Trends in aerosol optical properties over Eastern Europe based on MODIS-Aqua     

《地学前缘(英文版)》2020,11(6):2169-2181

This study provides characteristics of aerosol columnar properties, measured over ten countries in Eastern Europe from 2002 to 2019. Aerosol optical depth (AOD) and Ångström exponent (AE) were obtained with the Moderate Resolution Imaging Spectroradiometer (MODIS) Collection 6.1 merged Dark Target and Deep Blue aerosol product. The product is validated using ground-based Aerosol Robotic Network (AERONET) situated at Minsk, Belsk, Moldova and Kyiv. The results showed that 76.15% of retrieved AOD data are within the expected error. It was established that 64.2% of AOD points are between 0 and 0.2 and 79.3% of all AE points are over 1. Mean AOD values in the region vary from 0.130 ​± ​0.04 (Moldova) to 0.193 ​± ​0.03 (Czech Republic) with mean value in the region 0.162 ​± ​0.05. Seasonal mean AOD (AE) values were at the maximum during the summer from 0.231 ​± ​0.05 (1.482 ​± ​0.09 in winter) to minimum 0.087 ​± ​0.04 during the winter (1.363 ​± ​0.17 in summer). Gradual AOD reduction is observed in all countries with annual trend from −0.0050 (Belarus) to −0.0029 (Russia). Finally, the relationship between AOD and AE was studied to classify various aerosol types and showed seasonal non-uniformity of their contribution depending on variation in sources. The entire region is under significant impact of various aerosol types, including clean continental (СС), mixed (MX) and anthropogenic/burning (AB) aerosols types that are at 59.77%, 24.72%, and 12.97% respectively. These results form an important basis for further regional studies of air quality and distribution of sources of pollution.  相似文献   

冰核观测中两种滤膜采样方法的比较     

周德平  张晋广  陈刚  李成龙  洪也  苏航  王扬锋 《气象与环境学报》2021,37(5):49-55

大气冰核观测是研究自然冷云降水和人工影响天气的一项基础性工作,滤膜—扩散云室法是观测冰核浓度的主要方法之一。为检测分析两种滤膜采集方法对冰核观测结果的影响,2011—2015年用自制的大气颗粒物采样器和FA-3型撞击式9级采样器开展了平行采样试验,采集的滤膜样本均在同一静力扩散云室中进行冰核活化显现分析。结果表明：自制采样器较9级采样器观测的冰核浓度高数倍甚至数十倍,但两者随季节和不同气象条件的变化表现出一致的起伏特征。自制采样器适用于对大气中总的冰核浓度分布及理化特征研究;9级采样器适用于对PM₁₀中不同粒径段大气冰核浓度和尺度分布以及理化特征的研究。滤膜法对冰核数量的低估与采样体积成正比,改变采样器气泵的抽气流量和控制采样体积对改进“体积效应”影响均有明显效果。  相似文献   

Evaluation and comparison of CMIP6 models and MERRA-2 reanalysis AOD against Satellite observations from 2000 to 2014 over China     

《地学前缘(英文版)》2022,13(2):101325

Rapid industrialization and urbanization along with a growing population are contributing significantly to air pollution in China. Evaluation of long-term aerosol optical depth (AOD) data from models and reanalysis, can greatly promote understanding of spatiotemporal variations in air pollution in China. To do this, AOD (550 nm) values from 2000 to 2014 were obtained from the Coupled Model Inter-comparison Project (CIMP6), the second version of Modern-Era Retrospective analysis for Research, and Applications (MERRA-2), and the Moderate Resolution Imaging Spectroradiometer (MODIS; flying on the Terra satellite) combined Dark Target and Deep Blue (DTB) aerosol product. We used the Terra-MODIS DTB AOD (hereafter MODIS DTB AOD) as a standard to evaluate CMIP6 Ensemble AOD (hereafter CMIP6 AOD) and MERRA-2 reanalysis AOD (hereafter MERRA-2 AOD). Results show better correlations and smaller errors between MERRA-2 and MODIS DTB AOD, than between CMIP6 and MODIS DTB AOD, in most regions of China, at both annual and seasonal scales. However, significant under- and over-estimations in the MERRA-2 and CMIP6 AOD were also observed relative to MODIS DTB AOD. The long-term (2000–2014) MODIS DTB AOD distributions show the highest AOD over the North China Plain (0.71) followed by Central China (0.69), Yangtse River Delta (0.67), Sichuan Basin (0.64), and Pearl River Delta (0.54) regions. The lowest AOD values were recorded over the Tibetan Plateau (0.13 ± 0.01) followed by Qinghai (0.19 ± 0.03) and the Gobi Desert (0.21 ± 0.03). Large amounts of sand and dust particles emitted from natural sources (the Taklamakan and Gobi Deserts) may result in higher AOD in spring compared to summer, autumn, and winter. Trends were also calculated for 2000–2005, for 2006–2010 (when China introduced strict air pollution control policies during the 11th Five Year Plan or FYP), and for 2011–2014 (during the 12th FYP). An increasing trend in MODIS DTB AOD was observed throughout the country during 2000–2014. The uncontrolled industrialization, urbanization, and rapid economic development that mostly occurred from 2000 to 2005 probably contributed to the overall increase in AOD. Finally, China's air pollution control policies helped to reduce AOD in most regions of the country; this was more evident during the 12th FYP period (2011–2014) than during the 11th FYP period (2006–2010). Therefore this study strongly advises the authority to retain or extend these policies in the future for improving air quality.  相似文献   

基于气象要素的气溶胶吸湿增长分析:以浙江省为例          下载免费PDF全文

祝好  王永前  陶金花  张自力  王子峰  曾巧林  陈良富 《气候与环境研究》2019,24(2):186-198

气溶胶粒子的吸湿增长对区域环境、气象与辐射收支都有巨大影响,精确的气溶胶吸湿特性观测对描述气溶胶吸湿增长特性,以及研究气溶胶对气候环境影响,拓展卫星气溶胶产品的应用有非常重要的意义。本研究提出一种基于常规气象观测（能见度、相对湿度）和空气质量观测（PM2.5浓度,即空气动力学当量直径小于等于2.5 μm的颗粒物浓度）相结合的气溶胶吸湿增长估算方法,在此基础上对浙江地区气溶胶吸湿特性的时空变化影响因素进行了探讨。研究发现,沿海的温州瓯海站的吸湿增长能力最高,长三角典型城市环境的杭州和睦小学站的吸湿增长能力次之,而地处较为洁净内陆的衢州实验学校站的吸湿增长能力最低。在时间变化中,同一站点不同湿度条件的吸湿增长变化趋势相同,温州瓯海站的吸湿性变化最为剧烈,杭州和睦小学站的吸湿性变化次之,衢州实验学校站变化较为平缓。本研究表明,浙江地区的气溶胶吸湿增长特性存在较大的时空差异,基于本方法能够在较大的时空范围内描述气溶胶的吸湿增长特性,为有限的精密观测提供重要补充。  相似文献   

大连市大气污染物质量浓度与气溶胶光学厚度的相关性分析     

顾吉林  汤宏山  刘淼  耿杨  于月  陶涛 《地理科学》2019,39(3):516-523

分别对2015年6~12月和2016年6~12月大连地区的大气污染物PM2.5、PM10、SO₂、NO₂、CO和O₃的浓度数据进行数据统计分析,基于ENVI软件平台利用MODIS数据反演大连地区的气溶胶光学厚度,通过回归建模研究气溶胶光学厚度与大连地区10个地面监测站点的大气污染物PM2.5、PM10、SO₂、NO₂、CO和O₃的浓度数据的相关性。回归建模以气溶胶光学厚度（AOD）为自变量,以大气污染物PM2.5、PM10、SO₂、NO₂、CO和O₃为因变量,在SPSS软件中分别选取线性、对数、三次、乘幂、指数5种函数类型进行研究,通过对比回归模型的拟合优度R²,选择最优拟合模型,探讨利用遥感数据反演气溶胶光学厚度监测大气污染的相关性。结果表明：气溶胶光学厚度与NO₂、PM2.5和PM10的最优拟合模型均为三次模型,其拟合优度R²分别是0.685、0.801和0.845;与O₃和SO₂的最优拟合模型为指数模型,其R²为0.367和0.482;与CO的最优拟合模型为对数模型,其拟合优度R²为0.810。该结果为分析大气气溶胶污染来源以及治理提供了数据。  相似文献   

气溶胶对雷暴云起电以及闪电发生率影响的数值模拟   总被引：5，自引：1，他引：4  

师正  谭涌波  唐慧强  杨忆  彭琳  郭秀峰  陈浩然 《大气科学》2015,39(5):941-952

本文利用二维耦合气溶胶模块的雷暴云起电模式,结合一次南京雷暴个例,进行250 m分辨率雷暴云起电模拟实验,探讨了气溶胶浓度对雷暴云空间电荷分布以及闪电发生率的影响。在这个气溶胶模块中,假定一个三模态的气溶胶对数分布,考虑了气溶胶活化过程。结果显示:(1)随着气溶胶浓度增大,雷暴云电荷结构保持为三极型。(2)当气溶胶浓度从50 cm-3增加至1000 cm-3时,水成物粒子浓度上升,雷暴云电荷量和闪电发生率增加明显。(3)气溶胶浓度在1000~3000 cm-3范围时,云水竞争限制了冰晶的增长,导致雷暴云上部主正电荷堆电荷量降低。云滴和霰粒子浓度缓慢上升促进中部主负电荷堆和底部次正电荷堆电荷量继续增大。闪电发生率保持稳定。(4)当气溶胶浓度大于3000 cm-3时,水成物粒子浓度稳定,云内的电荷量以及闪电发生率保持为一定量级。  相似文献   

沈阳大气气溶胶光学特性及其影响因子   总被引：4，自引：0，他引：4  

赵胡笳  马雁军  王扬锋  朱轶明 《气象与环境学报》2015,(3):43-49

利用2010年3—10月沈阳大气成分监测站CE－318太阳光度计观测资料,计算沈阳大气气溶胶光学厚度和波长指数等大气光学特性参数,结合地面气象观测资料,分析大气气溶胶光学特性及其影响因子。结果表明：沈阳气溶胶光学厚度在3—6月较高,8月较低,9—10月气溶胶光学厚度略有增加;除4月和8月外,气溶胶光学厚度与风速基本呈反相关;气溶胶光学厚度与可吸入颗粒物（particulate matter,PM）质量浓度变化趋势基本一致;气溶胶光学厚度日平均值距平的绝对值、改变率均与降水强度成正比;地面能见度与气溶胶光学厚度呈负相关。由气溶胶浑浊度系数计算的能见度在4—6月与实际观测的能见度基本吻合,由气溶胶标高计算的水平能见度整体小于实际观测的水平能见度。  相似文献   

利用激光雷达资料分析兰州远郊气溶胶光学特性   总被引：9，自引：1，他引：8       下载免费PDF全文

周碧  张镭  曹贤洁  韩霄  张武  冯广泓 《高原气象》2011,30(4):1011-1017

利用2007年1～4月兰州大学半干旱气候与环境观测站激光雷达资料,反演了晴空无云典型日和沙尘过程大气气溶胶消光系数和光学厚度。结果表明,兰州远郊榆中地区,1km以下大气气溶胶消光系数较大,为0.01～0.1km-1;平均气溶胶光学厚度〈0.5,光学厚度日变化呈双峰型,峰值分别出现在12：00和20：00。采暖期与非采暖...  相似文献   

An Aerosol Model of the Marine and Coastal Atmospheric Surface Layer     

G. A. Kaloshin  I. A. Grishin 《大气与海洋》2013,51(2):112-120

We present a microphysical model for the surface layer marine and coastal atmospheric aerosols that is based on long-term observations of size distributions for 0.01–100 µm particles. The fundamental feature of the model is a parameterization of amplitudes and widths for aerosol modes of the aerosol size distribution function (ASDF) as functions of fetch and wind speed. The shape of ASDF and its dependence on meteorological parameters, height above sea level (H), fetch (X), wind speed (U) and relative humidity (RH), are investigated. At present, the model covers the ranges H = 0–25 m, U?=?3–18 km s^?1, X?≤?120 km and RH?=?40–98%.

The latest version of the Marine Aerosol Extinction Profiles model (MaexPro) is described and applied to the computation and analysis of the spectral profiles of aerosol extinction coefficients α(λ) in the wavelength band λ?=?0.2–12 µm. MaexPro is based on the aforementioned aerosol model assuming spherically shaped aerosol particles and the well-known Mie theory.

The spectral profiles of α(λ) calculated by MaexPro are in good agreement with observational data and the numerical results obtained from the Navy Aerosol Model (NAM) and the Advanced Navy Aerosol Model (ANAM). Moreover, MaexPro was found to be an accurate and reliable tool for investigating the optical properties of atmospheric aerosols.  相似文献   

Removal of Elongated Particle Aggregates on Fibrous Filters     

Lucija Boskovic  Igor S. Altman  Roger D. Braddock  Igor E. Agranovski 《洁净——土壤、空气、水》2009,37(11):843-849

Elongated aerosol particle removal on fibrous filters has been investigated. It was shown that particle agglomerates are removed much more efficiently compared to the regularly shaped single particles with identical electrical mobility diameter at two filtration velocities tested. The experimental results were compared with the classical filtration theory and it was shown that the theoretical predictions, which are based on the assumption that the particles are spherical, are significantly different compared to an agglomerate filtration efficiency value. In order to account for a particle shape non-regularity, dominating nanoparticle removal mechanisms were firstly evaluated for a regular particle of certain size and then adjusted by fitting coefficients k₁ (for diffusion component) and k₂ (for interception). These coefficients were determined by fitting the theoretical values that gives the best coincidence with the measured data points. As was further demonstrated theoretically, the coefficient k₁ is identical to the ratio of the actual particle surface area to the surface area of the spherical particle of the equivalent diameter. On the other hand, the coefficient k₂ was found to be equal to the ratio of the projection of a given particle on a plane perpendicular to a streamline, to that of the spherical particle of the equivalent diameter. The reported findings would allow undertaking more accurate evaluation of the removal efficiency of non-regular aerosol particle, which is especially important for industrial applications where non-regular aerosols are frequently met.  相似文献