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131.
Samples of natural sodalite, Na8Al6Si6O24Cl2, submitted to gamma irradiation and to thermal treatments, have been investigated using the thermoluminescence (TL) and electron
paramagnetic resonance (EPR) techniques. Both, natural and heat-treated samples at 500°C in air for 30 min, present an EPR
signal around g = 2.01132 attributed to oxygen hole centers. The EPR spectra of irradiated samples show an intense line at g = 2.0008 superimposed by a hyperfine multiplet of 11 lines due to an O− ion in an intermediate position with respect to two adjacent Al nuclei. In the TL measurements, the samples were annealed
at 500°C for 30 min and then irradiated with γ doses varying from 0.001 to 20 kGy. All the samples have shown TL peaks at
110, 230, 270, 365, and 445°C. A correlation between the EPR g = 2.01132 line and the 365°C TL peak was observed. A TL model is proposed in which a Na+ ion acts as a charge compensator when an Al3+ ion replaces a Si4+ lattice ion. The γ ray destruction of the Al–Na complex provides an electron trapped at the Na and a hole trapped at a non-bridging
oxygen ion adjacent to the Al3+ ion. 相似文献
132.
The Iwami epithermal silver deposit consists of Ag-Cu veins in a dacitic intrusive body at the deep portion of the Eikyu area, and veinlets with disseminated Ag mineralization in dacitic tuff breccia at a shallow portion of the Fukuishi area. Hydrothermal alteration associated with the silver mineralization is characterized by intense potassium metasomatism with oxidizing conditions. An illite zone occurs around the pathways of uprising fluids in both the Eikyu and Fukuishi areas. It grades laterally into the illite/smectite zone, which is surrounded by a broad smectite zone. Because of boiling, abundant adularia associated with silver mineralization overlaps on the altered tuff breccia in the Fukuishi area. The alteration zoning suggests that the western Eikyu area and the eastern Fukuishi area belong to a single hydrothermal system. The data of fluid inclusion microthermometry indicate that the temperatures range 220–270°C, and salinities range 5–7 wt percent NaCl equivalent for the silver mineralization at the upper portion in the Eikyu area and the lower portion in the Fukuishi area. Radiometric ages for volcanic rocks in the area range from 2.19 to 1.64 Ma, and the dacitic intrusion formed at approximately 1.6 Ma. The silver-dominant mineralizing hydrothermal fluids system was active around 1.44 to 1.07 Ma, which formed the Eikyu Ag-Cu veins at depth, and the Fukuishi Ag ores at the shallower portion. 相似文献
133.
Sohiko Kameyama Satoshi Yoshida Hiroshi Tanimoto Satoshi Inomata Koji Suzuki Hisayuki Yoshikawa-Inoue 《Journal of Oceanography》2014,70(3):225-239
We measured dissolved isoprene (2-methyl-1,3-butadiene; C5H8) concentrations in a broad area of the southern Indian Ocean and in the Indian sector of the Southern Ocean from 35°S to 64°S and from 37°E to 111°E during austral summer 2010–2011. Isoprene concentrations were continuously measured by use of a proton-transfer-reaction mass spectrometer combined with a bubbling-type equilibrator. Concentrations of isoprene and its emission flux throughout the study period ranged from 0.2 to 395 pmol L?1 and from 181 to 313 nmol m?2 day?1, respectively, the averages being generally higher than those of previous studies. Although we found a significant linear positive relationship between isoprene and chlorophyll-a concentrations (r 2 = 0.37, n = 36, P < 0.001), the correlation coefficient was lower than previously reported. In contrast, in the high-latitude area (>53°S) we identified a significant negative correlation (r 2 = 0.59, n = 1263, P < 0.001) between isoprene and the temperature-normalized partial pressure of carbon dioxide (n-pCO2), used as an indicator of net community production in this study. This suggests that residence times and factors controlling variations in isoprene and n-pCO2 are similar within a physically stable water column. 相似文献
134.
Large-eddy simulations were conducted to investigate the mechanism of pollutant removal from a three-dimensional street canyon. Five block configurations with aspect ratios (building height to length) of 1, 2, 4, 8 and $\infty $ were used to create an urban-like array. A pollutant was released from a ground-level line source at the centre of the target canyon floor. For smaller aspect ratios, the relative contribution of the turbulent mass flux to net mass flux at the roof level, which was spatially averaged along the roof-level ventilation area, was closer to unity, indicating that turbulent motions mainly affected pollutant removal from the top of the canyon. As aspect ratio increased, the relative contribution became smaller, owing to strong upwind motions. However, the relative contribution again reached near unity for the infinite aspect ratio (i.e. a two-dimensional street canyon) because of lowered lateral flow convergence. At least 75 % of total emissions from the three-dimensional street canyon were attributable to turbulent motions. Pollutant removal by turbulent motions was related to the coherent structures of low-momentum fluid above the canyons. Though the coherent structure size of the low-momentum fluid differed, the positions of low-momentum fluid largely corresponded to instantaneous high concentrations of pollutant above the target canyon, irrespective of canyon geometry. 相似文献
135.
136.
Hikaru YABUTA Hiroshi NARAOKA Kinya SAKANISHI Hiroyuki KAWASHIMA 《Meteoritics & planetary science》2005,40(5):779-787
Abstract— Chemical structures of the insoluble organic matter (IOM) from the Antarctic CM2 chondrites (Yamato [Y‐] 791198, 793321; Belgica [B‐] 7904; Asuka [A‐] 881280, 881334) and the Murchison meteorite were analyzed by solid‐state 13C nuclear magnetic resonance (NMR) spectroscopy. Different types of carbons were characterized, such as aliphatic carbon (Ali‐C), aliphatic carbon linked to hetero atom (Hetero‐Ali‐C), aromatic carbon (Aro‐C), carboxyls (COOR), and carbonyls (C=O). The spectra of the IOM from Murchison and Y‐791198 showed two major peaks: Ali‐C and Aro‐C, while the spectra from the other meteorites showed only one major peak of Aro‐C. Carbon distribution was determined both by manual integration and deconvolution. For most IOM, the Aro‐C was the most abundant (49.8–67.8%) of all carbon types. When the ratios of Ali‐C to Aro‐C (Ali/Aro) were plotted with the atomic hydrogen to carbon ratio (H/C), a correlation was observed. If we use the H/C as a parameter for the thermal alteration event on the meteorite parent body, this result shows a different extent of thermal alteration. In addition, IOM with a lower Ali/Aro showed a lower ratio of Ali‐C to COOR plus C=O (Ali / (COOR + C=O)). This result suggests that the ratio of CO moieties to aliphatic carbon in IOM might reflect chemical oxidation that was involved in hydrothermal alteration. 相似文献
137.
Shinsuke Abe Noboru Ebizuka Hideyuki Murayama Katsuhito Ohtsuka Satoru Sugimoto Masa-yuki Yamamoto Hajime Yano Jun-ichi Watanabe Jiří Borovička 《Earth, Moon, and Planets》2004,95(1-4):265-277
Spectra of persistent meteor trains were observed at wavelength between 300 and 930 nm. Two obtained train spectra during
the 1998 and 2001 Leonid meteor showers are reported here. During the 1998 Leonids, one train was detected by a photographic
camera with a spectrograph covering 370–640 nm region. On the other hand, during the 2001 Leonids, video observations were
carried out using image intensified cameras in ultraviolet (UV), visible and near infrared (near-IR) wavelengths. Temperatures
in persistent trains have been measured by atmospheric O2 A(0,1) band at the wavelength near 864.5 nm. From a video spectrum obtained just 7 s after parent fireball’s flare, a rotational
temperature of 250 K at altitude of 88.0±0.5 km was estimated. We can say that the cooling time scale of train strongly depends
on the initial mass of its fireball at least for Leonids. Based on cooling constant calculated from our results, we estimated
a temperature of ∼
∼130 K as a final exothermic temperature at early stage of persistent trains. 相似文献
138.
Akira Yamaguchi Hiroshi Takeda Donald D. Bogard Daniel Garrison 《Meteoritics & planetary science》1994,29(2):237-245
Abstract— We have investigated 10 new specimens of the Millbillillie eucrite to study its textures and mineral compositions by electron probe microanalyser and scanning electron microscope. Although originally described as having fine-grained texture, the new specimens show diversity of texture. The compositions (Mg/Fe ratios) of the host pigeonites and augite lamellae are homogeneous, respectively, in spite of the textural variation. In addition to their chemical homogeneity, pyroxenes in coarse and fine-grained clasts are partly inverted to orthopyroxene. Chemical zoning of plagioclase during crystal growth is preserved. This eucrite includes areas of granulitic breccias and impact melts. Large scale textures show a subparallel layering suggesting incomplete mixing and deposition of impact melt and lithic fragments. An 39Ar-40Ar age determination for a coarse-grained clast indicates a strong degassing event at 3.55 ± 0.02 Ga. We conclude that Millbillillie is among the most equilibrated eucrites produced by thermal annealing after impact brecciation. According to the classification of impact breccias, Millbillillie can be classified as a mixture of granulitic breccias and impact melts. The last significant thermal event is characterized by network-like glassy veins that run through clasts and matrices. Consideration of textural observations and requirements for Ar-degassing suggests that the 39Ar-40Ar age could in principle date either the earilier brecciation and annealing event or the event which produced the veins. 相似文献
139.
We simulated the effects of irrigation on groundwater flow dynamics in the North China Plain by coupling the NIES Integrated Catchment‐based Ecohydrology (NICE) model with DSSAT‐wheat and DSSAT‐maize, two agricultural models. This combined model (NICE‐AGR) was applied to the Hai River catchment and the lower reach of the Yellow River (530 km wide by 840 km long) at a resolution of 5 km. It reproduced excellently the soil moisture, evapotranspiration and crop production of summer maize and winter wheat, correctly estimating crop water use. So, the spatial distribution of crop water use was reasonably estimated at daily steps in the simulation area. In particular, NICE‐AGR reproduced groundwater levels better than the use of statistical water use data. This indicates that NICE‐AGR does not need detailed statistical data on water use, making it very powerful for evaluating and estimating the water dynamics of catchments with little statistical data on seasonal water use. Furthermore, the simulation reproduced the spatial distribution of groundwater level in 1987 and 1988 in the Hebei Plain, showing a major reduction of groundwater level due mainly to overpumping for irrigation. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
140.
Measurements of size-separated aerosol number concentrations at Midagahara (altitude, 1,930 m), on the western slope of Mt. Tateyama near the coast of the Japan Sea, were performed each autumn from 2006 to 2011. High number concentrations of particles larger than 2 μm were frequently seen in 2006 and 2009 when the influence of Asian dust might have been significant. The pH and the ratio of Ca2+ to total ions were high in the rainwater bulk sampled when high number concentrations of coarse particles were observed. The mean pH of rainwater during the autumn in 2006 was significantly higher than that in 2007 and 2008. Acidic species might have been neutralized by the Asian dust particles. Dust particles may highly affect the natural environment, such as forest ecosystems, at high elevations during seasons without snow cover. 相似文献