大气冰核谱对雷暴云微物理过程及起电影响的数值模拟     

王梦旖  谭涌波  师正  刘俊  于梦颖  郑天雪 《高原气象》2019,38(3):593-603

利用已有的二维对流云模式,讨论了三种不同的冰核谱对雷暴云微物理、起电及电荷结构的影响。模拟结果表明:(1)不同的冰核谱环境对雷暴云中冰相粒子的含量及分布具有明显作用。冰核谱的垂直温区越大,产生的冰相粒子分布越广。在冰核浓度较大的个例中,冰晶和霰粒子的含量高,更多的小冰相粒子出现在海拔更高的区域;(2)高温区冰核的数量会对上升气流速度产生显著影响。高温区的冰核越多,冰相粒子在微物理发展过程中释放的潜热越多,上升气流强,对流发展越旺盛;(3)在低温区冰晶浓度高的谱环境个例中,雷暴云中的非感应起电率和感应起电率高,导致起电量增加。高温区冰核多的谱环境,大量冰晶和霰获得正电荷形成次正电荷区,电荷结构呈现三极性;而高温区冰核少的谱环境,参与起电的水成物粒子少,易形成偶极性电荷结构。  相似文献   

冰晶核化对雷暴云微物理过程和起电影响的数值模拟研究   总被引：2，自引：0，他引：2  

谭涌波  杨忆  师正  周博文  张冬冬  廖义慧 《大气科学》2015,39(2):289-302

本文在已有的二维对流云模式中采用了一种与气溶胶有关的冰晶核化方案替代原有的冰晶核化经验公式, 并选取个例, 分别就两种方案进行了模拟对比试验。模拟结果表明:(1)新方案所得冰晶比含水量主要分布在-0.1~-7.6℃温区之间, 高于原方案所得的-50.1~-24.2℃温区;在整个雷暴云的发展过程中新方案冰晶的分布高度、温度区间以及最大浓度值均大于原方案。(2)在新方案中, 温度相对较高的过冷区产生大量冰晶, 其争食云中水汽抑制了云滴、雨滴的增长。此外, 与原方案相比, 霰增长受雨滴大幅减小的影响进一步得到限制, 导致生成的霰小于原方案, 且空间分布具有较大区别。(3)两方案在雷暴云初期形成的电荷结构不同;在发展旺盛与消散阶段新方案中电荷空间分布区域和电荷量均大于原方案, 此外, 在不同时刻主正电荷区和主负电荷区的中心高度存在差异。本文对云微物理过程及起电的分析为后继探讨气溶胶与雷暴云起放电过程、电荷结构之间的相互关系提供了有利条件。  相似文献   

Transmission electron microscopy applied to fluid inclusion investigations   总被引：8，自引：0，他引：8  

Cecilia Viti  Maria-Luce Frezzotti 《Lithos》2001,55(1-4):125-138

The transmission electron microscope (TEM) allows a detailed characterization of textural and chemical features of fluid inclusions (shape, inner compositions and inner textures), at a resolution higher than that attainable with an optical microscope (OM). TEM investigation indicates that most fluid inclusions appear as perfectly euhedral negative crystals, with variable shape (from prismatic to equant) and size (typically from <0.02 to 0.15 μm). Inner texture (fluid phase/melt distribution) and composition are variable as well. Different kinds of negative crystals may coexist in the same trail of inclusions, possibly indicating locally variable trapping conditions.

A critical feature, revealed by TEM, is that inclusions are often connected to structural defects (in particular, to dislocation arrays), which are undetected by optical microscopy. The identification of these hidden nanostructures should be taken into account for the correct petrological interpretation of microthermometric results, particularly when controversial data have been obtained. In fact, these nanostructures may represent a possible path for fluid phase leakage, thus modifying the original composition and/or density of the inclusions.  相似文献   

On the efficiency with which aerosol particles of radius larger than 0.1 μm are collected by simple ice crystal plates     

J. J. Martin  P. K. Wang  H. R. Pruppacher  A. E. Hamielec 《Pure and Applied Geophysics》1980,118(2):1109-1129

A theoretical model is presented which allows computing the efficiency with which aerosol particles of radius 0.1r10 m are collected by simple ice crystal plates of radius 50a _c 640 m in air of various relative humidities, temperatures and pressures. Particle capture due to thermophoresis, diffusiophoresis and inertial impaction are considered. It is shown that the capture efficiency of an ice crystal in considerably affected by phoretic effects in the range 0.1r1 m. For aerosol particles ofr>1 m the efficiency is strongly controlled by the flow field around the crystal and the density of the aerosol material. Trajectory analysis also predicts that aerosol particles are preferentially captured by the ice crystal rim. Our theoretica results are found to agree satisfactorily with the laboratory studies presently available. Comparison shows that for the same pressure, temperature and relative humidity of the ambient air ice crystal plates are better aerosol particle scavengers than water drops.  相似文献   

甘肃省秋季层状云冰雪晶粒子特征个例分析   总被引：3，自引：0，他引：3  

李照荣  李宝梓  庞朝云  杨增梓 《干旱气象》2002,20(3):21-23

利用安装有PMS探头、温湿仪和GPS的飞机 ,对 2 0 0 1年 10月 12日甘肃河西地区降水性层状云进行了探测。根据获取的资料分析了此次降水性层状云的冰雪晶特征 ,包括不同粒子的分布特性 ,给出不同温度下的冰雪晶粒子谱 ,还分析了粒子谱型随温度的变化及其包含的微物理机制。与我国其它地区的冰雪晶浓度比较认为 ,在一定的云水条件下 ,甘肃秋季层状云有较大的增雨催化潜力  相似文献   

Nanoscience and technology: the next revolution in the Earth sciences     

Michael F. Hochella Jr.^{Author Vitae} 《Earth and Planetary Science Letters》2002,203(2):593-605

Nanoscience and technology are not exactly new, but nevertheless rapidly expanding fields that are providing revolutions in all sciences on the scale of what genomics and proteomics have done in recent years for the biological sciences. Nanoscience is based on the fact that properties of materials change as a function of the physical dimension of that material, and nanotechnology takes advantage of this by applying selected property modifications of this nature to some beneficial endeavor. The prefix ‘nano’ is used because the property dependence on physical size is generally observed close to the nanoscale, somewhere around 10⁻⁹ m. The dimensions at which changes are observed depend on the specific material and the property in question, as well as which of the three dimensions are restricted in real space (e.g. small particles vs. thin films vs. ‘one-dimensional’ phases). Properties change in these confined spaces because the electronic structure (i.e. the distribution of electron energies) of the material is modified here in the gray area between the bulk and atomistic/molecular realms, or equivalently between the continuum and strictly quantum domains. Earth materials with at least one dimension in the nanorange are essentially ubiquitous. Many have been known for several decades and more are being discovered all the time. But the scientific emphasis has now shifted to that of measuring, understanding and ultimately predicting the property changes from the bulk to nanodomains, and to the understanding of the significant ways that Earth processes are affected by these changes. In addition, where possible, Earth scientists are using nanoscience to develop nanotechnology that should play important roles in Earth sustainability issues of the future.  相似文献   

Mechanodestruction of minerals at the crack tip (<Emphasis Type="Italic">Overview</Emphasis>): 1. Experiment     

Farit Khisamutdinovich Urakaev 《Physics and Chemistry of Minerals》2007,34(5):351-361

The kinetics of the amount of volatiles emitted from synthetic and natural calcite single crystals while cleaving and grinding are determined using time-of-flight mass spectrometry. It is revealed that the CO₂ emission is a product of mechano destruction rather than the release of impurities trapped in the crystal. Irradiation of calcite increases the CO₂ emission. A diffusion–desorption model is suggested to explain the kinetics of volatile emission from cleaved surfaces and experimental results on the emission of volatile products during the mechano destruction of various single crystals are summarized. The effects of several sources of systematic errors are discussed. The yield of volatiles is correlated with the speed of the brittle crack propagation and the physicochemical properties of minerals.  相似文献   

Laboratory studies about the interaction of ammonia with ice crystals at temperatures between 0 and −20°C     

Ines Hoog  Subir K. Mitra  Karoline Diehl  Stephan Borrmann 《Journal of Atmospheric Chemistry》2007,57(1):73-84

In laboratory experiments the interactions of ammonia with ice crystals were studied within the temperature range between 0 and −20°C. In a first series of experiments dendritic ice crystals were grown from water vapor in presence of ammonia gas in various concentrations between 4 and 400 ppbv. In a second series of experiments pure ice crystals were exposed to a humidified ammonia–air mixture inside a horizontal flow tube. The influence of temperature, ammonia gas concentration (0.6, 1.5, and 10 ppmv), exposure time, and the presence of impurities such as sulfate on the ammonia uptake by the ice surface was investigated by determining the ammonium content in the melt water of the ice crystals by ion chromatography. During the growth of ice crystals significant amounts of ammonia (around 200 μg/l) were taken up even at small gas concentrations. In contrast, even at high gas concentrations the uptake of ammonia by non-growing ice crystals was lower by approximately one order of magnitude. The presence of sulfate on the ice surface affected an enhanced uptake of ammonia by a factor of 5–10. A model is presented which describes the uptake of ammonia by ice considering the chemical processes occurring in the ice surface layer and simultaneous diffusion of ammonia into bulk ice. Even the increased uptake of ammonia by growing ice is rather small compared to the uptake by water droplets; thus, the major process for scavenging of ammonia from the atmosphere via the ice phase might not be the direct uptake by ice crystals but the riming involving super-cooled droplets containing ammonia.  相似文献   

Fabric and crystal characteristics of Bohai and Arctic sea ice   总被引：1，自引：0，他引：1  

李志军  康建成  蒲毅彬 《极地研究(英文版)》2002,13(1)

1　ＩｎｔｒｏｄｕｃｔｉｏｎＢｏｈａｉｏｎｅ ｙｅａｒｉｃｅａｎｄＡｎｔａｒｃｔｉｃｏｎｅｈａｖｅｔｈｅｓｉｍｉｌａｒｓｕｒｆａｃｅ ｆｅａｔｕｒｅｓａｎｄｃｏｒｒｅ ｓｐｏｎｄｉｎｇｆａｂｒｉｃａｎｄｃｒｙｓｔａｌｃｈａｒａｃｔｅｒｉｓｔｉｃｓ (Ａｌｌｉｓｏｎ 1 997;Ｌｉｅｔａｌ.1 997;Ｑｉｎ 1 991 ) .ＤｕｒｉｎｇｔｈｅＣｈｉｎａＦｉｒｓｔＡｒｃｔｉｃＥｘｐｅｄｉｔｉｏｎ ,ｔｈｅｒｅｓｕｌｔｓｉｎｔｈｅｓｔｕｄｙｏｆｏｎｅ ｙｅａｒｉｃｅｆｒｏｍＢｏｈａｉａｎｄＡｎｔａｒｃｔｉｃｗｅｒｅｕｓｅｄｆｏ…  相似文献   

察尔汗盐湖地区盐渍土微观结构及其力学与强度表现   总被引：2，自引：0，他引：2  

刘军勇  ;张留俊 《盐湖研究》2014,(2):60-67

为探明察尔汗盐湖区盐渍土的微观结构特征及其力学与强度表现,从盐湖区采集9组不同含盐量的盐渍土样品,对盐渍土进行电镜扫描、直接剪切试验和抗压强度试验,从微观结构上分析了盐渍土的力学与强度表现,提出了察尔汗盐湖区盐渍土颗粒骨架的连结形式。研究结果表明,不同含盐量的盐渍土微观结构形式不同,盐渍土颗粒骨架之间的连结有3种形式:1)点式接触、2)堆叠接触、3)盐晶体胶结;微观结构越密实,盐晶体胶结作用越强,盐渍土表现出越高力学与强度特性;盐晶体的胶结作用是影响盐溃土力学与强度特性的显著因素;无侧限抗压强度显著变化的含盐量拐点为45.74%。  相似文献