Impact of Taihu Lake on City Ozone in the Yangtze River Delta     

Liang ZHANG  Bin ZHU  Jinhui GAO  Hanqing KANG 《大气科学进展》2017,34(2):226-234

The lake-breeze at Taihu Lake generates a different specific heat capacity between the water body and the surrounding land. Taihu Lake has a significant impact on the atmospheric conditions and the air quality in the Yangtze River Delta. This phenomenon is referred to as the Taihu Lake effect. In this study, two simulations were conducted to determine the impact of the Taihu Lake effect in the reference experiment(R-E) and sensitivity experiments(NO TH). The control simulations demonstrated that the meteorological field and the spatial distribution of ozone(O3) concentrations over Taihu lake obviously changed once the land-use type of water body was substituted by cropland. The surface temperature of Taihu Lake was reduced under the impact of Taihu Lake, and a huge temperature difference caused a strong lake-breeze effect. The results also showed that the difference in the average concentrations of O3 between the R-E and NO TH experiments reached 12 ppbv in most areas of Taihu Lake, all day, on 20 May 2014. During daytime(0800–1600 LST, LST=UTC+8), the influence of the Taihu Lake effect on O3 in the Suzhou region was not significant. However, the influence of the Taihu Lake effect on O3 in the Suzhou region was obvious during nighttime(1800–2400 LST). The larger changes in the physical and chemical processes were horizontal and vertical advections under the influence of the Taihu Lake effect in Taihu Lake.  相似文献   

北半球中纬度地区上层臭氧变化的合成分析研究   总被引：1，自引：1，他引：0  

陈辉 《气候与环境研究》1998,3(2):158-162

应用逆转方法（C）,对北半球中纬度地区8个观测质量较好的O3地面站的近30年地面遥感逆转资料进行标准处理。采用合成分析方法,对中纬度带上层O3进行了分析研究,发现上层O3总的长期演变趋势较为平坦,仅80年代初及90年代初在36km以上层O3含量有突降现象。这可能与EL Chichon大火山焊发和Pinatubo大火山爆发有较大关系。此外。在上层O3含量的长期演变过程中,还可看到准11年周期,并证实28～36km层及36km以上层O3含量季节变化位相相反。本研究结果可能对南极O3洞的形成机制及近年来O3层变浅薄的机制的认识提供依据并产生影响。    相似文献   

Observation of Filterable Bromine Variabilities During Arctic Tropospheric Ozone Depletion Events in High (1hour) Time Resolution     

U. Langendörfer  E. Lehrer  D. Wagenbach  U. Platt 《Journal of Atmospheric Chemistry》1999,34(1):39-54

The halogen ions Br^- and Cl^- together with NO₃ ^-, SO₄ ⁼, MSA^- (methane sulfonate), Na⁺ and NH₄ ⁺ were analysed by ion chromatography in extracts of more than 800 aerosol cellulose filter samples taken at Ny Ålesund, Svalbard (79°N, 12°E) in spring 1996 (March 27 - May 16) within the European Union project ARCTOC (Arctic Tropospheric Ozone Chemistry). Anticorrelated variations between f-Br (filterable bromine, i.e. water soluble bromine species that can be collected by aerosol filters) and ozone within the arctic troposphere were evaluated at a resolution of 1 or 2 hours for periods with depleted ozone and 4 hours at normal ozone. A mean f-Br concentration of 11 ng m^-3 (0.14 nmol m^-3) was observed for the whole campaign, while maximum concentrations of 80 ng m^-3 (1 nmol m^-3) were detected during two total O₃-depletion events (O₃ drop to mixing ratios below the detection limit of < 2 ppb). Anticorrelation between f-Br and O₃ was also seen during minor O₃-depletion episodes (sudden drop in O₃ by at least 10 ppb, but O₃ still exceeding the detection limit) and even for ozone variations near its background level (40-50 ppb). A time lag of about 10 hours between the change of ozone and of f-Br concentrations could only be found during a total ozone depletion event, when f-Br reached its maximum values several hours after ozone was totally destroyed. Bromine oxide (BrO) concentrations, measured by DOAS (Differential Optical Absorption Spectroscopy), and f-Br showed a coincident variability during almost the entire campaign (except in the case of total O₃-loss). Frequently enhanced anthropogenic nitrate and sulphate concentrations were observed during O₃-depletion periods. At O₃ concentrations < 10 ppb sulphate and nitrate exceed their typical mean level by 54% and 77%, respectively. This may indicate a possible connection between acidity and halogen release.  相似文献   

预测大气臭氧含量变化趋势的一种分析方法     

柳燕 《地球物理学进展》1999,14(1):115-122

本文探索了在预测臭氧含量演变趋势的一种分析方法,该方法将臭氧总量分为三到五个状态,并用状态间的转移频率近似地代替状态间的转移概率,预测其最大可能的变化方向,并给出了具体的应用实例。  相似文献   

青藏高原环境气象研究进展   总被引：7，自引：1，他引：6  

高登义  周立波 《地球物理学进展》1999,14(3):17-28

近十年来,青藏高原环境气象研究进展迅速,无论是观测研究还是理论研究方面均有新的发现。周秀骥和邹捍等先后发现夏季青藏高原上空的臭氧低值中心并提出了产生这种低值中心的可能原因。高登义等利用１９７５年以来对珠穆朗玛峰北坡水环境的监测资料,分析研究后发现,１９９０￣１９９１年爆发的中东战争油田燃烧曾污染了珠峰地区的水环境,带来珠峰北坡绒布河水十三种化学元素含量的剧烈增加,比其前后各年增加了５￣７倍。  相似文献   

北太平洋上空臭氧总量长期变化趋势及其影响因素分析          下载免费PDF全文

韩爽爽  黄富祥  陈希  夏学齐 《地球物理学报》2016,59(11):3974-3984

本文基于1979—2014年臭氧总量的卫星遥感数据,利用多元线性回归模型对臭氧总量数据序列进行模拟计算,考察了北太平洋上空臭氧总量长期变化趋势及其影响因素的作用.结果表明,北太平洋地区大气臭氧总量长期变化呈现减少趋势,但是减少速率随季节和纬度带表现出差异性,在各纬度带臭氧峰值季节臭氧下降趋势最为显著.在0°—15°N地区臭氧高值出现在夏秋季节并在8月达到峰值,峰值月份臭氧年均下降率约为0.2DU/a;15°—30°N亚热带地区臭氧高值出现在春夏季并在5月达到峰值,峰值月份臭氧年均下降速率约为0.22DU/a;而在30°—45°N中纬度地区臭氧高值出现在冬春季并在2月达到峰值,峰值月份臭氧年均下降率0.75DU/a.在臭氧分布年平均态基础上,影响臭氧总量分布变化的因素主要有臭氧损耗物质(EESC)、太阳辐射周期(Solar)、准两年振荡(QBO)和厄尔尼诺-南方涛动(ENSO)等.其中,EESC导致臭氧损耗效应随着纬度升高而增大,在从低到高的三个纬度带损耗最大值分别为11DU、16DU和66DU;Solar增强导致臭氧增加,在三个纬度带的增加效应最大值分别为16DU、17DU和19DU;QBO@10hPa和QBO@30hPa对臭氧影响幅度基本在±10DU内波动,只有QBO@10hPa对30°—45°N区域的影响作用达到14DU,值得注意的是QBO影响作用随着纬度变化存在相位差异,在0°—15°N区域臭氧变化与QBO呈现相同相位,而在15°—30°N和30°—45°N区域臭氧变化与QBO呈现相反相位;ENSO对各个纬度带臭氧影响幅度也在±10DU内,ENSO影响作用在不同纬度带也存在相位差异,臭氧总量变化在0°—15°N、15°—30°N区域与ENSO相位相反,在30°—45°N区域与ENSO相位一致.  相似文献   

近30年北半球冬季臭氧总量分布特征及其与平流层温度的关系   总被引：6，自引：1，他引：5       下载免费PDF全文

李刚  谭言科  李崇银  陈书驰  白涛  杨道勇  张滢 《地球物理学报》2015,58(5):1475-1491

臭氧的时空分布特征对气候和环境变化具有显著影响,随着臭氧资料数量的增加和质量的提高,有必要对臭氧时空分布特征及其与气候变化的关系进行详细研究.本文利用欧洲中期天气预报中心提供的1979—2013年的全球月平均臭氧总量资料、平流层温度场资料,采用旋转经验正交函数分解(REOF)、Morlet小波分析、合成分析等方法研究了20°N以北的北半球冬季(12—2月)臭氧总量异常的主要空间分布结构与时间演变特征,并进一步分析了主要模态与平流层上层(2hPa)、中层(30hPa)以及下层(100hPa)温度异常的关系.结果表明:近30年北半球冬季臭氧总量异常变化最显著的区域主要有5个,分别位于极地地区(75°N—90°N,0°—360°)、北半球副热带地区(20°N—40°N,0°—360°)、阿拉斯加地区(60°N—75°N,180°—260°E)、北大西洋地区(45°N—60°N,310°E—360°E)及西伯利亚地区(50°N—65°N,80°E—130°E).5个区域的冬季臭氧总量异常具有明显的年际和年代际变化特征.1980年代后期是各个区域的臭氧总量异常由年代际偏多转为偏少的转换时段.此外,各区域存在显著的年际变化周期,而且各个区域的年际周期存在明显的差异.臭氧总量异常变化与平流层温度异常变化的关系表明,臭氧总量异常的增加(减少)能够导致平流层上层温度异常偏冷(暖)和平流层中、下层温度异常偏暖(冷),其中平流层中层温度异常的偏暖(冷)程度要比下层更加明显.  相似文献   

A numerical study of tropospheric ozone in the springtime in East Asia   总被引：11，自引：0，他引：11  

ZHANG Meigen  XU Yongfu  Itsushi UNO  Hajime AKIMOTO 《大气科学进展》2004,21(2):163-170

The Models-3 Community Multi-scale Air Quality modeling system (CMAQ)coupled with the Regional Atmospheric Modeling System (RAMS)is applied to East Asia to study the transport and photochemical transformation of tropospheric ozone in March 1998．The calculated mixing ratios of ozone and carbon monoxide are compared with ground 1evel observations at three remote sites in Japan and it is found that the model reproduces the observed features very well．Examination of several high episodes of ozone and carbon monoxide indicates that these elevated levels are found in association with continental outflow,demonstrating the critical role of the rapid transport of carbon monoxide and other ozone precursors from the continental boundary layer．In comparison with available ozonesonde data,it is found that the model-calculated ozone concentrations are generally in good agreement with the measurements,and the stratospheric contribution to surface ozone mixing ratios is quite limited．  相似文献   

塔克拉玛干沙漠腹地冬季大气边界层O3廓线分析   总被引：3，自引：2，他引：1  

何清  刘强  杨兴华  艾力·买买提明  霍文  梁云 《中国沙漠》2010,30(4):909-916

为了揭示塔克拉玛干沙漠腹地冬季大气边界层O3的浓度变化特征,利用系留气艇于2008年1月18—25日在塔中地区进行了大气边界层O3观测试验,结合相关资料,初步分析了塔中地区冬季边界层O3浓度垂直分布特征及其与温度、湿度的关系。其结果是:①塔中地区臭氧浓度集中分布在10~50 ppb之间,其中试验期间观测到O3最大浓度值56.1 ppb,最小浓度为2.6 ppb,臭氧的最大浓度基本都在40 ppb左右,日平均浓度为34.4 ppb。②大气边界层O3的浓度廓线可分为峰值型、均匀型、增长型3种,其中均匀型所占比重最大。③大气边界层O3浓度与温度、湿度密切相关,逆温及空气中水汽的增加会导致臭氧浓度降低。④大气边界层O3有明显的日变化,越贴近地面日变化越明显,其变化特征与太阳辐射有着密切关系。臭氧浓度夜晚较低,日出后开始增加,午后达到一天中的最大值;随着日落,臭氧浓度开始减小,在清晨达到最小值;臭氧浓度日最大值出现在17:00,最小值出现在08:00。  相似文献   

Multi-scale variation characteristics of polar vortex at 10 hPa in the Southern Hemisphere     

LiPing Li  JuHui M  PanXing Wang  Dong Guo  MingKen Duan  ShuXuan Guan 《寒旱区科学》2010,2(1):0073-0081

By use of 1948-2007 NCEP/NCAR reanalysis monthly geopotential data, a set of circulation indices are defined to characterize the polar vortex at 10 hPa in the Southern Hemisphere, including area-(S), intensity-(P) and centre position-(λc , φc) indices. Sea-sonal variation, interannual anomalies and their possible causes of 10 hPa polar vortex in the Southern Hemisphere are analyzed by using these indices, the relationship between 10 hPa polar vortex strength and the Antarctic Oscillation are analyzed as well. The results show that: (1) the polar region at 10 hPa in the Southern Hemisphere is controlled by anticyclone (cyclone) from Dec. to Jan. (from Mar. to Oct.), Feb. and Nov. are circulation transition seasons. (2) Intensity index (P) and area index (S) of anticy-clone (cyclone) in Jan. (Jul.) show a significant spike in the late 1970s, the anticyclone (cyclone) enhances (weakens) from ex-tremely weak (strong) oscillation to near the climatic mean before a spike, anticyclone tends to the mean state from very strong oscillation and cyclone oscillates in the weaker state after the spike. (3) There is significant interdecadal change for the anticyclone center in Jan., while markedly interannual variation for cyclone center in July. (4) The ozone anomalies can cause the interannual anomaly of the polar anticyclone at 10 hPa in the Southern Hemisphere in Jan. (positive correlation between them), but it is not related to the polar cyclone anomalies. (5) There is notable negative correlation between the polar vortex intensity index P and the Antarctic Oscillation index (AAOI), thus AAOI can be represented by P.  相似文献