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971.
Stefan Jansen Eva Walpersdorf Ursula Werner Markus Billerbeck Michael E Böttcher Dirk de Beer 《Ocean Dynamics》2009,59(2):317-332
In this article, we describe the dynamics of pH, O2 and H2S in the top 5–10 cm of an intertidal flat consisting of permeable sand. These dynamics were measured at the low water line
and higher up the flat and during several seasons. Together with pore water nutrient data, the dynamics confirm that two types
of transport act as driving forces for the cycling of elements (Billerbeck et al. 2006b): Fast surface dynamics of pore water chemistry occur only during inundation. Thus, they must be driven by hydraulics (tidal
and wave action) and are highly dependent on weather conditions. This was demonstrated clearly by quick variation in oxygen
penetration depth: Seeps are active at low tide only, indicating that the pore water flow in them is driven by a pressure
head developing at low tide. The seeps are fed by slow transport of pore water over long distances in the deeper sediment.
In the seeps, high concentrations of degradation products such as nutrients and sulphide were found, showing them to be the
outlets of deep-seated degradation processes. The degradation products appear toxic for bioturbating/bioirrigating organisms,
as a consequence of which, these were absent in the wider seep areas. These two mechanisms driving advection determine oxygen
dynamics in these flats, whereas bioirrigation plays a minor role. The deep circulation causes a characteristic distribution
of strongly reduced pore water near the low water line and rather more oxidised sediments in the centre of the flats. The
two combined transport phenomena determine the fluxes of solutes and gases from the sediment to the surface water and in this
way create specific niches for various types of microorganisms. 相似文献
972.
Hervey Bay, a large coastal embayment situated off the central eastern coast of Australia, is a shallow tidal area (average
depth = 15 m), close to the continental shelf. It shows features of an inverse estuary, due to the high evaporation rate (approx.
2 m/year), low precipitation (less than 1 m/year) and on average almost no freshwater input from rivers that drain into the
bay. The hydro- and thermodynamical structures of Hervey Bay and their variability are presented here for the first time,
using a combination of four-dimensional modelling and observations from field studies. The numerical studies are performed
with the Coupled Hydrodynamical Ecological Model for Regional Shelf Seas (COHERENS). Due to the high tidal range (>3.5 m),
the bay is considered as a vertically well-mixed system, and therefore, only horizontal fronts are likely. Recent field measurements,
but also the numerical simulations, indicate characteristic features of an inverse/hypersaline estuary with low salinity (35.5 psu)
in the open ocean and peak values (>39.0 psu) in the head water of the bay. The model further predicts a nearly persistent
mean salinity gradient of 0.5 psu across the bay (with higher salinities close to the shore). The investigation further shows
that air temperature, wind direction and tidal regime are mainly responsible for the stability of the inverse circulation
and the strength of the salinity gradient across the bay. Due to an ongoing drying trend, the occurrence of severe droughts
at the central east coast of Australia and, therefore, a reduction in freshwater supply, the salinity flux out of the bay
has increased, and the inverse circulation has also strengthened. 相似文献
973.
Markus Röhricht Jürgen Krisam Ulrich Weise Uta R. Kraus Rolf‐A. Düring 《洁净——土壤、空气、水》2009,37(8):638-641
Most conventional wastewater treatment plants remove very small amounts of micropollutants, such as pharmaceuticals. Here, the ability of two different types of submerged nanofiltration flat sheet modules to remove pharmaceuticals from wastewater is analyzed. The two nanofiltration membranes were used at relatively low pressures of only 0.3 and 0.7 bar. At such low pressures, the membranes did not retain salts to a great extent. This is advantageous in wastewater treatment because no salt concentrate is produced. Carbamazepine was retained only slightly by the nanofiltration membranes, whereas approximately 60% of diclofenac and naproxen were retained by both membranes. This level of effectiveness might not be enough to justify the use of such a system as an additional treatment step in wastewater treatment plants. 相似文献
974.
The development of biorefineries is the key for access to an integrated production of food, feed, chemicals, materials, goods, fuels and energy of the future. This communication considers an integrated green biorefinery combined with today's production of feed in the green agriculture. Special attention is given to the combination of physical and biotechnological processes for the production of proteins as well as platform chemicals such as lactic acid and lysine. Mass and energy flows (steam and electricity) are given for the biorefining of green biomass to produce platform chemicals, proteins, feed and biogas from residues. 相似文献
975.
Claire L. Smith Ian J. Fairchild Christoph Spötl Silvia Frisia Andrea Borsato Steven G. Moreton Peter M. Wynn 《Quaternary Geochronology》2009,4(1):11-21
Determination of annual lamination provides important additional constraints to radiometric dates on speleothems, both for dating the duration of specific growth intervals and optimizing growth models. In the absence of visible laminae, however, speleothem age models are reliant upon curve fitting through discretely dated points and are therefore inherently more uncertain than annual chronologies from laminae. Given that the impact of seasonality on speleothems is expected to be strong enough to generate an annual pulse in trace element chemistry regardless of whether or not visible or fluorescent growth laminae are visible, we demonstrate the potential for deriving high-resolution stalagmite chronologies from non-laminated samples using annual chemical variations in stalagmites from two Alpine caves (Obir, Austria and Ernesto, NE Italy). Trace element data were obtained by ion microprobe analyses for H, P, Mg, Na, Sr and Ba and the annual signal was sought using spectral and wavelet analysis. An automated chemical peak-counting software tool was developed in MATLAB©. It counts significant annual peaks using criteria of minimum amplitude in relation to the local standard deviation of signal variation and minimum separation between peaks determined by the thickness of the preceding layers. Verification of the tool using visibly laminated samples suggests the software is a reliable and accurate method of chronology building, with hit ratios greater than 0.93 and less than 0.75% false alarm occurrences. Used in conjunction with other dating methods such as radiocarbon, U–Th and sulphur peak dating, the automated chemical laminae chronology-building approach provides a more meaningful alternative to simple age-depth curve fitting for non-laminated samples. 相似文献
976.
Cassandra R. Fenton Samuel Niedermann Mirjam M. Goethals Björn Schneider Jan Wijbrans 《Quaternary Geochronology》2009,4(6):475-492
Combining cosmogenic 3He and 21Ne (3Hec and 21Nec) measurements on both pyroxene and olivine from the Pleistocene Bar Ten flows (85–107 ka) greatly increases our ability to evaluate the accuracy of 3Hec and 21Nec production rates and, therefore, 3Hec and 21Nec surface exposure ages. Comparison of 3Hec and 21Nec age-pairs yielded by experimentally determined production rates and composition-based model calculations indicates that the former give more accurate surface exposure ages than the latter in this study. However, experimental production rates should be adjusted to the composition of the minerals being analyzed to obtain the best agreement between 3Hec and 21Nec ages for any given sample. 21Nec/3Hec values are 0.400 ± 0.029 and 0.204 ± 0.014 for olivine and pyroxene, respectively, in Bar Ten lava flows, in agreement with previously published values, and indicate that 21Nec/3Hec in olivine and pyroxene is not affected by erosion and remains constant with latitude, elevation, and time (up to 10 Myr). Samples with 21Nec/3Hec that do not agree with these values may indicate the presence of non-cosmogenic helium and/or neon. The neon three-isotope diagram can also indicate whether or not all excess neon in mineral separates comes from cosmogenic sources. An error-weighted regression for olivine defines a spallation line [y = (1.033 ± 0.031)x + (0.09876 ± 0.00033)], which is indistinguishable from that for pyroxene (Schäfer et al., 1999). We have derived a production rate of 25 ± 8 at/g/yr for 21Nec in clinopyroxene (En43–44) based on the 40Ar/39Ar age of the upper Bar Ten flow. Our study indicates that the production rate of 21Nec in olivine may be slightly higher than previously determined. Cosmogenic 3He and 21Ne remain extremely useful, particularly when paired, in determining accurate eruption ages of young olivine- and pyroxene-rich basaltic lava flows. 相似文献
977.
978.
Multistage Variscan magmatism in the central Tauern Window (Austria) unveiled by U/Pb SHRIMP zircon data 总被引:2,自引:0,他引:2
Roland Eichhorn Georg Loth Rudolf Höll Fritz Finger Andreas Schermaier Allen Kennedy 《Contributions to Mineralogy and Petrology》2000,139(4):418-435
U/Pb SHRIMP ages of nine Variscan leucocratic orthogneisses from the central Tauern Window (Austria) reveal three distinct pulses of magmatism in Early Carboniferous (Visean), Late Carboniferous (Stephanian) and Early Permian, each involving granitoid intrusions and a contemporaneous opening of volcano-sedimentary basins. A similar relationship has been reported for the Carboniferous parts of the basement of the Alps further to the west, e.g. the “External massifs” in Switzerland. After the intrusion of subduction-related, volcanic-arc granitoids (374?±?10?Ma; Zwölferkogel gneiss), collisional intrusive-granitic, anatectic and extrusive-rhyolitic/dacitic rocks were produced over a short interval at ca. 340?Ma (Augengneiss of Felbertauern: 340?±?4?Ma, Hochweißenfeld gneiss: 342?± 5?Ma, Falkenbachlappen gneiss: 343?±?6?Ma). This Early Carboniferous magmatism, which produced relatively small volumes of melt, can be attributed to the amalgamation of the Gondwana-derived “Tauern Window” terrane with Laurussia–Avalonia. Probably due to the oblique nature of the collision, transtensional phenomena (i.e. volcano-sedimentary troughs and high-level intrusives) and transpressional regimes (i.e. regional metamorphism and stacked nappes with anatexis next to thrust planes) evolved contemporaneously. The magmas are mainly of the high-K I-type and may have been generated during a short phase of decompressional melting of lithospheric mantle and lower crustal sources. In the Late Carboniferous, a second pulse of magmatism occurred, producing batholiths of calc-alkaline I-type granitoids (e.g. Venediger tonalite: 296?±?4?Ma) and minor coeval bodies of felsic and intermediate volcanics (Heuschartenkopf gneiss: 299?±?4?Ma, Peitingalm gneiss: 300?±?5?Ma). Prior to this magmatism, several kilometres of upper crust must have been eroded, because volcano-sedimentary sequences hosting the Heu- schartenkopf and Peitingalm gneisses rest unconformably on 340-Ma-old granitoids. The youngest (Permian) period of magma generation contains the intrusion of the S-type Granatspitz Central Gneiss at 271?±?4?Ma and the extrusion of the rhyolitic Schönbachwald gneiss protolith at 279?±?9?Ma. These magmatic rocks may have been associated with local extension along continental wrench zones through the Variscan orogenic crust or with a Permian rifting event. The Permian and the above-mentioned Late Carboniferous volcano-sedimentary sequences were probably deposited in intra-continental graben structures, which survived post-Variscan uplift and Alpine compressional tectonics. 相似文献
979.
In this study, we present Th–U disequilibria as well as radiogenic and trace element data for recent volcanic rocks from
the Nevados de Payachata volcano which erupted through ∼70 km of continental crust in the Central Volcanic Zone of the Andes
(18°S, 69°W). Both lavas and mineral separates were analyzed by mass spectrometry for 238U–230Th disequilibria. The lavas are characterized either by 230Th enrichment or depletion relative to its parent nuclide 238U. Mineral separates are used to derive U–Th isochron ages and these ages compare favorably with inferred stratigraphic ages
or K–Ar ages, although in one case the U–Th age is significantly older than the stratigraphic age. Despite relatively constant
Sr, Nd, and Pb isotope ratios, the lavas display inverse trends in 230Th/238U versus Ce/Yb or Ba/Hf diagrams. These trends cannot be interpreted by simple two-component mixing. Rather, there must be
three (and perhaps four components) involved in the genesis of the Parinacota lavas. A mantle wedge, a slab fluid, and a lower
crustal component can be identified. A sediment component is more difficult to detect as it is difficult to decipher its signature
because of the strong crustal influence. The existence of binary arrays can be explained by variable amounts of crustal material.
The process of crust–mantle interaction must have been short enough to preserve U–Th disequilibrium (<300 ka).
Received: 21 April 1999 / Accepted: 11 March 2000 相似文献
980.
Since 1980 when F. Lippmann's seminal paper appeared, ourunderstanding of solubility equilibria involving ionic solidsolutions has been advanced by theoretical considerations as wellas careful experimental studies designed to determine excess Gibbsfunctions. A unified theory of solid-solution aqueous-solutionequilibria as well as the thermodynamic background of thephenomenon of ``stoichiometric saturation' are reviewed.It is shown that Lippmann diagrams effectively summarize thethermodynamic basis of solid-solute aqueous-solution equilibria ofsparingly soluble metal carbonate systems. Clearly, the predictivepower of these diagrams may be limited due to kineticrestrictions. Only when dissolution and precipitation areessentially reversible, favourable conditions to synthesizehomogeneous solid phases can be derived from studies of equilibria. 相似文献