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101.
102.
Taotao Zhang Yang Xiao Dongfang Liang Hongwu Tang Junzeng Xu Saiyu Yuan Nairu Wang Bin Luan 《水文研究》2021,35(5):e14152
Dissolved pollutants in stormwater are a main contributor to water pollution in urban environments. However, many existing transport models are semi-empirical and only consider one-dimensional flows, which limit their predictive capacity. Combining the shallow water and the advection–diffusion equations, a two-dimensional physically based model is developed for dissolved pollutant transport by adopting the concept of a ‘control layer’. A series of laboratory experiments has been conducted to validate the proposed model, taking into account the effects of buildings and intermittent rainfalls. The predictions are found to be in good agreement with experimental observations, which supports the assumption that the depth of the control layer is constant. Based on the validated model, a parametric study is conducted, focusing on the characteristics of the pollutant distribution and transport rate over the depth. The hyetograph, including the intensity, duration and intermittency, of rainfall event has a significant influence on the pollutant transport rates. The depth of the control layer, rainfall intensity, surface roughness and area length are dominant factors that affect the dissolved pollutant transport. Finally, several perspectives of the new pollutant transport model are discussed. This study contributes to an in-depth understanding of the dissolved pollutant transport processes on impermeable surfaces and urban stormwater management. 相似文献
103.
JianZhong Xu Amanda Grannas CunDe Xiao ZhiHeng Du Amanda Willoughby Patrick Hatcher YanQing An 《寒旱区科学》2018,10(1):38-46
Dissolved organic matter(DOM) is an important component of ice cores but is currently poorly characterized. DOM from one Holocene sample(HS, aged at 1600–4500 B.P.) and one Last Glacial Maximum sample(LS, aged at 21000–25000 B.P.) from the North Greenland Eemian Ice Drilling(NEEM) ice core were analyzed by ultra-high resolution Fourier transform ion cyclotron resonance mass spectrometry(FT-ICR-MS). CHO compounds contributed 50% of the compounds identified in negative-ionization mode in these two samples, with significant contributions from organic N, S, and P compounds, likely suggesting that marine DOM was an important source in these samples. Overall, the chemical compositions are similar between these two samples, suggesting their consistent DOM sources. However, subtle differences in the DOM between these two samples are apparent and could indicate differences in source strength or chemistry occurring through both pre-and post-depositional processes. For example, higher relative amounts of condensed carbon compounds in the HS DOM(5%), compared to the LS DOM(2%), suggest potentially important contributions from terrestrial sources. Greater incorporation of P in the observed DOM in the LS DOM(22%), compared to the HS DOM(13%), indicate more active microbiological processes that likely contribute to phosphorus incorporation into the DOM pool. Although these two samples present only a preliminary analysis of DOM in glacial/interglacial periods, the data indicate a need to expand the analysis into a broader range of ice-core samples, geographical locations, and glacial/interglacial periods. 相似文献
104.
994年9月采集了珠江口表层海水水样,并对其溶解态的K+、Na+、Ca2+、Mg2+、SO2-4、Cl等化学要素进行了测定。结果表明,珠江口调查海域表层水中溶解态的K+、Na+、Ca2+、Mg2+、SO2-4主要受陆源淡水与外海水物理混合稀释的影响,与Cl具有良好的直线正相关;Ca2+/Cl、SO2-4/Cl明显高于大洋水相应比值,Na+/Cl、Mg2+/Cl略高,而K+/Cl比大洋比值低;在与中国其它各主要河口表层水对应Cl比较中,珠江口的SO2-4/Cl较高,而Ca2+/Cl,Mg2+/Cl比值居低;上述各主要常量离子和Cl的等值线均沿自北向南走向递增。 相似文献
105.
鸭绿江口溶解有机碳的研究 总被引:3,自引:2,他引:1
1996年5月采样测定鸭绿江口溶解有机碳(DOC)的含量,得出分布变化特征,并同其它一些河口的溶解有机碳进行了比较。鸭绿江口表层水溶解有机碳的平均含量为208μmolC/L。在盐度大于1.6的河口区,溶解有机碳的分布主要受海水稀释作用控制;在盐度0~1.6的区域溶解有机碳的浓度随盐度的增加而明显增加。在最大混浊带,DOC的浓度最高,表明有颗粒有机碳转化为溶解有机碳。丹东市以上流段,河水中溶解有机碳的含量相对较低,说明由丹东市引入的工业及生活污水对鸭绿江水体中溶解有机碳的含量有一定的影响。 相似文献
106.
107.
Eutrophication Dynamics of Tolo Harbour, Hong Kong 总被引:8,自引:0,他引:8
The time and spatial variation of water quality in Tolo Harbour, a eutrophic landlocked semi-enclosed bay frequented by algal blooms, is studied using a dynamic eutrophication model. Hourly changes of tide levels and currents are computed by a link-node model assuming M2 tidal forcing. Phytoplankton growth is assumed to be limited by solar radiation, nitrogen and temperature. The model incorporates light acclimation by algae, self-shading, photosynthetic production, nutrient uptake, and a dynamic determination of the carbon to chlorophyll ratio. In particular, sediment-water-pollutant interactions are modelled via an anaerobic benthic layer segment. Using recorded pollution loads and environmental forcing as input, the model predictions of daily-averaged water quality are compared with the extensive water quality monitoring data of the Environmental Protection Department (EPD). The predicted spatial distribution and trends of algal biomass, inorganic nitrogen, dissolved oxygen (DO), as well as sediment oxygen demand (SOD), are in general agreement with field observations. 相似文献
108.
M. Thangarajan 《Environmental Geology》1999,38(3):209-222
Palar River Basin, a crystalline rock region in North Arcot District (Tamil Nadu), India, possesses vast groundwater potential
along and near the river course and its lands are fertile. Serious contamination of both surface water and groundwater has
been reported in this basin as a result of uncontrolled discharge of untreated effluents by the tanning industries for the
last three decades. The health of the rural farming community and people working in the tanning industries has been seriously
affected and they are suffering from occupational diseases such as asthma, chromium ulcers and skin diseases. About an 11000
hectares area of fertile land has lost its fertility. Total dissolved solids (TDS) concentration in groundwater at some pockets
varies from 3000 to 10000 mg/l. As the discharge of effluents is continuing, a prognosis of further pollutant migration is
carried out using a mathematical model. A numerical model of the Upper Palar River Basin was developed using the finite difference
technique coupled with method of characteristics and used to predict TDS migration for the next 20 years. Sensitivity analysis
was carried out to identify the parameters which are influencing the contaminant migration. Sensitivity analysis shows that
advection and not dispersion is the predominant mode of solute migration in Palar Basin. Prognosis using the model confirms
that the polluted area zone as well as the concentration of pollutants in the groundwater will continue to increase in future.
The study also indicated that even if the pollutant sources are reduced to 25% of the present level, the TDS concentration
level in the groundwater, even after 20 years, will not be reduced below 50% of its 1992 level.
Received: 20 June 1998 · Accepted: 26 October 1998 相似文献
109.
报道一种合成2,2-二甲基-4-戊烯酸的新方法。由异丁醛与烯丙醇缩合得到2,2-二甲基-4-戊烯醛,后者经氧化银选择氧化生成2,2-二甲基-4-戊烯酸。此法氧化产率(96%)高于分子氧氧化法(61%)和歧化法(41%)。反应中析出的金属银能定量回收,循环使用。 相似文献
110.
南极洲万达盐湖为饱和方解石湖水。计算出的方解石饱和指数随水深增加而变化。在Ca~(2+)及HCO_3~-活度值均一的上部氧化环境湖水中,pH及溶解氧(DO)是控制该变化的主要因素,在下部还原环境湖水中,Ca~(2+)及HCO_3~-的活度对方解石的饱和指数SI的变化起主要作用。这充分揭示了湖底部近代沉积物中分布较多方解石矿物的原因。 相似文献