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131.
不同浓度的Na2SO4水溶液的拉曼光谱显示了SO42-的四个拉曼活性带:980 cm-1处的SO42-的对称伸缩振动模式v1带,1 106 cm-1处的反对称伸缩振动模式v3带,448 cm-1处的变形振动模式v2带和617 cm-1处的变形振动模式v4带。482 cm-1处的肩膀峰是由于NaSO4-离子对的形成对448 cm-1的v2带的影响而形成的SO42-的一个新的振动峰。浓Na2SO4水溶液中,水共享离子对[Na+.H2O.SO42-]-是主要的离子对物种。随着Na2SO4水溶液浓度的增加,Na+和SO42-的相互作用增强,NaSO4-离子对所占的摩尔分数增加。 相似文献
132.
A tree‐ring width based drought reconstruction for southeastern China: links to Pacific Ocean climate variability
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Feng Chen Shulong Yu Yujiang Yuan Huiqin Wang Mary Gagen 《Boreas: An International Journal of Quaternary Research》2016,45(2):335-346
We present a drought reconstruction for southeastern China based on a tree‐ring width chronology of Cryptomeria fortunei developed from two sampling sites in central Fujian. A reconstruction of July–February drought variability, spanning AD 1855–2011, was developed by calibrating total tree‐ring width data with the self‐calibrating Palmer drought severity index (scPDSI). The reconstruction was verified against an independent data set, and accounts for 36% of the actual scPDSI variance during the period 1955–2011. Relatively dry intervals were reconstructed between AD 1859–1880, 1899–1911, 1927–1933, 1946–1959, 1964–1970 and 1987–1997. Relatively wet conditions prevailed during 1855–1858, 1881–1898, 1912–1926, 1934–1945, 1960–1963, 1971–1986 and 1998–2011. Comparisons between our scPDSI reconstruction and a moisture‐sensitive tree‐ring width record from Vietnam revealed consistencies between the two data sets, suggesting similar drought regimes. Spectral peaks of 2.2–6.4 years may be indicative of El Niño‐Southern Oscillation (ENSO) activity, as also suggested by the significant correlations with sea surface temperatures (SSTs) in the eastern equatorial and southeastern Pacific Ocean and an extreme event analysis. The analysis of links between our scPDSI reconstruction and the large‐scale regional climatic variation shows that there is a relationship between regional drought variation and East Asian summer monsoon (EASM) intensity. 相似文献
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Accepting the concept of standardization introduced by the standardized precipitation index, similar methodologies have been developed to construct some other standardized drought indices such as the standardized precipitation evapotranspiration index (SPEI). In this study, the authors provided deep insight into the SPEI and recognized potential deficiencies/limitations in relating to the climatic water balance it used. By coupling another well‐known Palmer drought severity index (PDSI), we proposed a new standardized Palmer drought index (SPDI) through a moisture departure probabilistic approach, which allows multi‐scalar calculation for accurate temporal and spatial comparison of the hydro‐meteorological conditions of different locations. Using datasets of monthly precipitation, temperature and soil available water capacity, the moisture deficit/surplus was calculated at multiple temporal scales, and a couple of techniques were adopted to adjust corresponding time series to a generalized extreme value distribution out of several candidates. Results of the historical records (1900–2012) for diverse climates by multiple indices showed that the SPDI was highly consistent and correlated with the SPEI and self‐calibrated PDSI at most analysed time scales. Furthermore, a simple experiment of hypothetical temperature and/or precipitation change scenarios also verified the effectiveness of this newly derived SPDI in response to climate change impacts. Being more robust and preferable in spatial consistency and comparability as well as combining the simplicity of calculation with sufficient accounting of the physical nature of water supply and demand relating to droughts, the SPDI is promising to serve as a competent reference and an alternative for drought assessment and monitoring. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献
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An analytical study on three‐dimensional versus two‐dimensional water table‐induced flow patterns in a Tóthian basin
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Jun‐Zhi Wang Xiao‐Wei Jiang Zhi‐Yuan Zhang Li Wan Xu‐Sheng Wang Hailong Li 《水文研究》2017,31(22):4006-4018
Although it has been increasingly acknowledged that groundwater flow pattern is complicated in the three‐dimensional (3‐D) domain, two‐dimensional (2‐D) water table‐induced flow models are still widely used to delineate basin‐scale groundwater circulation. However, the validity of 2‐D cross‐sectional flow field induced by water table has been seldom examined. Here, we derive the analytical solution of 3‐D water table‐induced hydraulic head in a Tóthian basin and then examine the validity of 2‐D cross‐sectional models by comparing the flow fields of selected cross sections calculated by the 2‐D cross‐sectional model with those by the 3‐D model, which represents the “true” cases. For cross sections in the recharge or discharge area of the 3‐D basin, even if head difference is not significant, the 2‐D cross‐sectional models result in flow patterns absolutely different from the true ones. For the cross section following the principal direction of groundwater flow, although 2‐D cross‐sectional models would overestimate the penetrating depth of local flow systems and underestimate the recharge/discharge flux, the flow pattern from the cross‐sectional model is similar to the true one and could be close enough to the true one by adjusting the decay exponent and anisotropy ratio of permeability. Consequently, to determine whether a 2‐D cross‐sectional model is applicable, a comparison of hydraulic head difference between 2‐D and 3‐D solutions is not enough. Instead, the similarity of flow pattern should be considered to determine whether a cross‐sectional model is applicable. This study improves understanding of groundwater flow induced by more natural water table undulations in the 3‐D domain and the limitations of 2‐D models accounting for cross‐sectional water table undulation only. 相似文献
138.
Spatial heterogeneity is ubiquitous in nature, which may significantly affect the soil hydraulic property curves. The models of a closed‐form functional relationship of soil hydraulic property curves (e.g. VG model or exponential model) are valid at point or local scale based on a point‐scale hydrological process, but how do scale effects of heterogeneity have an influence on the parameters of these models when the models are used in a larger scale process? This paper uses a two‐dimensional variably saturated flow and solute transport finite element model (VSAFT2) to simulate variations of pressure and moisture content in the soil flume under a constant head boundary condition. By changing different numerical simulation block sizes, a quantitative evaluation of parameter variations in the VG model, resulting from the scale effects, is presented. Results show that the parameters of soil hydraulic properties are independent of scale in homogeneous media. Parameters of α and n in homogeneous media, which are estimated by using the unsaturated hydraulic conductivity curve (UHC) or the soil water retention curve (WRC), are identical. Variations of local heterogeneities strongly affect the soil hydraulic properties, and the scale affects the results of the parameter estimations when numerical experiments are conducted. Furthermore, the discrepancy of each curve becomes considerable when moisture content becomes closer to a dry situation. Parameters estimated by UHC are totally different from the ones estimated by WRC. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
139.
Hao Liu Qinglong Xia Ian D. Somerville Yuan Wang Xinhuai Zhou Chengmin Niu Xiaofeng Du Xintao Zhang 《Geological Journal》2015,50(1):71-92
The sequence architecture and depositional systems of the Paleogene lacustrine rift succession in the Huanghekou Sag, Bohai Bay Basin, NE China were investigated based on seismic profiles, combined with well log and core data. Four second‐order or composite sequences and seven third‐order sequences were identified. The depositional systems identified in the basin include: fan delta, braid delta, meander fluvial delta, lacustrine and sublacustrine fan. Identification of the slope break was conducted combining the interpretation of faults of each sequence and the identification of syndepositional faults, based on the subdivision of sequence stratigraphy and analysis of depositional systems. Multiple geomorphologic units were recognized in the Paleogene of the Huanghekou Sag including faults, flexures, depositional slope break belts, ditch‐valleys and sub‐uplifts in the central sag. Using genetic division principles and taking into consideration tectonic features of the Paleogene of the Huanghekou Sag, the study area was divided into the Northern Steep Slope/Fault Slope Break System, the Southern Gentle Slope Break System and T10 Tectonic Slope Break System/T10 Tectonic Belt. Responses of slope break systems to deposition–erosion are shown as: (1) basin marginal slope break is the boundary of the eroded area and provenance area; (2) ditch‐valley formed by different kinds of slope break belts is a good transport bypass for source materials; (3) shape of the slope break belt of the slope break system controls sediments types; (4) the ditch‐valley and sub‐sag of a slope break system is an unloading area for sediments; and (5) due to their different origins, association characteristics and developing patterns, the Paleogene slope break belt systems in the Huanghekou Sag show different controls on depositional systems. The Northern Fault Slope Break system controls the deposition of a fan delta‐lacustrine‐subaqueous fan, the Southern Gentle Slope Break system controls the deposition of a fluvial–deltaic–shallow lacustrine and sublacustrine fan, and the T10 Tectonic Slope Break System controls the deposition of shallow lacustrine beach bar sandbodies. The existence of a slope break system is a necessary but not a sufficient condition for studying sandbody development. The formation of effective sandbodies along the slope break depends on the reasonable coupling of effective provenance, necessary association patterns of slope break belt, adequate unloading space and creation of definite accommodation space. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献
140.
目前常用的古构造图的制作方法为"厚度图法"和"断层平移法",这两种方法对断控圈闭为主的古构造恢复具有一定的局限性,且不能定量化的研究古构造生长发育情况。本论文首次将三维古构造恢复技术应用于珠江口盆地番禺-流花地区。三维古构造恢复技术在应用时,避免了厚度异常现象,实现了去压实恢复,能够更真实的反映古构造情况。该技术在珠江口盆地番禺流花地区"A"构造的应用,达到了定量分析古构造发育的效果,并且认识到了A构造在关键时期T32时期古构造幅度较小,后期构造幅度增大是A构造充满度过低的重要原因之一。 相似文献