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The photocatalytic decolorization and mineralization of Reactive Black 5 (RB5) dye in presence of TiO2 Degussa P25 has been studied using artificial light radiation in a shallow pond slurry reactor. The equilibrium adsorption of dye, influence of pH (3–11), catalyst load (0.5–3.0 g/L), and dye concentration (20–100 mg/L) on decolorization kinetics were studied. The effect of area to volume ratio of photoreactor on decolorization kinetics has been also studied. Mineralization studies were performed at optimized conditions of pH (3) and catalyst load (1.5 g/L). The maximum adsorption (26.5 mg/g) of dye was found to occur at pH 3. The apparent pseudo first order decolorization rate constant (kapp) value followed the order pH 3 > pH 11 > pH 9 > pH 7. As compared to available literature reduction in total organic carbon (TOC) was minimal by the time there was complete decolorization. Initial reduction in TOC was followed by subsequent increasing trend till complete decolorization. Final decreasing trend in TOC was observed only after complete decolorization. Twelve hours of treatment under experimental conditions reduced TOC content by 70% only. Discussion of results suggest that photocatalytic treatment of colored effluent under low UV intensity, and low A/V ratio may result in completely decolorized effluent but still having high COD. 相似文献
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Four bacterial isolates (two resistant and two sensitive to chromium) were isolated from soil contaminated with tannery effluents at Jajmau (Kanpur), India, and were identified by 16S rDNA gene sequencing as Stenotrophomonas maltophilia, Exiguobacterium sp., Pantoea sp., and Aeromonas sp. Biosorption of chromium by dried and living biomasses was determined in the resistant and sensitive isolates. The effect of pH, initial metal concentration, and contact time on biosorption was studied. At pH 2.5 the living biomass of chromium resistant isolate Exiguobacterium sp. ZM‐2 biosorbed maximum amount of Cr6+ (29.8 mg/g) whereas the dried biomass of this isolate biosorbed 20.1 mg/g at an initial concentration of 100 mg/L. In case of chromate sensitive isolates, much difference was not observed in biosorption capacities between their dried and living biomasses. The maximum biosorption of Cr3+ was observed at pH 4.5. However, biosorption was identical in resistant and sensitive isolates. The data on chromium biosorption were analyzed using Langmuir and Freundlich isotherm model. The biosorption data of Cr6+ and Cr3+ from aqueous solution were better fitted in Langmuir isotherm model compared to Freundlich isotherm model. Metal recovery through desorption was observed better with dried biomasses compared to the living biomasses for both types of chromium ions. Bioaccumulation of chromate was found higher in chromate resistant isolates compared to the chromate sensitive isolates. Transmission electron microscopy confirmed the accumulation of chromium in cytoplasm in the resistant isolates. 相似文献
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Quantifying preferential flow in soils: A review of different techniques 总被引：19，自引：0，他引：19
Preferential flow (PF) in soil has both environmental and human health implications since it favours contaminant transport to groundwater without interaction with the chemically and biologically reactive upper layer of soil. PF is, however, difficult to measure and quantify. This paper reviews laboratory and field techniques, such as breakthrough curves, dye tracing, and scanning techniques, for evaluating PF in soil at different scales. Advanced technologies, such as scanning techniques, have increased our capability to quantify transport processes within the soil with minimal soil disturbance. Important issues with respect to quantifying PF concern large-scale studies, frozen soil conditions, tracing techniques for particles and gases, a lack of simple mathematical tools for interpreting field data, and the lack of a systematic approach for comparing PF data resulting from different measurement techniques. Also, more research is required to quantify the relative importance of the various PF processes that occur in soil rather than the integrated result of all PF processes in soils. 相似文献
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Surface water/groundwater interaction in the Piora Aquifer,Switzerland: evidence from dye tracing tests 总被引：5，自引：2，他引：3
Martin?H.?OtzEmail author Heinz?K.?Otz Ines?Otz Donald?I.?Siegel 《Hydrogeology Journal》2003,11(2):228-239
Results of seven dye tracing tests done from 1993–1997 to investigate the extent to which lakes and surface water interact
with the underlying Triassic Piora Aquifer, Switzerland, are reported here. Two of the dye tracing tests showed that groundwater
flows in the Piora Aquifer from the Piora Valley to springs in the adjacent Santa Maria Valley, and even further east to the
di Campo Valley considerably outside of the Piora Valley surface water divide.
Lake Ritom located in the Piora Valley loses water only to the Canaria Valley outside of the lake's surface-water watershed
at the lake's western margin when lake levels are above 1,835 m above sea level. Dye tracing tests show that a major sinkhole
in the Piora Valley, Calderoni Sinkhole, is located precisely on the water divide where subsurface flow in the Piora Valley
and surface water diverge and move in opposite directions. The dye tracing results also showed no hydraulic connection between
surface water in the Piora Valley and the famous Pertusio Spring, located in the upper Santa Maria Valley. Only a small amount
of dye from the two dye tracing tests done in 1993 and 1997 entered an exploratory gallery built to test the viability of
the AlpTransit tunnel, being built in competent rock under the Triassic Piora Aquifer, effectively perched above.
Electronic Publication 相似文献
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Occurrence of priority pollutants in WWTP effluents and Mediterranean coastal waters of Spain 总被引：1，自引：0，他引：1
A comprehensive study aimed at evaluating the occurrence, significance of concentrations and spatial distribution of priority pollutants (PPs) along the Comunidad Valenciana coastal waters (Spain) was carried out in order to fulfil the European Water Framework Directive (WFD). Additionally, PP concentrations were also analysed in the effluent of 28 WWTPs distributed along the studied area. In coastal waters 36 organic pollutants of the 71 analysed, including 26 PPs were detected although many of them with low frequency of occurrence. Only 13 compounds, which belong to four different classes (VOCs, organochlorinated pesticides, phthalates and tributyltin compounds (TBT)) showed a frequency of occurrence above 20% in coastal waters. In the results obtained until now, octylphenol, pentachlorobenzene, DEHP and TBT exceeded the annual average concentration (EQS-AAC), and only TBT surpassed the maximum allowable concentration (EQS-MAC). The most frequent contaminants determined in coastal waters were also present in WWTP effluents. 相似文献
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Mohammad Ali Zanjanchi Hassan Sajjadi Majid Arvand Ali Mohammad‐Khah Bahram Ghalami‐Choobar 《洁净——土壤、空气、水》2011,39(11):1007-1013
The potential of MCM‐41 for the removal of cationic dyes from water solution was evaluated using sodium dodecyl sulfate (SDS) for the surface modification of this mesoporous material. Admicelle structures formed on the surface of the calcined MCM‐41 are capable of removing organic pollutants and cationic species from water environment. The structural, textural, and surface chemical characteristics of the prepared SDS‐modified MCM‐41 (SDS‐MCM‐41) were studied. The adsorption capacity of SDS‐MCM‐41 was evaluated for methylene blue (MB) as a target cationic dye. Equilibrium adsorption isotherm data were manipulated employing nonlinear regression analysis. The Langmuir, Freundlich, and Sips isotherm models were examined. The adsorption data were well fitted to both Langmuir and Sips isotherm models. The maximum adsorption capacity of SDS‐MCM‐41 for MB, based on Langmuir and Sips models, were 290.8 and 297.3 mg g?1, respectively. Ethanol was found to be an effective solvent for partial regeneration of the adsorbent. 相似文献