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1.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
2.
介绍了云南天文台天体测量工作的发展过程,论述了在空间时代地面光学基本天体测量的必要性和应具备的条件,并且叙述了在新的要求和条件下,地面光学基本天体测量工作应该发挥的作用和广阔的发展前景。 相似文献
3.
海岩的长篇小说《河流如血》再创出版高记录,但作家仍局限于特有的小说叙述模式,这部作品设能做到相应的创新。概言之,模式第一面是“刑侦+恋爱”;模式第二面是“财子+佳人”;模式第三面是“道德+法制”。文学创作需要不断创新,创新的过程也是对创作模式的不断突破过程。作家应该警惕的是,不要让模式成为创作的桎梏。 相似文献
4.
Tidal effects on temperature front in the Yellow Sea 总被引:5,自引:0,他引:5
Temperature front (TF) is one of the important features in the Yellow Sea, which forms in spring, thrives in summer, and fades
in autumn as thermocline declines. TF intensity ⋎S
T
⋎ is defined to describe the distribution of TF. Based on the MASNUM wave-tide-circulation coupled model, temperature distribution
in the Yellow Sea was simulated with and without tidal effects. Along 36°N, distribution of TF from the simulated results
are compared with the observations, and a quantitative analysis is introduced to evaluate the tidal effects on the forming
and maintaining processes of the TF. Tidal mixing and the circulation structure adapting to it are the main causes of the
TF.
Supported by the National Basic Research Program of China (No. G1999043809) and the National Science Foundation of China (No.
49736190). 相似文献
5.
PALEOSOLSOFSANDYLANDSANDENVIRONMENTALCHANGESINTHEWESTERNPARTOFNORTHEASTPLAINOFCHINAWESTERNDURINGHOLOCENE¥QiuShanwen(裘善文)LiQus... 相似文献
6.
In this paper, two factors — the redistribution of the density and the variation in the angular velocity of the Earth rotation, that affect the adopted value of the flattening for equidensity surface within the Earth, are discussed. The computational results show that the contribution of the redistribution of the density in the Earth interior (especially in the core) on the change of the flattening at the core-mantle boundary (CMB) is marginal, and that the calculated value of the flattening at the CMB can be in good agreement with the VLBI observed value so long as the fact that the angular velocity of the Earth rotation has undergone the tidal evolution is taken into account. As a result, this paper presents a set of recommended values of the dynamical parameters of the Earth (see Table III) for computing Earth's forced nutation series. 相似文献
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9.
企鹅珍珠贝人工苗生长的初步观察 总被引:3,自引:0,他引:3
为了解企鹅珍珠贝生长规律,观察了壳高2.5~5.0mm的出池幼苗,按月测量其生长参数和成活率,以及环境因子。结果表明,企鹅珍珠贝生长最快的月份为7~11月和次年4~6月,壳长,壳高和壳宽月均增加量分别为3.8~13.0mm、4.7~11.2mm、2.3~3.8mm,月成活率97.8%~98.6%。企鹅珍珠贝生长最慢月份是11月至次年3月。 相似文献
10.
Quasi-electrostatic electron and ion-cyclotron instabilities are studied. The result indicates that the higher harmonic ion cyclotron instabilities (ICI) can be excited while the fast ions produced from reconnection are injected into a coronal loop. Part of the energetic ions can be dragged out of the magnetic mirror turning points and a negative plasma potential is generated. The plasma potential may directly accelerate the electrons up to the relativistic velocity within a short time. This acceleration is similar to the processes occurring in the magnetic mirror devices of controlled thermonuclear fusion. The spectrum and flux of accelerated electrons have also been obtained. Some observational results during the solar flare might be explained by this acceleration mechanism. 相似文献