PM10 Source Apportionment in Ahvaz,Iran, Using Positive Matrix Factorization     

Mohammad Hossein Sowlat  Kazem Naddafi  Masud Yunesian  Peter L. Jackson  Saeedeh Lotfi  Abbas Shahsavani 《洁净——土壤、空气、水》2013,41(12):1143-1151

Source apportionment of particulate matter <10 µm in diameter (PM₁₀), having considerable impacts on human health and the environment, is of high priority in air quality management. The present study, therefore, aimed at identifying the potential sources of PM₁₀ in an arid area of Ahvaz located in southwest of Iran. For this purpose, we collected 24‐h PM₁₀ samples by a high volume air sampler. The samples were then analyzed for their elemental (Al, As, B, Ba, Be, Ca, Cd, Co, Cr, Cu, Fe, Hg, K, Mg, Mn, Na, Ni, Pb, Se, Si, Sn, Sr, Li, Ti, V, Zn, Mo, and Sb) and ionic (NH, Cl^?, NO, and SO) components using inductively coupled plasma optical emission spectrometry and ion chromatography instruments, respectively. Eight factors were identified by positive matrix factorization: crustal dust (41.5%), road dust (5.5%), motor vehicles (11.5%), marine aerosol (8.0%), secondary aerosol (9.5%), metallurgical plants (6.0%), petrochemical industries and fossil fuel combustion (13.0%), and vegetative burning (5.0%). Result of this study suggested that the natural sources contribute most to PM₁₀ particles in the area, followed closely by the anthropogenic sources.  相似文献   

Observational Subseasonal Variability of the PM_2.5 Concentration in the Beijing-Tianjin-Hebei Area during the January 2021 Sudden Stratospheric Warming     

Qian LU  Jian RAO  Chunhua SHI  Dong GUO  Ji WANG  Zhuoqi LIANG  Tian WANG 《大气科学进展》2022,39(10):1623-1636

It is still not well understood if subseasonal variability of the local PM_2.5 in the Beijing-Tianjin-Hebei (BTH) region is affected by the stratospheric state. Using PM_2.5 observations and the ERA5 reanalysis, the evolution of the air quality in BTH during the January 2021 sudden stratospheric warming (SSW) is explored. The subseasonal variability of the PM_2.5 concentration after the SSW onset is evidently enhanced. Stratospheric circumpolar easterly anomalies lasted for 53 days during the January–February 2021 SSW with two evident stratospheric pulses arriving at the ground. During the tropospheric wave weakening period and the intermittent period of dormant stratospheric pulses, the East Asian winter monsoon weakened, anomalous temperature inversion developed in the lower troposphere, anomalous surface southerlies prevailed, atmospheric moisture increased, and the boundary layer top height lowered, all of which favor the accumulation of pollutant particulates, leading to two periods of pollution processes in the BTH region. In the phase of strengthened East Asian winter monsoon around the very beginning of the SSW and another two periods when stratospheric pulses had reached the near surface, opposite-signed circulation patterns and meteorological conditions were observed, which helped to dilute and diffuse air pollutants in the BTH region. As a result, the air quality was excellent during the two periods when the stratospheric pulse had reached the near surface. The increased subseasonal variation of the regional pollutant particulates after the SSW onset highlights the important role of the stratosphere in the regional environment and provides implications for the environmental prediction.  相似文献   

1961-2020年郑州主城区大气自净能力变化特征分析     

刘美  姬兴杰  田力  丁亚磊  左璇 《气象与环境学报》2022,38(3):93-100

利用郑州市主城区1961—2020年气象观测资料和2014—2018年空气质量监测数据,分析了郑州主城区大气自净能力指数的长期变化趋势与影响因子以及2014—2018年主城区大气自净能力与PM_(2.5)的关系。结果表明:郑州主城区大气自净能力指数30 a气候均值为4.42 t·(d·km^(2))^(-1),春季大气自净能力最强,为5.20 t·(d·km^(2))^(-1);秋季大气自净能力最弱,为3.88 t·(d·km^(2))^(-1),不利于对大气污染物的清除。1961—2020年郑州主城区大气自净能力呈显著的减弱趋势,其中1969年最强为6.85 t·(d·km^(2))^(-1),2020年最弱为3.06 t·(d·km^(2))^(-1)。影响因子中,1961—1980年混合层厚度与大气自净能力指数呈正相关;日平均风速≥2.5 m·s^(-1)的日数和小风日数与大气自净能力分别呈正、负显著相关;大气自净能力指数与降水日数显著相关,2015年后偏强降水日数的增加对大气自净能力在同时期的增强有一定影响。此外,研究还表明主城区大气自净能力和PM_(2.5)浓度存在显著的负相关,说明大气自净能力强时,对应的PM_(2.5)浓度低,环境空气质量趋好。  相似文献   

西安市PM_2.5城乡差异及与城市热岛的关联研究          下载免费PDF全文

李煜斌  姜蕴聪  杨元建  张建彬  赵纯  高志球 《大气科学学报》2022,45(6):904-916

依据一种基于建筑用地比例和土地利用信息熵的城乡站点划分方法,将西安市环境与气象站点划分为城区、郊区和两类乡村站,讨论其PM_2.5的城乡分布特征及与城市热岛效应强度(Urban Heat Island Intensity,UHII)间的相关关系。结果表明,不同季节西安市呈现不同的PM_2.5城乡分布特征和日变化特征,两类乡村站点PM_2.5差异明显且下风向乡村站点(乡村D)对应的UHII_D对城区和乡村的影响程度大于上风向乡村站点(乡村U)对应的UHII_U。在城区较多本地排放的影响下,乡村PM_2.5浓度与 UHII_U(或UHII_D)相关系数均大于城区。随着UHII_D的增加,城乡PM_2.5相对浓度差值(RUPII_D)整体呈下降趋势且UHII_D与RUPII_D在春夏秋季显著负相关。UHII_D增大,城区近地面PM_2.5的水平扩散能力减弱,但PM_2.5的垂直扩散能力较乡村更强,从而UHII_D通过影响PM_2.5的传输扩散特征,进一步影响西安市RUPII_D。  相似文献   

The Interannual Variation of Transboundary Contributions from Chinese Emissions of PM_(2.5) to South Korea     

Xiao HAN  Meigen ZHANG 《大气科学进展》2021,38(5):701-706

In recent years,several studies pointed out that anthropogenic emission sources in China which significantly contribute to the PM_2.5mass burden was an important cause of particulate pollution in South Korea.However,most studies generally focused upon a single pollution event.It is rare to see comprehensive research that captures those features prone to interannual variations concerning the transboundary pollutant contribution in South Korea using a unified method.In this paper,we establish the emission inventories covering East Asia in 2010,2015,and 2017,and then conduct the source apportionment by applying a coupled regional air quality model called the Integrated Source Apportionment Module(ISAM).Comparison of simulated and observed PM_2.5mass concentration at 165 CNEMC(China National Environmental Monitoring Center)sites suggests that the PM_2.5concentrations are well represented by the modeling system.The model is used to quantitatively investigate the contribution from emission sources in China to PM_2.5concentrations over South Korea and those features found to be prone to interannual variations are then discussed.The results show that the average annual contribution of PM_2.5has dropped significantly from 28.0%in 2010 to 15.7%in 2017,which strongly suggests that China has achieved remarkable results in the treatment of atmospheric particulates.  相似文献   

气象-气溶胶资料联合同化对秋季PM_2.5浓度模拟的影响研究     

宋佳琨  陈耀登  陈丹 《气象学报》2021,79(3):477-491

相比冬季大范围静稳条件下的污染堆积过程,秋季气象条件更加复杂和局地化,气象条件模拟不确定性给秋季气溶胶模拟带来了更大难度,且目前研究较少考虑气象-气溶胶因素在线模拟和联合同化。使用WRF/Chem模式和格点统计差值（GSI）三维变分同化系统,2015年10月进行了为期1个月的气象-气溶胶资料联合同化及模拟试验,并基于此讨论了气象-气溶胶资料联合同化对秋季PM_2.5浓度模拟的影响。结果表明,WRF/Chem模式可以模拟出秋季污染天气过程,但对华北平原和中东部地区存在高估、西北部存在低估现象;同化地面PM_2.5浓度观测资料可以改进对PM_2.5浓度的模拟,上述两个地区的偏差均得到订正,6 h预报偏差均降低至6 μg/m3以内;重点针对华北地区的分析表明,秋季PM_2.5污染过程与特殊气象条件（湿度升高、风场辐合、区域输送）密切相关,因此在地面PM_2.5观测资料同化基础上增加常规气象资料同化,能进一步提高对华北平原气象-污染过程的表达,PM_2.5浓度预报相关系数从0.86提高至0.89。气象-气溶胶联合资料同化能更加准确地模拟秋季气溶胶污染过程,为更好地开展污染成因和在气象预报框架下开展气象-气溶胶相互影响研究提供了基础。   相似文献   

利用FY-4A卫星光学数据对中国近地面PM_2.5浓度的估算和检验分析     

江琪  迎春  王飞  张天航  何佳宝  桂海林  张碧辉  徐冉 《气象学报》2021,79(3):492-508

对FY-4A卫星的气溶胶光学厚度（AOD）产品进行检验,并根据卫星相关观测资料,通过改进后的PMRS方法,反演得到中国近地面PM_2.5质量浓度网格化分布。结果表明,FY-4A卫星反演不同站点AOD与地基观测网（AERONET）观测结果吻合较好,但存在一定的低估或高估现象,相关系数区间为0.54—0.87。将细粒子比（FMF）以0.4为界进行划分,FMF＞0.4时,拟合结果较FMF≤0.4时更接近于AERONET观测结果;但FMF≤0.4时,卫星反演的AOD稳定性优于FMF＞0.4时。通过引入AOD的大小,改进FMF＞0.4时对细粒子柱状体积消光比（VE_f）的估算算法,并通过改进后的PMRS方法对中国近地面PM_2.5浓度进行逐时反演,其反演结果和地面观测结果相关较好,其中,乌鲁木齐、石家庄和徐州观测点的相关系数均高于0.7,但数值上仍存在高估或低估,误差结果由多种因素决定。空间分布中,卫星反演的中国2019年近地面PM_2.5浓度月均值与近地面观测的结果有较好的对应关系,二者逐月演变趋势基本一致,基本可以反映出中国近地面大气细粒子的空间分布,特别是秋、冬季京津冀周边区域、汾渭平原等污染高值区均与地面观测对应较好。   相似文献   

饱和土体中空沟对移动荷载被动隔振的 2.5D边界元法分析   总被引：1，自引：1，他引：0  

徐斌  雷晓燕  徐满清  刘林芽 《岩土力学》2012,33(4):1079-1086

根据饱和土Biot理论及移动荷载特性,采用积分变换方法,推导了半无限饱和土体频域-波数内的边界积分方程,讨论了2.5D边界积分方程中Cauchy的奇异性,并分析了空沟对移动荷载引起饱和土体振动的被动隔振效果。通过与已知文献结果比较,验证了算法的正确性。数值结果表明,采用2.5D BEM不仅可以解决具有复杂表面的移动荷载作用下动力响应问题,而且可极大减小计算工作量。对于饱和土体受高速移动荷载作用,空沟更能有效减小土体孔压、竖向位移的振幅;当荷载速度较小时,空沟对土体表面的水平向位移几乎不起衰减作用,甚至有放大效应。另外,随空沟距振源的距离增大,空沟能够更好阻隔土体表面波传播。  相似文献   

Influence of Uneven Trace Spacing on Rayleigh Wave Dispersion     

张双喜  李孟奎 《中国地质大学学报(英文版)》2011,(2)

Rayleigh wave dispersion signals are significant to underground investigation.Tradition-ally,uniformed trace spacing is employed in surface wave surveys.In some cases,however,uneven trace spacing is often encountered because of the limitations of the site condition.In order to study the influence of uneven trace spacing on the dispersion data construction of Rayleigh waves,data acquisi-tion is performed based on a 2.5D field layout with a linear array of geophones fixed and a mobile source.The observation d...  相似文献   

2.5-D DC Resistivity Modeling Considering Flexibility and Accuracy     

汤井田  王飞燕  肖晓  张林成 《中国地质大学学报(英文版)》2011,(1)

We highlighted the flexibility of using unstructured mesh together with the local refinement by a resistivity model with complicated topography. The effect of topography is emphasized. Based on this, we calculated a specific class of layered models and found that the accuracy is not always satisfactory by utilizing the standard approach. As an improvement, we employed the layered earth as the reference model to calculate the wavenumbers. The comparison demonstrates that the accuracy is considerably improved...  相似文献