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101.
The Baikal Rift is a zone of active lithospheric extension adjacentto the Siberian Craton. The 6–16 Myr old Vitim VolcanicField (VVF) lies approximately 200 km east of the rift axisand consists of 5000 km3 of melanephelinites, basanites, alkaliand tholeiitic basalts, and minor nephelinites. In the volcanicpile, 142 drill core samples were used to study temporal andspatial variations. Variations in major element abundances (e.g.MgO = 3·3–14·6 wt %) reflect polybaric fractionalcrystallization of olivine, clinopyroxene and plagioclase. 87Sr/86Sri(0·7039–0·7049), 143Nd/144Ndi (0·5127–0·5129)and 176Hf/177Hfi (0·2829–0·2830) ratiosare similar to those for ocean island basalts and suggest thatthe magmas have not assimilated significant amounts of continentalcrust. Variable degrees of partial melting appear to be responsiblefor differences in Na2O, P2O5, K2O and incompatible trace elementabundances in the most primitive (high-MgO) magmas. Fractionatedheavy rare earth element (HREE) ratios (e.g. [Gd/Lu]n > 2·5)indicate that the parental magmas of the Vitim lavas were predominantlygenerated within the garnet stability field. Forward major elementand REE inversion models suggest that the tholeiitic and alkalibasalts were generated by decompression melting of a fertileperidotite source within the convecting mantle beneath Vitim.Ba/Sr ratios and negative K anomalies in normalized multi-elementplots suggest that phlogopite was a residual mantle phase duringthe genesis of the nephelinites and basanites. Relatively highlight REE (LREE) abundances in the silica-undersaturated meltsrequire a metasomatically enriched lithospheric mantle source.Results of forward major element modelling suggest that meltingof phlogopite-bearing pyroxenite veins could explain the majorelement composition of these melts. In support of this, pyroxenitexenoliths have been found in the VVF. High Cenozoic mantle potentialtemperatures (1450°C) predicted from geochemical modellingsuggest the presence of a mantle plume beneath the Baikal RiftZone. KEY WORDS: Baikal Rift; mafic magmatism; mantle plume; metasomatism; partial melting  相似文献   
102.
The Chernobyl plume contaminated vast lands of Europe with radiocaesium (137Cs) in 1986 because of the deposition of radionuclides on the ground by wet and dry deposition processes. Nevertheless, in a nuclear emergency, contamination data may be very sparse and there is need to make rapid and scientifically supported decisions. Here we analyze the rainfall field, an important precursor of the wet deposition, during the passage of the plume. Thus, estimating rainfall spatial variability can help to identify possible contaminated areas and associated risks when rainfall exceeded a given threshold. In this paper, we show that the conditional probabilities of exceeding threshold rainfall values could be spatially assessed using the mutual benefits of linking geostatistical and geographical information system (GIS) to quantify the evaluation of the risk involved in decision making. In particular, the non-parametric geostatistic technique, termed Indicator Kriging (IK), enables one to efficiently estimate the probability that the true value exceeds the threshold values by means of the indicator coding transform. Afterward, GIS has been used to find the areas probably affected by wash-out (probability >0.5 that rainfall is above a certain threshold). The experimental study has been focused on a test site in Beneventan agroecosystem (Southern Italy) to model the spatial uncertainty over a continuous area from sparse rainfall data. This enabled to generate probability maps delineating area potentially affected by to contamination to be monitored after wet deposition of Chernobyl releases.  相似文献   
103.
Our understanding on how ash particles in volcanic plumes react with coexisting gases and aerosols is still rudimentary, despite the importance of these reactions in influencing the chemistry and dynamics of a plume. In this study, six samples of fine ash (<100 m) from different volcanoes were measured for their specific surface area, as, porosity and water adsorption properties with the aim to provide insights into the capacity of silicate ash particles to react with gases, including water vapour. To do so, we performed high-resolution nitrogen and water vapour adsorption/desorption experiments at 77 K and 303 K, respectively. The nitrogen data indicated as values in the range 1.1–2.1 m2/g, except in one case where a as of 10 m2/g was measured. This high value is attributed to incorporation of hydrothermal phases, such as clay minerals, in the ash surface composition. The data also revealed that the ash samples are essentially non-porous, or have a porosity dominated by macropores with widths >500 Å. All the specimens had similar pore size distributions, with a small peak centered around 50 Å. These findings suggest that fine ash particles have relatively undifferentiated surface textures, irrespective of the chemical composition and eruption type. Adsorption isotherms for water vapour revealed that the capacity of the ash samples for water adsorption is systematically larger than predicted from the nitrogen adsorption as values. Enhanced reactivity of the ash surface towards water may result from (i) hydration of bulk ash constituents; (ii) hydration of surface compounds; and/or (iii) hydroxylation of the surface of the ash. The later mechanism may lead to irreversible retention of water. Based on these experiments, we predict that volcanic ash is covered by a complete monolayer of water under ambient atmospheric conditions. In addition, capillary condensation within ash pores should allow for deposition of condensed water on to ash particles before water reaches saturation in the plume. The total mass of water vapour retained by 1 g of fine ash at 0.95 relative water vapour pressure is calculated to be ~10–2 g. Some volcanic implications of this study are discussed.Editorial responsibility: J. Gilbert  相似文献   
104.
We present the results of a comprehensive major element, traceelement and Sr–Nd–Pb–O isotopic study of post-glacialvolcanic rocks from the Neovolcanic zones on Iceland. The rocksstudied range in composition from picrites and tholeiites, whichdominate in the main rift systems, to transitional and alkalicbasalts confined to the off-rift and propagating rift systems.There are good correlations of rock types with geochemical enrichmentparameters, such as La/Sm and La/Yb ratios, and with long-termradiogenic tracers, such as Sr–Nd–Pb isotope ratios,indicating a long-lived enrichment/depletion history of thesource region. 87Sr/86Sr vs 143Nd/144Nd defines a negative array.Pb isotopes define well-correlated positive arrays on both 206Pb/204Pbvs 207Pb/204Pb and 208Pb/204Pb diagrams, indicating mixing ofat least two major components: an enriched component representedby the alkali basalts and a depleted component represented bythe picrites. In combined Sr–Nd–Pb isotopic spacethe individual rift systems define coherent mixing arrays withslightly different compositions. The enriched component hasradiogenic Pb (206Pb/204Pb > 19·3) and very similargeochemistry to HIMU-type ocean island basalts (OIB). We ascribethis endmember to recycling of hydrothermally altered upperbasaltic oceanic crust. The depleted component that is sampledby the picrites has unradiogenic Pb (206Pb/204Pb < 17·8),but geochemical signatures distinct from that of normal mid-oceanridge basalt (N-MORB). Highly depleted tholeiites and picriteshave positive anomalies in mantle-normalized trace element diagramsfor Ba, Sr, and Eu (and in some cases also for K, Ti and P),negative anomalies for Hf and Zr, and low 18Oolivine values(4·6–5·0) below the normal mantle range.All of these features are internally correlated, and we, therefore,interpret them to reflect source characteristics and attributethem to recycled lower gabbroic oceanic crust. Regional compositionaldifferences exist for the depleted component. In SW Icelandit has distinctly higher Nb/U (68) and more radiogenic 206Pb/204Pbratios (18·28–18·88) compared with the NErift (Nb/U 47; 206Pb/204Pb = 18·07–18·47).These geochemical differences suggest that different packagesof recycled oceanic lithosphere exist beneath each rift. A thirdand minor component with relatively high 87Sr/86Sr and 207Pb/204Pbis found in a single volcano in SE Iceland (Öræfajökullvolcano), indicating the involvement of recycled sediments inthe source locally. The three plume components form an integralpart of ancient recycled oceanic lithosphere. The slope in theuranogenic Pb diagram indicates a recycling age of about 1·5Ga with time-integrated Th/U ratios of 3·01. Surprisingly,there is little evidence for the involvement of North AtlanticN-MORB source mantle, as would be expected from the interactionof the Iceland plume and the surrounding asthenosphere in formof plume–ridge interaction. The preferential samplingof the enriched and depleted components in the off-rift andmain rift systems, respectively, can be explained by differencesin the geometry of the melting regions. In the off-rift areas,melting columns are truncated deeper and thus are shorter, whichleads to preferential melting of the enriched component, asthis starts melting deeper than the depleted component. In contrast,melting proceeds to shallower depths beneath the main rifts.The longer melting columns also produce significant amountsof melt from the more refractory (lower crustal/lithospheric)component. KEY WORDS: basalts; trace element and Sr, Nd, Pb, O isotope geochemistry; Iceland plume; isotope ratios; oceanic crustal recycling; partial melting; plume–ridge interaction  相似文献   
105.
Atmospheric deposition can provide a significant fraction of the nitrogen loading to coastal waters. The Delmarva Peninsula, on the eastern shore of the Chesapeake Bay, is a region with intense poultry production that may supply a significant source of atmospheric ammonia (NH3). There is a need to quantify ammonia NH3 from representative growing methods in this region in order to more accurately estimate agricultural NH3 emissions and to develop best management practices. In this study, NH3 emissions were determined at an 18,600-bird tunnel-ventilated chicken house using a modified sampling grid (a planar arrangement normal to the length of the house) with Ogawa passive samplers to characterize the emission plume downwind from the house. This improvement in the sampling strategy, compared to a previous study, simplified the inverse Gaussian plume analysis which improved the confidence in the emission factors. In this study, a total of four separate plume characterizations were conducted over the final 3 weeks of the 6-week broiler grow-out cycle. The mean emission factor observed at the tunnel-ventilated house, 0.13 g NH3–N/bird-day, was an order of magnitude lower than that previously observed at a nearby side-wall ventilated house. Although not all growing variables were measured, the large difference in emission factors between the two ventilation regimes suggest that modern, tunnel-ventilated houses may result in a significant decrease in NH3 emissions compared with traditional growing methods. This variability in emission factors underscores the need for characterizing chicken houses under various conditions and determining the factors that control these atmospheric emissions.  相似文献   
106.
In order to simulate the plume produced by large natural draft cooling towers, a semi-spectral warm cloud parameterization has been implemented in an anelastic and non-hydrostatic 3D micro-scale meteorological code. The model results are compared to observations from a detailed field experiment carried out in 1980 at Bugey (location of an electrical nuclear power plant in the Rhône valley in East Central France) including airborne dynamical and microphysical measurements. Although we observe a slight overestimation of the liquid-water content, the results are satisfactory for all the 15 different cases simulated, which include different meteorological conditions ranging from low wind speed and convective conditions in clear sky to high wind and very cloudy. Such parameterization, which includes semi-spectral determination for droplet spectra, seems to be promising to describe plume interaction with atmosphere especially for aerosols and cloud droplets.  相似文献   
107.
In this work, we present a comprehensive X-ray picture of the interaction between a super star cluster and the interstellar medium. In order to do that, we compare and combine the X-ray emission from the superwind driven by the cluster with the emission from the wind-blown bubble. Detailed analytical models for the hydrodynamics and X-ray luminosity of fast polytropic superwinds are presented. The superwind X-ray luminosity models are an extension of the results obtained in Paper I. Here, the superwind polytropic character allows us to parametrize a wide variety of effects, for instance, radiative cooling. Additionally, X-ray properties that are valid for all bubble models taking thermal evaporation into account are derived. The final X-ray picture is obtained by calculating analytically the expected surface brightness and weighted temperature of each component. All of our X-ray models have an explicit dependence on metallicity and admit general emissivities as functions of the hydrodynamical variables. We consider a realistic X-ray emissivity that separates the contributions from hydrogen and metals. The paper ends with a comparison of the models with observational data.  相似文献   
108.
The basin-and-range area in eastern North China is known for frequent occurrence of earthquakes, their great magnitudes and heavy losses thereby incurred. Seismic studies in the past usually emphasized the intersections, inflexions and branches of the faults. However, the intensities of many great earthquakes in this area do not show linear distribution, and the epicenters are horizontally dispersed at certain depths instead of along the strike of faults. Based on the sub-mantle plume studies made by authors in the past decade, it is thought that there exists an uplifted sub-mantle plume under the fault depression area in North China. The uplifting and intrusion of mantle materials caused the upper crust to be faulted, while low-velocity and high-velocity layers are alternatively distributed in the middle crust under the influence of the mantle and the lower crust. The middle and lower crust materials were detached from the top of the sub-mantle plume to the surroundings while the sub-mantle plume materi  相似文献   
109.
Aspects of two qualitative models of Enceladus’ dust plume—the so-called “Cold Faithful” [Porco, C.C., et al., 2006. Cassini observes the active south pole of Enceladus. Science 311, 1393-1401; Ingersoll, A.P., et al., 2006. Models of the Enceladus plumes. In: Bulletin of the American Astronomical Society, vol. 38, p. 508] and “Frigid Faithful” [Kieffer, S.W., et al., 2006. A clathrate reservoir hypothesis for Enceladus’ south polar plume. Science 314, 1764; Gioia, G., et al., 2007. Unified model of tectonics and heat transport in a Frigid Enceladus. Proc. Natl. Acad. Sci. 104, 13578-13591] models—are analyzed quantitatively. The former model assumes an explosive boiling of subsurface liquid water, when pressure exerted by the ice crust is suddenly released due to an opening crack. In the latter model the existence of a deep shell of clathrates below Enceladus’ south pole is conjectured; clathrates can decompose explosively when exposed to vacuum through a fracture in the outer icy shell. For the Cold Faithful model we estimate the maximal velocity of ice grains, originating from water splashing in explosive boiling. We find that for water near the triple point this velocity is far too small to explain the observed plume properties. For the Frigid Faithful model we consider the problem of momentum transfer from gas to ice particles. It arises since any change in the direction of the gas flow in the cracks of the shell requires re-acceleration of the entrained grains. While this effect may explain the observed speed difference of gas and grains if the gas evaporates from triple point temperature (273.15 K) [Schmidt, J., et al., 2008. Formation of Enceladus dust plume. Nature 451, 685], the low temperatures of the Frigid Faithful model imply a too dilute vapor to support the observed high particle fluxes in Enceladus’ plume.  相似文献   
110.
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