云层与气溶胶对大气吸收太阳辐射的影响   总被引：3，自引：4，他引：3  

胡丽琴  刘长盛 《高原气象》2001,20(3):264-270

云通过辐射过程对地气系统的能量平衡起着特别显著的调节作用 ,是影响天气、气候以及全球变化的重要因子。近年来 ,有云大气对太阳短波辐射的“异常吸收”又成为云—辐射研究中的一个争论热点。有云大气的短波吸收受到多种因素的影响 ,关于这方面的研究还不够充分。本文通过计算 ,从理论上探讨了若干因素的组合对大气吸收的综合影响。在计算中 ,同时考虑了不同太阳辐射波段、不同太阳入射天顶角、不同云顶高度以及不同下垫面的影响 ,并考虑了包含大气分子、气溶胶和云滴的吸收与散射 ,以及在近红外波段大气自身的热辐射等过程 ,阐明了云与气溶胶在不同波段对大气吸收太阳辐射的影响。  相似文献   

重庆地区降水对气溶胶浓度及雨水中离子浓度的影响   总被引：1，自引：0，他引：1  

吴玉霞  沈志来 《高原气象》1991,10(1):52-60

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荒漠地区直接太阳光谱的测量   总被引：2，自引：4，他引：2  

孔琴心  熊效振 《高原气象》1992,1(4):353-360

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Aerosol’s Impacts on the Indian Summer Monsoon and the East Asian Summer Monsoon:An Overview     

Lu Wenxi  Wu Jian 《地球科学进展》2016,31(3):248-257

India Peninsula and East Asia are high aerosol loading regions as well as major regions influenced by Asian monsoon. The changes of monsoon intensity and precipitation have great influence on economy, especially agricultural production of monsoon regions. There are many researches of impacts of aerosol on Indian monsoon, which have achieved many comprehensive progresses. Earlier researches show that atmospheric brown cloud caused negative radiative forcing and weakened the warming induced by greenhouse gases. Current researches show that absorbing aerosol enhanced the Indian monsoon and increased rainfall in pre-monsoon season, while the scattering effect of aerosol weakened the Indian summer monsoon and the East Asian summer monsoon and rainfall in monsoon season. Due to so many factors affecting the monsoon, researches of aerosol impacts on monsoon become more complex. Thus, these results remain uncertain. This paper reviews previous researches and generalizes the mechanisms of impacts of aerosols on Asian monsoon. By comparing the East Asian summer monsoon with the Indian summer monsoon, we discussed deficiencies of the prior researches, and pointed out the direction for future researches about the impact of aerosol on the Asian summer monsoon, especially on the East Asian summer monsoon.  相似文献   

黄山夏季气溶胶多尺度吸湿性的参数化方案构建研究     

王启花  杨素英  李艳伟  银燕  张泽锋  陈魁  赵丽君 《气象学报》2016,74(6):989-1001

利用2014年7月在黄山光明顶观测的气溶胶吸湿性参数（κ）和气溶胶离子化学组分、有机碳（OC,organic carbon）数据,对多尺度气溶胶吸湿性参数进行分析,并在此基础上建立了多尺度κ的参数化方案。研究结果表明,影响黄山夏季气溶胶来源的主要气团包括西南气团、北方气团以及东南气团。黄山夏季κ的变化范围为0.2-0.48,且随粒径增大成先增大后减小的分布特征;气溶胶粒径在0.15-1.1 μm的强吸湿段,κ>0.3,而在粒径小于0.15 μm和粒径大于1.1 μm弱吸湿段,κκ分布不同,气溶胶粒子在小于1.1 μm的粒径段,当受西南气团影响时,κ值最大,而受东南气团影响时,κ值最小;在气溶胶粒径大于1.1 μm时,κ在两个气团背景下呈现与气溶胶粒径小于1.1 μm时相反的分布特征。影响粒径小于1.1 μm气溶胶吸湿能力的主要水溶性化学组分为NH4+、SO42-、水溶性有机碳（WSOC,water soluble organic carbon）,而影响大于1.1 μm粒径范围气溶胶吸湿能力的主要水溶性化学组分为NH4+、SO42-、NO3-、WSOC和Ca2+。由气溶胶多尺度离子化学组分和WSOC构建的气溶胶κ的参数化方案,在小于1.1 μm和大于1.1 μm的粒径范围内的表达式分别为κreg=0.12+0.45fNH4++0.63fSO42-+0.18fWSOC和κreg=0.01+0.78fNH4++0.76fNO3-+0.8fSO42--0.28fCa2++0.14fWSOC（f为对应组分的质量份数）。两个参数化方案均能较好地预报κ,预报值κreg与κ的计算值间存在较好的相关关系,相关系数通过了置信度99%的显著性检验,且预报误差在30%范围内。   相似文献   

海洋大气气溶胶的离子色谱分析   总被引：2，自引：1，他引：2  

张远辉  黄自强 《台湾海峡》1994,13(2):144-150

对分析方法如采样滤膜的均匀性，滤膜上阴，阳离子的萑萃取率，方法的精密度和检出限等进行了基础性研究，并采用该方法测定了厦门海域大气中的Ｃｌ＾－，Ｆ＾－，ＳＯ＾２－４，ＮＯ＾－３，ＮＨ＾＋４和Ｎａ＾＋。本文法有较高的灵敏度，重现性好，可同时测定多种无机离子，适用于海洋大气气溶胶分析。  相似文献   

An improved atmospheric correction algorithm for applying MERIS data to very turbid inland waters     

《International Journal of Applied Earth Observation and Geoinformation》2015

Atmospheric correction (AC) is a necessary process when quantitatively monitoring water quality parameters from satellite data. However, it is still a major challenge to carry out AC for turbid coastal and inland waters. In this study, we propose an improved AC algorithm named N-GWI (new standard Gordon and Wang’s algorithms with an iterative process and a bio-optical model) for applying MERIS data to very turbid inland waters (i.e., waters with a water-leaving reflectance at 864.8 nm between 0.001 and 0.01). The N-GWI algorithm incorporates three improvements to avoid certain invalid assumptions that limit the applicability of the existing algorithms in very turbid inland waters. First, the N-GWI uses a fixed aerosol type (coastal aerosol) but permits aerosol concentration to vary at each pixel; this improvement omits a complicated requirement for aerosol model selection based only on satellite data. Second, it shifts the reference band from 670 nm to 754 nm to validate the assumption that the total absorption coefficient at the reference band can be replaced by that of pure water, and thus can avoid the uncorrected estimation of the total absorption coefficient at the reference band in very turbid waters. Third, the N-GWI generates a semi-analytical relationship instead of an empirical one for estimation of the spectral slope of particle backscattering. Our analysis showed that the N-GWI improved the accuracy of atmospheric correction in two very turbid Asian lakes (Lake Kasumigaura, Japan and Lake Dianchi, China), with a normalized mean absolute error (NMAE) of less than 22% for wavelengths longer than 620 nm. However, the N-GWI exhibited poor performance in moderately turbid waters (the NMAE values were larger than 83.6% in the four American coastal waters). The applicability of the N-GWI, which includes both advantages and limitations, was discussed.  相似文献   

The acid catalyzed nitration of methanol: formation of methyl nitrate via aerosol chemistry     

Laura T. Iraci  Brent G. Riffel  Carly B. Robinson  Rebecca R. Michelsen  Rachel M. Stephenson 《Journal of Atmospheric Chemistry》2007,58(3):253-266

The aqueous phase acid-catalyzed reaction of methanol (CH₃OH) with nitric acid (HNO₃) to yield methyl nitrate (CH₃ONO₂) under atmospheric conditions has been investigated using gas-phase infrared spectroscopy. Reactions were conducted in aqueous sulfuric acid solutions (50.5–63.6 wt.%) with [CH₃OH] = 0.00005–0.005 M and [HNO₃] = 0.02–0.21 M, at 278.2–328.6 K. Methyl nitrate production rates increased linearly with CH₃OH and HNO₃ concentrations and exponentially with sulfuric acid weight percent within the regime studied. Rates increased linearly with nitronium ion concentration, indicating that the reaction involves as the nitrating agent under these conditions. At 298 K, the rate of methyl nitrate production can be calculated from k _obs [CH₃OH][HNO₃], where k _obs  = 2.337 × 10⁻¹³(exp(0.3198*wt.% H₂SO₄)) when the solubility of CH₃ONO₂ in acidic solution is approximated by H* for pure water. The temperature dependence of the rate coefficient is related to solution composition, with activation energies of 59 and 49 kJ/mol at 51.1 and 63.6 wt.% H₂SO₄, respectively, when k is calculated from rate. The temperature dependence has also been parameterized for application to the atmosphere, but the small quantities of present in aerosol particles will result in methyl nitrate production rates too small to be of significance under most atmospheric conditions. An erratum to this article can be found at  相似文献   

地球静止卫星和网格化站点支持下的PM_2.5精细制图     

范东浩  秦凯  杜娟  何秦  辛世纪  刘鼎医 《遥感学报》2022,26(5):1015-1026

许多城市建立的相对稠密的网格化监测站点,为精细化监管城市空气质量奠定了基础。本文选用徐州市网格化监测数据、地球静止卫星Himawari-8/AHI及COMS/GOCI的表观反射率和气溶胶光学厚度数据、气象和其他辅助数据,开展了徐州地区0.005°空间分辨率网格的PM_2.5浓度精细化制图研究。本文使用了极端梯度提升（XGBoost）、随机森林（RF）及时空加权回归（GTWR）等3种方法,并选用多种特征参数组合进行对比分析。综合分析模型精度和过拟合程度,结果表明XGBoost模型表现最好,其R²为0.90,RMSE为11.65 μg/m³。进一步将本文结果与国控站点、清华大学的TAP数据集和马里兰大学的CHAP数据集的对比分析,结果表明基于网格化站点的PM_2.5制图结果能更好地反映城市内部不同区域的PM_2.5浓度分布差异性,弥补因国控站点稀疏带来的缺陷,更好地服务于城市空气质量精准管控。  相似文献   

Lidar depolarization measurements for aerosol source and property studies over Chungli (24.58° N, 121.1° E)     

C.W. Chiang  S.K. Das  J.B. Nee 《Atmospheric Research》2008,90(2-4):203-ICNAA07

Aerosol depolarization ratio and aerosol optical depth (AOD) were measured at Chungli (24.58° N, 121.1° E), Taiwan during the period from 2002–2004. The depolarization ratios of background aerosol have values mostly less than 0.06. The maximum AOD in the altitude range of 0.7 to 2km occurs in the summer (June–August) while between 2 and 5km, the spring (March–May) shows the maximum. The former is mainly related to strong convection and humidity; however the latter is due to anthropogenic aerosols transported from East China and Southeast Asia based on calculations of backward trajectories. This seasonal variation of AOD inferred from different transport mechanisms and aerosol compositions which are supported by the height distributions of aerosol extinction and origins.  相似文献