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Mass loading and chemical composition of atmospheric aerosols over the Arabian Sea during the pre-monsoon months of April and May have been studied as a part of the Integrated Campaign for Aerosols, gases and Radiation Budget (ICARB). These investigations show large spatial variabilities in total aerosol mass loading as well as that of individual chemical species. The mass loading is found to vary between 3.5 and 69.2 μg m?3, with higher loadings near the eastern and northern parts of Arabian Sea, which decreases steadily to reach its minimum value in the mid Arabian Sea. The decrease in mass loading from the coast of India towards west is estimated to have a linear gradient of 1.53 μg m?3/° longitude and an e?1 scale distance of ~2300 km. SO 4 2? , Cl? and Na+ are found to be the major ionic species present. Apart from these, other dominating watersoluble components of aerosols are NO 3 ? (17%) and Ca2+ (6%). Over the marine environment of Arabian Sea, the non-sea-salt component dominates accounting to ~76% of the total aerosol mass. The spatial variations of the various ions are examined in the light of prevailing meteorological conditions and airmass back trajectories. 相似文献
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Jonathan F. Stebbins Emily V. Dubinsky Koji Kanehashi Kimberly E. Kelsey 《Geochimica et cosmochimica acta》2008,72(3):910-925
Configurational changes with temperature are important for the thermodynamic and transport properties of most aluminosilicate melts, but in general are not well understood. Here, we present high-resolution 27Al and 17O NMR data on several calcium aluminosilicate glasses prepared with varying quench rates and thus with fictive temperatures that span ranges up to about 200 K. In all compositions the content of five-coordinated aluminum increases with fictive temperature, in agreement with recent high temperature NMR data on melts. In a glass of CaAl2Si2O8 (“anorthite”) composition, the content of non-bridging oxygens also increases with temperature; however this effect was not observed in a sample with a much higher CaO/Al2O3 ratio. We present a consistent notation for reactions among structural species in these systems that clarify why in some cases, high-coordinated network cations may appear on the same side of the reaction, while in others they occur on the opposite sides: the key difference is in accounting for all coordination changes for oxygens. Mixing of non-bridging oxygens and of high-coordinated aluminum make significant contributions to the overall configurational entropy and heat capacity of the melts, as does the mixing of various bridging oxygens and of tetrahedral network cations. Other, less well known, types of increase in disorder with temperature may be important as well. 相似文献
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Forces induced by regular waves on submarine pipelines resting on as well as near a plane boundary and aligned parallel to wave fronts of the oncoming waves are investigated experimentally. The inline hydrodynamic coefficients of drag and inertia are evaluated through the use of Morison equation and the least squares method. The transverse force is analysed in terms of maximum transverse force and transverse root mean square (r.m.s.) coefficients. The resulting inline and transverse hydrodynamic coefficients are correlated with the period parameter or Keulegan-Carpenter number and relative clearance of the pipeline from the plane boundary. The effect of depth parameter on these coefficients and the correlation between maximum transverse force and transverse r.m.s. coefficients are also reported. 相似文献
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Joseph M. Delesantro Jonathan M. Duncan Diego Riveros-Iregui Joanna R. Blaszczak Emily S. Bernhardt Dean L. Urban Lawrence E. Band 《水文研究》2021,35(9):e14339
Current land-use classifications used to assess urbanization effects on stream water quality date back to the 1980s when limited information was available to characterize watershed attributes that mediate non-point source pollution. With high resolution remote sensing and widely used GIS tools, there has been a vast increase in the availability and precision of geospatial data of built environments. In this study, we leverage geospatial data to expand the characterization of developed landscapes and create a typology that allows us to better understand the impact of complex developed landscapes across the rural to urban gradient. We assess the ability of the developed landscape typology to reveal patterns in stream water chemistry previously undetected by traditional land-cover based classification. We examine the distribution of land-cover, infrastructure, topography and geology across 3876 National Hydrography Dataset Plus catchments in the Piedmont region of North Carolina, USA. From this dataset, we generate metrics to evaluate the abundance, density and position of landscape features relative to streams, catchment outlets and topographic wetness metrics. While impervious surfaces are a key distinguishing feature of the urban landscape, sanitary infrastructure, population density and geology are better predictors of baseflow stream water chemistry. Unsupervised clustering was used to generate a distinct developed landscape typology based on the expanded, high-resolution landscape feature information. Using stream chemistry data from 37 developed headwater catchments, we compared the baseflow water chemistry grouped by traditional land-cover based classes of urbanization (rural, low, medium and high density) to our composition and structure-based classification (a nine-class typology). The typology based on 22 metrics of developed landscape composition and structure explained over 50% of the variation in NO3−-N, TDN, DOC, Cl−, and Br− concentration, while the ISC-based classification only significantly explained 23% of the variation in TDN. These results demonstrate the importance of infrastructure, population and geology in defining developed landscapes and improving discrete classes for water management. 相似文献
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AbstractNatural resource challenges often span administrative jurisdictions and include actors and processes operating at different spatial and political scales. We applied concepts of new environmental governance to analyze Oregon’s approach to greater sage-grouse conservation. Through one in-depth case study in Lake County, we traced features of new environmental governance (cross-scale interactions, decentralization, and capacities of actors) through different governance levels. Interviews and qualitative analysis revealed that decentralization of administrative functions facilitated cross-scale interactions and relied on intermediaries, gap-filling, and perceptions of legitimacy at lower levels. State and agency guidelines steered the effort and were accompanied by financial and technical resources from multiple arenas, which increased local capacity. This study adds to the understandings of environmental governance for implementing multi-actor, multi-level conservation arrangements in resource-dependent communities. Further exploration of connections between higher levels and local contexts will reveal important, new ways to link policies with on-the-ground outcomes. 相似文献
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Emily Cloyd Susanne C. Moser Edward Maibach Julie Maldonado Tinqiao Chen 《Climatic change》2016,136(1):39-55
This paper examines the dynamics of energy investments and clean energy Research and Development (R&D) using a scenario-based modeling approach. Starting from the global scenarios proposed in the RoSE model ensemble experiment, we analyze the dynamics of investments under different assumptions regarding economic and population growth as well as availability of fossil fuel resources, in the absence of a climate policy. Our analysis indicates that economic growth and the speed of income convergence across countries matters for improvements in energy efficiency, both via dedicated R&D investments but mostly through capital-energy substitution. In contrast, fossil fuel prices, by changing the relative competitiveness of energy sources, create an economic opportunity for radical innovation in the energy sector. Indeed, our results suggest that fossil fuel availability is the key driver of investments in low carbon energy innovation. However, this innovation, by itself, is not sufficient to induce emission reductions compatible with climate stabilization objectives. 相似文献
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