Migration and speciation transformation mechanisms of mercury in undercurrent zones of the Tongguan gold mining area,Shaanxi Loess Plateau and impact on the environment     

《China Geology》2021,4(2):311-328

In order to study the migration and transformation mechanism of Hg content and occurrence form in subsurface flow zone of gold mining area in Loess Plateau and its influence on water environment, the field in-situ infiltration test and laboratory test were carried out in three typical sections of river-side loess, alluvial and proluvial strata in Tongguan gold mining area of Shaanxi Province, and the following results were obtained: (1) The source of Hg in subsurface flow zone is mainly caused by mineral processing activities; (2) the subsurface flow zone in the study area is in alkaline environment, and the residual state, iron and manganese oxidation state, strong organic state and humic acid state of mercury in loess are equally divided in dry and oxidizing environment; mercury in river alluvial or diluvial strata is mainly concentrated in silt, tailings and clayey silt soil layer, and mercury has certain stability, and the form of mercury in loess is easier to transform than the other two media; (3) under the flooding condition, most of mercury is trapped in the silt layer in the undercurrent zone where the sand and silt layers alternate with each other and the river water and groundwater are disjointed, and the migration capacity of mercury is far less than that of loess layer and alluvial layer with close hydraulic connection; (4) infiltration at the flood level accelerates the migration of pollutants to the ground; (5) the soil in the undercurrent zone is overloaded and has seriously exceeded the standard. Although the groundwater monitoring results are safe this time, relevant enterprises or departments should continue to pay attention to improving the gold extraction process, especially vigorously rectify the small workshops for illegal gold extraction and the substandard discharge of the three wastes, and intensify efforts to solve the geological environmental problems of mines left over from history. At present, the occurrence form of mercury in the undercurrent zone is relatively stable, but the water and soil layers have been polluted. The risk of disjointed groundwater pollution can not be ignored while giving priority to the treatment of loess and river alluvial landform areas with close hydraulic links. The research results will provide a scientific basis for water conservancy departments to groundwater prevention and control in water-deficient areas of the Loess Plateau.  相似文献   

Hydro-geochemistry of groundwater and surface water in Dschang town(West Cameroon): Alkali and alkaline-earth elements ascertain lithological and anthropogenic constraints          下载免费PDF全文

Yemeli Elida Joelle  Temgoua Emile  Kengni Lucas  Ambrosi Jean-Paul  Momo-nouazi Mathieu  Silatsa-Tedou Francis Brice  Wamba Franck Robean  Tchakam-Kamtchueng Brice 《地下水科学与工程》2021,9(3):212-224

This study focuses on the sources of alkali and alkaline-earth elements based on the geochemistry of groundwater and surface water in Dschang concerning environmental and anthropogenic constraints. A comprehensive set of 50 samples from groundwater and surface water were analyzed by ICPMS and processed by spatial interpolation in a GIS environment. The results highlight a geochemical anomaly at the center of the densely inhabited area subject to a profusion of open dumps discharges. This anomaly with the highest spatial contents of Be(Cs, Rb, Mg) suggests an anthropogenic source that demarcates with the lowest alkali and alkaline-earth elements on the peripheral area of Dschang. Other findings include lithological constraints with volcanic rocks being the main source compared to granitoid.The study points out good correlations between Be, Cs, Rb and Mg spatial distributions and physicochemical parameters of waters(K, EC, TDS), and inversely with the lowest p H. p H is established as the most functioning physico-chemical constraint of alkali and alkaline-earth mobility in Dschang. The p H lowest values within the geochemical anomaly also highlight the impact of human activities on water acidity, which later enhance elements mobility and enrichment. Despite low elements contents relative to WHO standards, our findings point out an example of anthropogenic impact on water geochemistry linked to solid waste pollution; it also demonstrates significant anthropogenic changes of environmental physicochemical parameters of prime importance in the mobility and distribution of elements in the study area.Similar assessments should be extended in major towns in Cameroon.  相似文献   

六盘山区夏秋季大气水汽和液态水特征初步分析     

田磊  桑建人  姚展予  常倬林  单新兰  曹宁  孙艳桥 《气象与环境学报》2019,35(6):28-37

六盘山区是中国典型的农牧交错带和生态脆弱带,也是黄土高原重要的水源涵养地、生态保护区及国家级扶贫开发区。利用2017年6-11月隆德气象站地基多通道微波辐射计资料,结合同期平凉探空站及隆德地面降水等观测资料,分析了六盘山区夏秋季大气水汽、液态水变化特征。结果表明：六盘山区夏秋季在降水天气背景下,大气水汽含量和液态水含量均较高,分别为无降水天气背景下的1.4倍和7.0倍;降水天气背景下水汽在5000 m以下有明显的增加,且在此高度范围内的水汽密度随高度的递减率比无降水天气背景下明显偏小;各高度层的液态水相比无降水天气背景下均有明显增大,除6月外,主峰值均出现在0℃层高度层以下。六盘山区夏秋季各月中,6-9月。大气水汽含量高值区均出现在正午到傍晚时段,低值区均出现在日出前后;液态水含量在日出前、午后及傍晚分别出现峰值,最明显的峰值出现在午后。对一次对流性降水天气过程分析后发现,降水发生前40 min大气水汽含量和液态水含量出现两次明显的跃增,水汽向上输送不断加强,2500-7500 m高度的相对湿度明显增大。  相似文献   

阻塞形势下内蒙古东南部地区一次冷涡暴雨过程水汽特征分析     

马素艳  伊娜娜  赵斐  张旭 《气象与环境学报》2019,(2):1-8

使用常规观测资料、FY-2G卫星及1°×1°的NCEP再分析资料,对2017年7月6—7日内蒙古东南部地区一次冷涡暴雨天气过程进行分析。结果表明:在稳定的"一槽一脊"型环流背景下,阻塞高压稳定维持,西风槽东移受阻移动缓慢,加深为涡,暴雨发生在冷涡发展加强阶段;低空急流建立,一方面形成偏南水汽输送,为暴雨提供源源不断的水汽,水汽收支主要集中在700 hPa以下,暴雨发生前水汽净收入明显增大,南、北边界水汽贡献率大;另一方面,偏南暖湿气流的输送使不稳定层结建立,能量在暴雨区积聚,偏南低空急流与高空急流耦合,又为暴雨发生提供了动力条件;暴雨发生前后湿度场变化显著,大气可降水量最大达到55—60 kg·m^-2,且暴雨发生前增幅显著,增幅近2倍。暴雨区700 hPa (850 hPa)上比湿不低于7 g·kg^-1(12 g·kg^-1),强降水出现在水汽图上白亮区断裂消失后,高层比湿峰值附近和相当黑体温度<230 K为强降水高发区。  相似文献   

An Operational Precipitable Water Vapor Retrieval Algorithm for Fengyun-2F/VISSR Using a Modified Three-Band Physical Split-Window Method     

Juyang HU  Shihao TANG  Hailei LIU  Min MIN 《Journal of Meteorological Research》2019,(2):276-288

The Visible and Infrared Spin-Scan Radiometer(VISSR) onboard the Fengyun-2(FY-2) satellite can provide valuable thermal infrared observations to help create a precipitable water vapor(PWV) product with high spatial and temporal resolutions. The current FY-2/VISSR PWV product in operation is produced by using a traditional two-band physical split-window(PSW) method, which produces low quality results under dry atmospheric conditions. Based on the sensitivity characteristics of FY-2 F/VISSR water vapor channel and two split-window channels to atmospheric water vapor, this study developed a new, robust operational PWV retrieval algorithm for FY-2 F to improve the operational precision of the current PWV product. The algorithm uses a modified three-band PSW method, which adds a scale for the water vapor channel in the improved three-band PSW method. Integrated PWV products from the radiosonde data in 2016 are used here to validate the precision of the PWV retrieved by the modified three-band and traditional two-band PSW methods. The mean bias, root mean square error(RMSE), and correlation coefficient of the PWV retrieved by the modified three-band PSW method are 0.28 mm, 4.53 mm, and 0.969, respectively. The accuracy is much better than the PWV retrieved by the two-band method, whose mean bias, RMSE, and correlation coefficient are 12.67 mm, 29.35 mm, and 0.23. Especially, in mid-or high-latitude regions, the RMSE of the PWV is improved from 10 to 2 mm by changing the inversion in the two-band method to the modified three-band PSW method. Furthermore, the modified three-band PSW results show a better consistency with the radiosonde PWV at any zonal belt and season than the two-band PSW results. This new algorithm could significantly improve the quality of the current FY-2 F/VISSR PWV product, especially at sites where the actual PWV are lower than 15 mm.  相似文献   

三江源区大气可降水量时空特征及其与降水关系     

强安丰  汪妮  解建仓  姜仁贵 《干旱气象》2019,37(1):22-30

利用1979—2016年欧洲中期天气预报中心(ECMWF) ERA-Interim (1°×1°)再分析资料中的经、纬向水汽通量和大气可降水量(precipitation water vapor,PWV)数据,采用相关性分析、趋势分析法、累积距平、IDW等方法,分析三江源地区PWV与水汽通量的时空分布特征、降水转化率(precipitati-on conversion efficiency,PCE)变化规律。结果表明:过去的38 a,经、纬向多年平均水汽通量分别为50. 2、196. 7 kg·m-1·s^(-1),纬向水汽通量气候倾向率比经向大。南边界为纬向主要水汽输入边界,东边界为经向主要水汽输出边界,纬向水汽输送大于经向输送。多年平均PWV为1998. 3 mm,近38 aPWV呈现微弱增加趋势,1979—1997年,PWV呈下降趋势,1998年后PWV呈增加趋势,同期降水也在增加,说明该时段三江源地区气候转湿。PWV与水汽通量的年际变化趋势和转折年相一致。三江源区多年平均PCE为24. 57%,1989年PCE最高,达32. 76%,各季节平均PCE空间分布与年平均PCE分布一致,均表现出南部、东南部高,西部、东北部低的变化特征,各季节PCE大小差异明显,春季多年平均PCE为15. 92%,夏季25. 67%,秋季21. 01%,冬季仅7. 03%。  相似文献   

内蒙古东北部地区一次极端降雪过程的水汽输送特征     

王慧清  付亚男  孟雪峰 《干旱气象》2019,(2):277-287

利用内蒙古呼伦贝尔市常规观测资料和GDAS、NCEP/NCAR再分析资料,采用欧拉方法分析了2016年春季内蒙古东北部地区一次极端暴雪过程的水汽输送及收支特征,利用HYSPLIT模式和聚类分析模拟计算了此次暴雪天气过程的水汽源地、主要水汽输送通道及其对水汽输送的贡献,并与传统的欧拉方法结果进行对比。结果表明:(1)有3支不同源地的水汽流在内蒙古东北部地区交汇,对呼伦贝尔地区暴雪的发生与维持有重要影响;(2)经向和纬向输送为此次暴雪天气的发生提供了充足的水汽,暴雪区水汽主要源于中高层的南边界和随西风气流的西边界;(3)利用HYSPLIT模式模拟发现,在此次暴雪天气过程中水汽主要来源于新地岛以西洋面、日本海以及巴尔喀什湖,且三者贡献率大致相当。  相似文献   

近50多年来淮河流域气候水分盈亏时空变化   总被引：1，自引：0，他引：1  

颜雅琼  申双和 《气象科学》2019,39(4):457-466

水分盈亏是区域干湿气候划分的重要依据。基于淮河流域63个气象台站1957—2014年逐日观测数据,运用累积距平、Mann-Kendall突变分析、Morlet小波分析及ArcGIS反权重空间插值法,结合Penman-Monteith蒸散计算模型获得淮河流域水分盈亏量的周期特征、突变特征及其时空分布特征,并分析其主要影响因子。结果表明:(1)水分盈亏月变化基本符合5月最低,7月最高。(2)从季节分布来看,水分亏缺面积秋季春季冬季夏季,亏缺程度春季最强。从平均年水分盈亏量分布来看,水分盈亏量由南向北递减。且不论季节还是年状况,山地及河流对区域水分盈亏量的南北递减存在滞后作用。(3)从各因子气候倾向率的时空分布来看,江苏东南部、山东西部、河南大部、湖北中部水分盈亏量变化的主导因子为潜在蒸散量,其他区域的主导因子为降雨量。(4)淮河流域水分盈亏量存在周期特征,第一主周期为10 a。  相似文献   

Latitudinal and Scan-dependent Biases of Microwave Humidity Sounder Measurements and Their Dependences on Cloud Ice Water Path     

Anqi CAI  Xiaolei ZOU 《大气科学进展》2019,36(5):557-569

The relationship between differences in microwave humidity sounder(MHS)–channel biases which represent measured brightness temperatures and model-simulated brightness temperatures, and cloud ice water path(IWP) as well as the influence of the cloud liquid water path(LWP) on the relationship is examined. Seven years(2011–17) of NOAA-18 MHS-derived measured brightness temperatures and IWP/LWP data generated by the NOAA Comprehensive Large Array-data Stewardship System Microwave Surface and Precipitation Products System are used. The Community Radiative Transfer Model, version2.2.4, is used to simulate model-simulated brightness temperatures using European Center for Medium-Range Weather Forecasts reanalysis data as background fields. Scan-angle deviations of the MHS window channel biases range from-1.7 K to1.0 K. The relationships between channels 2, 4, and 5 biases and scan angle are symmetrical about the nadir. The latitudedependent deviations of MHS window channel biases are positive and range from 0–7 K. For MHS non-window channels,the latitudinal deviations between measured brightness temperatures and model-simulated brightness temperatures are larger when the detection height is higher. No systematic warm or cold deviations are found in the global spatial distribution of difference between measured brightness temperatures and model-simulated brightness temperatures over oceans after removing scan-angle and latitudinal deviations. The corrected biases of five different MHS channels decrease differently with respect to the increase in IWP. This decrease is stronger when LWP values are higher.  相似文献   

闽中南罕见冬季锋前暴雨个例特征分析     

陈健康  赵玉春  陈赛  黄惠镕  郑辉 《气象》2019,45(2):228-239

利用福建省逐小时加密自动站资料、风廓线、S波段双偏振雷达与雨滴谱等新型探测资料以及NCEP逐6 h的1°×1°大气再分析资料,分析了2017年2月21—22日福建中南部一次预报失败的冬季暴雨过程。结果表明:(1)此次暴雨过程类似于锋前暖区暴雨,自2000年以来仅此一例,十分罕见,是在低空急流偏强并长时间维持的背景下产生的,并未受到南支槽和冷空气的影响。(2)闽中大到暴雨带和闽南暴雨区的对流系统相互独立,有多个对流系统影响闽中地区,仅两个对流系统影响闽南地区。降水有较明显对流特征,属暖云弱对流降水,容易导致预报员对雨强估计不足。(3)此次冬季暴雨过程的水汽主要来自南海地区,低层水汽条件与汛期暴雨相当,但整层水汽条件较汛期略差;低空急流对暖湿气流的输送使暴雨区趋于不稳定,但对流不稳定度较汛期弱。(4)高空辐散低层辐合的配置为冬季暴雨带来了有利的动力抬升条件,但暴雨区涡旋性不强,无明显正涡度柱。其中,闽中大到暴雨主要与条件性对称不稳定有关,是在湿斜压作用下倾斜上升运动中产生,而闽南暴雨区既存在对流不稳定,也存在条件性对称不稳定。  相似文献