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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
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Zhi Xu Cheng Fang Wei-Qun Can Astronomy Department of Nanjing University Nanjing Purple Mountain Observatory Chinese Academy of Sciences Nanjing 《中国天文和天体物理学报》2005,5(5):519-530
Chromospheric lines, including Ha, Lyα, Lyβand CaⅡK, CaⅡ8542, are systemically and quantitatively investigated with respect to the non-thermal excitation and ionization due to particle beam bombardment for a series of solar semi-empirical atmospheric models. As a result we propose to use the contrast in the integrated intensity of hydrogen lines to estimate the total energy flux of the bombarding beam during the solar flare impulsive phase. Partial frequency redistribution is considered in the Lyαline calculation and a smaller intensity enhancement in the Ha line-centers is found than in the previous results of Fang et al. 相似文献
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为建立社会主义市场经济的地矿工作新秩序,本文对国有地矿企业的经营者(厂长、经理)这一特殊群体进行了分析。着重研究了新形势下企业经营者实行年薪制的问题。指出年薪制就是以企业一个生产经营周期为单位确定经营者的报酬,这一周期通常为一年。进而阐述了为什么要实行企业经营者年薪制;企业经营者的收入应与职工工资完全脱钩;采用基础报酬加效益报酬的方法确定收入等等。并构想了实行经营者年薪制所需要的外部环境:建立经营者人才市场、经营者要能进能出、实行任职资格制度、建立风险机制、按劳动力市场经济规律办事。 相似文献
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从ROSAT巡天和定点观测结果的对比出发,发现了几个低银纬的巡天源表中的X射线源在定点观测中没有出现.本文计算了在这些位置的定点观测中出现点源的流强上限,发现比巡天源表中这些源的流强值低很多,这表明它们的流强变化很大,可能是X射线双星系统中的一类———X射线暂现源. 相似文献
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STUDY ON GIS FOR YIELD ESTIMATION BY REMOTE SENSING IN JILIN MAIZE BELTSTUDYONGISFORYIELDESTIMATIONBYREMOTESENSINGINJILINMAIZ... 相似文献
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Three continuous marine fish cell lines of FG (i. e., Hounder Gill) from flounder (Paralichthys olivaceus) gill, SPH (i. e. , Sea Perch Heart) from sea perch (Lateolabrax japonicus) heart and RSBF (i.e., Red Sea Bream Fin) from red sea bream (Pagrosomus major) fin, were characterized by lactate dehydrogenase (LDH) isozyme and morphological analysis. The LDH isozyme patterns of these three cell lines and their corresponding tissues of origin were investigated and compared. The results showed: (1) No difference was found in the LDH isozyme patterns of FG and flounder gill tissue. However, the LDH isozyme patterns of SPH and RSBF were significantly different from their corresponding tissues of origin; (2) LDH isozyme patterns of FG, SPH and RSBF were markedly different from each other and could serve as genetic markers for species identification and detection of cross contamination. Morphological change analysis of these three cell lines in comparison to their original tissues indicated that FG cells still appeared epithelioid without morphological transformation. However, morphological changes were found in SPH and RSBF compared to their original tissues. Therefore, the cellular morphology was still plastic in the relatively stable culture conditions, and it was possible that change of LDH patterns wasrelated to morphological changes of fish cells in vitro. 相似文献
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本文叙述南天区 5GHzVLBI普查中新发现的视超光速射电源 ,0 4 2 0— 0 1 4,1 334—1 2 7和 2 345— 1 67,这些结果尚待进一步的观测加以证实 相似文献