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Zhongwu Li Hao Peng Binggeng Xie Chun Liu Xiaodong Nie Danyang Wang Mei Huang Haibing Xiao Lin Shi Xuqin Zhang Jieyu Jiang 《水文研究》2020,34(6):1446-1459
Exploring the chemical characterization of dissolved organic matter (DOM) is important for understanding the fate of laterally transported organic matter in watersheds. We hypothesized that differences in water-extractable organic matter (WEOM) in soils of varying land uses and rainfall events may significantly affect the quality and the quantity of stream DOM. To test our hypotheses, characteristics of rainfall-runoff DOM and WEOM of source materials (topsoil from different land uses and gullies, as well as typical vegetation) were investigated at two adjacent catchments in the Loess Plateau of China, using ultraviolet–visible absorbance and excitation emission matrix fluorescence with parallel factor analysis (PARAFAC). Results indicated that land-use types may significantly affect the chemical composition of soil WEOM, including its aromaticity, molecular weight, and degree of humification. The PARAFAC analysis demonstrated that the soils and stream water were dominated by terrestrial/allochthonous humic-like substances and microbial transformable humic-like fluorophores. Shifts in the fluorescence properties of stream DOM suggested a pronounced change in the relative proportion of allochthonous versus autochthonous material under different rainfall patterns and land uses. For example, high proportions of forestland could provide more allochthonous DOM input. This study highlights the relevance of soils and hydrological dynamics on the composition and fluxes of DOM issuing from watersheds. The composition of DOM in soils was influenced by land-use type. Precipitation patterns influenced the proportion of terrestrial versus microbial origins of DOM in surface runoff. Contributions of allochthonous, terrestrially derived DOM inputs were highest from forested landscapes. 相似文献
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在全球气候变化和人类活动影响加剧的背景下,作为河口海岸重要子系统的三角洲正在发生快速变化。长江三角洲地处长江入东海交汇处,是中国最重要的经济核心区之一,对邻近区域乃至整个长江经济带经济社会发展都起着重要作用。由于全球变暖、海面上升和强烈人类活动引发了三角洲系统状态转换,因此以往基于恒定系统状态而获得的有关长江三角洲的认识已不能满足未来需求,迫切需要对未来海面变化、极端事件、流域与河口工程影响下的三角洲物质循环条件、物理过程、地貌冲淤演化、源-汇格局调整等科学问题进行深入研究。在三角洲系统行为、未来演化趋势的预测能力建设中,应重视从海面到海底的综合立体观测系统的发展,以获取关键数据;基于三角洲系统的时、空演化特征,建立三角洲本征态和衍生态的谱系理论。未来需针对系统状态转换而调整原先的经济社会发展模式,以便保护自然资源、重建生态系统,更好地支撑长江经济带发展,重绘长江三角洲发展蓝图。 相似文献
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The summer Asian–Pacific Oscillation(APO) is a major teleconnection pattern that reflects the zonal thermal contrast between East Asia and the North Pacific in the upper troposphere. The performance of Beijing Climate Center Climate System Models(BCC CSMs) with different horizontal resolutions, i.e., BCC CSM1.1 and BCC CSM1.1(m), in reproducing APO interannual variability, APO-related precipitation anomalies, and associated atmospheric circulation anomalies, is evaluated.The results show that BCC CSM1.1(m) can successfully capture the interannual variability of the summer APO index. It is also more capable in reproducing the APO's spatial pattern, compared to BCC CSM1.1, due to its higher horizontal resolution. Associated with a positive APO index, the northward-shifted and intensified South Asian high, strengthened extratropical westerly jet, and tropical easterly jet in the upper troposphere, as well as the southwesterly monsoonal flow over North Africa and the Indian Ocean in the lower troposphere, are realistically represented by BCC CSM1.1(m), leading to an improvement in reproducing the increased precipitation over tropical North Africa, South Asia, and East Asia, as well as the decreased precipitation over subtropical North Africa, Japan, and North America. In contrast, these features are less consistent with observations when simulated by BCC CSM1.1. Regression analysis further indicates that surface temperature anomalies over the North Pacific and the southern and western flanks of the Tibetan Plateau are reasonably reproduced by BCC CSM1.1(m), which contributes to the substantial improvement in the simulation of the characteristics of summer APO compared to that of BCC CSM1.1. 相似文献
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Some Au deposits in southern Anhui Province have recently been found to be closely associated with Late Mesozoic intrusions. Typical examples include the Huashan Au (Sb) deposit and Au deposits at Zhaojialing, Wuxi, and Liaojia. In order to understand the mechanisms that led the formation of these Au deposits, we make detailed reviews on the geological characteristics of these Au deposits. Specifically, we present new LA-ICP-MS zircon U–Pb dating, along with elemental and Hf isotopic data from the Huashan Au (Sb) deposit. Our data suggests that the Huashan ore-related intrusions were emplaced during the Late Jurassic and Early Cretaceous periods (144–148 Ma). They are characterized by arc-magma features and high oxygen fugacity and are rich in inherited zircons. Zircon U–Pb ages and Lu–Hf isotopes from intrusions suggest that Proterozoic juvenile lithosphere is the main source of these intrusions. The regional geological history implies that lithosphere beneath southern Anhui was produced during a Proterozoic subduction and was fertilized with Au (Cu) in the process. Integrated with the results of previous studies, we inferred that Late Mesozoic intrusions formed by the remelting of the lithosphere could provide the metal endowment for the Au-rich deposits in southern Anhui. 相似文献
47.
探讨活性氧(reactive oxygen species,ROS)在温石棉激活线粒体通路诱导A549凋亡中的作用。采用不同浓度温石棉粉尘染毒人肺上皮细胞(A549)后,MTT法检测细胞存活率,流式细胞术检测ROS抑制剂N-乙酰半胱氨酸(N-acetyl-L-cysteine,NAC)预处理前后的细胞凋亡率、胞内ROS水平及线粒体膜电位,Western Blot法检测各组细胞半胱天冬氨酸蛋白酶3(caspase-3)、p53蛋白表达水平。实验结果显示,温石棉可降低A549细胞存活率,呈现时间-剂量效应关系;NAC可显著减少胞内ROS水平、阻止线粒体膜电位下降,并下调caspase-3、p53蛋白的表达水平,抑制部分细胞凋亡的发生。表明ROS可通过诱导p53蛋白过表达,激活线粒体凋亡通路,诱导A549细胞发生凋亡。 相似文献
48.
将不同浓度PM_(2.5)降尘作用于A549细胞后,利用MTT法检测其存活率,W-G染色观察细胞形态,荧光探针法检测细胞ROS和MMP相对水平,以探讨PM_(2.5)降尘对A549细胞线粒体氧化损伤的影响及作用机制。结果显示,经12. 5μg/m L的PM_(2.5)降尘作用A549细胞3 h后,细胞存活率为(81. 77±6. 15)%,并随作用浓度及时间增加呈递减趋势。PM_(2.5)染毒后可观察到细胞形态不规则,胞膜溶解破坏,细胞微核出现。PM_(2.5)降尘作用于细胞24 h后,胞内ROS相对含量随暴露浓度增加呈递增趋势,细胞MMP相对水平随染毒浓度增加而降低,且胞内ROS和MMP两者间存在显著相关关系(R2=0. 878)。提示PM_(2.5)降尘处理A549细胞后可通过刺激ROS的产生,诱导细胞MMP下降,造成细胞线粒体氧化损伤。 相似文献
49.
Landslide-prone slopes in earthquake-affected areas commonly feature heterogeneity and high permeability due to the presence of cracks and fissures that were caused by ground shaking. Landslide reactivation in heterogeneous slope may be affected by preferential flow that was commonly occurred under heavy rainfall. Current hydro-mechanical models that are based on a single-permeability model consider soil as a homogeneous continuum, which, however, cannot explicitly represent the hydraulic properties of heterogeneous soil. The present study adopted a dual-permeability model, using two Darcy-Richards equations to simulate the infiltration processes in both matrix and preferential flow domains. The hydrological results were integrated with an infinite slope stability approach, attempting to investigate the hydro-mechanical behavior. A coarse-textured unstable slope in an earthquake-affected area was chosen for conducting artificial rainfall experiment, and in the experiment slope, failure was triggered several times under heavy rainfall. The simulated hydro-mechanical results of both single- and dual-permeability model were compared with the measurements, including soil moisture content, pore water pressure, and slope stability conditions. Under high-intensity rainfall, the measured soil moisture and pore water pressure at 1-m depth showed faster hydrological response than its simulations, which can be regarded as a typical evidence of preferential flow. We found the dual-permeability model substantially improved the quantification of hydro-mechanical processes. Such improvement could assist in obtaining more reliable landslide-triggering predication. In the light of the implementation of a dual-permeability model for slope stability analysis, a more flexible and robust early warning system for shallow landslides hazard in coarse-textured slopes could be provided. 相似文献
50.
Huangling Gu Zhangxing Nie Jianghong Deng Liuan Duan Qing Hu 《International Geology Review》2018,60(11-14):1404-1434
ABSTRACTThe Guichi ore-cluster district in the Lower Yangtze River Metallogenic Belt hosts extensive Cu–Au–Mo polymetallic deposits including the Tongshan Cu–Mo, Paodaoling Au, Matou Cu–Mo, Anzishan Cu–Mo, Guilinzheng Mo and Zhaceqiao Au deposits, mostly associated with the late Mesozoic magmatic rocks, which has been drawn to attention of study and exploration. However, the metallogenic relationship between magmatic rocks and the Cu–Au-polymetallic deposits is not well constrained. In this study, we report new zircon U–Pb ages, Hf isotopic, and geochemical data for the ore-bearing intrusions of Guichi region. LA-ICP-MS U–Pb ages for the Anzishan quartz diorite porphyrite is 143.9 ± 1.0 Ma. Integrated with previous geochronological data, these late Mesozoic magmatic rocks can be subdivided into two stages of magmatic activities. The first stage (150–132 Ma) is characterized by high-K calc-alkaline intrusions closely associated with Cu–Au polymetallic ore deposits. Whereas, the second stage (130–125 Ma) produced granites and syenites and is mainly characterized by shoshonite series that are related to Mo–Cu mineralization. The first stage of magmatic rocks is considered to be formed by partial melting of subducted Palaeo-Pacific Plate, assimilated with Yangtze lower crust and remelting Meso-Neoproterozoic crust/sediments. The second stage of magmatism is originated from partial melting of Mesoproterozoic-Neoproterozoic crust, mixed with juvenile crustal materials. The depression cross to the uplift zone of the Jiangnan Ancient Continent forms a gradual transition relation, and the hydrothermal mineralization composite with two stages have certain characteristics along the regional fault (Gaotan Fault). Guichi region results from two episodes of magmatism probably related to tectonic transition from subduction of Palaeo-Pacific Plate to back-arc extensional setting between 150 and 125 Ma, which lead to the Mesozoic large-scale polymetallic mineralization events in southeast China. 相似文献