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Microcystins(MCs) are cyclic hepatotoxic peptides produced by the bloom-forming cyanobacterium Microcystis and present a public health hazard to humans and livestock. The removal of MCs from contaminated water with powdered activated carbon(PAC) has been employed as a simple and economic treatment strategy. In this study, PAC-Fe(Ⅲ) was prepared and utilized for the fast and efficient removal of MCs from water. PAC-Fe(Ⅲ) exhibited superior microcystin-LR(MC-LR) removal capacity and efficiency compared to the unmodified PAC. The MC-LR removal efficiency of PAC-Fe(Ⅲ) increased with decreasing p H within the pH range of 4.3 to 9.6. PAC-Fe(Ⅲ) could be reused for 3 times by methanol elution while the MC-LR removal efficiency was still over 70 percent. The removal efficiency was positively correlated to the ionic strength of water and negatively correlated to alkalinity. Natural organic matter(NOM) such as humic acid(HA) and salicylic acid(SA) generated low interference with MC-LR adsorption by PAC-Fe(Ⅲ). The complexation reaction between Fe~(3+) in PAC-Fe(Ⅲ) and the functional groups of MCLR was suggested as the key mechanism of MC-LR removal by PAC-Fe(Ⅲ). The results suggest that Femodified PAC is a promising material for the treatment of MC-contaminated waters. 相似文献
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鄱阳湖是我国最大淡水湖泊,湖泊水文节律变化显著影响着湖区生产生活、生态环境,但界定标准尚未形成统一认识。综合考虑水位变化规律、湖盆形态特点、水资源利用等特征指标,探讨鄱阳湖丰、平、枯水期界定标准。结果表明：以星子站作为鄱阳湖代表性测站,当星子站水位大于17.00 m时为丰水期,13.01～16.00 m为平水期,小于12.00 m（含12.00 m）为枯水期,16.01～17.00 m为平—丰过渡期,12.01～13.00 m为枯—平过渡期。枯水期多发生在10月下旬至次年4月上旬,发生日数平均为142 d;丰水期多发生在7月上旬至8月中旬,发生日数平均为40 d;平水期多发生在4月中旬至6月下旬、8月下旬至10月中旬,发生日数平均为117 d。 相似文献
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蓝藻水华及其释放的蓝藻毒素给我国很多地区的饮用水安全带来较大威胁.尽管去除蓝藻和净化藻毒素的技术目前已有较多报道,但能同时对二者起作用的技术方法还较少,发展能够同时去除蓝藻和蓝藻毒素的技术显得十分必要.根据前期Fe(Ⅲ)化合物去除微囊藻毒素的工作基础,选取4种不同的土壤对其进行Fe(Ⅲ)改性,并应用于微囊藻毒素的去除.结果表明,黏土含量高低决定土壤本身对毒素的吸附能力强弱;土壤经过离子改性后,其毒素吸附能力与其阳离子交换量大小直接相关,且毒素去除能力较未改性前有显著提高,其中效率提升最高的一种土壤离子改性后其吸附能力增加了约148倍.离子改性土壤对微囊藻细胞同样具有絮凝沉降功能,沉降能力同样随土壤对Fe(Ⅲ)负载能力的提高而上升,使用剂量提高时微囊藻沉降平衡时间明显缩短.在野外蓝藻水华去除实验中,蓝藻细胞去除可以保持与室内实验相近的高去除率,但蓝藻毒素的去除效率有一定的下降,可能与天然水体中其它杂质的竞争作用有关. 相似文献
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