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A multi-layer deposited ice film was prepared through water vapor deposition on a Ni plate in a vacuum chamber at 90 K, and was used as it was or after annealing at 140 K. NO2 was adsorbed as N2O4 approximately 90 K on the ice film prepared as above, and irradiated by 193 nm excimer laser light. The time-of-flight (TOF) spectra of the desorbed species, i.e., NO2, NO, O2 and O, were measured by a quadrupole mass spectrometer. The photochemical process obeyed an one-photon process. The relative yields of the products and their TOF spectra were dependent on the preparation condition of the ice film and also varied with the continuation of the laser irradiation. From the ice film annealed at 140 K, NO2, NO and O2 were desorbed with an approximate ratio of 1:1:0.01. From the non-annealed film, the relative yield of NO2 was much smaller than that of NO. The TOF spectrum of NO from the non-annealed ice film consisted of distinctly different two components corresponding to the 1700 and 100 K translational temperature, respectively. The fast component was lost when additional ice was deposited on the adsorbed N2O4. NO was supposed to be a predissociation product from the electronically excited NO2 prepared through the photodissociation of N2O4. 相似文献
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Shinya Iwasaki Kozo Takahashi Yusuke Ogawa Seiichiro Uehara Christoph Vogt 《Journal of Oceanography》2014,70(3):241-249
Accurate knowledge of the extent of biogenic opal preservation in marine sediment cores is important for paleoceanographic reconstructions. The alkaline leaching method is widely employed for %biogenic opal analysis due to its ease and speed. In this study, a revised method for measuring %biogenic opal in sediment from arctic coring expedition samples was suggested. The studied middle Eocene sediments from the central Arctic Ocean presented a problem in insufficiently leaching biogenic opal with a Na2CO3 solution. Based on XRD analysis, it was suggested that such an alkaline resistance results from slight diagenesis of biogenic opal. In order to solve this problem, an alkaline leaching method utilizing a 2 M NaOH solution was suggested for the accurate measurement of %biogenic opal in the Eocene sediments from the central Arctic. Furthermore, dissolution rates from lithogenic matter by NaOH solution were measured in order to correct the %biogenic opal values. 相似文献
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The sediment parameters and nematode assemblages in the intertidal zone of the Hichirippu shallow lagoon, Hokkaido, Japan, were investigated. The objectives of this study were to observe the seasonal variation in the nematodes in the sediment, and to investigate the relationships between the nematodes and environmental factors. Samples were collected bi-monthly from five stations on the tidal flat from April 2003 to February 2004. It was found that the sediment parameters (Chl a concentration, AVS, TOC and TN contents) varied throughout the 10-month study. Fifty-four species of nematodes were found in the study area. The density and biomass of the nematodes varied in accordance with the sediment temperature during the sampling period. In this study, there was a seasonal variation in the nematode assemblage found in the intertidal zone of this shallow lagoon. The important factors affecting this variation were sediment temperature, and food competition among the nematodes themselves. The seasonal variation of the nematode also showed a relationship with the Chl a concentration in the sediment during the sampling period. 相似文献
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Takeshi Tsuji Yasuyuki Nakamura Hidekazu Tokuyama Millard F. Coffin Keita Koda 《Island Arc》2007,16(3):361-373
Abstract To show the structure of oceanic crust and Moho around the eastern Ogasawara Plateau, we have analyzed industry-standard two-dimensional multichannel seismic reflection data. To obtain improved velocity models, phase information of seismic signals was used for velocity analysis and velocity models for oceanic crust above Moho were determined. We apply this velocity analysis technique to seismic reflection data around the eastern Ogasawara Plateau, with the result of clear images of structures within oceanic crust and Moho. South of the Ogasawara Plateau, Moho deepens proximal to the Plateau. Moho distal to the Plateau is ca 7 km below sea floor (bsf), whereas it is ca 10 km bsf near the Plateau. The characters of oceanic crust and Moho differ significantly north and south of the Plateau. To the north, the structure of oceanic crust is ambiguous, the sea floor is shallower and less smooth, and Moho is discontinuous. To the south, structures within oceanic crust and Moho are imaged clearly, and the sea floor is deeper. A strong Moho reflection south of the Plateau might represent a sharp boundary between layered gabbro and peridotite. However, discontinuous Moho reflections north of the Plateau might represent rough topography because of intensive magmatism or a gradual downward increase in velocity within a thick Moho transition zone. A fracture zone north of the Plateau also appears to separate oceanic crust and Moho of different characters, suggesting vigorous magmatism between the Plateau and the fracture zone, and that the Ogasawara Plateau and the fracture zone influenced the genesis of oceanic crust and upper mantle. Differences in acoustic characteristics to the north and south of the Plateau are apparent in profiles illuminated by seismic attributes. 相似文献
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Variation of crustal thickness in the Philippine Sea deduced from three-dimensional gravity modeling
Abstract Crustal thickness of the northern to central Philippine Sea was gravimetrically determined on the simple assumption of four layers: seawater, sediments, crust and lithospheric mantle, with densities of 1030, 2300, 2800 and 3300 kg/m3 , respectively. As for the correction of the regional gravity variation, a 15 km difference of the lithospheric thickness with a density difference of 50 kg/m3 against the asthenosphere below between both sides of the Kyushu-Palau Ridge was taken into consideration. Mantle Bouguer anomalies were calculated on the assumption of constant crustal thickness of 6 km, and then the crustal thickness was obtained by three-dimensional gravity inversion method. The results show occurrence of thin crust areas with a thickness of approximately 5 km in the southern part and at the western margin of the Shikoku Basin and also of thick crust areas in the northwestern and northeastern parts of the Parece Vela Basin. We suggest that these are because of the variation of magma supply at the time of sea floor spreading in the Shikoku and Parece Vela Basins, which is possibly related to the variation of spreading rate and enhanced magmatism near the past arc volcanic fronts. The results further show the occurrence of crust thinner than 5 km in the northeastern part of the West Philippine Basin, of crust thicker than 15 km in the Amami Plateau, the Daito and Oki-Daito Ridges, and also in the northern part of Kyushu-Palau Ridge, whereas the southern part of the Kyushu-Palau Ridge the crust is thicker than 10 km. It was also inferred that small basins in the Daito Ridge province have the thinnest oceanic crust of less than 5 km in the Kita-Daito Basin. 相似文献
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Fault configuration produced by initial arc rifting in the Parece Vela Basin as deduced from seismic reflection data 总被引：1，自引：0，他引：1
Mikiya Yamashita Tetsuro Tsuru Narumi Takahashi Kaoru Takizawa Yoshiyuki Kaneda Kantaro Fujioka Keita Koda 《Island Arc》2007,16(3):338-347
Abstract The Parece Vela Basin (PVB), which is a currently inactive back-arc basin of the Philippine Sea Plate, was formed by separation between the Izu-Ogasawara Arc (IOA) and the Kyushu-Palau Ridge (KPR). Elucidating the marks of the past back-arc opening and rifting is important for investigation of its crustal structure. To image its fault configurations and crustal deformation, pre-stack depth migration to multichannel seismic reflection was applied and data obtained by the Japan Agency for Marine-Earth Science and Technology and Metal Mining Agency of Japan and Japan National Oil Corporation (Japan Oil, Gas and Metals National Corporation). Salient results for the pre-stack depth-migrated sections are: (i) deep reflectors exist around the eastern margin of KPR and at the western margin of IOA down to 8 km depth; and (ii) normal fault zones distributed at the eastern margin of the KPR (Fault zone A) and the western margin of the IOA (Fault zone B) have a total displacement of greater than 500 m associated with synrift sediments. Additional normal faults (Fault zone C) exist 20 km east of the Fault zone B. They are covered with sediment, which indicates deposition of recent volcanic products in the IOA. According to those results: (i) the fault displacement of more than 500 m with respect to initial rifting was approximately asymmetric at 25 Ma based on PSDM profiles; and (ii) the faults had reactivated after 23 Ma, based on the age of deformed sediments obtained from past ocean drillings. The age of the base sediments corresponds to those of spreading and rotation after rifting in the PVB. Fault zone C is covered with thick and not deformed volcanogenic sediments from the IOA, which suggests that the fault is inactive. 相似文献
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Toshiyuki Ohtsuka Mitsuru Hirota Xianzhou Zhang Ayako Shimono Yukiko Senga Minguan Du Seiichiro Yonemura Shigeto Kawashima Yanhong Tang 《Polar Science》2008,2(4):277-285
To accurately estimate soil organic carbon (SOC) storage in upper alpine to nival zones on the Tibetan Plateau, we inventoried SOC pools in 0–0.3 m profiles along an altitudinal gradient (4400–5300 m asl). We also studied vegetation properties and decomposition activity along the gradient to provide insight into the mechanisms of SOC storage. The vegetation cover and belowground root biomass showed a gradual increased with altitude, reaching a peak in the upper alpine zone at 4800–4950 m before decreasing in the nival zone at 5200–5300 m.Decomposition activity was invariant along the altitudinal gradient except in the nival zone. SOC pools at lower sites were relatively small (2.6 kg C m−2 at 4400 m), but increased sharply with altitude, reaching a peak in the upper alpine zone (4950 m; 13.7 kg C m−2) before decreasing (1.0 kg C m−2 at 5300 m) with altitude in the nival zone. SOC pool varied greatly within individual alpine meadows by a factor of five or more, as did bulk density, partly due to the effect of grazing. Inventory data for both carbon density and bulk density along altitudinal gradients in alpine ecosystems are of crucial importance in estimating global tundra SOC storage. 相似文献
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Based on measured stream nitrogen concentrations at outlets of 12 small sub‐areas (1·3–54·7 km2) in a largely forested catchment during the base flow period, we investigated the influences of discharges and different catchment characteristics on stream nitrogen concentration. Our field surveys were carried out during the 11‐month's period from April 2001 to February 2002 and the correlations between nitrogen concentrations and catchment characteristics were studied. The results showed that the vegetation cover was strongly correlated to total nitrogen (TN) and nitrate + nitrite ? nitrogen (NOx‐N) concentrations. That is, the TN and NOx‐N concentrations had positive correlations with mean normalized difference vegetation cover index (NDVI) of each sub‐area during dormant seasons (mean NDVI < 0 · 70) and had negative correlations during the growing season (mean NDVI ≥ 0 . 70). The significance of catchment characteristics to TN and NOx‐N concentrations was ranked as vegetation cover > soil > topography > land use, and the best models can account for 55–64% of the variance of TN and NOx‐N concentrations. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献