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991.
Size-fractionated uranium isotopes in surface waters in the Jiulong Estuary in China 总被引:1,自引:1,他引:0
L E ZHANG Lei CHEN Min QIU Yusheng XING N YANG Weifeng LI Yanping HUANG Yipu 《海洋学报(英文版)》2008,27(1):29-41
Surface water was collected from the Jiulong Estuary for determination of activity concentrations of uranium isotopes in different size fractions, namely, greater than 53, 10 -53, 2 - 10, 0.4 -2 μm, 10 000 u -0.4 μm and less than 10 000 u fractions by microfihration and cross-flow uhrafiltration technologies. Results indicated that most of the dissolved uranium ( 〈 0.4 μm) exis- ted in the low molecular mass fraction ( 〈 10 000 u), and the colloidal uranium-238 (10 000 u -0.4 μm) only contributed less than 1% of the dissolved uranium-238. The fractions of colloidal uranium in the dissolved phases decreased with the increasing sa- linity. A positive linear relationship between uranium-238 activities and salinities was observed for the dissolved, colloidal and low molecular mass fractions, indicating a conservative behavior of uranium in the Jiulong Estuary. In the particulate phases ( 〉 0.4 μm), the partitioning of uranium isotopes among different size fractions was controlled by the partitioning of particle concentrations. In the regions with salinities below 20, the partitioning of uranium-238 among different size fractions was as follows: 10 - 53 μm 〉 2 - 10 μm 〉 0.4 - 2 μm greater than above 53 μm. However, the order at the offshore station with salinities above 30 changed as follows : 0.4 - 2 μm 〉 10 - 53 μm 〉 2 - 10 μm greater than above 53 μm. The fraction of the 0.4 - 2 μm particles increased at the offshore station, suggesting the increased contribution of the authigenic uranium. The activity ratio of uranium-234 to uranium-238 in the dissolved phases, including the low molecular mass fraction and the colloidal fraction, was larger than unity, showing the occurrence of excess uranium-234. In contrast, the activity ratio of uranium-234 to uranium-238 in all size fractions of the particulate phase was close to the equilibrium value (1.0). The observed different values of the activity ratio of uranium-234 to uranium-238 in the dissolved phase and the partic 相似文献
992.
HE Jianhu MA Hao CHEN Liqi XIANG Baoqiang ZENG Xianzhang YIN Mingduan ZENG Wenyi 《海洋学报(英文版)》2008,27(2):21-29
Dissolved and particulate thorium-234, particulate organic carbon in the upper 150 m of water columns from five stations in the Prydz Bay, the Southern Ocean were determined during the 22nd Chinese National Antarctic Research Expedition (from November 2005 to March 2006 ). The disequilibria between thorium-234 and its parent uranium-238 in upper layer was used to derive the averaged residence time of thorium-234, which decreased along with the latitude to the south and a minimum value, 1 - 8 d for particulate thorium-234 and 29 - 48 d for dissolved thorium-234, appeared at the medium latitude station, and the export fluxes of thorium-234 were calculated too and 'a maximum value, 0. 35 -0. 63 Bq/(m^3 · d) for the particulate thorium-234 and 0. 44 -0. 65 Bq/ (m^3 ·d) for the dissolved thorium-234, appeared at the same station. The export fluxes of particulate organic carbon at different water columns were derived by two methods with irreversible scavenging model, and the averaged values were 104. 7 mmol/ ( m2 · d ) ( E method) and 120. 6 mmol/( m2·d ) ( B method ), respectively, indicating that a relatively high new production would exist in summer in the Prydz Bay where it will play a potential significant role in sequestering the absorption CO2 to deeper ocean. 相似文献
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青城子矿田是一个大型金、银多金属综合矿田,矿田内具有(铜)铅锌-银-金的矿化分带现象。从含矿原岩建造-浊积岩建造、变质作用、岩浆作用、韧性剪切作用以及矿质分异作用角度对青城子矿田的矿化分带性做了初步研究,认为青城子矿田的矿化分带性是多种因素造成的。对矿田分带性的研究有利于青城子矿田乃至辽东地区的金、银多金属矿产找矿与勘查。 相似文献
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本文介绍了一种连续监测空气中氡同位素浓度的新技术。与其他方法相比,该技术可直接测量^220Rn、^222Rn衰变的α粒子。 相似文献
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