In situ cosmogenic Be in olivines and pyroxenes     

P.-H. Blard  D. Bourls  R. Pik  J. Lav 《Quaternary Geochronology》2008,3(3):196-205

This study proposes an efficient new cleaning procedure for measuring in situ cosmogenic ¹⁰Be in olivines and pyroxenes. This chemical routine is specially designed to decontaminate the abundant meteoric ¹⁰Be from these minerals. The method was tested on mafic minerals from basaltic flows of Mt. Etna volcano and from Hawaiian flows and moraines. A sequential dissolution test shows that ¹⁰Be concentrations decrease with the number of cleaning steps until reaching a constant value. This is a necessary condition to demonstrate the efficiency of the method in properly decontaminating samples of meteoric ¹⁰Be. Moreover, cross-calibration with cosmogenic ³He measured within the same samples yielded a sea level high-latitude production rate of 4.5±0.4 at g⁻¹ a⁻¹ for cosmogenic ¹⁰Be in mafic minerals. This rate is within 1σ uncertainty of empirically or model-derived rates for ¹⁰Be on the same targets. Such concordance supports the consistency of the new method.  相似文献   

The crater lake and hydrothermal system of Mount Pinatubo,Philippines: evolution in the decade after eruption     

James?A.?StimacEmail author  Fraser?Goff  Dale?Counce  Adrienne?C.?L.?Larocque  David?R.?Hilton  Uwe?Morgenstern 《Bulletin of Volcanology》2004,66(2):149-167

The June 1991 eruption of Mount Pinatubo, Philippines breached a significant, pre-eruptive magmatic-hydrothermal system consisting of a hot (>300 °C) core at two-phase conditions and surrounding, cooler (<260 °C) liquid outflows to the N and S. The eruption created a large, closed crater that accumulated hydrothermal upwellings, near-surface aquifer and meteoric inflows. A shallow lake formed by early September 1991, and showed a long-term increase in level of ~1 m/month until an artificial drainage was created in September 2001. Comparison of the temporal trends in lake chemistry to pre- and post-eruptive springs distinguishes processes important in lake evolution. The lake was initially near-neutral pH and dominated by meteoric influx and Cl–SO₄ and Cl–HCO₃ hydrothermal waters, with peaks in SO₄ and Ca concentrations resulting from leaching of anhydrite and aerosol-laden tephra. Magmatic discharge, acidity (pH~2) and rock dissolution peaked in late 1992, during and immediately after eruption of a lava dome on the crater floor. Since cessation of dome growth, trends in lake pH (increase from 3 to 5.5), temperature (decline from 40 to 26 °C), and chemical and isotopic composition indicate that magmatic degassing and rock dissolution have declined significantly relative to the input of meteoric water and immature hydrothermal brine. Higher concentrations of Cl, Na, K, Li and B, and lower concentrations of Mg, Ca, Fe, SO₄ and F up to 1999 highlight the importance of a dilute hydrothermal contribution, as do stable-isotope and tritium compositions of the various fluids. However, samples taken since that time indicate further dilution and steeper trends of increasing pH and declining temperature. Present gas and brine compositions from crater fumaroles and hot springs indicate boiling of an immature Cl–SO₄ geothermal fluid of near-neutral pH at approximately 200 °C, rather than direct discharge from magma. It appears that remnants of the pre-eruptive hydrothermal system invaded the magma conduit shortly after the end of dome emplacement, blocking the direct degassing path. This, along with the large catchment area (~5 km²) and the high precipitation rate of the area, led to a rapid transition from a small and hot acid lake to a large lake with near-ambient temperature and pH. This behavior contrasts with that of peak-activity lakes that have more sustained volcanic gas influx (e.g., Kawah Ijen, Indonesia; Poas and Rincón de la Vieja, Costa Rica).Editorial responsibility: H. Shinohara  相似文献   

Activation energy for diffusion of helium in water-saturated, compacted Na-montmorillonite     

Tomohiro Higashihara  Tamotsu Kozaki 《Engineering Geology》2005,81(3):365-370

It is important to clarify the migration behavior of hydrogen gas dissolved in water-saturated, compacted bentonite, which is a promising material for geologic disposal of high-level waste and TRU waste disposal. The diffusion coefficients of helium, which can be detected under extremely low background conditions, in water-saturated, compacted Na-montmorillonite were determined as a function of temperature by a transient diffusion method. The activation energies for diffusion of helium were then obtained. The activation energies were from 6.9 ± 4.8 to 19 ± 2.8 kJ mol^− 1 and were regarded to be independent of dry density. The activation energies of helium in water-saturated Na-montmorillonite were roughly equal to those in bulk water, 14.9 kJ mol^− 1, and in ice, from 11 to 13 kJ mol^− 1. It is possible that helium diffuses not only in pore water but also in interlayer water.  相似文献   

Helium, radon and radiocarbon studies on a regional aquifer system of the North Gujarat-Cambay region, India     

Meetu Agarwal  R.D. Deshpande 《Chemical Geology》2006,228(4):209-232

The study reports the age evolution of groundwater as it flows from the recharge area through a regional alluvial aquifer system in North Gujarat-Cambay region in western India. Radiocarbon (¹⁴C), ⁴He and ⁴He / ²²²Rn dating methods have been employed. Sediments from a drill core in the Cambay Basin were also analysed for uranium (U) and thorium (Th) concentrations and the measured values have been used to estimate the ⁴He and ²²²Rn production rate for groundwater age calculations. Additionally, factors controlling the distribution of ²²²Rn, ⁴He and temperature anomalies in groundwater, vis-à-vis their relation to the tectonic framework and lithology of the study area, have also been examined.The multi-isotope study indicated a reasonable correspondence in groundwater age estimates by the three methods employed. The groundwater ¹⁴C ages increased, progressively, in the groundwater flow direction: from the foothills of Aravalli Mountains in the east, and reached a value of ∼35 ka towards the region of lowest elevation, linking Little Rann of Kachchh (LRK)-Nalsarovar (NS)-Gulf of Khambhat (GK) in the western part of the study area. In this region, groundwater ages obtained for free flowing thermal wells and springs employing ⁴He and ⁴He / ²²²Rn systematics are in the order of million years. Such anomalous ages are possibly due to enhanced mobilisation and migration of ‘excess helium’ from hydrothermal circulation vents along deep-seated faults. Excluding such anomalous cases and considering all uncertainties, presently estimated ⁴He and ⁴He / ²²²Rn groundwater ages are in reasonable agreement with ¹⁴C age estimates in the Cambay Basin for helium release factor (Λ_He) value of 0.4 ± 0.3. The ⁴He method also indicated west-southwards progression of groundwater ages up to ∼100 ka beyond the Cambay Basin.Large ‘excess helium’ concentrations are also seen to be generally associated with anomalous groundwater temperatures (> 35 °C) and found to overlie some of the basement faults in the study area, particularly along the east and the west flanks of the Cambay Basin. Groundwater ²²²Rn activities in most of the study area are 800 ± 400 dpm/l. But, a thermal spring at Tuwa on the east flank of the Cambay Basin, having granitic basement at shallow depth, recorded the highest ²²²Rn activity (∼63,000 dpm/l).  相似文献   

Spatial variations in 3He/4He ratios along a high strain rate zone,central Japan     

《Journal of Asian Earth Sciences》2013

A linear zone with high strain rates along the Japan Sea coast, the Niigata-Kobe Tectonic Zone (NKTZ), is considered to be associated with rheological heterogeneities in the lower crust and/or upper mantle. Helium isotope variations along the NKTZ reveal a close association with the geophysical evidence for rheological heterogeneities in the crust and mantle. In the southern NKTZ, the ³He/⁴He ratios lower than 3.4 Ra (Ra denotes the atmospheric ³He/⁴He ratio of 1.4 × 10⁻⁶) could be interpreted as a two-component mixture of helium stored in aqueous fluids driven off the subducting oceanic crust and radiogenic crustal helium. Higher ³He/⁴He ratios are observed in the central NKTZ where Quaternary volcanoes and high-temperature hot springs are concentrated, suggesting that the ³He emanation manifest in the central NKTZ results from the effective transfer of mantle helium by intrusion and degassing of mantle-derived magma in the crust. In the northern NKTZ where two large inland earthquakes occurred recently, there appears to be many samples with ³He/⁴He ratios significantly higher than those observed in the fore-arc side of northeast Japan. A plausible source of mantle helium could be attributed to upward mobilization of aqueous fluids generated by dehydration of the subducting Pacific Plate slab.  相似文献   

http://www.sciencedirect.com/science/article/pii/S1674987112000412     

Arie Lev Gilat  Alexander Vol 《地学前缘(英文版)》2012,3(6)

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Inferences of plasma parameters from coronal hole observations     

Shadia Rifai Habbal 《Astrophysics and Space Science》1996,243(1):49-56

The temperature in the acceleration region of the solar wind remains one of the most elusive parameters to measure. Knowledge of the temperature as well as its gradient in the inner corona is fundamental for placing constraints on physical mechanisms thought to be responsible for the coronal heating process, as well as for understanding the flow properties of the solar wind. Estimates of the helium abundance is essential for understanding the puzzling behavior of heavier ions in the solar wind. As an illustration of the difficulties and uncertainties involved in the inferences of plasma parameters in the wolar wind acceleration region, The inference of electron temperature and helium abundance will be described. Prospects for future observations will be briefly discussed.  相似文献   

Symbolic analytical solutions for the abundances differential equations of the Helium burning phase     

M.I. Nouh  M.A. Sharaf  A.S. Saad 《Astronomische Nachrichten》2003,324(5):432-436

In this paper, a literal analytical solution is developed for the abundances differential equations of the helium burning phase in hot massive stars. The abundance for each of the basic elements ⁴He,¹²C,¹⁶O and ²⁰Ne is obtained as a recurrent power series in time, which facilitates its symbolic and numerical evaluations. Numerical comparison between the present solution and the numerical integration of the differential equations for the abundances show good agreement.  相似文献