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81.
贵阳地表水—地下水的硫和氯同位素组成特征及其污染物示踪意义 总被引:5,自引:0,他引:5
喀斯特地表水和地下水的交换活跃,地下水系统容易受到地表污染物的污染。为了解喀斯特城市地表水—地下水系统污染特征和污染物质来源,对贵阳市地表水、地下水、雨水和城市排污污水的硫同位素和氯同位素组成变化进行了研究。贵阳市不同类型水体的δ37Cl值在-4.07‰~+2.03‰之间变化,δ34SSO4值变化为-20.4‰~+20.9‰。大气输入物质和城市排污污水的δ37Cl、δ34S及Cl-/SO42-比值与地表水和地下水的不同,稳定硫和氯同位素的结合研究为示踪地下水污染物来源提供了有效研究手段。贵阳市地下水中的Cl-和SO42-至少有4种来源,人为活动通过城市排污和大气输入向地下水系统大量输入了硫酸盐和氯离子。 相似文献
82.
83.
Based on the theory of thermal conductivity, in this paper we derived a formula to estimate the prolongation period (AtL) of cooling-crystallization process of a granitic melt caused by latent heat of crystallization as follows:△tL=QL×△tcol/(TM-TC)×CP where TM is initial temperature of the granite melt, Tc crystallization temperature of the granite melt, Cp specific heat, △tcol cooling period of a granite melt from its initial temperature (TM) to its crystallization temperature (Tc), QL latent heat of the granite melt.
The cooling period of the melt for the Fanshan granodiorite from its initial temperature (900℃) to crystallization temperature (600℃) could be estimated -210,000 years if latent heat was not considered. Calculation for the Fanshan melt using the above formula yields a AtL value of -190,000 years, which implies that the actual cooling period within the temperature range of 900°-600℃ should be 400,000 years. This demonstrates that the latent heat produced from crystallization of the granitic melt is a key factor influencing the cooling-crystallization process of a granitic melt, prolongating the period of crystallization and resulting in the large emplacement-crystallization time difference (ECTD) in granite batholith. 相似文献
The cooling period of the melt for the Fanshan granodiorite from its initial temperature (900℃) to crystallization temperature (600℃) could be estimated -210,000 years if latent heat was not considered. Calculation for the Fanshan melt using the above formula yields a AtL value of -190,000 years, which implies that the actual cooling period within the temperature range of 900°-600℃ should be 400,000 years. This demonstrates that the latent heat produced from crystallization of the granitic melt is a key factor influencing the cooling-crystallization process of a granitic melt, prolongating the period of crystallization and resulting in the large emplacement-crystallization time difference (ECTD) in granite batholith. 相似文献
84.
Benthic nutrient fluxes in the intertidal flat within the Changjiang (Yangtze River) Estuary 总被引:1,自引:0,他引:1
GAO Lei LI Daoji WANG Yanming YU Lihua KONG Dingjiang LI Mei LI Yun and FANG Tao State Key Laboratory of Marine Geology Tongji University Shanghai China State Key Laboratory of Estuarine Coastal Research East China Normal University Shanghai China 《中国地球化学学报》2008,27(1):58-71
In an annual cycle from March 2005 to February 2006, benthic nutrient fluxes were measured monthly in the Dongtan intertidal flat within the Changjiang (Yangtze River) Estuary. Except for NH4^+, there always showed high fluxes from overlying water into sediment for other four nutrients. Sediments in the high and middle marshes, covered with halophyte and consisting of macrofauna, demonstrated more capabilities of assimilating nutrients from overlying water than the low marsh. Sampling seasons and nutrient concentrations in the overlying water could both exert significant effects on these fluxes. Additionally, according to the model provided by previous study, denitrification rates, that utilizing NO3- transported from overlying water (Dw) in Dongtan sediments, were estimated to be from -16 to 193 μmol·h^-1·m^-2 with an average value of 63 μmol·h^-1·m^-2 (n=18). These estimated values are still underestimates of the in-situ rates owing to the lack of consideration of DN, i.e., denitrification supported by the local NO3^- production via nitrification. 相似文献
85.
Christoph Förste Roland Schmidt Richard Stubenvoll Frank Flechtner Ulrich Meyer Rolf König Hans Neumayer Richard Biancale Jean-Michel Lemoine Sean Bruinsma Sylvain Loyer Franz Barthelmes Saskia Esselborn 《Journal of Geodesy》2008,82(6):331-346
The recent improvements in the Gravity Recovery And Climate Experiment (GRACE) tracking data processing at GeoForschungsZentrum
Potsdam (GFZ) and Groupe de Recherche de Géodésie Spatiale (GRGS) Toulouse, the availability of newer surface gravity data
sets in the Arctic, Antarctica and North-America, and the availability of a new mean sea surface height model from altimetry
processing at GFZ gave rise to the generation of two new global gravity field models. The first, EIGEN-GL04S1, a satellite-only
model complete to degree and order 150 in terms of spherical harmonics, was derived by combination of the latest GFZ Potsdam
GRACE-only (EIGEN-GRACE04S) and GRGS Toulouse GRACE/LAGEOS (EIGEN-GL04S) mean field solutions. The second, EIGEN-GL04S1 was
combined with surface gravity data from altimetry over the oceans and gravimetry over the continents to derive a new high-resolution
global gravity field model called EIGEN-GL04C. This model is complete to degree and order 360 and thus resolves geoid and
gravity anomalies at half- wavelengths of 55 km at the equator. A degree-dependent combination method has been applied in
order to preserve the high accuracy from the GRACE satellite data in the lower frequency band of the geopotential and to form
a smooth transition to the high-frequency information coming from the surface data. Compared to pre-CHAMP global high-resolution
models, the accuracy was improved at a spatial resolution of 200 km (half-wavelength) by one order of magnitude to 3 cm in
terms of geoid heights. The accuracy of this model (i.e. the commission error) at its full spatial resolution is estimated
to be 15 cm. The model shows a reduced artificial meridional striping and an increased correlation of EIGEN-GL04C-derived
geostrophic meridional currents with World Ocean Atlas 2001 (WOA01) data. These improvements have led to select EIGEN-GL04C
for JASON-1 satellite altimeter data reprocessing.
Electronic Supplementary Material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
86.
北京市土壤Hg污染的区域生态地球化学评价 总被引:8,自引:1,他引:7
城市土壤Hg异常/污染是中国普遍存在的重大生态环境问题。文章对北京市近1000km2范围内的地表土壤、壤中气、大气干湿沉降、大气颗粒物、大气中的Hg含量水平和空间分布模式进行了系统研究,查明北京地表土壤Hg平均含量为0.41mg/kg,大气干湿沉降物中的Hg平均含量为0.194mg/kg,壤中气Hg的平均含量为559.65ng/m3,大气颗粒物PM10和PM2.5中的Hg含量分别为0.59和0.67ng/m3,大气中的Hg平均含量为3.13ng/m3。北京市自2000年起实现了由燃煤转变为燃气的减排措施,导致干湿沉降物中的Hg沉降通量显著减少,2006年大气干湿沉降物中Hg的沉降通量1.837mg·m-2·a-1,北京市城区(近1000km2)Hg全年沉降为1837kg,空气中总Hg浓度由1998年的8.3~24.7ng/m3下降到2006年的3.13ng/m3,大气颗粒物中Hg含量由2003年的1.18ng/m3下降到2006年的0.59ng/m3(PM10)和0.67ng/m3(PM2.5),表明北京市煤改气减排措施的实施显著改善了大气环境质量。通过对土壤中Hg的存在形式研究,发现土壤中有硫化物(辰砂)及各种Hg盐(HgCl2)的含Hg矿物,Hg也可以各种吸附方式或壤中气方式存在。研究证实北京壤中气Hg与大气Hg存在显著的相关性(n=131,R=0.267,p<0.01),表明壤中气Hg是大气Hg的重要来源之一。利用2005年地表土壤总Hg与Hg释放速率的线性方程估算,土壤Hg平均释放速率为102.42ng·m-2·h-1,2005年土壤释放进大气的Hg通量为936.70kg。在查明土壤中存在大量辰砂矿物的同时,还分布有大量具有高温熔融特征的金属微球粒和玻璃质微球粒,证明燃煤和冶金烟尘是地表土壤Hg的主要来源。土壤中Hg、S、pH和辰砂颗粒浓度在空间上的高度耦合性表明,碱性条件下,土壤中高含量的S和Hg是辰砂形成的重要原因。按国家土壤环境质量标准,北京市I级土壤Hg环境质量的面积为176km2,Ⅱ级为808km2,Ⅲ级为24km2,超Ⅲ为36km2。Ⅲ级、超Ⅲ级主要分布在二环路以内的中心城区。城南(长安街为界)大气Hg环境质量明显优于城北,在北四、北五环之间的部分地区,大气颗粒Hg的环境质量为Ⅲ级或超Ⅲ级。在地表土壤Hg含量较高的中心城区,居民每天因呼吸摄入的Hg高达364ng,对人体健康构成潜在风险。根据我国"十一五"规划中每年实现10%节能减排的目标,对北京市未来50年土壤Hg含量的时空演变趋势预测,预测2050年北京因干湿沉降带来的Hg输入量为16.03kg,地表土壤释放Hg的输出量为37.36kg,明显大于Hg的输入通量,土壤Hg的环境质量将得到根本改善。预测到2040年Ⅲ级土壤Hg环境质量的区域将完全消失,到2060年以Ⅰ级土壤为主。 相似文献
87.
Sukanta Roy Labani Ray Anurup Bhattacharya R. Srinivasan 《International Journal of Earth Sciences》2008,97(2):245-256
The Late Archaean Closepet Granite batholith in south India is exposed at different crustal levels grading from greenschist
facies in the north through amphibolite and granulite facies in the south along a ∼400 km long segment in the Dharwar craton.
Two areas, Pavagada and Magadi, located in the Main Mass of the batholith, best represent the granitoid of the greenschist
and amphibolite facies crustal levels respectively. Heat flow estimates of 38 mW m−2 from Pavagada and 25 mW m−2 from Magadi have been obtained through measurements in deep (430 and 445 m) and carefully sited boreholes. Measurements made
in four boreholes of opportunity in Pavagada area yield a mean heat flow of 39 ± 4 (s.d.) mW m−2, which is in good agreement with the estimate from deep borehole. The study, therefore, demonstrates a clear-cut heat flow
variation concomitant with the crustal levels exposed in the two areas. The mean heat production estimates for the greenschist
facies and amphibolite facies layers constituting the Main Mass of the batholith are 2.9 and 1.8 μW m−3, respectively. The enhanced heat flow in the Pavagada area is consistent with the occurrence of a radioelement-enriched 2-km-thick
greenschist facies layer granitoid overlying the granitoid of the amphibolite facies layer which is twice as thick as represented
in the Magadi area. The crustal heat production models indicate similar mantle heat flow estimates in the range 12–14 mW m−2, consistent with the other parts of the greenstone-granite-gneiss terrain of the Dharwar craton. 相似文献
88.
89.
90.
Carsten Blindauer Vladimir Rozanov John Philip Burrows 《Journal of Atmospheric Chemistry》1996,24(1):1-21
The accurate radiative transfer model GOMETRAN, initially designed to yield radiances at TOA in the wavelength range 240–790 nm, has been extended to allow for the computation of actinic fluxes down to 175 nm and for the calculation of photolysis frequencies in the atmosphere. The capability of the extended model PHOTOGT (PHOTOGOMETRAN) is demonstrated in a number of successful comparison studies both with recent experiments (ground-based, balloonborne, airborne) and model calculations of radiances, actinic fluxes and photolysis frequencies in the stratosphere and troposphere. In an atmospheric case study, the impact of new quantum yield data for the O3 » O2+O(1
d) photodissociation channel on the photolytic production of O(1
d) atoms in the lower atmosphere has been quantified. 相似文献