海洋沉积物重金属生态风险评价方法比较及实例验证——以莱州湾为例     

赵玉庭  董晓晓  王立明  齐延民  由丽萍  孙珊  马元庆 《海洋通报》2019,38(3)

利用2016年8月份莱州湾沉积物中Hg、Cd、Pb、Cu、As、Cr、Zn监测数据,分别利用单因子污染指数法、潜在生态风险指数法、地积累指数法、沉积物质量基准法、尼梅罗综合指数法、污染负荷指数法等6种沉积物重金属风险评价方法进行评价,以比较沉积物重金属生态风险评估方法的适用性与局限性。结果表明,莱州湾表层沉积物中,重金属Hg、Cd、Pb、Cu、As、Cr和Zn含量分别为0.077 4 mg/kg、0.169 mg/kg、12.1 mg/kg、11.9 mg/kg、11.6 mg/kg、31.1 mg/kg、45.3 mg/kg。不同方法在莱州湾沉积物风险评价结果上存在差异。单因素评价方法中,单因子污染指数法、潜在生态危害指数法、尼梅罗综合指数法的评价结果适中,地累积指数法评价结果偏轻,沉积物质量基准法评价结果偏重。Hg、As、Cd元素的污染评价结果均较大,为主要的污染元素;综合因素评价方法中,污染负荷指数法评价结果风险偏轻,潜在生态危害指数法评价结果适中,内梅罗综合指数法评价结果则倾向偏重。沉积物重金属含量与底栖生物的丰度、生物量的pearson相关系数表明,Hg与底栖生物的生物量呈现显著负相关。6种方法都有自身优缺点和适用范围,但潜在生态危害指数法更适合莱州湾沉积物重金属风险评价。  相似文献   

Quantifying sand delivery to deep water during changing sea-level: Numerical models from the Quaternary Brazos Icehouse continental margin     

Oriol Falivene  Bradford E. Prather  John Martin 《Basin Research》2020,32(6):1711-1733

Sequence stratigraphy for clastic continental margins predicts the development of sand-rich turbidite deposits during specific times in relation to base-level cycles. It is now widely understood that deltas can extend to the shelf-edge forced by high sediment flux and/or base level, providing a direct connection to transfer sediment and sand to the slope and basin floor even during high base level periods. Herein, we build a stratigraphic forward model for the last 120 kyr of the fluvio-deltaic to deep-water Brazos system (USA) where sediment partitioning along an Icehouse continental margin can be evaluated. The reduced-complexity stratigraphic forward model employs geologically constrained input parameters and mass balance. The modelled architecture is consistent with the location of depositional units previously mapped in the shelf. Sand bypasses the shelf and upper slope between 35 to 15 kyr before present and only about 20%–30% of all the sediment and sand supplied to the system is transferred to deep water. Several scenarios based on the initial Brazos model investigate the relationships between base level and deep-water sand ratio (DWSR). DWSR is defined as the relative amount of sand transferred to the deep-water portions of the system subdivided by the total sand input to the model. Linear correlations between DWSR and base level change rates or base level are very poor. Short-term variability due to local processes (for example avulsions) is superimposed to the long-term trends and mask the base level signal. DWSR for an entire base-level cycle is mainly controlled by the proportion of time the delta stays docked at the shelf-edge. Stratigraphic forward models are useful to complement field observations and quantify how different processes control stratigraphy, which is important for making predictions in areas with limited information.  相似文献   

Using LM‐OSL of quartz to distinguish sediments derived from surface‐soil and channel erosion          下载免费PDF全文

Arman Haddadchi  Jon Olley  Timothy Pietsch 《水文研究》2016,30(4):637-647

This study describes the use of linearly modulated optically stimulated luminescence (LM‐OSL) to distinguish surface‐soil derived sediments from those derived from channel bank erosion. LM‐OSL signals from quartz extracted from 15 surface‐soil and five channel bank samples were analysed and compared to signals from samples collected from two downstream river sites. Discriminant analysis showed that the detrapping probabilities of fast, first slow and second slow components of the LM‐OSL signal can be used to differentiate between the samples collected from the channel bank and surface‐soil sources. We show that for each of these source end members these components are all normally distributed. These distributions are then used to estimate the relative contribution of surface‐soil derived and channel bank derived sediment to the river bed sediments. The results indicate that channel bank derived sediments dominate the sediment sources at both sites, with 90.1 ± 3% and 91.9 ± 1.9% contributions. These results are in agreement with a previous study which used measurements of ¹³⁷Cs and ²¹⁰Pb_ex fallout radionuclides to estimate the relative contribution from these two sources. This result shows that LM‐OSL may be a useful method, at least in the studied catchment, to estimate the relative contribution of surface soil and channel erosion to river sediments. However, further research in different settings is required to test the difference of OSL signals in distinguishing these sediment sources. And if generally acceptable, this technique may provide an alternative to the use of fallout radionuclides for source tracing. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

潮致泥沙全沙净输运解析模式     

储鏖  徐怡  陈永平  郁夏琰  王彪 《海洋工程》2020,38(4):61-72

泥沙运动作为水流和底床相互作用的纽带,是河流、河口及海岸工程研究的重要内容。在潮波作用明显的河口、海岸地区,周期性的动力作用下的泥沙运动具有往复和可逆的特征,因此研究这类水域的泥沙的净输运更具有实际的意义。基于泥沙输运和流速呈指数关系假设,建立潮流环境下的泥沙全沙净输运的解析解公式,并对该公式的计算结果和数值计算以及数学模型的结果进行了检验和验证,结果表明本研究提出的公式能较好地反应潮流环境下的泥沙净输运。由此,基于本公式采用潮流分潮调和常数可计算得到全沙净输运,并可以分析各分潮流及其相互作用与泥沙净输运的关系。研究结果显示,在受径流影响较大的半日潮河口,S2、MS4、M2三潮相互作用对全沙净输运的贡献显著高于通常的潮流不对称作用,即M2、M4的相互作用。此外,河口区域径流导致的余流对泥沙净输运的贡献不可忽略,特别是在洪季,大径流量条件下往往导致余流较大,其对泥沙净输运的贡献所占比例较大。  相似文献   

Hydraulics of overland flow influenced by litter incorporation under extreme rainfall     

Lunjiang Wang  Guanghui Zhang  Xue Wang  Xiaoyan Li 《水文研究》2019,33(5):737-747

Water erosion on hillslopes is a worldwide environmental problem, which is a rainfall‐induced process, especially extreme rainfall. The great intensity of extreme rainfall strongly enhances the power of overland flow to detach soil and transport sediment. Plant litter is one of the most important constituents of ecosystems that often covers the soil surface and can be incorporated into topsoil. However, little attention has been paid to its effect on flow hydraulics owing to the veiled nature. This study aimed to examine the effects of incorporated litter on the hydraulic properties under extreme rainfall condition. To reach this goal, six litter rates of 0, 0.05, 0.10, 0.20, 0.35, and 0.50 kg m^?2 and four litter types collected from deciduous trees, coniferous trees, shrubs, and herbs were incorporated into topsoil. Then, simulated rainfall experiments were performed on five slope gradients (5°, 10°, 15°, 20°, and 25°) with an extreme rainfall intensity of 80 mm h^?1. The results showed that Froude number and flow velocity of the overland flow decreased, whereas flow resistance increased exponentially with litter incorporation rate. Litter type had an influence on flow hydraulics, which can mainly be attributed to the variations in surface coverage of the exposed litter and the litter morphology. Flow velocity and Darcy–Weisbach coefficient increased markedly with slope gradient. However, the variation of slope gradient did not modify the relationships between flow hydraulics and incorporated litter rate. The random roughness, resulting from heterogeneous erosion due to the uneven protection of surface exposed litter, increased linearly with litter incorporated rate. As rainfall proceeded, flow hydraulics varied with incorporated litter rate and slope gradient complicatedly due to the increases in flow rate and coverage of the exposed litter and the modification of soil surface roughness.  相似文献   

基于GF-1号的舟山近岸悬浮泥沙浓度反演研究          下载免费PDF全文

章敏超  郭碧云 《海洋开发与管理》2018,35(1):126-131

文章利用舟山近岸实测光谱数据和国产卫星GF-1号宽视场成像仪(WFV)遥感数据,反演该海域悬浮泥沙浓度。结果表明:(1)线性模型和二次模型相比,二次模型的精确度略高于线性模型,但对于悬沙低浓度区,反演误差过大,故线性模型更适用于舟山近岸水体悬浮泥沙浓度反演;(2)GF-1号B2和B3是悬沙浓度变化的敏感波段,B3/B2波段组合的线性模型反演效果较好;(3)GF-1号遥感数据能够较理想地实现定量反演近岸水体的悬浮物。  相似文献   

Impacts of climate variability on water quality with best management practices in sub‐tropical climate of USA          下载免费PDF全文

Priyantha Jayakody  Prem B. Parajuli  Thomas P. Cathcart 《水文研究》2014,28(23):5776-5790

Efficiency of non‐point source pollution control methods may be altered in future climate. This study investigated climate change impacts on sediment and nutrient transport, and efficiency of best management practices (BMPs), in the Upper Pearl River Watershed (UPRW) in Mississippi. The Soil and Water Assessment Tool was applied to the UPRW using observed flow, sediment and nutrient data. Water quality samples were collected at three US geological survey gauging stations. The model was successfully calibrated and validated for daily time steps (Nash Sutcliffe efficiency and coefficient of determination – R² up to 0.7) using manual and automatic (sequential uncertainty fitting version 2) methods from February 2010 to May 2011. Future weather scenarios were simulated using the LARS‐WG model, a stochastic weather generator, with Community Climate System Model, global climate model, which was developed by the National Center for Atmospheric Research in the USA. On the basis of the Special Report on Emissions Scenarios A1B, A2 and B1 of the Intergovernmental Panel on Climate Change, climate change scenarios were simulated for the mid (2046–2065) and late (2080–2099) century. Effectiveness of four BMPs (Riparian buffer, stream fencing, sub‐surface manure applications and vegetative filter strips) on reducing sediment and nutrient were evaluated in current and future climate conditions. Results show that sediment, nitrogen and phosphorus loadings will be increased up to a maximum of 26.3%, 7.3% and 14.3%, respectively, in future climate conditions. Furthermore, the effectiveness of BMPs on sediment removal will be reduced in future climate conditions, and the efficiency of nitrogen removal will be increased, whereas phosphorus removal efficiency will remain unchanged. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

Temporal variation of suspended sediment transport in the Koga catchment,North Western Ethiopia and environmental implications          下载免费PDF全文

Eleni Yeshaneh  Alexander Eder  Günter Blöschl 《水文研究》2014,28(24):5972-5984

Event sediment transport and yield were studied for 45 events in the upstream part of the 260 km² agricultural Koga catchment that drains to an irrigation reservoir. Discharge and turbidity data were collected over a period of more than a year, accompanied by grab sampling. Turbidity was very well correlated with the sediment concentrations from the samples (r = 0.99), which allowed us to estimate the temporal patterns of sediment concentrations within events. The hysteresis patterns between discharge and sediment concentrations were analysed to provide insight into the different sediment sources. Anticlockwise patterns are the dominant hysteresis patterns in the area, suggesting smaller contributions of suspended sediment from the river channels than from the hillslopes and agricultural areas. Complicated types of hysteresis patterns were mostly observed for long events with multiple peaks. For a given discharge, sediment yields in August and September, when the catchment was almost completely covered with vegetation, were much smaller than during the rest of the rainy season. The hysteresis patterns and timing suggest that the sediment availability from the agricultural areas and hillslopes affects sediment yields more strongly than does peak discharge. Two distinct types of sediment rating curves were observed for the season when the agricultural land was covered with vegetation and when it was not, indicating the dominating contribution of land use/cover to sediment yields in the catchment. The rate of suspended sediment transport in the area was estimated as 25.6 t year^?1 ha^?1. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

Rainstorm-generated sediment yield model based on soil moisture proxies (SMP)     

Sushindra Kumar Gupta  Pushpendra K. Singh  Jaivir Tyagi  Gunwant Sharma  Ajay Singh Jethoo 《水文研究》2020,34(16):3448-3463

This study develops improved Soil Moisture Proxies (SMP) based suspended sediment yield (SMPSY) models corresponding to three antecedent moisture conditions (AMCs) (i.e., AMC-I-AMC-III) by coupling the improved initial abstraction (I_a-λ) model, the SMA procedure and the SMP concept for modelling the rainfall generated suspended sediment yield. The SMPSY models specifically incorporate a watershed storage index (S) model to accentuate the transformation from storm to storm and to avoid the sudden jumps in sediment yield computation. The workability of the SMPSY models is tested using a large dataset of rainfall and sediment yield (98 storm events) from twelve small watersheds and a comparison has been made with the existing MSY model. The goodness-of-fit (GOF) statistics is evaluated in terms of the Nash Sutcliffe efficiency (NSE), and error indices, i.e., root mean square error (RMSE), normalized root mean square error (nRMSE), standard error (SE), mean absolute error (MAE), and RMSE-observations standard deviation ratio (RSR). The NSE values vary from 74.31% to 96.57% and from 75.21% to 91.78%, respectively for the SPMSY and MSY model. The NSE statistics indicate that the SMPSY model has lower uncertainty in simulating sediment yield as compared to the MSY model. The error indices are lower for the SMPSY model than the MSY model for most of the watersheds. These results show that the SMPSY model has less uncertainty and performs better than the MSY model. A sensitivity analysis of the SMPSY model shows that the parameter β is most sensitive followed by parameter S, α and A. Overall, the results show that the characterization of soil moisture variability in terms of SMPs and incorporation of improved delivery ratio and runoff coefficient relationship improves the simulation of the erosion and sediment yield generation process.  相似文献   

菲与纳米银对胶州湾表层沉积物反硝化作用的复合毒性效应评价     

孙鹏飞  白洁  李岿然  白晓岩  田延昭  赵阳国 《中国海洋大学学报(自然科学版)》2020,(1):104-114

多环芳烃(PAHs)与纳米材料污染已对沉积物生态系统和人类生存环境构成严重威胁,其复合污染的毒性效应环境危害可能更大。为了深入探讨PAHs与纳米材料对近岸表层沉积物反硝化作用的复合毒性效应,本文选取位于胶州湾(JZB)的大沽河河口区(DRE)E站和湾内S站,分别以菲和纳米银代表PAHs和纳米材料,通过测定不同剂量单一及复合污染下沉积物反硝化潜势(PDA)的变化,结合浓度相加模型(CA)、独立作用模型(IA)和中效/联合指数等效图法(CI)三种复合毒性评价方法,评价菲和纳米银对沉积物反硝化潜势的复合毒性效应,并对评价方法进行了优选。结果表明,两种污染物浓度越高,对研究区域反硝化潜势的抑制作用越大。菲、纳米银单一及复合作用下对河口区沉积物反硝化潜势的EC50值分别为44.62、112.49和64.86 mg·kg-1,对湾内分别为61.79、147.05和96.18 mg·kg-1。菲单一作用对反硝化潜势的抑制效应强于纳米银,但复合污染的抑制效应更强。两种污染物对河口区的沉积物反硝化潜势抑制效应强于湾内,可能与河口区具有较高Eh和沉积物颗粒度及较低的pH、盐度和有机质含量有关。三种毒性效应评价方法的结果表明,菲和纳米银的复合污染对2个站位反硝化潜势的毒性效应均为协同作用,且对大沽河河口区的协同作用更强。此外,CI法对复合效应的预测结果比CA和IA法更为接近实际观测值,且CI不需要考虑污染物作用模式的限制,因此认为CI法更适用于评价混合污染对沉积物反硝化作用复合影响的效果。本研究结果表明,菲和纳米银会增强彼此对反硝化菌及反硝化功能的毒性效应,由此推断,PAHs和纳米材料在环境中同时存在时比其单独存在对沉积环境的危害更大。  相似文献