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101.
氮气、氧气和空气水合物的合成及其拉曼光谱特征 总被引:1,自引:0,他引:1
在-20℃和不同的压力下,在实验室内分别合成了氮气水合物(16MPa)、氧气水合物(13MPa)和空气水合物(15MPa),并对其N—N和O—O键伸缩振动的拉曼光谱特征进行了研究。结果表明,人工合成的水合物中的N—N和O—O键的拉曼位移与天然的空气水合物中的数据十分接近。在氮气水合物和空气水合物中,N—N键的拉曼峰值均为2322.4cm-1;O—O键的拉曼峰值在氧气水合物和空气水合物保持一致,均为1547.8cm-1。空气水合物分解的拉曼谱图表明,它不是氮气水合物和氧气水合物组成的混合物,而是由氮分子和氧分子共同生成的单一水合物,氮分子和氧分子同时进入水合物的大笼和小笼中。与空气中的氮、氧比例相比,水合物中氧分子明显富集,氮分子和氧分子的比例为2.4∶1。 相似文献
102.
103.
通过对西湖茶园的植物和土壤样品进行一系列的调查,以着力寻找茶叶的铅污染源。利用铅同位素技术对西湖茶园的土壤、茶叶和城区的燃煤、大气气溶胶、汽车尾气进行铅同位素示踪研究。研究表明,茶园土壤铅物质的可溶相具同源性和残查态偏于多源性。清洗后的茶叶铅含量显著降低,但其同位素组成不发生明显改变,显示出茶叶中的铅与叶面空气沉降物中的铅同源。不同介质铅同位素对比值平均值呈现表土、大气(气溶胶)、煤的w(206Pb)/w(207Pb)与茶叶趋于相近,汽油低之;表土、大气(气溶胶)、汽油的w(208Pb)/〔w(206Pb)+w(207Pb)〕与茶叶趋于相近,煤略高之。不同区域茶叶铅物质具同源性,与种植的农业地质背景无关。在煤燃烧、气化过程中,Pb进入大气,通过大气沉降或被茶树吸收或附着在茶叶叶面;汽车尾气的排放是茶树铅污染的重要原因之一。 相似文献
104.
105.
Geochemical characteristics and source analysis of inflow of mine water in Wang’ershan Gold Mine, Shandong 总被引:1,自引:0,他引:1
QIAN Jianping LI Shuangli and CAO Chao Guilin University of Technology Guilin China 《中国地球化学学报》2008,(1)
Through a systematic observation of water level and temperature, and a comprehensive analysis of the data on major/trace elements, nitrite, hydrogen-oxygen isotopes, the conclusion has been drawn that there are two relatively independent groundwater systems (cool water and hot water), and the geochemical indicators of hot/cool waters are described. The cool water system is relatively enriched in Ca2 , Mg2 and HCO3-. Its TDS is relatively low, about 1400–1800 mg/L. The hot water system is relatively enriched in K , Na , Cl- and SO42-. Its TDS is relatively high, about 2200–2300 mg/L. The cool water system is enriched in Ba, Ga, Cd, and the hot water system is enriched in B, Ti, Cr, Ni, Cu, Mo, Rb, and Cs, relatively. Especially, the contents of Rb and Cs in the hot water system are more than five times as high as those in the cool water system. The NO3- contents of cool water discharged from the gold mine are relatively high, and those of hot water are extremely low. The δD and δ18O values follow an increasing order of surface water>mine cool water>mine hot water. The cool water comes mainly from the lateral supply of phreatic water, while the hot water comes mainly from the vertical supply of deeply circulating structure-fracture water. The ratio of cool water over hot water was estimated to be about 1:1 by a water quality model.. 相似文献
106.
Benjamin A ALLOU Huanzhang LU Jayanta GUHA Jacques CARIGNAN 《大地构造与成矿学》2008,32(2):195-211
在西非的象牙海岸Issia地区分布着许多铌钽矿床,包括原生矿和砂矿。原生矿产在分带很好的伟晶岩中。这个地区发育着许多花岗岩和花岗伟晶岩。伟晶岩可分为:(1)分异不好的伟晶岩,无矿化;(2)含Be伟晶岩,分带较好,见绿柱石;(3)含Be-Nb-Ta的伟晶岩,分带很好,是矿体;(4)Be-Nb-Ta-Li伟晶岩,分带很好,是矿体。除了10多个原生矿外,还有许多砂矿。砂矿有两种类型:一种近原生矿的坡积砂矿,另一种是经河流冲刷搬运后的冲积砂矿。我们选择了Etienne-Meguhe砂矿作为近原生矿的坡积砂矿的代表,Bemadi矿作为河流冲积型的砂矿的代表,对这两种类型的砂矿的风化、搬运、沉积机理进行了比较研究。研究发现不同的搬运距离和搬运模式对铌钽砂矿的主要矿物——铌钽铁矿的化学性质没有什么影响,而其物理形态则发生了变化。坡积型砂矿的铌钽铁矿常与石英、长石等矿物连生,其颗粒大小与原生的Nb-Ta伟晶岩中的铌钽铁矿一致;经河流冲积而形成的砂矿中,铌钽铁矿颗粒变小、轮廓变得圆滑,几乎无连生矿物,但矿体集中,常在河流的冲积扇中分布,易开采。 相似文献
107.
Environmental Investigation and Evaluation of Land Subsidence in the Datong Coalfield Based on InSAR Technology 总被引:1,自引:0,他引:1
Heavy mining of Jurassic and Carboniferous horizontal coal seams in the Datong coalfield has seriously affected the local geological environment, which is mainly manifested by such geohazards as soil avalanches, landslides, mudflows, surface subsidence, surface cracks, surface solid waste accumulation and surface deformation. More seriously, coal mining causes groundwater to leak. Overpumping of groundwater has resulted in substantial land subsidence of the urban area in Datong City. Based on the previous geo-environmental investigation in the work area, the authors used radar remote sensing techniques such as InSAR (synthetic aperture radar interferometry) and D-InSAR (differential synthetic aperture radar interferometry), supplemented by the optical remote sensing method, for geo-environmental investigation to ascertain the geo-environmental background of the Datong Jurassic and Carboniferous-Permian coalfield and evaluate the effects of the geohazards, thus providing a basis for the geo-environmental protection, geohazard control and prevention, land improvement and optimization of the human environment. In this study 8 cog-nominal ERS-1/2 SAR data frames during 1992 to 2003 were used, but the following processing was made: (1) the multitemporal SAR magnitude images were used to interpret the geological structure, vegetation, microgeomorphology and drainage system; (2) the multi-temporal InSAR coherent images were used to make a classification of surface features and evaluate the coherence change due to coal mining; and (3) the multi-temporal cog-nominal SAR images were used to complete D-InSAR processing to remove the information of differential deformation areas (sites). In the end, a ten-year time series of differential interferograms were obtained using the multi-temporal cog-nominal SAR images. In the tests, 84 deformed areas (sites) were obtained, belonging to those in 1993-1996, 1996-1997, 1997-1998, 1998-2001, 1998-2002 and 2001-2003 respectively. Of the 84 areas, 44 are m 相似文献
108.
Petroleum Migration Direction of the Silurian Paleo-pools in the Tarim Basin, Northwest China 总被引:1,自引:0,他引:1
LIU Luofu ZHAO Ye HUO Hong CHEN Lixin CHEN Yuanzhuang ZHAO Suping LI Chao LI Shuangwen GUO Yongqiang LI Yan 《《地质学报》英文版》2008,82(1):174-183
The results obtained in this paper indicate that carbazole-type compounds have high thermal stability and also show stability in oxidation and bio-degradation. This kind of compounds still has a high concentration and complete distribution in the analyzed dry asphalt samples, showing that they are particularly useful in studying petroleum migration of paleo-pool. During the basin's first-stage of oil-gas pool formation in the Silurian in Tazhong and Tabei areas of Tarim Basin (at the end of Silurian period) and the second-stage in the Awati area (in Permian), the petroleum experienced a long-distance migration. During the formation of the Silurian paleo-pools in Tazhong Uplift at the end of Silurian, the petroleum mainly came from the lower and middle Cambrian source rocks in the Manjiaer sag. The petroleum migrated towards the southwest-south entering the Silurian reservoir beds in Tazhong first. Then, it further migrated within Silurian from northwest to southeast along the highs of the Structural Belts to the region of the Silurian pinchout boundary in Tazhong. In Tabei Uplift, during the first-stage of pool formation, the petroleum was also from the lower and middle Cambrian source rocks in the Manjiaer sag. It migrated northwest entering the Silurian reservoir beds in the Tabei Uplift firstly, and then the migration continued in the same direction within the Silurian reservoirs and finally the petroleum was trapped in higher positions. During the second-stage pool formation in the Silurian beds in the areas around Awati sag, the petroleum mainly came from the lower-middle Cambrian source rocks in the Awati sag. The petroleum migrated from the generation center to Silurian reservoirs in all directions around the sag through major paths, and the petroleum was finally trapped in higher locations. 相似文献
109.
Late Cenozoic Stratigraphy and Paleomagnetic Chronology of the Zanda Basin, Tibet, and Records of the Uplift of the Qinghai-Tibet Plateau 总被引:1,自引:0,他引:1
MENG Xiangang ZHU Dagang SHAO Zhaogang YANG Chaobin HAN Jianen YU Ji MENG Qingwei LU Rongping 《《地质学报》英文版》2008,82(1):63-72
The characteristics of Late Cenozoic tectonic uplift of the southern margin of the Qinghai- Tibet Plateau may be inferred from fluvio-lacustrine strata in the Zanda basin, Ngari, Tibet. Magnetostratigraphic study shows that the very thick fluvio-lacustrine strata in the basin are 5.89- 0.78 Ma old and that their deposition persisted for 5.11 Ma, i.e. starting at the end of the Miocene and ending at the end of the early Pleistocene, with the Quaternary glacial stage starting in the area no later than 1.58 Ma. Analysis of the sedimentary environment indicates that the Zanda basin on the southern Qinghai-Tibet Plateau began uplift at -5.89 Ma, later than the northern Qinghai-Tibet Plateau. Presence of gravel beds in the Guge and Qangze Formations reflects that strong uplift took place at -5.15 and -2.71 Ma, with the uplift peaking at -2.71 Ma. 相似文献
110.