ (relative to NIST SRM 976) and are thus enriched in heavy isotopes relative to their possible parent sedimentary sources (δ66Zn = ?0.07 to +0.64‰; δ65Cu = ?0.4 to +0.7‰). In particular, the Cheb Basin moldavites show some of the highest δ65Cu values (up to 12.5‰) ever observed in natural samples. The relative magnitude of isotope fractionation for Cu and Zn seen here is opposite to oxygen‐poor environments such as the Moon where Zn is significantly more isotopically fractionated than Cu. One possibility is that monovalent Cu diffuses faster than divalent Zn in the reduced melt and diffusion will not affect the extent of Zn isotope fractionation. These observations imply that the capability of forming a redox environment may aid in volatilizing some elements, accompanied by isotope fractionation, during the impact process. The greater extent of elemental depletion, coupled with isotope fractionation of more refractory Cu relative to Zn, may also hinge on the presence of carbonyl species of transition metals and electromagnetic charge, which could exist in the impact‐induced high‐velocity jet of vapor and melts. 相似文献
62.
63.
Two sedimentary units are recognized by means of stratigraphic and sedimentological analyses at Monte Verde, a late Pleistocene archeological site with stone tools and well-preserved wood artifacts and botanical remains, that lies southwest of Lago Llanquihue and north of the Golfo de Reloncavi in the southern end of the Chilean Central graben. the geological evidence shows that at no time after 33,000 yr B.P., and perhaps since the first Llanquihue advance (before 56,000 yr B.P.), was the Monte Verde area covered by ice. Influences of two glacial advances at 20,000 and 15,000-14,500 yr B.P. are recognized at the site; effects of the Varas Interstade, however, are not identified. Rapid climatic change took place after the end of the Llanquihue Glaciation. It was shortly interrupted by a cool, wet period around 10,000 yr B.P., after which a well-documented Hypsithermal (8270-4750 yr B.P.) accompanied by pyroclastic vulcanism followed. The evidence indicates that around 13,000 yr B.P. 1) the site occupants settled on the sandy point bars and beaches of the old creek channel and 2) the area was habitated during cool and wet conditions similar to those that prevail in the area today. Evidence for reconstruction of the paleo-environment and climate of the terminal Pleistocene and the preliminary implications of these findings for understanding the human occupation at Monte Verde are discussed. 相似文献
64.
65.
Tom D. Brewer Joshua E. Cinner Rebecca Fisher Alison Green Shaun K. Wilson 《Global Environmental Change》2012,22(2):399-406
There is overwhelming evidence that many local-scale human activities (e.g. fishing) have a deleterious effect on coral reef fish assemblages. Our understanding of how broad social phenomena (e.g. socioeconomic development) affect the diversity and function of coral reef fish assemblages however, is still poor. Here, we use structural equation models to reveal how human population density, socioeconomic development, and market access affect fishing pressure and coral cover to, in turn, explain the diversity and biomass of key functional groups of reef fish assemblages within Solomon Islands. Fishing pressure is predominantly driven by both market access and local population density, and has a clear negative effect on the diversity and function of coral reef fishes. The strong positive effect of market access on fishing pressure makes clear the importance of understanding social-ecological linkages in the context of increasingly connected societies. This study highlights the need to address broad social phenomena rather than focusing on proximate threats such as fishing pressure, to ensure the continued flow of coral reef goods and services in this time of rapid global social and environmental change. 相似文献
66.
Modelling magnetization processes in single-and multi-domain rock samples using the preisach diagram
Summary The paper presents the results of identifying a model of the Preisach type for haematite grains of the single-domain as well as multi-domain size. Due to the phenomenological conception of the model, the relations between the parameters of the model and actual parameters are very complex, however, impressive accuracy and stability of the modified model indicate the need to resume studies of this problem. The model parameters also confirm the adequate properties of the vibrating-sample magnetometr (VSM) used and developed in our laboratories. 相似文献
67.
Employing clean and quantitative techniques, a marine monitoring programme succeeded in detecting large surface elevations in the concentrations of dissolved Cu, Zn and Pb in the marine surface waters of Puget Sound adjacent to Seattle and Tacoma, Washington. Physical mixing with cleaner waters was the controlling factor in reducing the dissolved concentrations of Cu downstream of these contaminated regions. Comparisons between Puget Sound waters and coastal waters adjacent to Puget Sound suggest that a portion of this Cu, Zn and Pb pollution is being advected out of Puget Sound. The low Ni and Cd concentrations found in this study indicate that these trace metals are not a significant pollution problem in the main basin of Puget Sound. 相似文献
68.
Improved regional and interregional stratigraphic correlations of Pennsylvanian strata permit comparisons of vegetational changes in Euramerican coal swamps. The coal-swamp vegetation is known directly from in situ coal-ball peat deposits from more than 65 coals in the United States and Europe. Interpretations of coal-swamp floras on the basis of coal-ball peat studies are extended to broader regional and stratigraphic patterns by use of coal palynology. Objectives of the quantitative analyses of the vegetation in relation to coal are to determine the botanical constituents at the peat stage and their environmental implications for plant growth and peat accumulation. Morphological and paleoecological analyses provide a basis for deducing freshwater regimes of coal swamps.Changes in composition of Pennsylvanian coal-swamp vegetation are quire similar from one paralic coal region to another and show synchrony that is attributable to climate. Paleobotany and paleogeography of the Euramerican province indicate a moist tropical paleoclimate. Rainfall, runoff and evapotranspiration were the variable climatic controls in the distribution of coal-swamp vegetation, peat accumulation and coal resources. In relative terms of climatic wetness the Pennsylvanian Period is divisible into five intervals, which include two relatively drier intervals that developed during the Lower-Middle and Middle-Upper Pennsylvanian transitions. The climate during Early Pennsylvanian time was moderately wet and the median in moisture availability. Early Middle Pennsylvanian was drier, probably seasonally dry-wet; late Middle Pennsylvanian was the wettest in the Midcontinent; early Late Pennsylvanian was the driest; and late Late Pennsylvanian was probably the wettest in the Dunkard Basin. The five climatic intervals represent a general means of dividing coal resources within each region into groups with similar botanical constituents and environments of peat accumulation. Regional differences in basinal geology and climate were significant variables, but the synchronous control of paleoclimate was of primary importance. 相似文献
69.
Benjamin D. Santer Karl E. Taylor Tom M. L. Wigley Joyce E. Penner Philip D. Jones Ulrich Cubasch 《Climate Dynamics》1995,12(2):77-100
It has been hypothesized recently that regional-scale cooling caused by anthropogenic sulfate aerosols may be partially obscuring
a warming signal associated with changes in greenhouse gas concentrations. Here we use results from model experiments in which
sulfate and carbon dioxide have been varied individually and in combination in order to test this hypothesis. We use centered
[R (t)] and uncentered [C (t)] pattern similarity statistics to compare observed time-evolving surface temperature change patterns with the model-predicted
equilibrium signal patterns. We show that in most cases, the C (t) statistic reduces to a measure of observed global-mean temperature changes, and is of limited use in attributing observed
climate changes to a specific causal mechanism. We therefore focus on R (t), which is a more useful statistic for discriminating between forcing mechanisms with different pattern signatures but similar
rates of global mean change. Our results indicate that over the last 50 years, the summer (JJA) and fall (SON) observed patterns
of near-surface temperature change show increasing similarity to the model-simulated response to combined sulfate aerosol/CO2 forcing. At least some of this increasing spatial congruence occurs in areas where the real world has cooled. To assess the
significance of the most recent trends in R (t) and C (t), we use data from multi-century control integrations performed with two different coupled atmosphere-ocean models, which
provide information on the statistical behavior of 'unforced' trends in the pattern correlation statistics. For the combined
sulfate aerosol/CO2 experiment, the 50-year R (t) trends for the JJA and SON signals are highly significant. Results are robust in that they do not depend on the choice of
control run used to estimate natural variability noise properties. The R (t) trends for the CO2-only signal are not significant in any season. C (t) trends for signals from both the CO2-only and combined forcing experiments are highly significant in all seasons and for all trend lengths (except for trends
over the last 10 years), indicating large global-mean changes relative to the two natural variability estimates used here.
The caveats regarding the signals and natural variability noise which form the basis of this study are numerous. Nevertheless,
we have provided first evidence that both the largest-scale (global-mean) and smaller-scale (spatial anomalies about the global
mean) components of a combined CO2/anthropogenic sulfate aerosol signal are identifiable in the observed near-surface air temperature data. If the coupled-model
noise estimates used here are realistic, we can be highly confident that the anthropogenic signal that we have identified
is distinctly different from internally generated natural variability noise. The fact that we have been able to detect the
detailed spatial signature in response to combined CO2 and sulfate aerosol forcing, but not in response to CO2 forcing alone, suggests that some of the regional-scale background noise (against which we were trying to detect a CO2-only signal) is in fact part of the signal of a sulfate aerosol effect on climate. The large effect of sulfate aerosols found
in this study demonstrates the importance of their inclusion in experiments designed to simulate past and future climate change.
Received: 10 November 1994 / Accepted: 19 July 1995 相似文献
70.
The most appropriate indices with which to quantify Australian bushfire danger are the McArthur fire danger meters. These meters use meteorological information to produce a fire danger index that is directly related to the chance of a fire starting - and to the severity of a fire once it has started. The Mark 5 forest-fire danger meter uses air temperature, relative humidity and wind speed, plus a drought factor that is calculated using daily rainfall and temperature information.Three years of daily data generated from the CSIRO four-level general circulation model, and thirty years of daily data generated from the CSIRO nine-level model were used to estimate the daily McArthur forest fire danger index for simulations corresponding to present conditions, and to those corresponding to doubled atmospheric CO2. The performance of these models with respect to fire danger was tested by comparing the fire danger index for Sale (in the Eastern part of Victoria, South-eastern Australia) calculated from analysis of daily climatological data with the modelled annual cumulative forest fire danger index for the grid point that was representative of Sale. Data from both models for all Australian grid points were also examined. Both models predict an increase in fire danger over much of Australia for their doubled CO2 scenarios.The results from the models confirm that annually averaged daily relative humidity is the single most important variable in the estimation of forest fire danger on an annual basis, yet the models tend to produce relative humidities that are slightly too low so that the fire danger is overestimated. A simple one-box model of evaporation indicates that the value of relative humidity to be expected under an altered climatic regime depends on the modelled relation between actual and potential evaporation, the present values of relative humidity and evaporation rate, as well as on the expected changes in wind speed. 相似文献